arXiv subjects

Stefan Scheel

Publications and source records attributed to Stefan Scheel.

At least 19 recordsLinked to original sources

arXiv2026

Non-Markovian interactions with pulses of quantum radiation

The interaction of a traveling pulse of quantum light with a localized quantum system shows non-Markovian features when scattering takes place in a structured environment. Here, we devise a non-Markovian input-output theory by coherently coupling the scatterer to a pseudomode, which decays into a Markovian reservoir. This incorporates memory effects of a structured environment without altering the cascaded nature of the Lindblad master equation, whose solution provides the quantum state of the output field of any desired mode. We apply our theory to the stimulated emission by a two-level atom, and to transmission of a Gaussian pulse through a cavity. We observe that the non-Markovian revival of coherence in the scatterer distorts the single-mode nature of the incoming pulse, thus resulting in a multimode output field.

quant-ph↗

arXiv2026

Even-harmonic generation through nonequilibrium steady-state symmetry breaking

High-harmonic generation (HHG) in inversion-symmetric systems is typically restricted to odd harmonics by symmetry. Here, we show that this selection rule can be broken without modifying the underlying Hamiltonian. We investigate a boundary-driven Su-Schrieffer-Heeger (SSH) chain coupled to source and sink reservoirs and demonstrate that dissipative dynamics generates a nonequilibrium steady state carrying a finite DC current. While the SSH Hamiltonian retains inversion symmetry, the current-carrying steady-state density matrix does not, leading to the emergence of even harmonics in the emitted spectrum. Using a correlation-matrix approach based on the Lindblad master equation, we obtain the steady state and calculate the resulting HHG response. We find that the intensity of the even harmonics is directly controlled by the transport current, establishing a link between nonequilibrium charge transport and HHG selection rules. Our results uncover a mechanism for even-harmonic generation that relies solely on nonequilibrium steady-state symmetry breaking and provide a route to probing transport currents through ultrafast nonlinear spectroscopy in centrosymmetric quantum systems.

quant-ph↗

arXiv2026

Vector Magnetometry with Broadband Microwave Fields in Nitrogen-Vacancy Centers in Diamond

We present a novel method for full vector magnetometry using nitrogen-vacancy (NV) centers. In contrast to conventional optically detected magnetic resonance techniques, our method employs two distinct broadband microwave pulses and measures them after transmission through the NV sensor medium, thus capturing the line splitting of the ground state triplet due to the Zeeman effect. Two orthogonally polarized microwave pulses allow resolving all magnetic field components independently by reading out differently oriented NV centers. Simulated data is analyzed using deep neural networks, whose efficacy we expect to translate very well to experiments. Our method yields sensitivities between $5~\mathrm{pT}/\sqrt{\mathrm{Hz}}$ and $100~\mathrm{pT}/\sqrt{\mathrm{Hz}}$ across different magnetic field vector components, while achieving approximately $\mathrm{nT}$ accuracy at a signal-to-noise (SNR) ratio of $70~\mathrm{dB}$. By being capable of accurately measuring magnetic fields down to $25~\mathrm{\mu T}$, the need for a bias field beyond Earth's magnetic field is eliminated.

quant-ph↗

arXiv2026

Path integral quantization of the electromagnetic field in nonlinear dielectric materials

We construct a quantum theory of light in nonlinear dielectric media with dispersion and absorption. We employ a mesoscopic model for the light-matter interaction that include a fourth-order nonlinearity in the material response. Quantization is performed by constructing an effective action in a path-integral formalism by integrating out matter and bath degrees of freedom. We show how a nonlinear response function associated with Kerr nonlinearity is obtained through the model and, after full field quantization, we derive the Feynman rules from this theory.

quant-ph↗

arXiv2026

Impact of the valence band on Rydberg excitons in cuprous oxide quantum wells

The complex valence band structure of bulk cuprous oxide necessitates going beyond the parabolic approximation to precisely estimate exciton binding energies. The same is true for excitons in cuprous oxide quantum wells, for which many effects have been obtained so far only qualitatively within a hydrogenlike two-band model. Here, we derive the complete Hamiltonian for excitons in cuprous oxide quantum wells based on the Luttinger-Kohn model, taking into account the full complex valence band structure. Symmetry properties of the system are discussed. Numerical results based on the diagonalization of the Hamiltonian using B-spline functions reveal the energy shifts and the lifting of degeneracies due to the nondiagonal coupling terms of the complex valence band. The relative oscillator strengths of the excitonic transitions induced by circularly polarized light are also calculated.

cond-mat.mes-hall↗

arXiv2025

Unlocking klockmannite: formation of colloidal quasi-2D CuSe nanocrystals and photo-physical properties arising from crystal anisotropy

Copper selenide is an exceptional quasi-layered monolithic material that exhibits both semiconducting and metallic properties in adjacent visible and near-infrared (NIR) spectral ranges. Here we introduce a thiol-free colloidal synthesis for generating quasi-2D klockmannite copper selenide nanocrystals via hot injection method, achieving shape control by tuning the injection temperature and precursor concentrations without any additional ligands. This approach produces large klockmannite nanosheets with lateral sizes from 200 nm to several micrometres, as well as uniform triangular nanoplatelets with sizes of 12-25 nm that are monocrystalline and display strong NIR plasmonic absorption. The spectral features of the anisotropic klockmannite phase in the NIR have been analysed using complex-scaled discrete dipole approximation (CSDDA) calculations, which reveal pronounced optical anisotropy and the emergence of hyperbolic regime. The combined effect of propagating and evanescent fields is regarded as the underlying reason of such modes in the hyperbolic domain. Finally, the ultrafast photophysical behaviour of the material in klockmannite phase is examined, including hot-hole cooling, trapping, and coherent phonons generation. Our findings emphasize the important role of the intrinsic crystal anisotropy in governing the physical properties of nanoscale klockmannite.

cond-mat.mtrl-sci↗

arXiv2025

Gate Sequence Optimization for Parameterized Quantum Circuits using Reinforcement Learning

Current experimental quantum computing devices are limited by noise, mainly originating from entangling gates. If an efficient gate sequence for an operation is unknown, one often employs layered parameterized quantum circuits, especially hardware-efficient ansätze, with fixed entangling layer structures. We demonstrate a reinforcement learning algorithm to improve on these by optimizing the entangling gate sequence in the task of quantum state preparation. This allows us to restrict the required number of CNOT gates while taking the qubit connectivity architecture into account. Recent advancements using reinforcement learning have already demonstrated the power of this technique when optimizing the circuit for a sequence of non-parameterized gates. We extend this approach to parameterized gate sets by incorporating general single-qubit unitaries, thus allowing us to consistently reach higher state preparation fidelities at the same number of CNOT gates compared to a hardware-efficient ansatz.

quant-ph↗

arXiv2025

Multipole expansion for dispersion forces -- watch this trace

Light-matter interaction models invariably rely on the multipole expansion of the electromagnetic potentials generated by complex charge distributions. These multipoles are typically taken to be traceless, however, for a correct evaluation of dispersion forces at all distances, the validity of this assumption has to be checked carefully. Here, we revisit the concept of dispersion forces on an atom near a dielectric surface from the perspective of macroscopic quantum electrodynamics and find that, beyond the quadrupole, the multipoles cannot always be taken as fully traceless. In particular, we show that the trace of the octupole moment contributes to Casimir-Polder interactions beyond the electrostatic regime.

quant-ph↗

arXiv2025

Wavefunctions and oscillator strengths of Rydberg excitons in cuprous oxide quantum wells

We investigate the eigenstates, that is, the wavefunctions of Rydberg excitons in cuprous oxide quantum wells and derive expressions relating them to the oscillator strengths of different exciton states. Using the B-spline expansion, we compute the wavefunctions in coordinate space and estimate the oscillator strengths. The symmetry properties of the states and the non-separability of the wavefunctions are illustrated. Wavefunctions associated with resonances above the scattering threshold, in particular those of bound states in the continuum as well as their partner states, are also given.

cond-mat.mes-hall↗

arXiv2025

Bound states in the continuum in cuprous oxide quantum wells

We propose a realistic semiconductor system containing bound states in the continuum (BICs) which allows for a practical realization. By varying the confinement strength of excitons in cuprous oxide quantum wells, we show that long-lived Rydberg states of the confined electron-hole pairs appear in the continuum background. The accuracy of calculations of the linewidths based on the coupled-channel Schrödinger equation with three channels and only few basis states is confirmed by a numerically exact solution employing a B-spline basis and the complex coordinate-rotation method. We argue that finite-sized cuprous oxide crystals, due to their large exciton binding energies, are a convenient platform for experimental identification of BICs.

cond-mat.mes-hall↗

arXiv2024

Energy states of Rydberg excitons in finite crystals: From weak to strong confinement

Due to quantum confinement, excitons in finite-sized crystals behave rather differently than in bulk materials. We investigate the dependence of energies of Rydberg excitons on the strengths of parabolic as well as rectangular confinement potentials in finite-sized crystals. The evolution of the energy levels of hydrogen-like excitons in the crossover region from weak to strong parabolic confinement is analyzed for different quantum numbers by numerical solution of the two-dimensional Schrödinger equation. The energy spectrum of hydrogen-like excitons in Cu$_{2}$O-based rectangular quantum wells is, in turn, obtained numerically from the solution of the three-dimensional Schrödinger equation as a function of the quantum well width. Various crossings and avoided crossings of Rydberg energy levels are observed and categorized based on the symmetry properties of the exciton wave function. Particular attention is paid to the two limiting cases of narrow and wide quantum wells attributed to strong and weak confinement, respectively. The energies obtained with the pure Coulomb interaction are compared with the results originating from the Rytova-Keldysh potential, i.e., by taking into account the dielectric contrast in the quantum well and in the barrier.

cond-mat.mes-hall↗

arXiv2024

Effects of higher-order Casimir-Polder interactions on Rydberg atom spectroscopy

In the extreme near-field, when the spatial extension of the atomic wavefunction is no longer negligible compared to the atom-surface distance, the dipole approximation is no longer sufficient to describe Casimir-Polder interactions. Here we calculate the higher-order, quadrupole and octupole, contributions to Casimir-Polder energy shifts of Rydberg atoms close to a dielectric surface. We subsequently investigate the effects of these higher-order terms in thin-cell and selective reflection spectroscopy. Beyond its fundamental interest, this new regime of extremely small atom surface separations is relevant for quantum technology applications with Rydberg or surface-bound atoms interfacing with photonic platforms.

physics.atom-ph↗

arXiv2024

Manipulating the Dipolar Interactions and Cooperative Effects in Confined Geometries

To facilitate the transition of quantum effects from the controlled laboratory environment to practical real-world applications, there is a pressing need for scalable platforms. One promising strategy involves integrating thermal vapors with nanostructures designed to manipulate atomic interactions. In this tutorial, we aim to gain deeper insights into this by examining the behavior of thermal vapors that are confined within nanocavities or waveguides and exposed to near-resonant light. We explore the interactions between atoms in confined dense thermal vapors. Our investigation reveals deviations from the predictions of continuous electrodynamics models, including density-dependent line shifts and broadening effects. In particular, our results demonstrate that by carefully controlling the saturation of single atoms and the interactions among multiple atoms using nanostructures, along with controlling the geometry of the atomic cloud, it becomes possible to manipulate the effective optical nonlinearity of the entire atomic ensemble. This capability renders the hybrid thermal atom-nanophotonic platform a distinctive and valuable one for manipulating the collective effect and achieving substantial optical nonlinearities.

physics.atom-ph↗

arXiv2024

Non-adiabatic holonomies as photonic quantum gates

One of the most promising nascent technologies, quantum computation faces a major challenge: The need for stable computational building blocks. We present the quantum-optical realization of non-adiabatic holonomies that can be used as single-qubit quantum gates. The hallmark topological protection of non-Abelian geometric phases reduces the need for quantum error correction on a fundamental physical level, while the inherent non-adiabaticity of the structures paves the way for unprecedented miniaturization. To demonstrate their versatility, we realize the Hadamard and Pauli-X gates, experimentally show their non-Abelian nature, and combine them into a single-qubit quantum algorithm, the PQ penny flipover. The planar geometry of such designs enables them to be substituted for the conventional directional coupler meshes currently in wide-spread use in photonic quantum architectures across all platforms.

quant-ph↗

arXiv2023

Particle-Number Threshold for Non-Abelian Geometric Phases

When a quantum state traverses a path, while being under the influence of a gauge potential, it acquires a geometric phase that is often more than just a scalar quantity. The variety of unitary transformations that can be realised by this form of parallel transport depends crucially on the number of particles involved in the evolution. Here, we introduce a particle-number threshold (PNT) that assesses a system's capabilities to perform purely geometric manipulations of quantum states. This threshold gives the minimal number of particles necessary to fully exploit a system's potential to generate non-Abelian geometric phases. Therefore, the PNT might be useful for evaluating the resource demands of a holonomic quantum computer. We benchmark our findings on bosonic systems relevant to linear and nonlinear quantum optics.

quant-ph↗

arXiv2023

Order-invariant two-photon quantum correlations in PT-symmetric interferometers

Multiphoton correlations in linear photonic quantum networks are governed by matrix permanents. Yet, surprisingly few systematic properties of these crucial algebraic objects are known, while their calculation is a computationally hard task. As such, predicting the overall multiphoton behavior of a network from its individual building blocks typically defies intuition. In this work we identify sequences of concatenated two-mode linear optical transformations whose two-photon behavior is invariant under reversal of the order. We experimentally verify this systematic behavior in parity-time-symmetric complex interferometer arrangements of varying composition. Our results underline new ways in which quantum correlations may be preserved in counterintuitive ways even in small-scale non-Hermitian networks.

quant-ph↗

arXiv2022

Geometrically robust linear optics from non-Abelian geometric phases

We construct a unified operator framework for quantum holonomies generated from bosonic systems. For a system whose Hamiltonian is bilinear in the creation and annihilation operators, we find a holonomy group determined only by a set of selected orthonormal modes obeying a stronger version of the adiabatic theorem. This photon-number independent description offers deeper insight as well as a computational advantage when compared to the standard formalism on geometric phases. In particular, a strong analogy between quantum holonomies and linear optical networks can be drawn. This relation provides an explicit recipe how any linear optical quantum computation can be made geometrically robust in terms of adiabatic or nonadiabatic geometric phases.

quant-ph↗

arXiv2021

Interseries dipole transitions from yellow to green excitons in cuprous oxide

We study dipole interseries transitions between the yellow and green exciton series in cuprous oxide including the complex valence band structure. To this end, we extend previous studies of the spectrum of complex green exciton resonances [Phys. Rev. B 101, 075208 (2020)] to optical transitions between different exciton states in addition to transitions from the crystal ground state. This allows us to augment the calculations on interseries transitions using a hydrogen-like model [Phys. Rev. B 100, 085201 (2019)] by a more comprehensive treatment of the valence band structure.

cond-mat.mes-hall↗