arXiv subjects

Stefan Schumacher

Publications and source records attributed to Stefan Schumacher.

At least 55 records · Page 3Linked to original sources

arXiv2022

Circularly polarized electroluminescence from a single-crystal organic microcavity light-emitting diode based on photonic spin-orbit interactions

Circularly polarized (CP) electroluminescence from organic light-emitting diodes (OLEDs) has aroused considerable attention for their potential in future display and photonic technologies. The development of CP-OLEDs relies largely on chiral-emitters, which not only remain rare owing to difficulties in design and synthesis but also limit the performance of electroluminescence. When the polarization (pseudospin) degrees of freedom of a photon interact with its orbital angular momentum, photonic spin-orbit interaction (SOI) emerges such as Rashba-Dresselhaus (RD) effect. Here, we demonstrate a chiral-emitter-free microcavity CP-OLED with a high dissymmetry factor (gEL) and high luminance by embedding a thin two-dimensional organic single crystal (2D-OSC) between two silver layers which serve as two metallic mirrors forming a microcavity and meanwhile also as two electrodes in an OLED architecture. In the presence of the RD effect, the SOIs in the birefringent 2D-OSC microcavity result in a controllable spin-splitting with CP dispersions. Thanks to the high emission efficiency and high carrier mobility of the OSC, chiral-emitter-free CP-OLEDs have been demonstrated exhibiting a high gEL of 1.1 and a maximum luminance of about 60000 cd/m2, which places our device among the best performing CP-OLEDs. This strategy opens a new avenue for practical applications towards on-chip microcavity CP-OLEDs.

physics.optics↗

arXiv2022

Strain Induced Indirect-to-Direct Bandgap Transition, Photoluminescence Enhancement, and Linewidth Reduction in Bilayer MoTe2

Two-dimensional (2D) layered materials provide an ideal platform for engineering electronic and optical properties through strain control because of their extremely high mechanical elasticity and sensitive dependence of material properties on mechanical strain. In this paper, a combined experimental and theoretical effort is made to investigate the effects of mechanical strain on various spectral features of bilayer MoTe2 photoluminescence (PL). We found that bilayer MoTe2 can be converted from an indirect-to direct-bandgap material through strain engineering, resulting in a photoluminescence enhancement by a factor of 2.24. Over 90% of the PL comes from photons emitted by the direct excitons at the maximum strain applied. Importantly, we show that strain effects lead to a reduction of the overall linewidth of PL by as much as 36.6%. We attribute the dramatic decrease of linewidth to a strain-induced complex interplay among various excitonic varieties such as direct bright excitons, trions, and indirect excitons. Our experimental results on direct and indirect exciton emission features are explained by theoretical exciton energies that are based on first-principle electronic band structure calculations. The consistent theory-experimental trend shows that the enhancement of PL and the reduction of linewidth are the consequences of the increasing direct exciton contribution with the increase of strain. Our results demonstrate that strain engineering can lead to a PL quality of the bilayer MoTe2 comparable to that of the monolayer counterpart. The additional benefit of a longer emission wavelength makes the bilayer MoTe2 more suitable for Silicon-photonics integration due to the reduced Silicon absorption.

cond-mat.mtrl-sci↗

arXiv2022

Tracking quantum coherence in polariton condensates with time-resolved tomography

Long-term quantum coherence constitutes one of the main challenges when engineering quantum devices. However, easily accessible means to quantify complex decoherence mechanisms are not readily available, nor are sufficiently stable systems. We harness novel phase-space methods - expressed through non-Gaussian convolutions of highly singular Glauber-Sudarshan quasiprobabilities - to dynamically monitor quantum coherence in polariton condensates with significantly enhanced coherence times. Via intensity- and time-resolved reconstructions of such phase-space functions from homodyne detection data, we probe the systems's resourcefulness for quantum information processing up to the nanosecond regime. Our experimental findings are confirmed through numerical simulations for which we develop an approach that renders established algorithms compatible with our methodology. In contrast to commonly applied phase-space functions, our distributions can be directly sampled from measured data, including uncertainties, and yield a simple operational measure of quantum coherence via the distribution's variance in phase. Therefore, we present a broadly applicable framework and a platform to explore time-dependent quantum phenomena and resources.

quant-ph↗

arXiv2022

Unidirectional vortex waveguides and multistable vortex pairs in polariton condensates

Vortices carrying quantized topological charges have potential application in information processing. In this work, we investigate vortex carriers and waveguides in microcavity polariton condensates, nonresonantly excited by a homogeneous pump with intensity grooves. An intensity groove with a ring shape in the pump gives rise to dark-ring states of the condensate with a $π$-phase jump, akin to dark solitons. The dark-ring states can be destroyed by a stronger density of the surrounding condensate and reduce into vortex-antivortex pairs. Multiple vortex-pair states are found to be stable in the same dark ring of the pump. When the pump ring is broader, higher-order dark states with multiple $π$-phase jumps can be obtained and interestingly they can be used to construct vortex waveguides. If a single vortex is imprinted in such waveguides, it can travel in a particular direction, showing one-way transportation. In other words, an imprinted vortex with a certain charge in a specifically designed higher-order dark state is only allowed to propagate unidirectionally.

physics.optics↗

arXiv2021

Dynamics of phase defects trapped in optically imprinted orbits in dissipative binary polariton condensate

We study the dynamics of phase defects trapped in a finite optically imprinted ring lattice in binary polariton condensates, under the influence of the cross-interaction (CI) between the condensates in different spin components and the spin-orbit interaction (SOI). In this configuration, we find that a vortex circulates unidirectionally in optically induced orbits because of the Magnus force acting in the polariton fluid, and the vortex' angular velocity is influenced by the SOI and CI. Interestingly, in our system, these two interactions can also lead to elongated and frozen phase defects, forming a frozen dark solution with similarity to a dark soliton but with finite size in both spin components. When the dark solution is stretched further to occupy the entire orbit of a condensate ring, the phase defect triggers a snake instability and induces the decay of the dark ring solution. The circulation direction of a single vortex is determined by the Magnus force. This situation is more complex for the group motion of multiple vortices because of significant vortex-antivortex interaction. The collective motion of such vortex constellations, however, can be determined by the SOI.

cond-mat.quant-gas↗

arXiv2021

Helical polariton lasing from topological valleys in an organic crystalline microcavity

Topological photonics provides an important platform for the development of photonic devices with robust disorder-immune light transport and controllable helicity. Mixing photons with excitons (or polaritons) gives rise to nontrivial polaritonic bands with chiral modes, allowing the manipulation of helical lasers in strongly coupled light-matter systems. In this work, we demonstrate helical polariton lasing from topological valleys of an organic anisotropic microcrystalline cavity based on tailored local nontrivial band geometry. This polariton laser emits light of different helicity along different angular directions. The significantly enhanced chiral characteristics are achieved by the nonlinear relaxation process. Helical topological polariton lasers may provide a perfect platform for the exploration of novel topological phenomena that involve light-matter interaction and the development of polariton-based spintronic devices.

physics.optics↗

arXiv2021

Quantifying quantum coherence in polariton condensates

We theoretically and experimentally investigate quantum features of an interacting light-matter system from a multidisciplinary perspective, unifying approaches from semiconductor physics, quantum optics, and quantum information science. To this end, we quantify the amount of quantum coherence that results from the quantum superposition of Fock states, constituting a measure of the resourcefulness of the produced state for modern quantum protocols. As an archetypal example of a hybrid light-matter interface, we study a polariton condensate and implement a numerical model to predict its properties. Our simulation is confirmed by our proof-of-concept experiment in which we measure and analyze the phase-space distributions of the emitted light. Specifically, we drive a polariton microcavity across the condensation threshold and observe the transition from an incoherent thermal state to a coherent state in the emission, thus confirming the build-up of quantum coherence in the condensate itself.

quant-ph↗

arXiv2021

Tilting flat bands in an empty microcavity

Recently microcavities with anisotropic materials are shown to be able to create novel bands with non-zero local Berry curvature. The anisotropic refractive index of the cavity layer is believed to be critical in opening an energy gap at the tilted Dirac points. In this work, we show that an anticrossing between a cavity mode and a Bragg mode can also form within an empty microcavity without any birefringent materials. Flat bands are observed within the energy gap due to the particular refractive index distribution of the sample. The intrinsic TE-TM splitting and XY splitting induce the squeezing of the cavity modes in momentum space, so that the flat bands are spin-dependently tilted. Our results pave the way to investigate the spin orbit coupling of photons in a simple microcavity without anisotropic cavity layers.

physics.optics↗

arXiv2021

Ultrafast electric control of cavity mediated single-photon and photon-pair generation with semiconductor quantum dots

Employing the ultrafast control of electronic states of a semiconductor quantum dot in a cavity, we introduce a novel approach to achieve on-demand emission of single photons with almost perfect indistinguishability and photon pairs with near ideal entanglement. Our scheme is based on optical excitation off-resonant to a cavity mode followed by ultrafast control of the electronic states using the time-dependent quantum-confined Stark effect, which then allows for cavity-resonant emission. Our theoretical analysis takes into account cavity-loss mechanisms, the Stark effect, and phonon-induced dephasing allowing realistic predictions for finite temperatures.

cond-mat.mes-hall↗

arXiv2021

Pulse shaping for on-demand emission of single Raman photons from a quantum-dot biexciton

Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and the ground state of a quantum dot. The advantage of this process is that it allows all-optical control of the properties of the emitted single photon with a laser pulse. However, with the presence of other decay channels and excitation-induced quantum interference, on-demand emission of the single Raman photon is generally difficult to achieve. Here we show that laser pulses with non-trivial shapes can be used to maintain excitation conditions for which with increasing pulse intensities the on-demand regime is reached. To provide a realistic picture of the achievable system performance, we include phonon-mediated processes in the theoretical caluclations. While preserving both high photon purity and indistinguishability, we find that although based on a higher-order emission process, for realistic system parameters on-demand Raman photon emission is indeed achievable with suitably tailored laser pulses.

quant-ph↗

arXiv2021

Realization of exciton-mediated optical spin-orbit interaction in organic microcrystalline resonators

The ability to control the spin-orbit interaction of light in optical microresonators is of fundamental importance for future photonics. Organic microcrystals, due to their giant optical anisotropy, play a crucial role in spin-optics and topological photonics. Here we realize controllable and wavelength-dependent Rashba-Dresselhaus spin-orbit interaction, attributed to the anisotropic excitonic response in an optical microcavity filled with an organic microcrystalline. We also investigate the transition of the spin-orbit interaction from dominant photonic type caused by the splitting of the transverse-electric and transverse-magnetic modes to spin-orbit interaction of the Rashba-Dresselhaus type. The interplay of the two allows us to engineer the spin-orbit interaction of light in organic microcavities, which besides its fundamental interest promises applications in spin-controlled on-chip integrated nanophotonic elements, towards exploiting non-magnetic and low-cost spin-photonic devices.

physics.optics↗

arXiv2021

All-optical beam steering using the polariton lighthouse effect

We demonstrate theoretically and experimentally that a specifically designed microcavity driven in the optical parametric oscillation regime exhibits lighthouse-like emission, i.e., an emission focused around a single direction. Remarkably, the emission direction of this micro-lighthouse is continuously controlled by the linear polarization of the incident laser, and angular beam steering over \unit{360}{\degree} is demonstrated. Theoretically, this unprecedented effect arises from the interplay between the nonlinear optical response of microcavity exciton-polaritons, the difference in the subcavities forming the microcavity, and the rotational invariance of the device.

physics.optics↗

arXiv2021

Switching off microcavity polariton condensate near the exceptional point

Gain and loss modulation are ubiquitous in nature. An exceptional point arises when both the eigenvectors and eigenvalues coalesce, which in a physical system can be achieved by engineering the gain and loss coefficients, leading to a wide variety of counter-intuitive phenomena. In this work we demonstrate the existence of an exceptional point in an exciton polariton condensate in a double-well potential. Remarkably, near the exceptional point, the polariton condensate localized in one potential well can be switched off by an additional optical excitation in the other well with very low (far below threshold) laser power which surprisingly induces additional loss into the system. Increasing the power of the additional laser leads to a situation in which gain dominates in both wells again, such that the polaritons re-condense with almost the same density in the two potential wells. Our results offer a simple way to optically manipulate the polariton lasing process in a double-well potential structure. Extending such configuration to complex potential well lattices offers exciting prospects to explore high-order exceptional points and non-Hermitian topological photonics in a non-equilibrium many-body system.

physics.optics↗

arXiv2021

Atomically thin sheets of lead-free one-dimensional hybrid perovskites feature tunable white-light emission from self-trapped excitons

Low-dimensional organic-inorganic perovskites synergize the virtues of two unique classes of materials featuring intriguing possibilities for next-generation optoelectronics: they offer tailorable building blocks for atomically thin, layered materials while providing the enhanced light harvesting and emitting capabilities of hybrid perovskites. Here, we go beyond the paradigm that atomically thin materials require in-plane covalent bonding and report single layers of the one-dimensional organic-inorganic perovskite [C$_7$H$_{10}$N]$_3$[BiCl$_5$]Cl. Its unique 1D-2D structure enables single layers and the formation of self-trapped excitons which show white light emission. The thickness dependence of the exciton self-trapping causes an extremely strong shift of the emission energy. Thus, such two-dimensional perovskites demonstrate that already 1D covalent interactions suffice to realize atomically thin materials and provide access to unique exciton physics. These findings enable a much more general construction principle for tailoring and identifying two-dimensional materials that are no longer limited to covalently bonded 2D sheets.

cond-mat.mtrl-sci↗

arXiv2021

Externally Controlled Lotka-Volterra Dynamics in a Linearly Polarized Polariton Fluid

Spontaneous formation of transverse patterns is ubiquitous in nonlinear dynamical systems of all kinds. An aspect of particular interest is the active control of such patterns. In nonlinear optical systems this can be used for all-optical switching with transistor-like performance, for example realized with polaritons in a planar quantum-well semiconductor microcavity. Here we focus on a specific configuration which takes advantage of the intricate polarization dependencies in the interacting optically driven polariton system. Besides detailed numerical simulations of the coupled light-field exciton dynamics, in the present paper we focus on the derivation of a simplified population competition model giving detailed insight into the underlying mechanisms from a nonlinear dynamical systems perspective. We show that such a model takes the form of a generalized Lotka-Volterra system for two competing populations explicitly including a source term that enables external control. We present a comprehensive analysis both of the existence and stability of stationary states in the parameter space spanned by spatial anisotropy and external control strength. We also construct phase boundaries in non-trivial regions and characterize emerging bifurcations. The population competition model reproduces all key features of the switching observed in full numerical simulations of the rather complex semiconductor system and at the same time is simple enough for a fully analytical understanding of the system dynamics.

cond-mat.other↗

arXiv2020

Structuring co- and counter-flowing currents of polariton condensates in concentric ring-shaped potentials

We investigate the current flow of microcavity polariton condensates loaded into concentric ring-shaped potentials. The tunneling of the condensates between different potential rings results in different phase-locked states, depending on the separation of the potential rings. As a consequence, the condensate currents in different rings can flow either in the same or opposite direction depending on the specific configuration of the ring-shaped potentials. In two concentric standard ring-shaped potentials, the condensates always circulate in the same direction (co-flowing current) and the vortices formed in the two rings share the same topological charge because of the azimuthally uniform distribution of their phase difference. In this case, increasing the number of the potential rings enables the excitation of Bessel-like solutions. If the two ring-shaped potentials are engineered into an eye shape with the inner ring being standard ring-shaped and the outer ring being elliptically ring-shaped, the phase differences of the condensates in the two rings along the major and minor axes of the ellipse can be opposite, which gives rise to a counter-flowing condensate currents.

physics.optics↗

arXiv2020

Chiral condensates in a polariton hexagonal ring

We model generation of vortex modes in exciton-polariton condensates in semiconductor micropillars, arranged into a hexagonal ring molecule, in the presence of TE-TM splitting. This splitting lifts the degeneracy of azimuthally modulated vortex modes with opposite topological charges supported by this structure, so that a number of non-degenerate vortex states characterized by different combinations of topological charges in two polarization components appears. We present a full bifurcation picture for such vortex modes and show that because they have different energies, they can be selectively excited by coherent pump beams with specific frequencies and spatial configurations. At high pumping intensity, polariton-polariton interactions give rise to the coupling of different vortex resonances and a bistable regime is achieved.

cond-mat.quant-gas↗

arXiv2020

Topological edge states of nonequilibrium polaritons in hollow honeycomb arrays

We address topological currents in polariton condensates excited by uniform resonant pumps in finite honeycomb arrays of microcavity pillars with a hole in the center. Such currents arise under combined action of the spin-orbit coupling and the Zeeman splitting that break the time-reversal symmetry and open a topological gap in the spectrum of the structure. The most representative feature of this structure is the presence of two interfaces, inner and outer ones, where the directions of topological currents are opposite. Due to the finite size of the structure polariton-polariton interactions lead to the coupling of the edge states at the inner and outer interfaces, which depends on the size of the hollow region. Moreover, switching between currents can be realized by tuning the pump frequency. We illustrate that currents in this finite structure can be stable and study bistability effects arising due to the resonant character of the pump.

physics.optics↗