arXiv subjects

Shuyuan Shi

Publications and source records attributed to Shuyuan Shi.

14 recordsLinked to original sources

arXiv2025

Nonreciprocal spin-charge interconversion in topological insulator/ferromagnet heterostructures

The process of spin-charge interconversion is critical in modern spintronics. Nonetheless, experiments conducted on a wide variety of magnetic heterostructures consistently report that charge-to-spin and spin-to-charge conversion efficiencies can be vastly different, especially in the case of topological insulators (TI). This discrepancy between the two "reciprocal" effects remains unexplained, hampering the development of spin devices based on spin-charge conversion. In this study, we investigate both spin-charge and charge-spin interconversion processes in TI Bi2Te3/Py and Pt/Py bilayers experimentally using spin-torque ferromagnetic resonance and spin pumping techniques. We find that the measured charge-to-spin conversion efficiency (C-S) in TI/Py is ~26 times larger than the measured spin-to-charge conversion efficiency (S-C), whereas C-S and S-C are comparable in the case of Pt/Py. Using a theoretical model enforcing Onsager reciprocity, we show that spin-to-charge and charge-to-spin conversions in bilayers are genuinely inequivalent, and explain our results as arising from the distinct spin current leakage that takes place during the interconversion. This work clarifies previous conflicting reports on spin-charge interconversion processes and highlights the potential of interface engineering to achieve efficient spin transport in TI-based ferromagnetic heterostructures, paving the way for highly efficient spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Investigation of Sub-configurations Reveals Stable Spin-Orbit Torque Switching Polarity in Polycrystalline Mn3Sn

Previous studies have demonstrated the switching of octupole moment in Mn3Sn driven by spin-orbit torque (SOT). However, they have not accounted for the polycrystalline nature of the sample when explaining the switching mechanism. In this work, we use samples with various atomic orientations to capture this polycrystalline nature. We thoroughly investigate their SOT-induced spin dynamics and demonstrate that the polycrystalline structure leads to distinct outcomes. Our findings reveal that configuration II, where the Kagome plane is perpendicular to the spin polarization, exhibits robust switching with stable polarity, whereas the signals from various sub-configurations in configuration I cancel each other out. By comparing our findings with experimental results, we pinpoint the primary sources contributing to the measured AHE signals. Additionally, we establish a dynamic balance model that incorporates the unique properties of Mn3Sn to elucidate these observations. Our study highlights the essential role of the polycrystalline nature in understanding SOT switching. By clarifying the underlying physical mechanisms, our work resolves the longstanding puzzle regarding the robust SOT switching observed in Mn3Sn.

cond-mat.mes-hall↗

arXiv2024

Spin current leakage and Onsager reciprocity in interfacial spin-charge interconversion

Experimental investigations of spin-charge interconversion in magnetic bilayers comprising a ferromagnet adjacent to a topological insulator have reported scattered results on the spin-charge and charge-spin conversion efficiency. Attempting to reconcile these contradicting experimental results, we develop a phenomenological theory of spin-charge interconversion accounting for both interfacial interconversion through the spin galvanic effect, also called the Rashba-Edelstein effect, as well as bulk interconversion via the spin Hall effect. We find that the spin current leakage into the nonmagnetic metal plays a central role during the spin-to-charge and charge-to-spin conversion, leading to dissymmetric interconversion processes. In particular, spin-to-charge conversion is much less sensitive to the spin current absorption in the nonmagnetic metal than charge-to-spin conversion. This suggests that spin pumping is a more trustable technique to extract the interfacial Rashba parameter than spin-orbit torque.

cond-mat.mes-hall↗

arXiv2023

Deterministic Spin-Orbit Torque Switching of Mn3Sn with the Interplay between Spin Polarization and Kagome Plane

Previous studies have demonstrated spin-orbit torque (SOT) switching of Mn3Sn where the spin polarization lies in the kagome plane (configuration I). However, the critical current density ($ J_{crit}$) is unrealistically large ($ J_{crit}$=$ 10^{14}$ A/$ m^2$) and independent on the external field ($ H_{ext}$). The stabilized magnetic state also depends on the initial state. These features conflict with the ferromagnet (FM) switching scheme as claimed in those studies, and thus call for other explanations. Alternatively, the system with the spin polarization perpendicular to the kagome plane (configuration II) is more like the FM based system since the spin polarization is orthogonal to all magnetic moments. In this work, we show SOT switching of Mn3Sn in configuration II. Similar to the FM, Jcrit and Hext are in the order of $ 10^{10}$ A/$ m^2$ and hundreds of Oersted, respectively. The switching result is also independent of the initial state. Interestingly, the unique spin structure of Mn3Sn also leads to distinct features from FM systems. We demonstrate that Jcrit increases linearly with Hext, and extrapolation gives ultralow $ J_{crit}$ for the field-free switching system. In addition, the switching polarity is opposite to the FM. We also provide the switching phase diagram as a guideline for experimental demonstration. Our work provides comprehensive understanding for the switching mechanism in both configurations. The switching protocol proposed in this work is more advantageous in realistic spintronic applications. We also clearly reveal the fundamental difference between FM and noncollinear antiferromagnetic switching.

cond-mat.mes-hall↗

arXiv2023

Efficient domain wall motion driven by the out-of-plane spin polarization

Fast domain wall motion in systems with perpendicular magnetization is necessary for many novel applications such as the racetrack memory, domain wall logic devices and artificial synapses. The domain wall speed has been greatly improved after the demonstration of current driven domain wall motion using the spin transfer torque, and later achieved another leap due to the combined effect of spin-Hall effect and Dzyaloshinskii-Moriya interaction (DMI). However, only Neel wall can be effectively driven in the latter system. In this paper, we show that both Bloch and Neel domain walls can be effectively moved by exploiting the field-like torque with the out-of-plane spin polarization, which can be generated in materials with reduced symmetry. In addition, we find that the Neel wall and Bloch walls stabilized by the magnetostatic energy are easily distorted by the spin-orbit torque and they then enter the Walker breakdown region. External magnetic field and DMI are introduced to stabilize the domain wall, and a very high domain wall velocity over 500 m/s is obtained at a moderate current density of $2\times 10^{11} A/m^2$. In principle, this mechanism can be used to drive any types of domain walls. This work thus provides new degrees of freedom in the control of domain wall motion.

cond-mat.mes-hall↗

arXiv2022

Field-free spin-orbit torque switching of an antiferromagnet with perpendicular Néel vector

The field-free spin-orbit torque induced 180° reorientation of perpendicular magnetization is beneficial for the high performance magnetic memory. The antiferromagnetic material (AFM) can provide higher operation speed than the ferromagnetic counterpart. In this paper, we propose a trilayer AFM/Insulator/Heavy Metal structure as the AFM memory device. We show that the field-free switching of the AFM with perpendicular Néel vector can be achieved by using two orthogonal currents, which provide the uniform damping-like torque and stagger field-like torque, respectively. The reversible switching can be obtained by reversing either current. A current density of 1.79 10^11A/m^2 is sufficient to induce the switching. In addition, the two magnetic moments become noncollinear during the switching. This enables an ultrafast switching within 40 picoseconds. The device and switching mechanism proposed in this work offer a promising approach to deterministically switch the AFM with perpendicular Néel vector. It can also stimulate the development of ultrafast AFM-based MRAM.

cond-mat.mes-hall↗

arXiv2021

Room temperature energy-efficient spin-orbit torque switching in wafer-scale all-vdW heterostructure

The emergent two-dimensional (2D) ferromagnetic materials with unique magnetic properties have endowed great potential for next-generation spintronic devices with extraordinary merits of high flexibility, easy controllability, and high heretointegrability, which is expected to promote the development of Moore's Law continuously. However, it is extremely challenging to realize magnetic switching with ultra-low power consumption at room temperature. Here, we demonstrate the room-temperature spin-orbit torque (SOT) driven magnetization switching in a well-epitaxial all-van der Waals (vdW) heterostructure. The topological insulator Bi2Te3 not only helps to elevate the Curie temperature of Fe3GeTe2 (FGT) through interfacial exchange coupling but also works as a spin current source allowing to switch FGT at a low current density of 2.2 * 106 A cm2. A large SOT efficiency of 0.7 is measured at room temperature, and the thickness of FGT is further adjusted to reduce the influence of the thermal contribution on the second-harmonic signal. Furthermore, the temperature and thickness-dependent SOT efficiency prove that the large SOT in our system mainly originates from the nontrivial origin of topological materials. Our experiment has enabled an all-vdW SOT structure and lays a solid foundation for the implementation of room-temperature all-vdW spintronic devices in the future.

physics.app-ph↗

arXiv2021

Observation of the out-of-plane polarized spin current from CVD grown WTe2

Weyl semimetal Td-phase WTe2 possesses the spin-resolved band structure with strong spin-orbit coupling, holding promises as a useful spin source material. The noncentrosymmetric crystalline structure of Td-WTe2 endows the generation of the out-of-plane polarized spin, which is of great interest in magnetic memory applications. Previously, WTe2 was explored in spin devices based on mechanically exfoliated single crystal flakes with a size of micrometers. For practical spintronics applications, it is highly desirable to implement wafer-scale thin films. In this work, we utilize centimeter-scale chemical vapor deposition (CVD)-grown Td-WTe2 thin films and study the spin current generation by the spin torque ferromagnetic resonance technique. We find the in-plane and out-of-plane spin conductivities of 7.36 x 10^3 (h/2e) (ohm-m)^-1 and 1.76 x 10^3 (h/2e) (ohm-m)^-1, respectively, in CVD-growth 5 nm-WTe2. We further demonstrate the current-induced magnetization switching in WTe2/NiFe at room temperature in the domain wall motion regime, which may invigorate potential spintronic device innovations based on Weyl semimetals.

cond-mat.mtrl-sci↗

arXiv2020

Spin-orbit torque magnetization switching in MoTe2/permalloy heterostructures

The ability to switch magnetic elements by spin-orbit-induced torques has recently attracted much attention for a path towards high-performance, non-volatile memories with low power consumption. Realizing efficient spin-orbit-based switching requires harnessing both new materials and novel physics to obtain high charge-to-spin conversion efficiencies, thus making the choice of spin source crucial. Here we report the observation of spin-orbit torque switching in bilayers consisting of a semimetallic film of 1T'-MoTe2 adjacent to permalloy. Deterministic switching is achieved without external magnetic fields at room temperature, and the switching occurs with currents one order of magnitude smaller than those typical in devices using the best-performing heavy metals. The thickness dependence can be understood if the interfacial spin-orbit contribution is considered in addition to the bulk spin Hall effect. Further threefold reduction in the switching current is demonstrated with resort to dumbbell-shaped magnetic elements. These findings foretell exciting prospects of using MoTe2 for low-power semimetal material based spin devices.

cond-mat.mtrl-sci↗

arXiv2019

Nonlinear planar Hall effect

An intriguing property of three-dimensional (3D) topological insulator (TI) is the existence of surface states with spin-momentum locking, which offers a new frontier of exploration in spintronics. Here, we report the observation of a new type of Hall effect in a 3D TI Bi2Se3 film. The Hall resistance scales linearly with both the applied electric and magnetic fields and exhibits a π/2 angle offset with respect to its longitudinal counterpart, in contrast to the usual angle offset of π/4 between the linear planar Hall effect and the anisotropic magnetoresistance. This novel nonlinear planar Hall effect originates from the conversion of a nonlinear transverse spin current to a charge current due to the concerted actions of spin-momentum locking and time reversal symmetry breaking, which also exists in a wide class of non-centrosymmetric materials with a large span of magnitude. It provides a new way to characterize and utilize the nonlinear spin-to-charge conversion in a variety of topological quantum materials.

cond-mat.mes-hall↗

arXiv2019

Nonlinear magnetotransport shaped by Fermi surface topology and convexity in WTe2

The nature of Fermi surface defines the physical properties of conductors and many physical phenomena can be traced to its shape. Although the recent discovery of a current-dependent nonlinear magnetoresistance in spin-polarized non-magnetic materials has attracted considerable attention in spintronics, correlations between this phenomenon and the underlying fermiology remain unexplored. Here, we report the observation of nonlinear magnetoresistance at room temperature in a semimetal WTe2, with an interesting temperature-driven inversion. Theoretical calculations reproduce the nonlinear transport measurements and allow us to attribute the inversion to temperature-induced changes in Fermi surface convexity. We also report a large anisotropy of nonlinear magnetoresistance in WTe2, due to its low symmetry of Fermi surfaces. The good agreement between experiments and theoretical modeling reveals the critical role of Fermi surface topology and convexity on the nonlinear magneto-response. These results lay a new path to explore ramifications of distinct fermiology for nonlinear transport in condensed-matter.

cond-mat.mtrl-sci↗

arXiv2018

Long spin coherence length and bulk-like spin-orbit torque in ferrimagnetic multilayers

Ferromagnetic spintronics has been a main focus as it offers non-volatile memory and logic applications through current-induced spin-transfer torques. Enabling wider applications of such magnetic devices requires a lower switching current for a smaller cell while keeping the thermal stability of magnetic cells for non-volatility. As the cell size reduces, however, it becomes extremely difficult to meet this requirement with ferromagnets because spin-transfer torque for ferromagnets is a surface torque due to rapid spin dephasing, leading to the 1/ferromagnet-thickness dependence of the spin-torque efficiency. Requirement of a larger switching current for a thicker and thus more thermally stable ferromagnetic cell is the fundamental obstacle for high-density non-volatile applications with ferromagnets. Theories predicted that antiferromagnets have a long spin coherence length due to the staggered spin order on an atomic scale, thereby resolving the above fundamental limitation. Despite several spin-torque experiments on antiferromagnets and ferrimagnetic alloys, this prediction has remained unexplored. Here we report a long spin coherence length and associated bulk-like-torque characteristic in an antiferromagnetically coupled ferrimagnetic multilayer. We find that a transverse spin current can pass through > 10 nm-thick ferrimagnetic Co/Tb multilayers whereas it is entirely absorbed by 1 nm-thick ferromagnetic Co/Ni multilayer. We also find that the switching efficiency of Co/Tb multilayers partially reflects a bulk-like-torque characteristic as it increases with the ferrimagnet-thickness up to 8 nm and then decreases, in clear contrast to 1/thickness-dependence of Co/Ni multilayers. Our results on antiferromagnetically coupled systems will invigorate researches towards energy-efficient spintronic technologies.

cond-mat.mtrl-sci↗

arXiv2018

Efficient Charge-Spin Conversion and Magnetization Switching though Rashba Effect at Topological Insulator/Ag Interface

We report the observation of efficient charge-to-spin conversion in the three-dimensional topological insulator (TI) Bi2Se3 and Ag bilayer by the spin-torque ferromagnetic resonance technique. The spin orbit torque ratio in the Bi2Se3/Ag/CoFeB heterostructure shows a significant enhancement as the Ag thickness increases to ~2 nm and reaches a value of 0.5 for 5 nm Ag, which is ~3 times higher than that of Bi2Se3/CoFeB at room temperature. The observation reveals the interfacial effect of Bi2Se3/Ag exceeds that of the topological surface states (TSS) in the Bi2Se3 layer and plays a dominant role in the charge-to-spin conversion in the Bi2Se3/Ag/CoFeB system. Based on the first-principles calculations, we attribute our observation to the large Rashba-splitting bands which wrap the TSS band and has the same net spin polarization direction as TSS of Bi2Se3. Subsequently, we demonstrate for the first time the Rashba induced magnetization switching in Bi2Se3/Ag/Py with a low current density of 5.8 X 10^5 A/cm2.

cond-mat.mtrl-sci↗

arXiv2017

Room temperature magnetization switching in topological insulator-ferromagnet heterostructures by spin-orbit torques

Topological insulators (TIs) with spin momentum locked topological surface states (TSS) are expected to exhibit a giant spin-orbit torque (SOT) in the TI/ferromagnet systems. To date, the TI SOT driven magnetization switching is solely reported in a Cr doped TI at 1.9 K. Here, we directly show giant SOT driven magnetization switching in a Bi2Se3/NiFe heterostructure at room temperature captured using a magneto-optic Kerr effect microscope. We identify a large charge to spin conversion efficiency of ~1-1.75 in the thin TI films, where the TSS is dominant. In addition, we find the current density required for the magnetization switching is extremely low, ~6x10^5 A cm-2, which is one to two orders of magnitude smaller than that with heavy metals. Our demonstration of room temperature magnetization switching of a conventional 3d ferromagnet using Bi2Se3 may lead to potential innovations in TI based spintronic applications.

cond-mat.mtrl-sci↗