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Shiyu Zhu

Publications and source records attributed to Shiyu Zhu.

At least 19 recordsLinked to original sources

Decoupled domain-texture switching from magnetic easy axis in kagome ferromagnet EuTi3Bi4

Magnetic anisotropy defines the easy axis of a magnetic material and governs the spatial arrangement of its domains. To date, anisotropy engineering has focused on reorienting the easy axis or tuning the anisotropy energy, both of which demand substantial energy input. Here, we demonstrate that magnetic domain textures can be switched without reorienting the easy axis, as observed in a kagome ferromagnet EuTi3Bi4 crystal. Using low-temperature magnetic force microscopy, we observe that the preferred orientation of magnetic domains switches from the a-axis to the b-axis upon temperature variation, and that this switching can also be triggered by an out-of-plane magnetic-field reset. Magnetization measurements and density functional theory calculations confirm a robust c-axis easy magnetization, ruling out a conventional spin-reorientation transition. Instead, the texture switching is governed by the temperature dependence of the in-plane variation of the Magnetic anisotropy energy landscape, which arises from two competing interactions with different decay rates: single-ion anisotropy favors a-oriented spin components, while nearest-neighbor anisotropic exchange favors b-oriented ones. Furthermore, the critical switching temperature is substantially elevated in a mechanically exfoliated EuTi3Bi4 flake. Our findings establish that macroscopic magnetic textures can be effectively manipulated by tuning the competition between in-plane anisotropic interactions, without the energy cost of reorienting the easy axis.

cond-mat.mtrl-sci

Simultaneous nanoscale imaging of local conductivity and chemical potential in a quantum Hall isospin ferromagnet

Quantum Hall isospin ferromagnetism in multilayer graphene offers a versatile playground for exploring flat band correlated physics, driven by the intricate coupling of spin, valley, orbital, and layer degrees of freedom. However, a nanoscale probe capable of simultaneously mapping local conductivity and chemical potential in these exotic phases has yet to be realized. Here, we introduce scanning conductivity and chemical potential microscopy (SCCM), a technique integrating scanning microwave impedance microscopy and Kelvin probe force microscopy. We demonstrate SCCM by probing the quantum Hall states and many-body Landau level energy spectrum in bilayer graphene. Applied to marginally twisted double bilayer graphene, SCCM then reveals a cascade of quantum Hall isospin ferromagnetic states with unexpected re-emergence behaviors. Significantly, experimental many-body Landau level energy spectrum further uncovers the intricate connections of these complex phenomena to inter-subband Landau level crossings and Landau level single-particle wavefunctions. These insights enable the construction of a comprehensive quantum Hall phase diagram. Our results demonstrate SCCM's capability in decoding complex quantum phenomena, establishing it as a versatile nanoscale probe for electron correlation and topology.

cond-mat.mes-hall

Capacitive Touchscreens at Risk: A Practical Side-Channel Attack on Smartphones via Electromagnetic Emanations

Capacitive touchscreens in modern smartphones introduce severe side-channel vulnerabilities. However, existing attacks often require restrictive conditions or invasive measurements. This paper presents TESLA, a novel, contactless electromagnetic (EM) side-channel attack that exploits inherent EM emanations during touchscreen scanning. We demonstrate that these emanations encode the spatiotemporal evolution of touch interactions, forming a unified leakage basis. By secretly placing an EM probe near the victim's device, TESLA enables attackers to extract highly sensitive information, including screen-unlocking PIN codes, keyboard inputs, interacting application categories, and continuous handwriting trajectories. Compared to existing attacks, TESLA offers a broader range of attack targets, more efficient sample acquisition, and operations in practical attack scenarios. Extensive evaluations on popular commercial smartphones, specifically the iPhone X, Xiaomi 10 Pro, Samsung S10, and Huawei Mate 30 Pro, validate the effectiveness of TESLA. It achieves remarkable inference accuracy in diverse settings such as private meeting rooms and public libraries, with success rates of 99.3% for PIN code recognition, 97.6% for keyboard input reconstruction, and 95.0% for application inference, respectively. Simultaneously, it attains a 76.8% character recognition accuracy and a high geometric similarity (Jaccard index of 0.74) for 2D handwriting trajectory reconstruction.

cs.CR

Controllable highly oriented skyrmion track array in Fe3GaTe2

Magnetic skyrmions are emerging as promising candidates for next-generation information technologies, while the realization of scalable skyrmion lattices with tailored configurations is essential for advancing fundamental skyrmion physics and developing future applications. Here we achieved the controllable generation and regulation of a large-area, highly oriented skyrmion track array (STA) in ferromagnetic Fe3GaTe2 using a vector magnetic field manipulation technique. The orientation and ordering of STA, along with the types and density of skyrmions, are precisely controlled by modulating parameters during the manipulation. The critical roles of in-plane magnetic fields and Dzyaloshinskii-Moriya interaction in STA generation is further confirmed by micromagnetic simulation. Our findings develop a strategy for engineering large-area and highly-oriented skyrmion configurations, offering a new pathway for the future application of next-generation spintronic and information technologies.

cond-mat.mtrl-sci

Spin-mediated hysteretic switching of unidirectional charge density waves by rotating magnetic fields

Charge density waves (CDWs) are a widespread collective electronic order in quantum materials, furnishing key insights into symmetry breaking and competing phases. However, their dynamic control with external fields remains a pivotal challenge. Here, we report deterministic and hysteretic switching of unidirectional CDW orientation via in-plane magnetic field rotation in magnetic kagome metal GdTi3Bi4. Atomically resolved spectroscopy shows two types of 3a0*1a0 CDW domains, Q1 and Q2 oriented 60 degree apart along two distinct crystallographic directions and separated by atomically sharp domain walls. Rotating the magnetic field drives reversible transitions between these CDW configurations, exhibiting a robust C2-symmetric phase diagram with pronounced hysteresis. This hysteretic switching is mediated by a field-dependent reorientation of underlying antiferromagnetic spins, revealing a tunable energy landscape with stable and metastable states and modulates the electronic charge order via spin-lattice coupling. Our findings not only demonstrate the switching of CDW configurations by in-plane magnetic field but also reveal the mechanism of coupling between CDW and magnetic fields, offering new insights into CDW manipulation and versatile platform for developing a spin-mediated multistate spin-charge coupling memory and programmable quantum devices.

cond-mat.str-el

Tunable bifurcation of magnetic anisotropy and bi-oriented antiferromagnetic order in kagome metal GdTi3Bi4

The novel kagome family RTi3Bi4 (R: rare-earth) offers a unique platform for exploring distinctive physical phenomena such as anisotropy, spin density wave, and anomalous Hall effect. In particular, the magnetic frustration and behavior of magnetic anisotropy in antiferromagnetic (AFM) kagome materials are of great interest for the fundamental studies and hold promise for next-generation device applications. Here, we report a tunable bifurcation of magnetic anisotropic and bi-oriented AFM order observed in the quasi-1D kagome antiferromagnet GdTi3Bi4. The magnetic domain evolutions during two plateau transition processes are directly visualized, unveiling a pronounced in-plane anisotropy along the a-axis. Temperature-dependent characterization reveals a bifurcation transition of anisotropy at approximately 2 K, where the a-axis anisotropy splits into two special orientations, revealing a hidden bi-oriented in-plane AFM order deviating from the high-symmetry direction by 7 degree. More intriguingly, the characteristics of the bifurcated anisotropy are clearly illustrated through vector magnetic field modulation, revealing three distinct in-plane domain phases in the transverse magnetic field phase diagram. Our results not only provide valuable insights into the tunable bifurcation of magnetic anisotropic in GdTi3Bi4, but also pave a novel pathway for AFM spintronics development.

cond-mat.str-el

Capacitive Touchscreens at Risk: Recovering Handwritten Trajectory on Smartphone via Electromagnetic Emanations

This paper reveals and exploits a critical security vulnerability: the electromagnetic (EM) side channel of capacitive touchscreens leaks sufficient information to recover fine-grained, continuous handwriting trajectories. We present Touchscreen Electromagnetic Side-channel Leakage Attack (TESLA), a non-contact attack framework that captures EM signals generated during on-screen writing and regresses them into two-dimensional (2D) handwriting trajectories in real time. Extensive evaluations across a variety of commercial off-the-shelf (COTS) smartphones show that TESLA achieves 77% character recognition accuracy and a Jaccard index of 0.74, demonstrating its capability to recover highly recognizable motion trajectories that closely resemble the original handwriting under realistic attack conditions.

cs.CR

Unveiling the delicate "hidden" interface conditions in WS2 flakes by advanced atomic force microscopy

The delicate interfacial conditions and behaviors play critical roles in determining the valuable physical properties of two-dimensional materials and their heterostructures on substrates. However, directly probing these complex interface conditions remains challenging. Here, we reveal the coupled in-plane strain and out-of-plane bonding conditions in strain-engineered WS2 flakes by combining dual-harmonic electrostatic force microscopy (DH-EFM) and scanning microwave impedance microscopy (sMIM). A striking contradiction is observed between the compressive-strain-induced larger bandgap (lower electrical conductivity) detected by DH-EFM, and the enhanced conductivity probed by sMIM. Comparative measurements under different sMIM modes demonstrate that this contradiction originates from a tip-loading-force-induced dynamic puckering effect, which is governed by the interfacial bonding strength. Furthermore, the progressive accumulation and subsequent release of conductivity during forward/backward sMIM-contact scans further confirms this dynamic puckering behavior, revealing pronounced differences in interface conditions between the open- and closed-ring regions of WS2. This work resolves the correlation between electrical properties and interface conditions, and provides fundamental insights for interface-engineered devices.

cond-mat.mtrl-sci

AdaReTaKe: Adaptive Redundancy Reduction to Perceive Longer for Video-language Understanding

Multimodal Large Language Models (MLLMs) have revolutionized video understanding, yet are still limited by context length when processing long videos. Recent methods compress videos by leveraging visual redundancy uniformly, yielding promising results. Nevertheless, our quantitative analysis shows that redundancy varies significantly across time and model layers, necessitating a more flexible compression strategy. We propose AdaReTaKe, a training-free method that flexibly reduces visual redundancy by allocating compression ratios among time and layers with theoretical guarantees. Integrated into state-of-the-art MLLMs, AdaReTaKe improves processing capacity from 256 to 2048 frames while preserving critical information. Experiments on VideoMME, MLVU, LongVideoBench, and LVBench datasets demonstrate that AdaReTaKe outperforms existing methods by 2.3% and 2.8% for 7B and 72B models, respectively, with even greater improvements of 5.9% and 6.0% on the longest LVBench. Our code is available at https://github.com/SCZwangxiao/video-FlexReduc.git.

cs.CV

Tailoring composite skyrmionic spin textures in an above-room-temperature ferromagnet Fe3-xGaTe2

Realizing room-temperature tunable skyrmionic objects in van der Waals ferromagnet offers unparalleled prospects for future spintronics. Here, we report an experimental investigation on the emergence and evolution of skyrmionic spin textures in the non-stoichiometric Fe3-xGaTe2 using magnetic force microscopy. The iron-deficiency-specific magnetic states of stripe, striped skyrmionium and striped skyrmion sack are observed. Through zero-field-cooling and field-cooling measurements, we observed distinct topological transitions and trivial transitions (distinguished by changes in topological charge) emerging during the stepwise evolution of topological spin textures, which enabled us to develop an evolution pathway model. Leveraging this model, the room-temperature stable composite topological spin textures of skyrmionium, skyrmion bag and sack states are further controllably realized via the exclusive topological-transition path (regulated by magnetic field and DMI intensity). Our work provides valuable insights into the room-temperature realization of topological spin textures in Fe3-xGaTe2, and inspires further exploration of their potential applications in heterostructure spintronics.

cond-mat.mtrl-sci

ReTaKe: Reducing Temporal and Knowledge Redundancy for Long Video Understanding

Video Large Language Models (VideoLLMs) have made significant strides in video understanding but struggle with long videos due to the limitations of their backbone LLMs. Existing solutions rely on length extrapolation, which is memory-constrained, or visual token compression, which primarily leverages low-level temporal redundancy while overlooking the more effective high-level knowledge redundancy. To address this, we propose $\textbf{ReTaKe}$, a training-free method with two novel modules DPSelect and PivotKV, to jointly reduce both temporal visual redundancy and knowledge redundancy for video compression. To align with the way of human temporal perception, DPSelect identifies keyframes based on inter-frame distance peaks. To leverage LLMs' learned prior knowledge, PivotKV marks the keyframes as pivots and compress non-pivot frames by pruning low-attention tokens in their KV cache. ReTaKe enables VideoLLMs to process 8 times longer frames (up to 2048), outperforming similar-sized models by 3-5% and even rivaling much larger ones on VideoMME, MLVU, LongVideoBench, and LVBench. Moreover, by overlapping compression operations with prefilling, ReTaKe introduces only ~10% prefilling latency overhead while reducing decoding latency by ~20%. Our code is available at https://github.com/SCZwangxiao/video-ReTaKe.

cs.CV

Discovery of unconventional charge-spin-intertwined density wave in magnetic kagome metal GdTi3Bi4

The symmetry breaking and its interplay among spin, charge, and lattice degrees of freedom is crucial for understanding correlated quantum states such as charge density waves (CDWs) and unconventional superconductivity. Here, we report the discovery by low-temperature scanning tunneling microscopy/spectroscopy of unconventional charge-spin-intertwined density waves in magnetic kagome metal GdTi3Bi4, which exhibits the one-third magnetization plateau. We reveal the emergence of 3Q CDWs incommensurate with the crystalline lattice in both periodicity and orientation, breaking all mirror and rotation symmetries. The CDW exhibits incommensurate-commensurate transitions in an applied magnetic field and transitions between 3Q and 1Q CDWs as a function of field and temperature, accompanied by changes in the spatial symmetries. Remarkably, the quantum and classic melting of the CDWs exhibits a phase structure which is consistent with the magnetization phase diagram of bulk GdTi3Bi4, providing strong evidence for the intertwined charge-spin density wave order. The origin of the charge-spin intertwinement is further evidenced by the observed hybridization between itinerant electrons and Gd local moments. Our findings uncover an unconventional form of charge-spin orders and offer new insights into a broad class of multi-components density wave formation in kagome and other correlated quantum materials.

cond-mat.str-el

Electrothermal manipulation of current-induced phase transitions in ferrimagnetic Mn$_3$Si$_2$Te$_6$

Phase transitions driven by external stimuli are central to condensed matter physics, providing critical insights into symmetry breaking and emergent phenomena. Recently, ferrimagnetic (FiM) Mn$_3$Si$_2$Te$_6$ has attracted considerable attention for its magnetic-field-induced insulator-metal transitions (IMTs) and unconventional current-driven phase transitions, yet the role of applied currents in the magnetic phase remains poorly understood. Here, by combining local magnetization probes and time-resolved transport measurements, we uncover an electrothermal origin for the current-induced first-order-like phase transitions, characterized by abrupt voltage jumps and distinct magnetic domain evolution. Current-voltage (I-V) characteristics measured under triangular waveforms exhibit strong non-reciprocal and hysteretic behaviors, which are significantly suppressed at frequencies ~1000 Hz. Time-resolved studies using rectangular pulsed currents demonstrate that the resistance dynamics closely mirror the equilibrium resistance-temperature profile, directly implicating Joule heating as the driving mechanism. Furthermore, we reveal that the intrinsic I-V response adheres to Ohm's law, displaying linearity across various magnetic fields and temperatures. Our work advocates for a cautious approach in distinguishing between genuine current-induced nonequilibrium quantum states and thermal effects.

cond-mat.mtrl-sci

Site-ordering/disordering-induced magnetic textures in a vdW ferromagnet by competing global and broken inversion-symmetry

Fe5GeTe2 single crystals can be divided into nonquenched (NQ) and quench-cooled (QC) phases with different magnetic properties. A comprehensive understanding of the magnetic property variations in the NQ and QC phases is imperative for guiding Fe5GeTe2 towards spintronics applications; however, it remains elusive. Here, we report a real-space study on the structural and magnetic properties of these two magnetic phases using cryogenic magnetic force microscopy and scanning tunneling microscopy. The thermal history introduces disorder and order to the Fe(1) sites, resulting in the NQ and QC phases exhibiting global and broken inversion symmetry, respectively. The observed magnetic domain transitions (branching to labyrinthine) in the spin reorientation process and the distinct 3D spin textures stabilized by magnetic dipolar interaction observed in field-dependent studies allow the NQ phase to exhibit a more resilient global magnetic state. In contrast, the QC phase exhibits enhanced magnetic anisotropy, resulting in a higher TC. Meanwhile, the Dzyaloshinskii-Moriya interaction (DMI) introduced by the broken inversion symmetry causes the QC phase to exhibit a localized magnetic state: no domain transformation occurs during spin reorientation, and irregular domain states are observed in field-related studies. Our work provides an important reference for understanding the complex magnetic properties in Fe5GeTe2.

cond-mat.mtrl-sci

Discovery and construction of surface kagome electronic states induced by p-d electronic hybridization

Kagome-lattice materials possess attractive properties for quantum computing applications, but their synthesis remains challenging. Herein, we show surface kagome electronic states (SKESs) on a Sn-terminated triangular Co3Sn2S2 surface, which are imprinted by vertical p-d electronic hybridization between the surface Sn (subsurface S) atoms and the buried Co kagome lattice network in the Co3Sn layer under the surface. Owing to the subsequent lateral hybridization of the Sn and S atoms in a corner-sharing manner, the kagome symmetry and topological electronic properties of the Co3Sn layer is proximate to the Sn surface. The SKESs and both hybridizations were verified via qPlus non-contact atomic force microscopy (nc-AFM) and density functional theory calculations. The construction of SKESs with tunable properties can be achieved by the atomic substitution of surface Sn (subsurface S) with other group III-V elements (Se or Te), which was demonstrated theoretically. This work exhibits the powerful capacity of nc-AFM in characterizing localized topological states and reveals the strategy for synthesis of large-area transition-metal-based kagome lattice materials using conventional surface deposition techniques.

cond-mat.mtrl-sci

Dynamic wavefront transformer based on a two-degree-of-freedom control system for 6-kHz mechanically actuated beam steering

Vast tunable optical components are realized based on dynamic reconfigurations of the incident wavefronts, such as beam steering and tunable lens. However, the dominant paradigm of current wavefront reconfiguration technologies relies on complex control systems with degrees of freedom much larger than output wavefronts, e.g. beam steering based on spatial light modulator or phased array antennas. Here, we propose a new paradigm for dynamic reconfiguration of arbitrary output wavefronts using control systems with the same degrees of freedom. As an example, a wavefront transformer is demonstrated using an in-plane two-degree-of-freedom (2DOF) mechanical actuation system of metasurface doublet for semi-omnidirectional beam steering, which measured a 6-kHz modulation speed and a "+-65.6 degree" field of view. This paradigm can be applied to metasurface transformers for dynamic wavefront reconfiguration with any control system for vast applications, such as tunable lens, beam steering, and dynamic beam profiler, just to name a few.

physics.optics

Two distinct superconducting states controlled by orientation of local wrinkles in LiFeAs

We observe two types of superconducting states controlled by orientations of local wrinkles on the surface of LiFeAs. Using scanning tunneling microscopy/spectroscopy, we find type-I wrinkles enlarge the superconducting gaps and enhance the transition temperature, whereas type-II wrinkles significantly suppress the superconducting gaps. The vortices on wrinkles show a C2 symmetry, indicating the strain effects on the wrinkles. A discontinuous switch of superconductivity occurs at the border between two different wrinkles. Our results demonstrate that the local strain effect could affect superconducting order parameter of LiFeAs with a possible Lifshitz transition, by alternating crystal structure in different directions.

cond-mat.supr-con

Tunable vortex Majorana zero modes in LiFeAs superconductor

The recent realization of pristine Majorana zero modes (MZMs) in vortices of iron-based superconductors (FeSCs) provides a promising platform for long-sought-after fault-tolerant quantum computation. A large topological gap between the MZMs and the lowest excitations enabled detailed characterization of vortex MZMs in those materials. Despite those achievements, a practical implementation of topological quantum computation based on MZM braiding remains elusive in this new Majorana platform. Among the most pressing issues are the lack of controllable tuning methods for vortex MZMs and inhomogeneity of the FeSC Majorana compounds that destroys MZMs during the braiding process. Thus, the realization of tunable vortex MZMs in a truly homogeneous compound of stoichiometric composition and with a charge neutral cleavage surface is highly desirable. Here we demonstrate experimentally that the stoichiometric superconductor LiFeAs is a good candidate to overcome these two obstacles. Using scanning tunneling microscopy, we discover that the MZMs, which are absent on the natural surface, can appear in vortices influenced by native impurities. Our detailed analysis and model calculations clarify the mechanism of emergence of MZMs in this material, paving a way towards MZMs tunable by controllable methods such as electrostatic gating. The tunability of MZMs in this homogeneous material offers an unprecedented platform to manipulate and braid MZMs, the essential ingredients for topological quantum computation.

cond-mat.supr-con