arXiv subjects

Sophie A. Morley

Publications and source records attributed to Sophie A. Morley.

10 recordsLinked to original sources

arXiv2026

Lightfall: An API-first, LLM-addressable control platform for synchrotron beamlines

Synchrotron beamlines differ in hardware, technique, and workflow, making customized control interfaces necessary; bespoke per-beamline graphical user interfaces (GUIs) do not scale well, one-size-fits-all facility software forces compromises that leave most of the interface unused, and even recent component-library approaches keep per-scientist tweaks on a developer's queue. We present Lightfall, a control platform designed for facility-wide use, whose API-first architecture exposes every panel, device, and scan plan through a single uniform addressable interface. An embedded language-model agent drives experiments through that interface, from a single move-and-read to a Gaussian-process-driven autonomous scan, while beamline staff extend the interface during operation via skills: plugin modules the agent invokes to compose and modify panels in the running application. The result is a closed development loop: a beamline scientist authors a panel change in natural language, the agent emits and applies it, and the commit lands in the beamline's plugin repository as a side effect. The per-iteration cost of a scientist-driven change is then fixed in the scientist's own time rather than in developer hours the facility must supply. Lightfall is in testing at the COSMIC-Scattering beamline at the Advanced Light Source.

physics.ins-det↗

arXiv2026

Beyond conventional skyrmions in synthetic antiferromagnets

Magnetic skyrmions are topologically protected spin textures that can act as reconfigurable nanoscale information carriers. In synthetic antiferromagnets (SAFs), interlayer exchange coupling offers an additional control parameter beyond the interfacial Dzyaloshinskii-Moriya interaction (DMI) and magnetic anisotropy. Here, we engineer a SAF composed of two chemically distinct ferromagnets (CoB and CoFeB), in which the external magnetic field and interlayer exchange act asymmetrically on the sublattices. The competition of these effects, acting as a resultant effective-field, gives rise to two distinct skyrmion families in different field regimes. In large fields, conventional-polarity skyrmions nucleate, with core antiparallel to the external field, whereas in smaller fields an inverse-polarity skyrmion state emerges as the effective-field reverses sign and almost saturates the CoFeB layers. Return-point memory measurements confirm independent nucleation pathways for the two families. Using element-resolved x-ray magnetometry, correlative magnetic force and Lorentz transmission electron microscopies, and parameter-matched micromagnetic modelling, we show that all textures reside only in the CoFeB layers, which experience a Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange field originating from the CoB layers. This effective-field method provides a robust route to programmable three-dimensional spin textures with controlled polarity in selected layers of a multilayer with potential for applications in skyrmion-based computing and spin-logic architectures.

cond-mat.mes-hall↗

arXiv2026

Soft X-ray Reflection Ptychography

Scanning transmission X-ray microscopy and ptychography have become mature tools for high-resolution, element-specific imaging of nanoscale structures. However, transmission geometries impose stringent constraints on sample thickness and preparation, thereby limiting investigations of extended or bulk specimens, especially in the soft X-ray region. Here, we demonstrate reflection geometry soft X-ray ptychography as a robust imaging mode. Instrumental feasibility and spatial resolution are established using a lithographically defined Siemens star and barcode test pattern on a multilayer substrate. We empirically demonstrate a full-pitch spatial resolution of ca. 45 nm from Fourier ring correlation analysis of the reconstructed object. The results highlight the potential of the reflection geometry for nondestructive X-ray studies of materials without the need for transmissive samples.

physics.optics↗

arXiv2023

Antiferromagnetic real-space configuration probed by dichroism in scattered x-ray beams with orbital angular momentum

X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity--an azimuthally varying phase--which leads to a gradient of the light field. New material properties can be probed by utilizing the helicity of an OAM beam. Here, we demonstrate a novel dichroic effect in resonant diffraction from an artificial antiferromagnet with a topological defect. We found that the scattered OAM beam has circular dichroism at the antiferromagnetic Bragg peak whose sign is coupled to its helicity, which reveals the real-space configuration of the antiferromagnetic ground state. Thermal cycling of the artificial antiferromagnet can change the ground state, as indicated by reversal of the sign of circular dichroism. This result is one of the first demonstrations of a soft x-ray spectroscopy characterization technique utilizing the OAM of x-rays. This helicity-dependent circular dichroism exemplifies the potential to utilize OAM beams to probe matter in a way that is inaccessible using currently available x-ray techniques.

cond-mat.mtrl-sci↗

arXiv2020

Subterahertz spin pumping from an insulating antiferromagnet

Spin-transfer torque and spin Hall effects combined with their reciprocal phenomena, spin-pumping and inverse spin Hall (ISHE) effects, enable the reading and control of magnetic moments in spintronics. The direct observation of these effects remains elusive in antiferromagnetic-based devices. We report sub-terahertz spin-pumping at the interface of a uniaxial insulating antiferromagnet MnF2 and platinum. The measured ISHE voltage arising from spin-charge conversion in the platinum layer depends on the chirality of the dynamical modes of the antiferromagnet, which is selectively excited and modulated by the handedness of the circularly polarized sub-THz irradiation. Our results open the door to the controlled generation of coherent pure spin currents at THz frequencies.

cond-mat.mtrl-sci↗

arXiv2019

Heisenberg pseudo-exchange and emergent anisotropies in field-driven pinwheel artificial spin ice

Rotating all islands in square artificial spin ice (ASI) uniformly about their centres gives rise to the recently reported pinwheel ASI. At angles around 45$^\mathrm{o}$, the antiferromagnetic ordering changes to ferromagnetic and the magnetic configurations of the system exhibit near-degeneracy, making it particularly sensitive to small perturbations. We investigate through micromagnetic modelling the influence of dipolar fields produced by physically extended islands in field-driven magnetisation processes in pinwheel arrays, and compare the results to hysteresis experiments performed in-situ using Lorentz transmission electron microscopy. We find that magnetisation end-states induce a Heisenberg pseudo-exchange interaction that governs both the inter-island coupling and the resultant array reversal process. Symmetry reduction gives rise to anisotropies and array-corner mediated avalanche reversals through a cascade of nearest-neighbour (NN) islands. The symmetries of the anisotropy axes are related to those of the geometrical array but are misaligned to the array axes as a result of the correlated interactions between neighbouring islands. The NN dipolar coupling is reduced by decreasing the island size and, using this property, we track the transition from the strongly coupled regime towards the pure point dipole one and observe modification of the ferromagnetic array reversal process. Our results shed light on important aspects of the interactions in pinwheel ASI, and demonstrate a mechanism by which their properties may be tuned for use in a range of fundamental research and spintronic applications.

cond-mat.mes-hall↗

arXiv2018

Thermally and field-driven mobility of emergent magnetic charges in square artificial spin ice

Designing and constructing model systems that embody the statistical mechanics of frustration is now possible using nanotechnology. We have arranged nanomagnets on a two-dimensional square lattice to form an artificial spin ice, and studied its fractional excitations, emergent magnetic monopoles, and how they respond to a driving field using X-ray magnetic microscopy. We observe a regime in which the monopole drift velocity is linear in field above a critical field for the onset of motion. The temperature dependence of the critical field can be described by introducing an interaction term into the Bean-Livingston model of field-assisted barrier hopping. By analogy with electrical charge drift motion, we define and measure a monopole mobility that is larger both for higher temperatures and stronger interactions between nanomagnets. The mobility in this linear regime is described by a creep model of zero-dimensional charges moving within a network of quasi-one-dimensional objects.

cond-mat.mes-hall↗

arXiv2018

Superferromagnetism and domain-wall topologies in artificial 'pinwheel' spin ice

For over ten years, arrays of interacting single-domain nanomagnets, referred to as artificial spin ices, have been engineered with the aim to study frustration in model spin systems. Here, we use Fresnel imaging to study the reversal process in 'pinwheel' artificial spin ice, a modified square ASI structure obtained by rotating each island by some angle about its midpoint. Our results demonstrate that a simple 45° rotation changes the magnetic ordering from antiferromagnetic to ferromagnetic, creating a superferromagnet which exhibits mesoscopic domain growth mediated by domain wall nucleation and coherent domain propagation. We observe several domain-wall configurations, most of which are direct analogues to those seen in continuous ferromagnetic films. However, novel charged walls also appear due to the geometric constraints of the system. Changing the orientation of the external magnetic field allows control of the nature of the spin reversal with the emergence of either 1-D or 2-D avalanches. This unique property of pinwheel ASI could be employed to tune devices based on magnetotransport phenomena such as Hall circuits.

cond-mat.dis-nn↗

arXiv2017

Effect of FePd alloy composition on the dynamics of artificial spin ice

Artificial spin ices (ASI) are arrays of single domain nano-magnetic islands, arranged in geometries that give rise to frustrated magnetostatic interactions. It is possible to reach their ground state via thermal annealing. We have made square ASI using different FePd alloys to vary the magnetization via co-sputtering. From a polarized state the samples were incrementally heated and we measured the vertex population as a function of temperature using magnetic force microscopy. For the higher magnetization FePd sample, we report an onset of dynamics at $T = 493$ K, with a rapid collapse into $>90\%$ ground state vertices. In contrast, the low magnetization sample started to fluctuate at lower temperatures, $T = 393$ K and over a wider temperature range but only reached a maximum of $25\%$ of ground state vertices. These results indicate that the interaction strength, dynamic temperature range and pathways can be finely tuned using a simple co-sputtering process. In addition we have compared our experimental values of the blocking temperature to those predicted using the simple Néel-Brown two-state model and find a large discrepancy which we attribute to activation volumes much smaller than the island volume.

cond-mat.mes-hall↗

arXiv2017

Frustration and thermalisation in an artificial magnetic quasicrystal

We have created and studied artificial magnetic quasicrystals based on Penrose tiling patterns of interacting nanomagnets that lack the translational symmetry of spatially periodic artificial spin ices. Vertex-level degeneracy and frustration induced by the network topology of the Penrose pattern leads to a low energy configuration that we propose as a ground state. Topologically induced emergent frustration means that this ground state cannot be constructed from vertices in their ground states. It has two parts, a quasi-one-dimensional rigid "skeleton" that spans the entire pattern and is capable of long-range order, and "flippable" clusters of macrospins within it. These lead to macroscopic degeneracy for the array as a whole. Magnetic force microscopy imaging of Penrose tiling arrays revealed superdomains that are larger for more strongly coupled arrays. The superdomain size is larger after AC-demagnetisation and especially after annealing the array above its blocking temperature.

cond-mat.dis-nn↗