arXiv · 2004.10845
The Excitation Ladder of Cavity Polaritons
Abstract
Multidimensional coherent spectroscopy directly unravels multiply excited states that overlap in a linear spectrum. We report multidimensional coherent optical photocurrent spectroscopy in a semiconductor polariton diode and explore the excitation ladder of cavity polaritons. We measure doubly and triply avoided crossings for pairs and triplets of exciton-polaritons, demonstrating the strong coupling between light and dressed doublet and triplet semiconductor excitations. These results demonstrate that multiply excited excitonic states strongly coupled to a microcavity can be described as two coupled quantum-anharmonic ladders.
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Travis M. Autry, Gaël Nardin, Christopher L. Smallwood, Kevin Silverman, Daniele Bajoni, Aristide Lemaître, Sophie Bouchoule, Jacqueline Bloch, Steven Cundiff. 2020-04-22. The Excitation Ladder of Cavity Polaritons. https://doi.org/10.1103/physrevlett.125.067403
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