arXiv subjects

Stephan W. Koch

Publications and source records attributed to Stephan W. Koch.

21 records · Page 2Linked to original sources

arXiv2011

Terahertz excitation of a coherent three-level Λ-type exciton-polariton microcavity mode

Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique Λ-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.

cond-mat.mes-hall↗

arXiv2009

A classical theory for second-harmonic generation from metallic nanoparticles

In this article, we develop a classical electrodynamic theory to study the optical nonlinearities of metallic nanoparticles. The quasi-free electrons inside the metal are approximated as a classical Coulomb-interacting electron gas, and their motion under the excitation of an external electromagnetic field is described by the plasma equations. This theory is further tailored to study second-harmonic generation. Through detailed experiment-theory comparisons, we validate this classical theory as well as the associated numerical algorithm. It is demonstrated that our theory not only provides qualitative agreement with experiments, it also reproduces the overall strength of the experimentally observed second-harmonic signals.

physics.optics↗

arXiv2003

Dynamics of short time--scale energy relaxation of optical excitations due to electron--electron scattering in the presence of arbitrary disorder

A non--equilibrium occupation distribution relaxes towards the Fermi--Dirac distribution due to electron--electron scattering even in finite Fermi systems. The dynamic evolution of this thermalization process assumed to result from an optical excitation is investigated numerically by solving a Boltzmann equation for the carrier populations using a one--dimensional disordered system. We focus on the short time--scale behavior. The logarithmically long time--scale associated with the glassy behavior of interacting electrons in disordered systems is not treated in our investigation. For weak disorder and short range interaction we recover the expected result that disorder enhances the relaxation rate as compared to the case without disorder. For sufficiently strong disorder, however, we find an opposite trend due to the reduction of scattering probabilities originating from the strong localization of the single--particle states. Long--range interaction in this regime produces a similar effect. The relaxation rate is found to scale with the interaction strength, however, the interplay between the implicit and the explicit character of the interaction produces an anomalous exponent.

cond-mat.dis-nn↗