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Susumu Minami

Publications and source records attributed to Susumu Minami.

14 recordsLinked to original sources

Topological transition and emergent elasticity of dislocation in skyrmion lattice: Beyond Kittel's magnetic-polar analogy

Magnetic and polar skyrmions exhibit topologically protected quasiparticle behavior, including emergent fields, deformation, and the formation of a densely packed skyrmion lattice, beyond conventional domain configurations described by Kittel's law. Analogous to atomic crystals, lattice defects, especially dislocations and their associated strain fields, are crucial for understanding the lattice behavior of skyrmions; however, their features and roles remain insufficiently understood. Here, we show that magnetic skyrmion dislocations develop a core-split structure due to a significant skyrmion elongation up to 180% of their original length, reaching a topological transition from a single skyrmion to two half-skyrmions. Despite such a distinct structure, the long-range strain fields around the dislocation perfectly obey conventional Volterra's elasticity theory, in contrast to polar skyrmion lattices, where skyrmion deformations cause a breakdown of the elasticity theory. Furthermore, an energetic analysis shows that Dzyaloshinskii-Moriya interaction drives the large skyrmion deformation of the dislocation core. Our findings not only clarify the coexistence of topological core-reconstruction and a robust long-range elastic field of dislocations in magnetic skyrmion lattices, but also reveal that magnetic and electric domains, long regarded as dual and analogous, exhibit fundamental differences when extended into the regime of collective topological quasiparticles.

cond-mat.mtrl-sci

Ab initio study of magnetoresistance effect in $\mathrm{Mn_{3}Sn}/\mathrm{MgO}/\mathrm{Mn_{3}Sn}$ antiferromagnetic tunnel junction

The antiferromagnets with the time-reversal symmetry broken magnetic structures possess a finite spin splitting in the momentum space, and may contribute to a realization of a finite tunnel magnetoresistance (TMR) effect even with magnets with zero net spin polarization. In this paper, we study the TMR effect with the noncollinear antiferromagnet $\mathrm{Mn_{3}Sn}$ whose inverse $120^{\circ}$ antiferromagnetic order breaks the time-reversal symmetry. In particular, we employ the representative barrier material $\mathrm{MgO}$ as the tunnel insulator, and calculate the TMR effect in the $\mathrm{Mn_{3}Sn}(01\bar{1}0)/\mathrm{MgO}(110)/\mathrm{Mn_{3}Sn}$ magnetic tunnel junctions (MTJs), which has an optimal geometry for the spin-orbit torque switching of the magnetic configurations. We show that a finite TMR ratio reaching $\gtrsim 1000\%$ appears in the $\mathrm{Mn_{3}Sn}/\mathrm{MgO}/\mathrm{Mn_{3}Sn}$ MTJs, which is due to the spin splitting properties of $\mathrm{Mn_{3}Sn}$ in the momentum space combined with the screening effect of $\mathrm{MgO}$.

cond-mat.mes-hall

Topological Electronic Structure and Transport Properties of the Distorted Rutile-type WO$_2$

We elucidate the transport properties and electronic structures of distorted rutile-type WO2. Electrical resistivity and Hall effect measurements of high-quality single crystals revealed the transport property characteristics of topological materials; these characteristics included an extremely large magnetoresistance of 13,200% (2 K and 9 T) and a very high carrier mobility of 25,700 cm2 V-1 s-1 (5 K). First-principles calculations revealed Dirac nodal lines (DNL) near the Fermi energy in the electronic structure when spin-orbit interactions (SOIs) were absent. Although these DNLs mostly disappeared in the presence of SOIs, band crossings at high-symmetry points in the reciprocal space existed as Dirac points. Furthermore, DNLs protected by nonsymmorphic symmetry persisted on the ky = π/b plane. The unique transport properties originating from the topological electronic structure of chemically and thermally stable WO2 could represent an opportunity to investigate the potential electronic applications of the material.

cond-mat.mtrl-sci

Large anomalous Nernst effect in the ferromagnetic Fe3Si polycrystal

The high-throughput calculation predicts that the Fe-based cubic ferromagnet Fe$_3$Si may exhibit a large anomalous Nernst effect (ANE). Here, we report our experimental observation of the large Nernst coefficient $S_{yx}\sim$2 $μ$V/K and the transverse thermoelectric coefficient $-α_{yx}$ $\sim$ 3 Am$^{-1}$K$^{-1}$ for Fe$_3$Si polycrystal at room temperature. The large $-α_{yx}$ indicates that the large ANE originates from the intrinsic Berry curvature mechanism. The high Curie temperature of 840 K and the most abundant raw elements of Fe and Si make Fe$_3$Si a competitive candidate for Nernst thermoelectric generations.

cond-mat.mtrl-sci

High-throughput calculations of antiferromagnets hosting anomalous transport phenomena

We develop a high-throughput computational scheme based on cluster multipole theory to identify new functional antiferromagnets. This approach is applied to 228 magnetic compounds listed in the AtomWork-Adv database, known for their elevated Néel temperatures. We conduct systematic investigations of both stable and metastable magnetic configurations of these materials. Our findings reveal that 34 of these compounds exhibit antiferromagnetic structures with zero propagation vectors and magnetic symmetries identical to conventional ferromagnets, rendering them potentially invaluable for spintronics applications. By cross-referencing our predictions with the existing MAGNDATA database and published literature, we verify the reliability of our findings for 26 out of 28 compounds with partially or fully elucidated magnetic structures in the experiments. These results not only affirm the reliability of our scheme but also point to its potential for broader applicability in the ongoing quest for the discovery of new functional magnets.13

cond-mat.mtrl-sci

Electron-doped magnetic Weyl semimetal LixCo3Sn2S2 by bulk-gating

Manipulating carrier density through gate effects, both in electrostatic charge storage and electrochemical intercalation mode, offers powerful control over material properties, although commonly restricted to ultra-thin films or van der Waals materials. Here we demonstrate the application of gate-driven carrier modulation in the microdevice of magnetic Weyl semimetal Co3Sn2S2, fabricated from a bulk single crystal via focused ion beam (FIB). We discovered a Li-intercalated phase LixCo3Sn2S2 featuring electron doping exceeding 5*1021 cm-3, resulting in the Fermi energy shift of 200 meV. The carrier density dependent anomalous Hall conductivity shows fair agreement with density functional theory (DFT) calculation, which also predicts intercalated Li+ ion stabilization within the anion layer while maintaining the kagome-lattice intact. This likely explains the observed rigid band behavior and constant Curie temperature, contrasting with magnetic site substitution experiments. Our findings suggest ionic gating on FIB devices broadens the scope of gate-tuning in quantum materials.

cond-mat.mtrl-sci

Maximizing intrinsic anomalous Hall effect by controlling the Fermi level in simple Weyl semimetal films

Large intrinsic anomalous Hall effect (AHE) originating in the Berry curvature has attracted growing attention for potential applications. Recently proposed magnetic Weyl semimetal EuCd$_2$Sb$_{\mathrm{2}}$ provides an excellent platform for controlling the intrinsic AHE because it only hosts a Weyl-points related band structure near the Fermi energy. Here we report the fabrication of EuCd$_2$Sb$_{\mathrm{2}}$ single-crystalline films and control of their anomalous Hall effect by film technique. As also analyzed by first-principles calculations of energy-dependent intrinsic anomalous Hall conductivity, the obtained anomalous Hall effect shows a sharp peak as a function of carrier density, demonstrating clear energy dependence of the intrinsic AHE.

cond-mat.str-el

First-principles calculation of anomalous Hall and Nernst conductivity by local Berry phase

In this study, we implemented a finite-difference algorithm for computing anomalous Hall and Nernst conductivity. Based on the expression to evaluate the Berry curvature in an insulating system [J. Phys. Soc. Jpn. 74 1674(2005)], we extended the methods to a metallic system. We calculated anomalous Hall conductivity and Nernst conductivity in a two-dimensional ferromagnetic material FeCl$_2$ and three-dimensional ferromagnetic transition metals bcc-Fe, hcp-Co, and fcc-Ni. Our results are comparable to previously reported results computed by Kubo-formula or Wannier representation. To evaluate anomalous Nernst coefficients, the detailed Fermi-energy dependence of the anomalous Hall conductivity is required. Nonetheless, previous methods based on Wannier representation or Kubo-formula have numerical instability due to the ${\boldsymbol k}$-space Dirac monopole. The present method will open an efficient thermoelectric material design based on the high-throughput first-principles screening.

cond-mat.mtrl-sci

Large anomalous Hall effect induced by weak ferromagnetism in the noncentrosymmetric antiferromagnet $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$

We study the mechanism of the exceptionally large anomalous Hall effect (AHE) in the noncentrosymmetric antiferromagnet $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ by angle-resolved photoemission spectroscopy (ARPES) and magnetotransport measurements. From ARPES measurements of $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ and its family compounds ($\mathrm{Fe}\mathrm{Nb}_3\mathrm{S}_6$ and $\mathrm{Ni}\mathrm{Nb}_3\mathrm{S}_6$), we find a band dispersion unique to the Co intercalation existing near the Fermi level. We further demonstrate that a slight deficiency of sulfur in $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ eliminates the ferromagnetism and the AHE simultaneously while hardly changing the band structure, indicating that the weak ferromagnetism is responsible for the emergence of the large AHE. Based on our results, we propose Weyl points near the Fermi level to cause the large AHE.

cond-mat.mtrl-sci

Logarithmic Criticality in Transverse Thermoelectric Conductivity of the Ferromagnetic Topological Semimetal CoMnSb

We report the results of our experimental studies on the magnetic, transport and thermoelectric properties of the ferromagnetic metal CoMnSb. Sizable anomalous Hall conductivity $σ_{yx}$ and transverse thermoelectric conductivity $α_{yx}$ are found experimentally and comparable in size to the values estimated from density-functional theory. Our experiment further reveals that CoMnSb exhibits $-T\ln T$ critical behavior in $α_{yx}(T)$, deviating from Fermi liquid behavior $α_{yx}\sim T$ over a decade of temperature between 10 K to 400 K, similar to ferromagnetic Weyl and nodal-line semimetals. Our theoretical calculation for CoMnSb also predicts the $-T\ln T$ behavior when the Fermi energy locates near the Weyl nodes in momentum space.

cond-mat.mtrl-sci

Quantum transport observed in films of magnetic topological semimetal EuSb$_2$

We report fabrication of EuSb$_2$ single-crystalline films and investigation of their quantum transport. First-principles calculations demonstrate that EuSb$_2$ is a magnetic topological nodal-line semimetal protected by nonsymmorphic symmetry. Observed Shubnikov-de Haas oscillations with multiple frequency components exhibit small effective masses and two-dimensional field-angle dependence even in a 250 nm thick film, further suggesting possible contributions of surface states. This finding of the high-mobility magnetic topological semimetal will trigger further investigation of exotic quantum transport phenomena by controlling magnetic order in topological semimetal films.

cond-mat.mtrl-sci

Anomalous transport due to Weyl fermions in the chiral antiferromagnets Mn$_3$$X$, $X$ = Sn, Ge

The recent discoveries of strikingly large zero-field Hall and Nernst effects in antiferromagnets Mn$_3$$X$, ($X$ = Sn, Ge) have brought the study of magnetic topological states to the forefront of condensed matter research and technological innovation. These effects are considered fingerprints of Weyl nodes residing near the Fermi energy, promoting Mn$_3$$X$, ($X$ = Sn, Ge) as a fascinating platform to explore the elusive magnetic Weyl fermions. In this review, we provide recent updates on the insights drawn from experimental and theoretical studies of Mn$_3$$X$, ($X$ = Sn, Ge) by combining previous reports with our new, comprehensive set of transport measurements of high-quality Mn$_3$Sn and Mn$_3$Ge single crystals. In particular, we report magnetotransport signatures specific to chiral anomalies in Mn$_3$Ge and planar Hall effect in Mn$_3$Sn, which have not yet been found in earlier studies. The results summarized here indicate the essential role of magnetic Weyl fermions in producing the large transverse responses in the absence of magnetization.

cond-mat.mtrl-sci

Enhancement of transverse thermoelectric conductivity originating from stationary points in nodal line

Motivated by the recent discovery of a large anomalous Nernst effect in Co$_2$MnGa, Fe$_3X$ ($X$=Al, Ga) and Co$_3$Sn$_2$S$_2$, we performed a first-principles study to clarify the origin of the enhancement of the transverse thermoelectric conductivity ($α_{ij}$) in these ferromagnets. The intrinsic contribution to $α_{ij}$ can be understood in terms of the Berry curvature ($Ω$) around the Fermi level, and $Ω$ is singularly large along nodal lines (which are gapless in the absence of the spin-orbit coupling) in the Brillouin zone. We find that not only the Weyl points but also stationary points in the energy dispersion of the nodal lines play a crucial role. The stationary points make sharp peaks in the density of states projected onto the nodal line, clearly identifying the characteristic Fermi energies at which $α_{ij}$ is most dramatically enhanced. We also find that $α_{ij}/T$ breaks the Mott relation and show a peculiar temperature dependence at these energies. The present results suggest that the stationary points will give us a useful guiding principle to design magnets showing a large anomalous Nernst effect.

cond-mat.mtrl-sci

First-principles study on thermoelectric properties of half-Heusler compounds CoMSb(M=Sc, Ti, V, Cr, and Mn)

We have performed systematic density functional calculations and evaluated thermoelectric properties, See- beck coefficient and anomalous Nernst coefficient of half-Heusler comounds CoMSb(M=Sc, Ti, V, Cr, and Mn). The carrier concentration dependence of Seebeck coefficients in nonmagnetic compounds are in good agreement with experimental values. We found that the half-metallic ferromagnetic CoMnSb show large anomalous Nernst effect originating from Berry curvature at the Brillouin zone boundary. These results help to understanding for the mechanism of large anomalous Nernst coefficient and give us a clue to design high performance magnetic thermoelectric materials.

cond-mat.mtrl-sci