arXiv subjects

Sumiran Pujari

Publications and source records attributed to Sumiran Pujari.

At least 19 recordsLinked to original sources

arXiv2026

Diodes and capacitors for the transport of monopoles in fragmented spin ice

Spin-ice materials are famous for their quasi-particle excitations that behave like magnetic monopoles. Magnetricity is the concept that these monopoles can conduct an AC magnetic current, in analogy with conduction electrons. While monopole dynamics has been intensively studied and is reasonably well understood, very little has been done to design devices in order to control magnetricity. Here we develop a theoretical proof of concept for the design of diodes and capacitors for the transport of monopoles. We use the property of systems with magnetic fragmentation, where spin-ice physics co-exists with long-range antiferromagnetic order. The key point is that magnetic order allows for the existence of domain walls. Under certain conditions of preparation, this domain wall is equivalent to an asymmetric filter for monopoles. In a given direction, positive charges can go through while negative ones are repelled; the opposite applies in the opposite direction. This asymmetry effectively functions like a diode for monopole current. Successive domain walls separate positive from negative charges with a vacuum of charge in between, producing a capacitor for monopoles. Once the capacitor is charged, it can in principle be used as a battery for monopoles. All microscopic mechanisms are explained and our proof of concept is validated by simulations of more than a million spins. Application to experiments are discussed for rare-earth pyrochlore oxides and artificial spin ice. Finally, we discuss in general terms how a domain wall in fragmented spin ice can also be seen as an emergent boundary separating two mirror "worlds" separated by time-reversal symmetry. Beyond spin ice, our work opens a promising direction of investigation for the dynamics of emergent quasi-particles crossing domain walls in chiral and nematic spin liquids, which also possess a broken symmetry.

cond-mat.str-el↗

arXiv2026

Critical SO(5) scaling of entanglement entropy at honeycomb lattice deconfined criticality

The deconfined quantum critical point (DQCP) in square lattice S=1/2 quantum antiferromagnets has been extensively studied with a large body of evidence pointing to a weakly first-order transition scenario. Recent studies, which focused on entanglement at this nearly continuous DQCP in square lattice J-Q models, have observed conflicting bipartite entanglement entropy (EE) scaling behavior. One bipartition choice gave scaling coefficients in remarkable agreement with predictions from the unitary CFT corresponding to the putative DQCP. While another equally natural choice gave scaling coefficients in complete violation of unitary CFT that may be attributed to lack of scale invariance at the known weakly first-order behavior of the model. This motivates the exploration of DQCP behavior via entanglement measures in lattice models with distinct crystalline symmetries. Here we study a S=1/2 honeycomb model that hosts a nearly continuous transition between N\'eel and valence-bond-solid ground states relevant to probing DQCP. Using large-scale quantum Monte Carlo simulations, we compute the R\'enyi EE for a variety of bipartitions and test the CFT based description of the DQCP on the honeycomb lattice. For smooth bipartitions, we find no evidence of logarithmic corrections, in accordance with CFT, thereby essentially ruling out contributions from Goldstone modes. For subsystems with corners, CFT predicts universal logarithmic contributions, which we extract for corners with 60 and 120 degree angles and find close agreement with an emergent SO(5) CFT. While we observe scaling consistent with a critical system in the majority of cases, we also demonstrate an intriguing counterexample of the hexagon subsystem that exhibits a subtle period three oscillation. This results in three separate finite-size series, where the sign of the logarithmic term apparently changes depending on the series.

cond-mat.str-el↗

arXiv2026

Toric code made subsystem: a framework for topological subsystem codes using anticommuting quantum spin liquids

We introduce a framework of constructing topological subsystem codes based on the class of anticommuting quantum spin liquids described in [Phys. Rev. B 113, 064402 (2026)]. A canonical model from this class can be considered as a spatial modification of the toric code that voids its stabilizer code property. Rather, these models contain an extensive set of anticommuting local conserved operators that lead to an extensive ground state degeneracy. This degeneracy forms the basis of the subsystem degrees of freedom in the associated quantum error correcting code. The code inherits the many-body topological order of the quantum spin liquid, making it a topological subsystem code. We present two concrete and detailed examples for constructing these codes on a square lattice and a kagome lattice geometry, requiring weight-4 and weight-3 local check operator measurements respectively. In contrast to other subsystem codes, a unique property of these codes is the presence of an extensive number of local gauge qubits that are left undisturbed by the check operators apart from the logical qubits. Our construction provides a template for generating this new category of topological subsystem codes on different lattice or graph geometries, suitable for implementation on various quantum hardware platforms.

cond-mat.str-el↗

arXiv2025

Pseudocriticality in antiferromagnetic spin chains

Weak first-order pseudocriticality with approximate scale invariance has been observed in a variety of settings, including the intriguing case of deconfined criticality in 2+1 dimensions. Recently, this has been interpreted as extremely slow flows ("walking behavior") for real-valued couplings in proximity to a bona fide critical point with complex-valued couplings, described by a complex conformal field theory (CFT). Here we study an SU($N$) generalization of the the Heisenberg antiferromagnet, which is a familiar model for deconfined criticality in 2+1 dimensions. We show that in 1+1 dimensions the model is located near a complex CFT, whose proximity can be tuned as a function of $N$. We employ state-of-the-art quantum Monte Carlo simulations for continuous $N$ along with an improved loop estimator for the R\'{e}nyi entanglement entropy based on a nonequilibrium work protocol. These techniques allow us to track the central charge of this model in detail as a function of $N$, where we observe excellent agreement with CFT predictions. Notably, this includes the region $N>2$, where the CFT moves into the complex plane and pseudocritical drifts enable us to recover the real part of the complex central charge with remarkable accuracy. Since the present model with $N=3$ is also equivalent to the spin-1 biquadratic model, our work sheds new light on the dimerized phase of the spin-1 chain, demonstrating that it is pseudocritical and proximate to a complex CFT.

cond-mat.str-el↗

arXiv2025

{\guillemotleft}Anticommuting{\guillemotright} $\mathbb{Z}_2$ quantum spin liquids

We discuss a class of lattice $S=\frac{1}{2}$ quantum Hamiltonians with bond-dependent Ising couplings and a mutually {\guillemotleft}anticommuting{\guillemotright} algebra of extensively many local $\mathbb{Z}_2$ conserved charges that was explicated in [arXiv:2407.06236]. This mutual algebra is reminiscent of the spin-$\frac{1}{2}$ Pauli matrix algebra but encoded in the structure of \emph{local conserved charges}. These models have finite residual entropy density in the ground state with a simple but non-trivial degeneracy counting and concomitant quantum spin liquidity as proved in [arXiv:2407.06236]. The spin liquidity relies on a geometrically site-interlinked character of the local conserved $\mathbb{Z}_2$ charges that is rather natural in presence of an {\guillemotleft}anticommuting{\guillemotright} structure, as opposed to for example the bond-interlinked character of the local conserved $\mathbb{Z}_2$ hexagonal plaquette charges of the Kitaev honeycomb spin-$\frac{1}{2}$ model which leads to a mutually commuting local algebra. In this work, we make several exact statements on the many-body order that can be present within the class of {\guillemotleft}anticommuting{\guillemotright} quantum spin liquids. We elucidate the differences between the many-body order in these models and that found in some gapped quantum spin liquids with mutually commuting local algebras, e.g. the Kitaev toric code or Levin-Wen models. We also point out a mutually commuting algebra with local support that are naturally expressed as multi-linear Majorana forms in the Kitaev representation of these quantum spin liquids. They capture non-trivial quantum resonances throughout the lattice in these {\guillemotleft}anticommuting{\guillemotright} $\mathbb{Z}_2$ quantum spin liquid Hamiltonians.

cond-mat.str-el↗

arXiv2024

Rational Control of Magnonic and Electronic Band Splittings

We provide a theoretical demonstration of controllable non-relativistic spin splitting in both electronic and magnonic bands via targeted structural distortions tied to specific phonon modes. Using MnF$_2$ as a model system, we identify a $d$-wave magnon band splitting between magnon modes of specific handedness, directly correlated with the non-relativistic spin splitting observed in the electronic structure. Crucially, we show that structural distortions associated with the A$_{2u}$ and A$_{1g}$ phonon modes (8.52 and 9.74 THz) modulate these splittings without altering the antiferromagnetic order. The effect originates from changes in the nonmagnetic ligand environment, highlighting the key role of lattice degrees of freedom in governing spin dynamics. Our findings establish a novel route for structure-mediated control of spin splitting, opening possibilities for tunable magnonic and spintronic functionalities in antiferromagnetic materials.

cond-mat.mtrl-sci↗

arXiv2024

Tomonaga-Luttinger liquid and quantum criticality in spin-1/2 antiferromagnetic Heisenberg chain C14H18CuN4O10 via Wilson ratio

The ground state of a one-dimensional spin-1/2 uniform antiferromagnetic Heisenberg chain (AfHc) is a Tomonaga-Luttinger liquid which is quantum-critical with respect to applied magnetic fields upto a saturation field Hs beyond which it transforms to a fully polarised state. Wilson ratio has been predicted to be a good indicator for demarcating these phases [Phys. Rev. B 96, 220401 (2017)]. From detailed temperature and magnetic field dependent magnetisation, magnetic susceptibility and specific heat measurements in a metalorganic complex and comparisons with field theory and quantum transfer matrix method calculations, the complex was found to be a very good realisation of a spin-1/2 AfHc. Wilson ratio obtained from experimentally obtained magnetic susceptibility and magnetic contribution of specific heat values was used to map the magnetic phase diagram of the uniform spin-1/2 AfHc over large regions of phase space demarcating Tomonaga-Luttinger liquid, saturation field quantum critical, and fully polarised states. Luttinger parameter and spinon velocity were found to match very well with the values predicted from conformal field theory.

cond-mat.str-el↗

arXiv2024

Transverse resistance due to electronic inhomogeneities in superconductors

Phase transitions in many-body systems are often associated with the emergence of spatial inhomogeneities. Such features may develop at microscopic lengthscales and are not necessarily evident in measurements of macroscopic quantities. In this work, we address the topic of distribution of current paths in superconducting films. Typical lengthscales associated with superconductivity are in the range of nanometres. Accordingly, measurements of electrical resistance over much larger distances are supposed to be insensitive to details of spatial inhomogeneities of electronic properties. We observe that, contrary to expectations, current paths adopt a highly non-uniform distribution at the onset of the superconducting transition which is manifested in the development of a finite transverse resistance. The anisotropic distribution of current density is unrelated to the structural properties of the superconducting films, and indicates the emergence of electronic inhomogeneities perceivable over macroscopic distances. Our experiments reveal the ubiquitous nature of this phenomenon in conventional superconductors.

cond-mat.supr-con↗

arXiv2024

A theorem on extensive ground state entropy, spin liquidity and some related models

An exact mechanism is written down to guarantee extensive residual ground state entropy and spin liquidity in spin-1/2 lattice models with bond-dependent couplings. It is based on the presence of extensively large and mutually non-commuting (``\guillemotleft anticommuting\guillemotright'') sets of local conserved quantities with a gauge-like character. This mutual algebra is similar to those of spin-1/2 degrees of freedom however arising in the structure of local conserved charges whose support is not restricted to a single lattice site. The general theorem is first pedagogically illustrated through a variant of the familiar one-dimensional quantum Ising model featuring such an \guillemotleft anticommuting\guillemotright$~$structure. This leads to classical spin liquidity co-existing with quantum Ising order. The rest of the paper is then devoted to applications in higher dimensions with more general \guillemotleft anticommuting\guillemotright$~$structures which voids spin or magnetic ordering altogether. Proofs of the resultant quantum spin liquidity are given through an analysis of static and dynamic $n$-point spin correlators relying solely on the \guillemotleft anticommuting\guillemotright$~$algebraic structure of the constructed models. It is not evident if they admit exact solutions using known techniques. The precise nature of these quantum spin liquids is thus an open question including the existence of a quasiparticle description for these models. We compare and contrast them with other well-known quantum spin liquids.

cond-mat.stat-mech↗

arXiv2024

A solvable embedding mechanism for one-dimensional spinless and Majorana fermions in higher-dimensional spin-1/2 magnets

We write down a class of two-dimensional quantum spin-1/2 Hamiltonians whose eigenspectra are exactly solvable via the Jordan-Wigner transformation. The general structure corresponds to a suitable grid composed of XY or XX-Ising spin chains and ZZ-Ising spin chains and is generalizable to higher dimensions. They can host stacks of one-dimensional spinless fermion liquids with gapless excitations and power-law correlations coexisting with ordered spin moments (localized spinless fermions). Bond-dependent couplings thus can be an alternate mechanism than geometric frustration of SU(2)-symmetric couplings to obtain spinless fermionic excitations. Put in a different way, bond-dependent couplings allow for an embedding of one-dimensional spinless fermion (Tomonoga-Luttinger) liquids and solids and also Majorana excitations in higher dimensions. They can accommodate a simpler set of site-local conserved quantities apart from the more intricate, interlocked set of plaquette-local or bond-local conserved quantities in Kitaev's honeycomb model with Majorana excitations. The proposed grid structure may provide an architecture for quantum engineering with controllable qubits.

cond-mat.str-el↗

arXiv2024

A Class of Exactly Solvable Hamiltonians for S=1/2 Quantum Magnets with Spinless Fermionic Excitations in Higher Dimensions

This contribution summarizes the main results of a work on exactly solvable Hamiltonians for quantum magnets. A class of Hamiltonians which supports fractionalized spinless fermionic excitations in dimensions greater than one is written down. A well-known one-dimensional example is that of S=1/2 spin chains with Luttinger liquid physics and spinless fermionic excitations that are also called spinons. A well-known two-dimensional example is that of Kitaev's S=1/2 honeycomb model with bond-dependent magnetic couplings which supports Majorana fermionic excitations. The class of models to be discussed here also exploits bond-dependent couplings in a different way to non-perturbatively stabilize spinless fermionic spinons and also Majorana fermions. A more detailed account of these results is being prepared for publication elsewhere.

cond-mat.str-el↗

arXiv2024

(H,Li)$_{6}$Ru$_{2}$O$_{6}$ : a possible zero-field Ru$^{3+}$-based Kitaev Quantum Spin Liquid

We report the synthesis and properties of (H,Li)$_{6}$Ru$_{2}$O$_{6}$, which is shown to be a $J_{\text{eff}}=\frac{1}{2}$ system made out of Ru$^{3+}$ moments in a honeycomb geometry. Bulk magnetization, heat capacity, nuclear magnetic resonance (NMR), and muon spin relaxation ($\mu$SR) rule out the presence of static moments or any spin glass phase down to 84 mK. All techniques suggest a crossover to a liquid-like state below about 40 K. The $^{7}$Li nuclear magnetic resonance (NMR) shift data suggest a non-zero $T$-independent spin susceptibility at low $T$. In zero field, $C_m/T$ shows $T^{-0.9}$ divergence which is consistent with vacancy-induced effects on low-energy excitations of the pristine Kitaev spin liquid. With field, power-law variations in the $^{7}$Li NMR spin-lattice relaxation rate 1/T$_{1}$ and magnetic heat capacity $C_{m}$ show quantitatively new scaling behaviors. A two-step entropy release in heat capacity is also observed putatively from $Z_{2}$ flux (low-$T$ step) and itinerant Majorana fermions (high-$T$ step). Based on these findings, we propose that (H,Li)$_{6}$Ru$_{2}$O$_{6}$ realizes a Kitaev spin liquid with no evidence of inherent magnetic ordering in zero field unlike $\alpha$-RuCl$_{3}$ where approximately $8$ Tesla field is required to suppress magnetic order.

cond-mat.str-el↗

arXiv2023

Deconfined pseudocriticality in a model spin-1 quantum antiferromagnet

Berry phase interference arguments that underlie the theory of deconfined quantum criticality (DQC) for spin-$\frac{1}{2}$ antiferromagnets have also been invoked to allow for continuous transitions in spin-1 magnets including a N\'eel to (columnar) valence bond solid (cVBS) transition. We provide a microscopic model realization of this transition on the square lattice consisting of Heisenberg exchange ($J_H$) and biquadratic exchange ($J_B$) that favor a N\'eel phase, and a designed $Q$-term ($Q_B$) interaction which favors a cVBS through large-scale quantum Monte Carlo (QMC) simulations. For $J_H=0$, this model is equivalent to the $SU(3)$ $JQ$ model with a N\'eel-cVBS transition that has been argued to be DQC through QMC. Upon turning on $J_H$ which brings down the symmetry to $SU(2)$, we find multiple signatures -- a single critical point, high quality collapse of correlation ratios and order parameters, "$U(1)$-symmetric" cVBS histograms and lack of double-peak in order parameter histograms for largest sizes studied near the critical point -- that are highly suggestive of a continuous transition scenario. However, Binder analysis finds negative dips that grow sub-extensively that we interpret as these transitions rather being pseudocritical. This along with recent results on spin-$\frac{1}{2}$ models suggests that deconfined pseudocriticality is the more generic scenario.

cond-mat.str-el↗

arXiv2023

Decoupling Nuclear Spins via Interaction-Induced Freezing in Nitrogen Vacancy Centers in Diamond

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol for an NV center to isolate its intrinsic nuclear spin from a noisy electromagnetic environment. Any initial state of the nuclear spin can be frozen when the hyperfine-coupled electron and nuclear spins are simultaneously driven with unequal Rabi frequencies. Through numerical simulations, we show that our protocol can effectively shield the nuclear spin from strong drive or noise fields. We also observe a clear suppression of quantum correlations in the frozen nuclear spin regime by measuring the quantum discord of the electron-nuclear spin system. These features can be instrumental in extending the storage times of NV nuclear-spin based quantum memories in hybrid quantum systems.

quant-ph↗

arXiv2022

Punctured-Chern topological invariants for semi-metallic bandstructures

Topological insulator-based methods underpin the topological classification of gapped bands, including those surrounding semi-metallic nodal defects. However, multiple bands with gap-closing points can also possess non-trivial topology. We construct a general wavefunction-based ``punctured-Chern" invariant to capture such topology. To show its general applicability, we analyze two systems with disparate gapless topology: 1) a recent two-dimensional fragile topological model to capture the various band-topological transitions and 2) a three-dimensional model with a triple-point nodal defect to characterize its semi-metallic topology with \emph{half-integers} that govern physical observables such as anomalous transport. This invariant also gives the classification for Nexus triple-points ($\mathbb{Z}\times\mathbb{Z}$) with certain symmetry restrictions, which is re-confirmed by abstract algebra.

cond-mat.mes-hall↗

arXiv2022

Role of Majorana Fermions in high-harmonic generation from Kitaev chain

The observation of Majorana fermions as collective excitations in condensed-matter systems is an ongoing quest, and several state-of-the-art experiments have been performed in the last decade. As a potential avenue in this direction, we simulate the high-harmonic spectrum of Kitaev's superconducting chain model that hosts Majorana edge modes in its topological phase. It is well-known that this system exhibits a topological--trivial superconducting phase transition. We demonstrate that high-harmonic spectroscopy is sensitive to the phase transition in presence of open boundary conditions due to the presence or absence of these edge modes. The population dynamics of the Majorana edge modes are different from the bulk modes, which is the underlying reason for the distinct harmonic profile of both the phases. On the contrary, in presence of periodic boundary conditions with only bulk modes, high-harmonic spectroscopy becomes insensitive to the phase transition with similar harmonic profiles in both phases.

cond-mat.str-el↗

arXiv2022

Notes on resummation-based quantum Monte Carlo vis-à-vis sign-problematic Heisenberg models on canonical geometrically frustrated lattices

We show here that a direct application of resummation-based quantum Monte Carlo (QMC) -- implemented recently for sign-problem-free SU(2)-symmetric Hamiltonians in the stochastic series expansion (SSE) framework -- does not reduce the sign problem for frustrated SU(2)-symmetric Heisenberg antiferromagnets on canonical geometrically frustrated lattices composed of triangular motifs such as the triangular lattice. In the process, we demonstrate that resummation-based updates do provide an ergodic sampling of the SSE-based QMC configurations which can be an issue when using the standard SSE updates, however, severely limited by the sign problem as previously mentioned. The notions laid out in these notes may be useful in the design of better algorithms for geometrically frustrated magnets.

cond-mat.str-el↗

arXiv2021

Resummation-based updates for Stochastic Series Expansion Quantum Monte Carlo

For spin rotational symmetric models with a positive-definite high-temperature expansion of the partition function, a stochastic sampling of the series expansion upon partial resummation becomes logically equivalent to sampling an uncoloured closely-packed loop-gas model in one higher dimension. Based on this, we devise quantum Monte Carlo updates that importance-sample loop configurations for general $SU(N)$ in fundamental and higher-symmetric representations. The algorithmic performance systematically improves with increase in (continuous) $N$ allowing efficient simulation of quantum paramagnets. The underlying reason for the increased efficacy is the correspondence of quantum paramagnetic phases like valence bond solids to short-loop phases on the loop-gas side rather than the particular value of $N$. This also gives a connection between Sandvik's $JQ$ model class and classical loop-gas models in the deconfined universality class.

cond-mat.str-el↗