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Sven Höfling

Publications and source records attributed to Sven Höfling.

At least 163 records · Page 9Linked to original sources

A monolithic frequency comb platform based on interband cascade lasers and detectors

Optical frequency combs enable all-solid-state spectrometers that will trigger a breakthrough in miniaturization and on-chip integration of mid-infrared sensing technology. Interband cascade lasers (ICLs) are an ideal candidate for practical implementations due to their low power consumption and zero-bias detection functionality. Here, we demonstrate the generation of self-starting ICL frequency combs. We show that the gain is fast enough to respond to beating of the intracavity field, which hinders the formation of short pulses. Instead, the ICL operates in a comb state, where the phases of the fundamental intermode beatings are splayed over a range of $2π$. This state appears to be general to self-starting combs based on the inherent gain nonlinearity and minimizes oscillations of the population inversion. Using the same epi-layer material, we demonstrate efficient detector operation at room temperature up to several GHz bandwidth and thereby provide a complete and unmatched platform for monolithic and battery driven dual-comb spectroscopy.

physics.optics↗

Polarized indistinguishable single photons from a quantum dot in an elliptical micropillar

The key challenge to scalable optical quantum computing, boson sampling, and quantum metrology is sources of single photons with near-unity system efficiency and simultaneously near-perfect indistinguishability in all degrees of freedom (including spectral, temporal, spatial, and polarization). However, previous high-indistinguishability solid-state single-photon sources had to rely on polarization filtering that reduced the system efficiency by at least 50%. Here, we overcome this challenge by developing a new single-photon source based on a coherently driven quantum dot embedded in an elliptical micropillar. The asymmetric cavity lifts the polarization degeneracy into two orthogonal linearly polarized modes with a suitable energy separation. We design an excitation-collection scheme that allows the creation and collection of single photons with an indistinguishability of 0.976(1) and a degree of polarization of 91%. Our method provides a solution of combining near-unity system efficiency and indistinguishability compatible with background-free resonant excitation, and opens the way to truly optimal single-photon sources for scalable photonic quantum technologies.

physics.optics↗

Rabi oscillations of a quantum dot exciton coupled to acoustic phonons: coherence and population readout

While the advanced coherent control of qubits is now routinely carried out in low frequency (GHz) systems like single spins, it is far more challenging to achieve for two-level systems in the optical domain. This is because the latter evolve typically in the THz range, calling for tools of ultrafast, coherent, nonlinear optics. Using four-wave mixing micro-spectroscopy, we here measure the optically driven dynamics of a single exciton quantum state confined in a semiconductor quantum dot. In a combined experimental and theoretical approach, we reveal the intrinsic Rabi oscillation dynamics by monitoring both central exciton quantities, i.e., its occupation and the microscopic coherence, as resolved by the four-wave mixing technique. In the frequency domain this oscillation generates the Autler-Townes splitting of the light-exciton dressed states, directly seen in the four-wave mixing spectra. We further demonstrate that the coupling to acoustic phonons strongly influences the FWM dynamics on the picosecond timescale, because it leads to transitions between the dressed states.

cond-mat.mes-hall↗

Mutual coupling and synchronization of optically coupled quantum-dot micropillar lasers at ultra-low light levels

In this work we explore the limits of synchronization of mutually coupled oscillators at the crossroads of classical and quantum physics. In order to address this uncovered regime of synchronization we apply electrically driven quantum dot micropillar lasers operating in the regime of cavity quantum electrodynamics. These high-$β$ microscale lasers feature cavity enhanced coupling of spontaneous emission and operate at output powers on the order of 100 nW. We selected pairs of micropillar lasers with almost identical optical properties in terms of the input-output dependence and the emission energy which we mutually couple over a distance of about 1m and bring into spectral resonance by precise temperature tuning. By excitation power and detuning dependent studies we unambiguously identify synchronization of two mutually coupled high-$β$ microlasers via frequency locking associated with a sub-GHz locking range. A detailed analysis of the synchronization behavior includes theoretical modeling based on semi-classical stochastic rate equations and reveals striking differences from optical synchronization in the classical domain with negligible spontaneous emission noise and optical powers usually well above the mW range. In particular, we observe deviations from the classically expected locking slope and broadened locking boundaries which are successfully explained by the fact the quantum noise plays an important role in our cavity enhanced optical oscillators. Beyond that, introducing additional self-feedback to the two mutually coupled microlasers allows us to realize zero-lag synchronization. Our work provides important insight into synchronization of optical oscillators at ultra-low light levels and has high potential to pave the way for future experiments in the quantum regime of synchronization.

cond-mat.mes-hall↗

Electroluminescence on-off ratio control of n-i-n GaAs/AlGaAs-based resonant tunneling structures

We explore the nature of the electroluminescence (EL) emission of purely n-doped GaAs/AlGaAs resonant tunneling diodes (RTDs) and the EL evolution with voltage. A singular feature of such a device is unveiled when the electrical output current changes from high to low and the EL on-off ratio is enhanced by 2 orders of magnitude compared to the current on-off ratio. By combining the EL and current properties, we are able to identify two independent impact ionization channels associated with the coherent resonant tunneling current and the incoherent valley current. We also perform the same investigation with an associated series resistance, which induces a bistable electrical output in the system. By simulating a resistance variation for the current-voltage and the EL, we are able to tune the EL on-off ratio by up to 6 orders of magnitude. We further observe that the EL on and off states can be either direct or inverted compared to the tunneling current on and off states. This electroluminescence, combined with the unique RTD properties such as the negative differential resistance (NDR) and high frequency operation, enables the development of high speed functional opto-electronic devices and optical switches.

cond-mat.mtrl-sci↗

Deterministic coupling of quantum emitters in WSe$_2$ monolayers to plasmonic nanocavities

We discuss coupling of site-selectively induced quantum emitters in exfoliated monolayers of WSe$_2$ to plasmonic nanostructures. Squared and rectangular gold nanopillars, which are arranged in pitches of \SI{4}{\micro\meter} on the surface, have sizes of tens of nanometers, and act as seeds for the formation of quantum emitters in the atomically thin materials. We observe chraracteristic narrow-band emission signals from the monolayers, which correspond well with the positions of the metallic nanopillars with and without thin dielectric coating. Single photon emission from the emitters is confirmed by autocorrelation measurements, yielding $g^{2}(τ=0)$ values as low as 0.17. Moreover, we observe a strong co-polarization of our single photon emitters with the frequency matched plasmonic resonances, indicating deterministic light-matter coupling. Our work represents a significant step towards the scalable implementation of coupled quantum emitter-resonator systems for highly integrated quantum photonic and plasmonics applications.

cond-mat.mes-hall↗

Dynamics of liquid crystal on hexagonal lattice

Nematic liquid crystal (LC) molecules adsorbed on two dimensional materials are aligned along the crystal directions of the hexagonal lattice. It was demonstrated that short electric pulses can reorient the aligned LC molecules in the preferred armchair direction of hexagonal boron nitride (h-BN). Several states with a variety of colors were obtained by changing the direction and strength of the electric pulses. The ab initio calculations based on density functional theory was carried out to determine the favorable adsorption configurations of the LC molecules on the h-BN surface. A non-volatile display, in which pixel resolution can be determined by grains of hexagonal surface, is proposed, which can offer a pathway towards dynamic high-quality pixels with low power consumption, and could define a new paradigm for all non-volatile display applications.

cond-mat.soft↗

Observation of bosonic condensation in a hybrid monolayer MoSe2-GaAs microcavity

Condensation of bosons into a macroscopic quantum state belongs to the most intriguing phenomena in nature. It was first realized in quantum gases of ultra-cold atoms, but more recently became accessible in open-dissipative, exciton-based solid-state systems at elevated temperatures. Semiconducting monolayer crystals have emerged as a new platform for studies of strongly bound excitons in ultimately thin materials. Here, we demonstrate the formation of a bosonic condensate driven by excitons hosted in an atomically thin layer of MoSe2, strongly coupled to light in a solid-state resonator. The structure is operated in the regime of collective strong coupling, giving rise to hybrid exciton-polariton modes composed of a Tamm-plasmon resonance, GaAs quantum well excitons and two-dimensional excitons confined in a monolayer of MoSe2. Polariton condensation in a monolayer crystal manifests by a superlinear increase of emission intensity from the hybrid polariton mode at injection powers as low as 4.8 pJ/pulse, as well as its density-dependent blueshift and a dramatic collapse of the emission linewidth as a hallmark of temporal coherence. Importantly, we observe a significant spin-polarization in the injected polariton condensate, a fingerprint of the core property of monolayer excitons subject to spin-valley locking. The observed effects clearly underpin the perspective of building novel highly non-linear valleytronic devices based on light-matter fluids, coherent bosonic light sources based on atomically thin materials, and paves the way towards studying materials with unconventional topological properties in the framework of bosonic condensation.

cond-mat.quant-gas↗

High-concurrence time-bin entangled photon pairs from optimized Bragg-reflection waveguides

Semiconductor Bragg-reflection waveguides are well-established sources of correlated photon pairs as well as promising candidates for building up integrated quantum optics devices. Here, we use such a source with optimized non-linearity for preparing time-bin entangled photons in the telecommunication wavelength range. By taking advantage of pulsed state preparation and efficient free-running single-photon detection, we drive our source at low pump powers, which results in a strong photon-pair correlation. The tomographic reconstruction of the state's density matrix reveals that our source exhibits a high degree of entanglement. We extract a concurrence of $88.9\pm 1.8\%$ and a fidelity of $94.2 \pm 0.9\%$ with respect to a Bell state.

quant-ph↗

Two-dimensional semiconductors in the regime of strong light-matter coupling

The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced optical transitions, which can be brought into resonance with electromagnetic fields in microcavities and plasmonic nanostructures. Due to the atomic thinness and robustness of the monolayers, their integration in van der Waals heterostructures provides unique opportunities for engineering strong light-matter coupling. We review first results in this emerging field and outline future opportunities and challenges.

cond-mat.mes-hall↗

Intrinsic and environmental effects on the interference properties of a high-performance quantum dot single photon source

We report a joint experimental and theoretical study of the interference properties of a single photon source based on a In(Ga)As quantum dot embedded in a quasi-planar GaAs-microcavity. Using resonant laser excitation with a pulse separation of 2 ns, we find near-perfect interference of the emitted photons, and a corresponding indistinguishability of $\mathcal{I} = (99.6\,^{+\,0.4}_{-\,1.4})\%$. For larger pulse separations, quasi-resonant excitation conditions, increasing pump power or with increasing temperature, the interference contrast is progressively and notably reduced. We present a systematic study of the relevant dephasing mechanisms, and explain our results in the framework of a microscopic model of our system. For strictly resonant excitation, we show that photon indistinguishability is independent of pump power, but strongly influenced by virtual phonon assisted processes which are not evident in excitonic Rabi oscillations.

quant-ph↗

Spontaneous emission enhancement in strain-induced WSe2 monolayer based quantum light sources on metallic surfaces

Atomic monolayers of transition metal dichalcogenides represent an emerging material platform for the implementation of ultra compact quantum light emitters via strain engineering. In this framework, we discuss experimental results on creation of strain induced single photon sources using a WSe2 monolayer on a silver substrate, coated with a very thin dielectric layer. We identify quantum emitters which are formed at various locations in the sample. The emission is highly linearly polarized, stable in linewidth and decay times down to 300 ps are observed. We provide numerical calculations of our monolayer-metal device platform to assess the strength of the radiative decay rate enhancement by the presence of the plasmonic structure. We believe, that our results represent a crucial step towards the ultra-compact integration of high performance single photon sources in nanoplasmonic devices and circuits.

cond-mat.mes-hall↗

Polariton condensation in $S$- and $P$-flatbands in a two-dimensional Lieb lattice

We study the condensation of exciton-polaritons in a two-dimensional Lieb lattice of micropillars. We show selective polariton condensation into the flatbands formed by S and P$_{x;y}$ orbital modes of the micropillars under non-resonant laser excitation. The real space mode patterns of these condensates are accurately reproduced by the calculation of related Bloch modes of S- and P-flatbands. Our work emphasizes the potential of exciton-polariton lattices to emulate Hamiltonians of advanced potential landscapes. Furthermore, the obtained results provide a deeper inside into the physics of flatbands known mostly within the tight-binding limit.

cond-mat.mes-hall↗

Quantum-optical spectroscopy of a two-level system using an electrically driven micropillar laser as resonant excitation source

Two-level emitters constitute main building blocks of photonic quantum systems and are model systems for the exploration of quantum optics in the solid state. Most interesting is the strict-resonant excitation of such emitters to generate close to ideal quantum light and to control their occupation coherently. Up till now related experiments have been performed exclusively using bulky lasers which hinders the application of resonantly driven two-level emitters in photonic quantum systems. Here we perform quantum-optical spectroscopy of a two-level system using a compact high-$β$ microlaser as excitation source. The two-level system is based on a semiconductor quantum dot (QD), which is excited resonantly by a fiber-coupled electrically driven micropillar laser. In this way we dress the excitonic state of the QD under continuous wave excitation and trigger the emission of single-photons with strong multi-photon suppression ($g^{(2)}(0)=0.02$) and high photon indistinguishably ($V=57\pm9\%$) via pulsed resonant excitation at 156 MHz.

cond-mat.mes-hall↗

Exploring the Photon-Number Distribution of Bimodal Microlasers

A photon-number resolving transition edge sensor (TES) is used to measure the photon-number distribution of two microcavity lasers. The investigated devices are bimodal microlasers with similar emission intensity and photon statistics with respect to the photon auto-correlation. Both high-$β$ microlasers show partly thermal and partly coherent emission around the lasing threshold. For higher pump powers, the strong mode of microlaser A emits Poissonian distributed photons while the emission of the weak mode is thermal. In contrast, laser B shows a bistability resulting in overlayed thermal and Poissonian distributions. While a standard Hanbury Brown and Twiss experiment cannot distinguish between simple thermal emission of laser A and the mode switching of laser B, a TES allows us to measure the photon-number distribution which provides important insight into the underlying emission processes. Indeed, our experimental data and its theoretical description by a master equation approach show that TESs are capable of revealing subtle effects like temporal mode switching of bimodal microlasers. As such our studies clearly demonstrate the huge benefit and importance of investigating nanophotonic devices via photon-number resolving sensors.

cond-mat.mes-hall↗

Dynamics of the Optical Spin Hall Effect

We study the time evolution of the Optical Spin Hall Effect (OSHE), which occurs when exciton-polaritons undergo resonant Rayleigh scattering. The resulting spin pattern in momentum space is quantified by calculating the degree of circular polarization of the momentum space image for each point in time. We find the degree of circular polarization performing oscillations, which can be described within the framework of the pseudospin model by Kavokin et al. (Ref. 1).

cond-mat.mes-hall↗

Observation of hybrid Tamm-plasmon exciton-polaritons with GaAs quantum wells and a MoSe2 monolayer

Strong light matter coupling between excitons and microcavity photons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of light and matter excitations. The regime of collective strong coupling arises, when various excitations from different host media are strongly coupled to the same optical resonance. This leads to a well-controllable admixture of various matter components in three hybrid polariton modes. Here, we study a cavity device with four embedded GaAs quantum wells hosting excitons that are spectrally matched to the A-valley exciton resonance of a MoSe2 monolayer. The formation of hybrid polariton modes is evidenced in momentum resolved photoluminescence and reflectivity studies. We describe the energy and k-vector distribution of exciton-polaritons along the hybrid modes by a thermodynamic model, which yields a very good agreement with the experiment.

cond-mat.quant-gas↗

Signatures of a dissipative phase transition in photon correlation measurements

Understanding and characterizing phase transitions in driven-dissipative systems constitutes a new frontier for many-body physics. A generic feature of dissipative phase transitions is a vanishing gap in the Liouvillian spectrum, which leads to long-lived deviations from the steady-state as the system is driven towards the transition. Here, we show that photon correlation measurements can be used to characterize the corresponding critical slowing down of nonequilibrium dynamics. We focus on the extensively studied phenomenon of optical bistability in GaAs cavity-polaritons, which can be described as a first-order dissipative phase transition. Increasing the excitation strength towards the bistable range results in an increasing photon-bunching signal along with a decay time that is prolonged by more than nine orders of magnitude as compared to that of low density polaritons. In the limit of strong polariton interactions leading to pronounced quantum fluctuations, the mean-field bistability threshold is washed out. Nevertheless, the scaling of the Liouvillian gap closing as thermodynamic limit is approached provides a signature of the emerging dissipative phase transition. Our results establish photon correlation measurements as an invaluable tool for studying dynamical properties of dissipative phase transitions without requiring phase-sensitive interferometric measurements.

quant-ph↗