arXiv subjects

Sven Höfling

Publications and source records attributed to Sven Höfling.

At least 181 records · Page 10Linked to original sources

arXiv2017

Relaxation Oscillations and Ultrafast Emission Pulses in a Disordered Expanding Polariton Condensate

Semiconductor microcavities are often influenced by structural imperfections, which can disturb the flow and dynamics of exciton-polariton condensates. Additionally, in exciton-polariton condensates there is a variety of dynamical scenarios and instabilities, owing to the properties of the incoherent excitonic reservoir. We investigate the dynamics of an exciton-polariton condensate which emerges in semiconductor microcavity subject to disorder, which determines its spatial and temporal behaviour. Our experimental data revealed complex burst-like time evolution under non-resonant optical pulsed excitation. The temporal patterns of the condensate emission result from the intrinsic disorder and are driven by properties of the excitonic reservoir, which decay in time much slower with respect to the polariton condensate lifetime. This feature entails a relaxation oscillation in polariton condensate formation, resulting in ultrafast emission pulses of coherent polariton field. The experimental data can be well reproduced by numerical simulations, where the condensate is coupled to the excitonic reservoir described by a set of rate equations. Theory suggests the existence of slow reservoir temporarily emptied by stimulated scattering to the condensate, generating ultrashort pulses of the condensate emission.

cond-mat.quant-gas↗

arXiv2017

Prototype of a bistable polariton field-effect transistor switch

Microcavity exciton polaritons are promising candidates to build a new generation of highly nonlinear and integrated optoelectronic devices. Such devices range from novel coherent light emitters to reconfigurable potential landscapes for electro-optical polariton-lattice based quantum simulators as well as building blocks of optical logic architectures. Especially for the latter, the strongly interacting nature of the light-matter hybrid particles has been used to facilitate fast and efficient switching of light by light, something which is very hard to achieve with weakly interacting photons. We demonstrate here that polariton transistor switches can be fully integrated in electro-optical schemes by implementing a one-dimensional polariton channel which is operated by an electrical gate rather than by a control laser beam. The operation of the device, which is the polariton equivalent to a field-effect transistor, relies on combining electro-optical potential landscape engineering with local exciton ionization to control the scattering dynamics underneath the gate. We furthermore demonstrate that our device has a region of negative differential resistance and features a completely new way to create bistable behavior.

cond-mat.mes-hall↗

arXiv2017

Cascaded emission of single photons from the biexciton in monolayered WSe2

Monolayers of transition metal dichalcogenide materials emerged as a new material class to study excitonic effects in solid state, since they benefit from enormous coulomb correlations between electrons and holes. Especially in WSe2, sharp emission features have been observed at cryogenic temperatures, which act as single photon sources . Tight exciton localization has been assumed to induce an anharmonic excitation spectrum, however, the evidence of the hypothesis, namely the demonstration of a localized biexciton, is elusive. Here, we unambiguously demonstrate the existence of a localized biexciton in a monolayer of WSe2, which triggers an emission cascade of single photons. The biexciton is identified by its time-resolved photoluminescence, superlinearity and distinct polarization in micro-photoluminescence experiments. We evidence the cascaded nature of the emission process in a cross-correlation experiment, which yields a strong bunching behavior. Our work paves the way to a new generation of quantum optics experiments with two-dimensional semiconductors.

cond-mat.mtrl-sci↗

arXiv2017

Experimental verification of the very strong coupling regime in a GaAs quantum well microcavity

When the coupling between light and matter becomes comparable to the energy gap between different excited states they hybridize, leading to the appearance of a rich and complex phenomenology which attracted remarkable interest in recent years. While the mixing between states with different number of excitations, so-called ultrastrong coupling regime, has been observed in various implementations, the effect of the hybridization between different single excitation states, referred to as very strong coupling regime, has remained elusive. In semiconductor quantum wells such a regime is predicted to manifest as a photon-mediated electron-hole coupling leading to different excitonic wavefunctions for the two polaritonic branches when the ratio of the coupling strength to exciton binding energy approaches unity. Here, we verify experimentally the existence of this regime in magneto-optical measurements on a microcavity with 28 GaAs quantum wells, showing that the average electron-hole separation of the upper polariton is significantly increased compared to the bare quantum well exciton Bohr radius. This manifests in a diamagnetic shift around zero detuning that exceeds the shift of the lower polariton by one order of magnitude and the bare quantum well exciton diamagnetic shift by a factor of two. The lower polariton exhibits a diamagnetic shift smaller than expected from the coupling of a rigid exciton to the cavity mode which suggests more tightly bound electron-hole pairs than in the bare quantum well.

cond-mat.quant-gas↗

arXiv2017

Exploring coherence of individual excitons in InAs quantum dots embedded in natural photonic defects: influence of the excitation intensity

The exact optical response of quantum few-level systems depends crucially on the exact choice of the incoming pulse areas. We use four-wave mixing (FWM) spectroscopy to infer the coherent response and dynamics of single InAs quantum dots (QDs) and study their pulse area dependence. By combining atomic force microscopy with FWM hyperspectral imaging, we show that the retrieved FWM signals originate from individual QDs enclosed in natural photonic defects. The optimized light-matter coupling in these defects allows us to perform our studies in a wide range of driving field amplitudes. When varying the pulse areas of the exciting laser pulses the so-called Rabi rotations can be resolved by the two-pulse FWM technique. We investigate these Rabi rotations within two- and three-level systems, both theoretically and experimentally, and explain their damping by the coupling to acoustic phonons. To highlight the importance of the pulse area influence, we show that the phonon-induced dephasing of QD excitons depends on the pulse intensity.

cond-mat.mes-hall↗

arXiv2017

Coherent coupling of individual quantum dots measured with phase-referenced two-dimensional spectroscopy: photon echo versus double quantum coherence

We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and non-rephasing four-wave mixing (FWM) configurations. We emphasize the non-rephasing case, allowing to monitor two-photon coherence dynamics. Respective Fourier transform yields a double quantum 2D FWM map, which is corroborated with its single quantum counterpart, originating from the rephasing sequence. We introduce referencing of the FWM phase with the one carried by the driving pulses, overcoming the necessity of its active-stabilization, as required in 2D spectroscopy. Combining single and double quantum 2D FWM, provides a pertinent tool in detecting and ascertaining coherent coupling mechanisms between individual quantum systems, as exemplified experimentally.

cond-mat.mes-hall↗

arXiv2017

Gate-tunable, normally-on to normally-off memristance transition in patterned LaAlO3/SrTiO3 interfaces

We report gate-tunable memristive switching in patterned LaAlO3/SrTiO3 interfaces at cryogenic temperatures. The application of voltages in the order of a few volts to the back gate of the device allows controlling and switching-on and -off the inherent memory functionality (memristance). For large and small gate voltages a simple non-linear resistance characteristic is observed while a pinched hysteresis loop and memristive switching occurs in an intermediate voltage range. The memristance is further controlled by the density of oxygen vacancies, which is tuned by annealing the sample at 300 °C in nitrogen atmosphere. Depending on the annealing time the memristance at zero gate voltage can be switched on and off leading to normally-on and normally-off memristors. The presented device offers reversible and irreversible control of memristive characteristics by gate voltages and annealing, respectively, which may allow to compensate fabrication variabilities of memristors that complicate the realization of large memristor-based neural networks.

cond-mat.mes-hall↗

arXiv2017

Substrate engineering for high quality emission of free and localized excitons from atomic monolayers in hybrid architectures

Atomic monolayers represent a novel class of materials to study localized and free excitons in two dimensions and to engineer optoelectronic devices based on their significant optical response. Here, we investigate the role of the substrate on the photoluminescense response of MoSe$_2$ and WSe$_2$ monolayers exfoliated either on SiO$_2$ or epitaxially grown InGaP substrates. In the case of MoSe$_2$, we observe a significant qualitative modification of the emission spectrum, which is widely dominated by the trion resonance on InGaP substrates. However, the effects of inhomogeneous broadening of the emission features are strongly reduced. Even more strikingly, in sheets of WSe$_2$, we could routinely observe emission lines from localized excitons with linewidths down to the resolution limit of 70\,$μ$ eV. This is in stark contrast to reference samples featuring WSe$_2$ monolayers on SiO$_2$ surfaces, where the emission spectra from localized defects are widely dominated by spectral diffusion and blinking behaviour. Our experiment outlines the enormous potential of III-V-monolayer hybrid architectures to obtain high quality emission signals from atomic monolayers, which are straight forward to integrate into nanophotonic and integrated optoelectronic devices.

cond-mat.mes-hall↗

arXiv2016

Deterministic implementation of a bright, on-demand single photon source with near-unity indistinguishability via quantum dot imaging

Deterministic techniques enabling the implementation and engineering of bright and coherent solid-state quantum light sources are key for the reliable realization of a next generation of quantum devices. Such a technology, at best, should allow one to significantly scale up the number of implemented devices within a given processing time. In this work, we discuss a possible technology platform for such a scaling procedure, relying on the application of nanoscale quantum dot imaging to the pillar microcavity architecture, which promises to combine very high photon extraction efficiency and indistinguishability. We discuss the alignment technology in detail, and present the optical characterization of a selected device which features a strongly Purcell-enhanced emission output. This device, which yields an extraction efficiency of $η=(49\pm4)~\%$, facilitates the emission of photons with $(94\pm2.7)~\%$ indistinguishability.

physics.optics↗

arXiv2016

Transition from Jaynes-Cummings to Autler-Townes ladder in a quantum dot-microcavity system

We study experimentally and theoretically a coherently-driven strongly-coupled quantum dot-microcavity system. Our focus is on physics of the unexplored intermediate excitation regime where the resonant laser field dresses a strongly-coupled single exciton-photon (polariton) system resulting in a ladder of laser-dressed Jaynes-Cummings states. In that case both the coupling of the emitter to the confined light field of the microcavity and to the light field of the external laser are equally important, as proved by observation of injection pulling of the polariton branches by an external laser. This intermediate interaction regime is of particular interest since it connects the purely quantum mechanical Jaynes-Cummings ladder and the semi-classical Autler-Townes ladder. Exploring the driving strength-dependence of the mutually coupled system we establish the maximum in the resonance fluorescence signal to be a robust fingerprint of the intermediate regime and observe signatures indicating the laser-dressed Jaynes-Cummings ladder. In order to address the underlying physics we excite the coupled system via the matter component of fermionic nature undergoing saturation - in contrast to commonly used cavity-mediated excitation.

cond-mat.mes-hall↗

arXiv2016

Injection locking of quantum dot microlasers operating in the few photon regime

We experimentally and theoretically investigate injection locking of quantum dot (QD) microlasers in the regime of cavity quantum electrodynamics (cQED). We observe frequency locking and phase-locking where cavity enhanced spontaneous emission enables simultaneous stable oscillation at the master frequency and at the solitary frequency of the slave microlaser. Measurements of the second-order autocorrelation function prove this simultaneous presence of both master and slave-like emission, where the former has coherent character with $g^{(2)}(0)=1$ while the latter one has thermal character with $g^{(2)}(0)=2$. Semi-classical rate-equations explain this peculiar behavior by cavity enhanced spontaneous emission and a low number of photons in the laser mode.

physics.optics↗

arXiv2016

An exciton-polariton laser based on biologically produced fluorescent protein

Under adequate conditions, cavity-polaritons form a macroscopic coherent quantum state, known as Bose-Einstein condensate (BEC). Compared to Wannier-Mott excitons in inorganic semiconductors, the localized Frenkel excitons in organic emitter materials show weaker interaction but stronger coupling, which recently enabled the first realization of BEC at room temperature. However, this required ultrafast optical pumping which limits the applications of organic BECs. Here, we demonstrate room-temperature BEC of cavity-polaritons in simple laminated microcavities filled with the biologically produced enhanced green fluorescent protein (eGFP). The unique molecular structure of eGFP prevents exciton annihilation even at high excitation densities, thus facilitating BEC under conventional nanosecond pumping. BEC is clearly evidenced by a distinct threshold, an interaction-induced blueshift of the condensate, long-range coherence and the presence of a second threshold at higher excitation density which is associated with the onset of photon lasing and results from thermalization of the exciton reservoir.

cond-mat.mes-hall↗

arXiv2016

GaAs integrated quantum photonics: Towards dense and fully-functional quantum photonic integrated circuits

The recent progress in integrated quantum optics has set the stage for the development of an integrated platform for quantum information processing with photons, with potential applications in quantum simulation. Among the different material platforms being investigated, direct-bandgap semiconductors and particularly gallium arsenide (GaAs) offer the widest range of functionalities, including single- and entangled-photon generation by radiative recombination, low-loss routing, electro-optic modulation and single-photon detection. This paper reviews the recent progress in the development of the key building blocks for GaAs quantum photonics and the perspectives for their full integration in a fully-functional and densely integrated quantum photonic circuit.

cond-mat.mes-hall↗

arXiv2016

Half-Skyrmion Spin Textures In Polariton Microcavities

We study the polarization dynamics of a spatially expanding polariton condensate under nonresonant linearly polarized optical excitation. The spatially and temporally resolved polariton emission reveals the formation of non-trivial spin textures in the form of a quadruplet polarization pattern both in the linear and circular Stokes parameters, and an octuplet in the diagonal Stokes parameter. The continuous rotation of the polariton pseudospin vector through the condensate due to TE-TM splitting exhibits an ordered pattern of half-skyrmions associated with a half-integer topological number. A theoretical model based on a driven-dissipative Gross-Pitaevskii equation coupled with an exciton reservoir describes the dynamics of the nontrivial spin textures through the optical spin-Hall effect.

physics.optics↗

arXiv2016

High-energy side-peak emission of exciton-polariton condensates in high density regime

In a standard semiconductor laser, electrons and holes recombine via stimulated emission to emit coherent light, in a process that is far from thermal equilibrium. Exciton-polariton condensates -- sharing the same basic device structure as a semiconductor laser, consisting of quantum wells coupled to a microcavity -- have been investigated primarily at densities far below the Mott density for signatures of Bose-Einstein condensation. At high densities approaching the Mott density, exciton-polariton condensates are generally thought to revert to a standard semiconductor laser, with the loss of strong coupling. Here, we report the observation of a photoluminescence sideband at high densities that cannot be accounted for by conventional semiconductor lasing. This also differs from an upper-polariton peak by the observation of the excitation power dependence in the peak-energy separation. Our interpretation as a persistent coherent electron-hole-photon coupling captures several features of this sideband whereas many remain elusive. Understanding the observation will lead to a development in non-equilibrium many-body physics.

cond-mat.quant-gas↗

arXiv2016

On-Demand Single Photons with High Extraction Efficiency and Near-Unity Indistinguishability from a Resonantly Driven Quantum Dot in a Micropillar

Scalable photonic quantum technologies require on-demand single-photon sources with simultaneously high levels of purity, indistinguishability, and efficiency. These key features, however, have only been demonstrated separately in previous experiments. Here, by s-shell pulsed resonant excitation of a Purcell-enhanced quantum dot-micropillar system, we deterministically generate resonance fluorescence single photons which, at pi pulse excitation, have an extraction efficiency of 66%, single-photon purity of 99.1%, and photon indistinguishability of 98.5%. Such a single-photon source for the first time combines the features of high efficiency and near-perfect levels of purity and indistinguishabilty, and thus open the way to multi-photon experiments with semiconductor quantum dots.

quant-ph↗

arXiv2016

Near Transform-Limited Single Photons from an Efficient Solid-State Quantum Emitter

By pulsed s-shell resonant excitation of a single quantum dot-micropillar system, we generate long streams of a thousand of near transform-limited single photons with high mutual indistinguishability. Hong-Ou-Mandel interference of two photons are measured as a function of their emission time separation varying from 13 ns to 14.7 μs, where the visibility slightly drops from 95.9(2)% to a plateau of 92.1(5)% through a slow dephasing process occurring at time scale of 0.7 μs. Temporal and spectral analysis reveal the pulsed resonance fluorescence single photons are close to transform limit, which are readily useful for multi-photon entanglement and interferometry experiments.

quant-ph↗

arXiv2016

Room temperature Tamm-Plasmon Exciton-Polaritons with a WSe2 monolayer

Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit1,2, enhancing light-matter coupling. They further serve as an architecture to design ultra-fast, non-linear integrated circuits with smallest footprints3. Transition metal dichalcogenides are ideally suited as the active material in such circuits as they interact strongly with light at the ultimate monolayer limit4. Here, we implement a Tamm-plasmon-polariton structure, and study the coupling to a monolayer of WSe2, hosting highly stable excitons5. Exciton-Polariton formation at room temperature is manifested in the characteristic energy-momentum dispersion relation studied in photoluminescence, featuring an anti-crossing between the exciton and photon modes with a Rabi-splitting of 23.5 meV. Creating polaritonic quasi-particles in plasmonic architectures with atomic monolayers under ambient conditions is a crucial step towards compact, highly non-linear integrated photonic and polaritonic circuits6,7.

cond-mat.mes-hall↗