arXiv subjects

Stefan Scheel

Publications and source records attributed to Stefan Scheel.

At least 37 records · Page 2Linked to original sources

arXiv2021

Symmetry-protected non-Abelian geometric phases in optical waveguides with nonorthogonal modes

The generation of non-Abelian geometric phases from a system of evanescently coupled waveguides is extended towards the framework of nonorthogonal coupled-mode theory. Here, we study an experimentally feasible tripod arrangement of waveguides that contain dark states from which a nontrivial U(2)-mixing can be obtained by means of an adiabatic parameter variation. We investigate the influence of higher-order contributions beyond nearest-neighbour coupling as well as self-coupling on the stability of a U(3)-phase generated from an optical tetrapod setup. Our results indicate that, despite the mode nonorthogonality, the symmetry of dark states protects the geometric evolution of light from distortion.

physics.optics↗

arXiv2021

Reconstruction of nanoscale particles from single-shot wide-angle FEL diffractions patterns with physics-informed neural networks

Single-shot wide-angle diffraction imaging is a widely used method to investigate the structure of non-crystallizing objects such as nanoclusters, large proteins or even viruses. Its main advantage is that information about the three-dimensional structure of the object is already contained in a single image. This makes it useful for the reconstruction of fragile and non-reproducible particles without the need for tomographic measurements. However, currently there is no efficient numerical inversion algorithm available that is capable of determining the object's structure in real time. Neural networks, on the other hand, excel in image processing tasks suited for such purpose. Here we show how a physics-informed deep neural network can be used to reconstruct complete three-dimensional object models of uniform, convex particles on a voxel grid from single two-dimensional wide-angle scattering patterns. We demonstrate its universal reconstruction capabilities for silver nanoclusters, where the network uncovers novel geometric structures that reproduce the experimental scattering data with very high precision.

physics.data-an↗

arXiv2020

A Passive $\mathcal{PT}$-Symmetric Floquet-Coupler

Based on a Liouville-space formulation of open systems, we present a solution to the quantum master equation of two coupled optical waveguides with varying loss. The periodic modulation of the Markovian loss of one of them yields a passive $\mathcal{PT}$-symmetric Floquet system that, at resonance, shows a strong reduction of the required loss for the $\mathcal{PT}$ symmetry to be broken. We showcase this transition for a multi-photon state, and we show how to physically implement the modulated loss with reservoir engineering of a set of bath modes.

quant-ph↗

arXiv2020

Asymmetric Rydberg blockade of giant excitons in Cuprous Oxide

The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4] and technology [5-7]. Rydberg excitons provide a promising solid-state realization of such highly excited states, for which record-breaking orbital sizes of up to a micrometer have indeed been observed in cuprous oxide semiconductors [8]. Here, we demonstrate the generation and control of strong exciton interactions in this material by optically producing two distinct quantum states of Rydberg excitons. This makes two-color pump-probe experiments possible that allow for a detailed probing of the interactions. Our experiments reveal the emergence of strong spatial correlations and an inter-state Rydberg blockade that extends over remarkably large distances of several micrometers. The generated many-body states of semiconductor excitons exhibit universal properties that only depend on the shape of the interaction potential and yield clear evidence for its vastly extended-range and power-law character.

cond-mat.mes-hall↗

arXiv2020

Fast reconstruction of single-shot wide-angle diffraction images through deep learning

Single-shot X-ray imaging of short-lived nanostructures such as clusters and nanoparticles near a phase transition or non-crystalizing objects such as large proteins and viruses is currently the most elegant method for characterizing their structure. Using hard X-ray radiation provides scattering images that encode two-dimensional projections, which can be combined to identify the full three-dimensional object structure from multiple identical samples. Wide-angle scattering using XUV or soft X-rays, despite yielding lower resolution, provides three-dimensional structural information in a single shot and has opened routes towards the characterization of non-reproducible objects in the gas phase. The retrieval of the structural information contained in wide-angle scattering images is highly non-trivial, and currently no efficient rigorous algorithm is known. Here we show that deep learning networks, trained with simulated scattering data, allow for fast and accurate reconstruction of shape and orientation of nanoparticles from experimental images. The gain in speed compared to conventional retrieval techniques opens the route for automated structure reconstruction algorithms capable of real-time discrimination and pre-identification of nanostructures in scattering experiments with high repetition rate -- thus representing the enabling technology for fast femtosecond nanocrystallography.

physics.atm-clus↗

arXiv2020

Collective dipole-dipole interactions in planar nanocavities

The collective response of an atomic ensemble is shaped by its macroscopic environment. We demonstrate this effect in the near-resonant transmission of light through a thermal rubidium vapor confined in a planar nanocavity. Our model reveals density-dependent line shifts and broadenings beyond continuous electrodynamics models that oscillate with cavity width and have been observed in recent experiments. We predict that the amplitudes of these oscillations can be controlled by coatings that modify the cavity's Finesse.

physics.atom-ph↗

arXiv2020

Interaction of charged impurities and Rydberg excitons in cuprous oxide

We investigate the influence of a static, uncorrelated distribution of charged impurities on the spectrum of bound excitons in the copper oxide Cu$_{\text{2}}$O. We show that the statistical distribution of Stark shifts and ionisation rates leads to the vanishing of Rydberg resonances into an apparent continuum. The appearance of additional absorption lines due to the broken rotational symmetry, together with spatially inhomogeneous Stark shifts, leads to a modification of the observed line shapes that agree qualitatively with the changes observed in the experiment.

cond-mat.mes-hall↗

arXiv2020

Highly-Degenerate Photonic Waveguide Structures for Holonomic Computation

We investigate an all-out optical setup allowing for generation of non-Abelian geometric phases on its large degenerate eigenspaces. The proposal has the form of an M -pod system and can be implemented in terms of integrated photonic waveguide structures. We show that by injecting a larger number of photons into the optical setup, the degeneracy of eigenspaces scales rapidly. After studying the spectral properties of our system for the general case, we show how arbitrary U(4) transformations can be generated on the dark subspace of an optical tripod filled with two photons. Moreover, a degeneracy in the bright subspaces of the system, absent in any atomic analogue, allows for the generation of universal single-qubit manipulations. Finally, we address the complexity issue of holonomic computation. Particularly, we show how two-qubit and three-qubit states can be implemented on a photonic tripod, where a natural multi-partite structure is inherited from the spatial mode structure of the waveguides.

quant-ph↗

arXiv2020

Solving the quantum master equation of coupled harmonic oscillators with Lie algebra methods

Based on a Liouville-space formulation of open systems, we present two methods to solve the quantum dynamics of coupled harmonic oscillators experiencing Markovian loss. Starting point is the quantum master equation in Liouville space which is generated by a Liouvillian that induces a Lie algebra. We show how this Lie algebra allows to define ladder operators that construct Fock-like eigenstates of the Liouvillian. These eigenstates are used to decompose the time-evolved density matrix and, together with the accompanying eigenvalues, provide insight into the transport properties of the lossy system. Additionally, a Wei-Norman expansion of the generated time evolution can be found by a structure analysis of the algebra. This structure analysis yields a construction principle to implement effective non-Hermitian Hamiltonians in lossy systems.

quant-ph↗

arXiv2019

Casimir--Polder induced Rydberg macrodimers

We theoretically investigate Rydberg atom pair potentials of Rb atoms in front of a perfectly conducting plate. The pair potentials are perturbed by both the Casimir--Polder potential acting on a single atom and the scattering contribution to the interatomic interaction. In contrast to the pair potentials in free space, at atom-surface distances $d_s \lesssim 4\,μ$m, avoided crossings appear. In the associated potential wells that are entirely due to dispersion interactions with the surface, there exist vibrational bound states, i.e. Rydberg macrodimers, with groundstate energies of up to $E = -68\,$MHz and radial expectation values of the order of several $μ$m.

physics.atom-ph↗

arXiv2019

Interseries transitions between Rydberg excitons in Cu$_{\mathrm{2}}$O

We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is inadequate and, in particular, that it breaks down in yellow-blue transitions even for moderate principal quantum numbers of $n \approx 10$. The interband matrix elements of the transition operator needed for the evaluation of the excitonic transition strengths are derived from known as well as from fitted band parameters.

cond-mat.mes-hall↗

arXiv2019

Holonomic Gates in Pseudo-Hermitian Quantum Systems

The time-dependent pseudo-Hermitian formulation of quantum mechanics allows to study open system dynamics in analogy to Hermitian quantum systems. In this setting, we show that the notion of holonomic quantum computation can equally be formulated for pseudo-Hermitian systems. Starting from a degenerate pseudo-Hermitian Hamiltonian we show that, in the adiabatic limit, a non-Abelian geometric phase emerges which realizes a pseudounitary quantum gate. We illustrate our findings by studying a pseudo-Hermitian gain/loss system which can be written in the form of a tripod Hamiltonian by using the biorthogonal representation. It is shown that this system allows for arbitrary pseudo-$\mathrm{U}(2)$ transformations acting on the dark subspace of the system.

quant-ph↗

arXiv2019

Observation of PT-symmetric quantum interference

Parity-Time (PT) symmetric quantum mechanics is a complex extension of conventional Hermitian quantum mechanics in which physical observables possess a real eigenvalue spectrum. However, an experimental demonstration of the true quantum nature of PT symmetry has been elusive thus far, as only single-particle physics has been exploited to date. In our work, we demonstrate two-particle quantum interference in a PT-symmetric system. We employ integrated photonic waveguides to reveal that PT-symmetric bunching of indistinguishable photons shows strongly counterintuitive features. We substantiate our experimental results by modelling the system by a quantum master equation, which we analytically solve using Lie algebra methods. Our work paves the way for nonlocal PT-symmetric quantum mechanics as a novel building block for future quantum devices.

quant-ph↗

arXiv2019

Optimal design strategy for non-Abelian geometric phases using Abelian gauge fields based on quantum metric

Geometric phases, which are ubiquitous in quantum mechanics, are commonly more than only scalar quantities. Indeed, often they are matrix-valued objects that are connected with non-Abelian geometries. Here we show how generalized, non-Abelian geometric phases can be realized using electromagnetic waves travelling through coupled photonic waveguide structures. The waveguides implement an effective Hamiltonian possessing a degenerate dark subspace, in which an adiabatic evolution can occur. The associated quantum metric induces the notion of a geodesic that defines the optimal adiabatic evolution. We exemplify the non-Abelian evolution of an Abelian gauge field by a Wilson loop.

physics.optics↗

arXiv2018

Eigenenergies of excitonic giant-dipole states in cuprous oxide

In this work we present the eigenspectra of a novel species of Wannier excitons when exposed to crossed electric and magnetic fields. In particular, we compute the eigenenergies of giant-dipole excitons in $\textrm{Cu}_2\textrm{O}$ in crossed fields. In our theoretical approach, we calculate the excitonic spectra within both an approximate as well as a numerically exact approach for arbitrary field configurations. We verify that stable bound excitonic giant-dipole states are only possible in the strong magnetic field limit, as this is the only regime providing sufficiently deep potential wells for their existence. Comparing both analytic as well as numerical calculations, we obtain excitonic giant-dipole spectra with level spacings in the range of $0.6\ldots100\, μ\textrm{eV}$.

cond-mat.mes-hall↗

arXiv2018

Interactions between Rydberg excitons in Cu$_2$O

Highly-excited states of excitons in cuprous oxide have recently been observed at a record quantum number of up to $n=25$. Here, we evaluate the long-range interactions between pairs of Rydberg excitons in Cu$_2$O, which are due to direct Coulomb forces rather than short-range collisions typically considered for ground state excitons. A full numerical analysis is supplemented by the van der Waals asymptotics at large exciton separations, including the angular dependence of the potential surfaces.

cond-mat.quant-gas↗

arXiv2018

Waveguides for Rydberg excitons in Cu$_\text{2}$O from strain traps

We investigate the formation of waveguides for Rydberg excitons in Cu$_\text{2}$O from cylindrical stressors as alternatives to optical traps. We show that the achievable potential depths can easily reach the meV and the trap frequencies the GHz regimes. For Rydberg excitons, we find that it is sufficient to consider only the shift of the band gap, whereas the excitonic binding energies remain almost unchanged.

cond-mat.mes-hall↗

arXiv2018

PT-symmetric photonic quantum systems with gain and loss do not exist

We discuss the impact of gain and loss on the evolution of photonic quantum states and find that PT-symmetric quantum optics in gain/loss systems is not possible. Within the framework of macroscopic quantum electrodynamics we show that gain and loss are associated with non-compact and compact operator transformations, respectively. This implies a fundamentally different way in which quantum correlations between a quantum system and a reservoir are built up and destroyed.

quant-ph↗