arXiv subjects

Sophie Bouchoule

Publications and source records attributed to Sophie Bouchoule.

15 recordsLinked to original sources

arXiv2026

Electrically-injected room-temperature waveguide polariton laser

Exciton-polariton lasers are coherent light sources which do not require the population inversion (transparency) condition to be fulfilled. They have been conceptualized at the end of the XXth century but until now they operate almost exclusively under optical injection, which severely limits the widespread integration of the polariton-based devices implemented so far. Here we tackle this issue by reporting an electrically-pumped exciton-polariton laser based on GaN and operating at room temperature in a mode-locked regime. The laser architecture is close to the geometry of commercial ridge-waveguide GaN lasers, but based on a bulk GaN active region instead of quantum wells. Unique features of polariton lasers are demonstrated, in particular the breakdown of the transparency condition, which enables our polariton lasers to operate even when only a small fraction (20\%) of the cavity length is injected. Moreover, the large polaritonic gain allows for the operation of a short cavity length (60$μm$) compared to commercial lasers. From the very same sample, we also achieve polariton lasing under optical injection, confirming that the doped layers necessary for electrical injection do not prevent strong-coupling nor polariton lasing. Our results open a new perspective for polariton-based devices.

physics.optics↗

arXiv2025

Time-resolved dynamics of GaN waveguide polaritons

We implement a new experimental approach to directly measure the lifetime of guided polaritons arising from the strong-coupling of GaN excitons and the guided photonic modes of a slab waveguide. Using a Fourier imaging setup, combined with spatial filtering of the emission, the emission associated to polaritonic modes with well-defined propagation constants can be selectively analyzed in the temporal domain. By directing it to the entrance slit of a streak camera, time-resolved photoluminescence (TRPL) measurements along the polariton dispersion branch were performed at 40 K, enabling to assess the time decay of polariton modes. By combining this information with the photonic/excitonic fraction corresponding to each polariton mode, extracted from a coupled-oscillators model that indicate a Rabi splitting of $Ω$ = 80 meV, we could extract the photon lifetime in the waveguide $τ_γ\, =\, 3\pm 1$ ps. This corresponds to a record $Q$-factor in the UV of 16 000. The excitonic reservoir lifetime, which contributes to polariton formation, was determined through TRPL measurements on excitonic luminescence. Finally, measurements conducted at lower temperature highlight secondary feeding mechanisms for the guided polaritonic mode, either via photon recycling from the AlGaN cladding layer or through resonant injection of photons from transitions below the band gap.

cond-mat.mtrl-sci↗

arXiv2025

On the importance of Ni-Au-Ga interdiffusion in the formation of a Ni-Au / p-GaN ohmic contact

The Ni-Au-Ga interdiffusion mechanisms taking place during rapid thermal annealing (RTA) under oxygen atmosphere of a Ni-Au/p-GaN contact are investigated by high-resolution transmission electron microscopy (HR-TEM) coupled to energy dispersive X-ray spectroscopy (EDX). It is shown that oxygen-assisted, Ni diffusion to the top surface of the metallic contact through the formation of a nickel oxide (NiOx) is accompanied by Au diffusion down to the GaN surface, and by Ga out-diffusion through the GaN/metal interface. Electrical characterizations of the contact by Transmission Line Method (TLM) show that an ohmic contact is obtained as soon as a thin, Au-Ga interfacial layer is formed, even after complete diffusion of Ni or NiOx to the top surface of the contact. Our results clarify that the presence of Ni or NiOx at the interface is not the main origin of the ohmic-like behavior in such contacts. Auto-cleaning of the interface during the interdiffusion process may play a role, but TEM-EDX analysis evidences that the creation of Ga vacancies associated to the formation of a Ga-Au interfacial layer is crucial for reducing the Schottky barrier height, and maximizing the amount of current flowing through the contact.

cond-mat.mtrl-sci↗

arXiv2023

Experimental demonstration of a Two-Dimensional Hole Gas (2DHG) in a GaN/AlGaN/GaN based heterostructure by optical spectroscopy

The polarization discontinuity across interfaces in polar nitride-based heterostructures can lead to the formation of two-dimensional electron and hole gases. In the past, the observation of these electron and hole gases has been achieved through various experimental techniques, most often by electronic measurements but occasionally by optical means. However, the occurrence of a two-dimensional hole gas has never been demonstrated optically. The objective of this article is to demonstrate, thanks to the combination of various optical spectroscopy techniques coupled to numerical simulations, the presence of a two-dimensional hole gas in a GaN/AlGaN/GaN heterostructure. This is made possible thanks to a GaN/AlGaN/GaN heterostructure displaying a micrometer-thick AlGaN layer and a GaN cap thicker than in conventional GaN-based HEMTs structures. The band structure across the whole heterostructure was established by solving self-consistently the Schrödinger and Poisson equations and by taking into account the experimentally determined strain state of each layer. Continuous and quasi-continuos photoluminescence reveal the presence of a broad emission band at an energy around 50 meV below the exciton emission and whose energy blueshifts with increasing excitation power density, until it is completely quenched due to the complete screening of the internal electric field. Time-resolved measurements show that the emission arising from the two-dimensional hole gas can be assigned to the recombination of holes in the potential well with electrons located in the top GaN as well as electron from the bottom AlGaN, each of them displaying different decay times due to unequal electric fields. Besides the optical demonstration of a two-dimensional hole gas in a nitride-based heterostructure, our work highlights the optical recombination processes involved in the emission from such a hole gas.

cond-mat.mtrl-sci↗

arXiv2023

Lasing in a ZnO waveguide: clear evidence of polaritonic gain obtained by monitoring the continuous exciton screening

The stimulated emission of exciton-polaritons was proposed as a means of lowering the lasing threshold because it does not require the dissociation of excitons to obtain an electron-hole plasma, as in a classical semiconductor laser based on population inversion. In this work we propose a method to prove unambiguously the polaritonic nature of lasing by combining experimental measurements with a model accounting for the permittivity change as a function of the carrier density. To do so we use angle resolved photoluminescence to observe the lasing at cryogenic temperature from a polariton mode in a zinc oxide waveguide structure, and to monitor the continuous shift of the polaritonic dispersion towards a photonic dispersion as the optical intensity of the pump is increased (up to 20 times the one at threshold). This shift is reproduced thanks to a model taking into account the reduction of the oscillator strength and the renormalization of the bandgap due to the screening of the electrostatic interaction between electrons and holes. Furthermore, the measurement of the carriers lifetime at optical intensities in the order of those at which the polariton lasing occurs enables us to estimate the carrier density, confirming it is lower than the corresponding Mott density for zinc oxide reported in the literature.

cond-mat.mtrl-sci↗

arXiv2020

The Excitation Ladder of Cavity Polaritons

Multidimensional coherent spectroscopy directly unravels multiply excited states that overlap in a linear spectrum. We report multidimensional coherent optical photocurrent spectroscopy in a semiconductor polariton diode and explore the excitation ladder of cavity polaritons. We measure doubly and triply avoided crossings for pairs and triplets of exciton-polaritons, demonstrating the strong coupling between light and dressed doublet and triplet semiconductor excitations. These results demonstrate that multiply excited excitonic states strongly coupled to a microcavity can be described as two coupled quantum-anharmonic ladders.

cond-mat.mes-hall↗

arXiv2018

Ultra-low noise dual-frequency VECSEL at telecom wavelength using fully correlated pumping

An ultra-low intensity and beatnote phase noise dual-frequency vertical-external-cavity surface-emitting laser is built at telecom wavelength. The pump laser is realized by polarization combining two single-mode fibered laser diodes in a single-mode fiber, leading to a 100 % in-phase correlation of the pump noises for the two modes. The relative intensity noise is lower than -140 dB/Hz, and the beatnote phase noise is suppressed by 30 dB, getting close to the spontaneous emission limit. The role of the imperfect cancellation of the thermal effect resulting from unbalanced pumping of the two modes in the residual phase noise is evidenced.

physics.optics↗

arXiv2016

Interplay between tightly focused excitation and ballistic propagation of polariton condensates in a ZnO microcavity

The formation and propagation of a polariton condensate under tightly focused excitation is investigated in a ZnO microcavity both experimentally and theoretically. 2D near-field and far-field images of the condensate are measured under quasi-continuous non-resonant excitation. The corresponding spatial profiles are compared to a model based on the Gross-Pitaevskii equation under cylindrical geometry. This work allows to connect the experiments performed with a small excitation laser spot and the previous kinetic models of condensation in a 2D infinite microcavity, and to determine the relevant parameters of both the interaction and the relaxation between the reservoir and the condensate. Two main parameters are identified: the exciton-photon detuning through the polariton effective mass and the temperature, which determines the efficiency of the relaxation from the reservoir to the condensate.

cond-mat.mes-hall↗

arXiv2015

Intensity and phase noise correlations in a dual-frequency VECSEL operating at telecom wavelength

The amplitude and phase noises of a dual-frequency vertical-external-cavity surface-emitting laser (DF-VECSEL) operating at telecom wavelength are theoretically and experimentally investigated in detail. In particular, the spectral behavior of the correlation between the intensity noises of the two modes of the DF-VECSEL is measured. Moreover, the correlation between the phase noise of the radio-frequency (RF) beatnote generated by optical mixing of the two laser modes with the intensity noises of the two modes is investigated. All these spectral behaviors of noise correlations are analyzed for two different values of the nonlinear coupling between the laser modes. We find that to describe the spectral behavior of noise correlations between the laser modes, it is of utmost importance to have a precise knowledge about the spectral behavior of the pump noise, which is the dominant source of noise in the frequency range of our interest (10 kHz to 35 MHz). Moreover, it is found that the noise correlation also depends on how the spatially separated laser modes of the DF-VECSEL intercept the noise from a multi-mode fiber-coupled laser diode used for pumping both the laser modes. To this aim, a specific experiment is reported, which aims at measuring the correlations between different spatial regions of the pump beam. The experimental results are in excellent agreement with a theoretical model based on modified rate equations.

physics.optics↗

arXiv2014

Quantum confinement of zero-dimensional hybrid organic-inorganic polaritons at room temperature

We report on the quantum confinement of zero-dimensional polaritons in perovskite-based microcavity at room temperature. Photoluminescence of discrete polaritonic states are observed for polariton localized in symmetric sphere-like defects which are spontaneously nucleated on the top dielectric Bragg mirror. The linewidth of these confined states are found much sharper (almost one order of magnitude) than that of photonic modes in the perovskite planar microcavity. Our results show the possibility to study organic-inorganic cavity polariton in confined microstructure and suggest a fabrication method to realize integrated polaritonic devices operating at room temperature.

cond-mat.mes-hall↗

arXiv2012

ZnO-Based Polariton Laser Operating at Room Temperature: From Excitonic to Photonic Condensate

A laser threshold is determined by the gain condition, which has been progressively reduced by the use of heterostructures and of quantum confinement. The polariton laser is the ultimate step of this evolution: coherent emission is obtained from the spontaneous decay of an exciton-polariton condensate, without the achievement of any gain condition. ZnO, with its unique excitonic properties, is the best choice for a blue/UV-emitting polariton laser device. We report on the fabrication of a new family of fully hybrid microcavities that combine the best-quality ZnO material available (bulk substrate) and two dielectric distributed Bragg reflectors, demonstrating large quality factors (>2500) and Rabi splittings (~200 meV). Low threshold polariton lasing is achieved between 4 and 300 K and for excitonic fractions ranging between 12% and 96 %. A phase diagram highlighting the role of LO phonon-assisted relaxation in this polar semiconductor is established, and a remarkable switching between polariton modes is demonstrated.

cond-mat.mtrl-sci↗

arXiv2011

Laser emission with excitonic gain in a ZnO planar microcavity

The lasing operation of a ZnO planar microcavity under optical pumping is demonstrated from T=80 K to 300 K. At the laser threshold, the cavity switches from the strong coupling to the weak coupling regime. A gain-related transition, which appears while still observing polariton branches and, thus, with stable excitons, is observed below 240K. This shows that exciton scattering processes, typical of II-VI semiconductors, are involved in the gain process.

physics.optics↗

arXiv2009

Relaxation and emission of Bragg-mode and cavity-mode polaritons in a ZnO microcavity at room temperature

The strong coupling regime in a ZnO microcavity is investigated through room temperature photoluminescence and reflectivity experiments. The simultaneous strong coupling of excitons to the cavity mode and the first Bragg mode is demonstrated at room temperature. The polariton relaxation is followed as a function of the excitation density. A relaxation bottleneck is evidenced in the Bragg-mode polariton branch. It is partly broken under strong excitation density, so that the emission from this branch dominates the one from cavity-mode polaritons.

cond-mat.other↗

arXiv2008

Optical bistability in a GaAs based polariton diode

We report on a new type of optical nonlinearity in a polariton p-i-n microcavity. Abrupt switching between the strong and weak coupling regime is induced by controlling the electric field within the cavity. As a consequence bistable cycles are observed for low optical powers (2-3 orders of magnitude less than for Kerr induced bistability). Signatures of switching fronts propagating through the whole 300 microns x 300 microns mesa surface are evidenced.

cond-mat.other↗

arXiv2007

Microcavity polariton light emitting diode

Cavity polaritons have been shown these last years to exhibit a rich variety of non-linear behaviors which could be used in new polariton based devices. Operation in the strong coupling regime under electrical injection remains a key step toward a practical polariton device. We report here on the realization of a polariton based light emitting diode using a GaAs microcavity with doped Bragg mirrors. Both photocurrent and electroluminescence spectra are governed by cavity polaritons up to 100 K.

cond-mat.mtrl-sci↗