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Stefan Yoshi Buhmann

Publications and source records attributed to Stefan Yoshi Buhmann.

103 records · Page 6Linked to original sources

Thermal Casimir vs Casimir-Polder forces: Equilibrium and non-equilibrium forces

We critically discuss the common belief that the thermal Casimir-Polder force can always be represented as a Matsubara sum, as it is true for the Casimir force. On the contrary, an exact treatment of the atom-field coupling reveals that for a ground-state atom, terms associated with virtual-photon absorption contribute to the force which are identified as a signature of non-equilibrium dynamics. Even the equilibrium force on a thermalized atom or molecule may be overestimated when using the ground-state polarizability instead of its thermal counterpart.

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Interatomic van der Waals potential in the presence of a magneto-electric sphere

On the basis of a general formula obtained earlier via fourth-order erturbation theory within the framework of macroscopic quantum electrodynamics, the van der Waals potential between two neutral, unpolarized, ground-state atoms in the presence of a homogeneous, dispersing and absorbing magnetoelectric sphere is studied. When the radius of the sphere becomes sufficiently large, the result asymptotically agrees with that for two atoms near a planar interface. In the opposite limit of a very small sphere, the sphere can effectively be regarded as being a third ground-state atom, and the nonadditive three-atom van der Waals potential is recovered. To illustrate the effect of a sphere of arbitrary radius, numerical results are presented for the triangular arrangement where the atoms are at equidistance from the sphere, and for the linear arrangement where the atoms and the sphere are aligned along a straight line. As demonstrated, the enhancement or reduction of the interaction potential in the presence of purely electric or magnetic spheres can be physically understood in terms of image charges.

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Two-atom van der Waals interaction between polarizable/magnetizable atoms near magneto-electric bodies

The van der Waals potential of two atoms in the presence of an arbitrary arrangement of dispersing and absorbing magnetodielectric bodies is studied. Starting from a polarizable atom placed within a given geometry, its interaction with a second polarizable/magnetizable atom is deduced from its Casimir-Polder interaction with a weakly polarizable/magnetizable test body. The general expressions for the van der Waals potential hence obtained are illustrated by considering first the case of two atoms in free space, with special emphasis on the interaction between (i) two polarizable atoms and (ii) a polarizable and a magnetizable atom. Furthermore, the influence of magnetodielectric bodies on the van der Waals interaction is studied in detail for the example of two atoms placed near a perfectly reflecting plate or a magnetodielectric half space, respectively.

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Microscopic origin of Casimir-Polder forces

We establish a general relation between dispersion forces. First, based on QED in causal media, leading-order perturbation theory is used to express both the single-atom Casimir-Polder and the two-atom van der Waals potentials in terms of the atomic polarizabilities and the Green tensor for the body-assisted electromagnetic field. Endowed with this geometry-independent framework, we then employ the Born expansion of the Green tensor together with the Clausius-Mosotti relation to prove that the macroscopic Casimir-Polder potential of an atom in the presence of dielectric bodies is due to an infinite sum of its microscopic many-atom van der Waals interactions with the atoms comprising the bodies. This theorem holds for inhomogeneous, dispersing, and absorbing bodies of arbitrary shapes and arbitrary atomic composition on an arbitrary background of additional magnetodielectric bodies.

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Dispersion forces in macroscopic quantum electrodynamics

The description of dispersion forces within the framework of macroscopic quantum electrodynamics in linear, dispersing, and absorbing media combines the benefits of approaches based on normal-mode techniques of standard quantum electrodynamics and methods based on linear response theory in a natural way. It renders generally valid expressions for both the forces between bodies and the forces on atoms in the presence of bodies, while showing very clearly the intimate relation between the different types of dispersion forces. By considering examples, the influence of various factors like form, size, electric and magnetic properties, or intervening media on the forces is addressed. Since the approach based on macroscopic quantum electrodynamics does not only apply to equilibrium systems, it can be used to investigate dynamical effects such as the temporal evolution of forces on arbitrarily excited atoms.

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Casimir-Polder forces: A non-perturbative approach

Within the frame of macroscopic QED in linear, causal media, we study the radiation force of Casimir-Polder type acting on an atom which is positioned near dispersing and absorbing magnetodielectric bodies and initially prepared in an arbitrary electronic state. It is shown that minimal and multipolar coupling lead to essentially the same lowest-order perturbative result for the force acting on an atom in an energy eigenstate. To go beyond perturbation theory, the calculations are based on the exact center-of-mass equation of motion. For a nondriven atom in the weak-coupling regime, the force as a function of time is a superposition of force components that are related to the electronic density-matrix elements at a chosen time. Even the force component associated with the ground state is not derivable from a potential in the ususal way, because of the position dependence of the atomic polarizability. Further, when the atom is initially prepared in a coherent superposition of energy eigenstates, then temporally oscillating force components are observed, which are due to the interaction of the atom with both electric and magnetic fields.

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The van der Waals energy of atomic systems near absorbing and dispersing bodies

Within the frame of macroscopic quantum electrodynamics in causal media, the van der Waals interaction between an atomic system and an arbitrary arrangement of dispersing and absorbing dielectric bodies including metals is studied. It is shown that the minimal-coupling scheme and the multipolar-coupling scheme lead to essentially the same formula for the van der Waals potential. As an application, the vdW potential of an atom in the presence of a sphere is derived. Closed expressions for the long-distance (retardation) and short-distance (non-retardation) limits are given, and the effect of material absorption is discussed.

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Local-field correction to the spontaneous decay rate of atoms embedded in bodies of finite size

The influence of the size and shape of a dispersing and absorbing dielectric body on the local-field corrected spontaneous-decay of an excited atom embedded in the body is studied on the basis of the real-cavity model. By means of a Born expansion of the Green tensor of the system it is shown that to linear order in the susceptibility of the body the decay rate exactly follows Tomas's formula found for the special case of an atom at the center of a homogeneous dielectric sphere [Phys. Rev. A 63, 053811 (2001)]. It is further shown that for an atom situated at the interior of an arbitrary dielectric body this formula remains valid beyond the linear order. The case of an atom embedded in a weakly polarizable sphere is discussed in detail.

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Body-assisted van der Waals interaction between two atoms

Using fourth-order perturbation theory, a general formula for the van der Waals potential of two neutral, unpolarized, ground-state atoms in the presence of an arbitrary arrangement of dispersing and absorbing magnetodielectric bodies is derived. The theory is applied to two atoms in bulk material and in front of a planar multilayer system, with special emphasis on the cases of a perfectly reflecting plate and a semi-infinite half space. It is demonstrated that the enhancement and reduction of the two-atom interaction due to the presence of a perfectly reflecting plate can be understood, at least in the nonretarded limit, by using the method of image charges. For the semi-infinite half space, both analytical and numerical results are presented.

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Born expansion of the Casimir-Polder interaction of a ground-state atom with dielectric bodies

Within leading-order perturbation theory, the Casimir-Polder potential of a ground-state atom placed within an arbitrary arrangement of dispersing and absorbing linear bodies can be expressed in terms of the polarizability of the atom and the scattering Green tensor of the body-assisted electromagnetic field. Based on a Born series of the Green tensor, a systematic expansion of the Casimir-Polder potential in powers of the susceptibilities of the bodies is presented. The Born expansion is used to show how and under which conditions the Casimir-Polder force can be related to microscopic many-atom van der Waals forces, for which general expressions are presented. As an application, the Casimir-Polder potentials of an atom near a dielectric ring and an inhomogeneous dielectric half space are studied and explicit expressions are presented that are valid up to second order in the susceptibility.

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Ground-state van der Waals forces in planar multilayer magnetodielectrics

Within the frame of lowest-order perturbation theory, the van der Waals potential of a ground-state atom placed within an arbitrary dispersing and absorbing magnetodielectric multilayer system is given. Examples of an atom situated in front of a magnetodielectric plate or between two such plates are studied in detail. Special emphasis is placed on the competing attractive and repulsive force components associated with the electric and magnetic matter properties, respectively, and conditions for the formation of repulsive potential walls are given. Both numerical and analytical results are presented.

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Casimir-Polder interaction of atoms with magnetodielectric bodies

A general theory of the Casimir-Polder interaction of single atoms with dispersing and absorbing magnetodielectric bodies is presented, which is based on QED in linear, causal media. Both ground-state and excited atoms are considered. Whereas the Casimir-Polder force acting on a ground-state atom can conveniently be derived from a perturbative calculation of the atom-field coupling energy, an atom in an excited state is subject to transient force components that can only be fully understood by a dynamical treatment based on the body-assisted vacuum Lorentz force. The results show that the Casimir-Polder force can be influenced by the body-induced broadening and shifting of atomic transitions - an effect that is not accounted for within lowest-order perturbation theory. The theory is used to study the Casimir-Polder force of a ground-state atom placed within a magnetodielectric multilayer system, with special emphasis on thick and thin plates as well as a planar cavity consisting of two thick plates. It is shown how the competing attractive and repulsive force components related to the electric and magnetic properties of the medium, respectively, can - for sufficiently strong magnetic properties - lead to the formation of potential walls and wells.

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Electromagnetic-field quantization and spontaneous decay in left-handed media

We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.

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