arXiv subjects

T. Chanelière

Publications and source records attributed to T. Chanelière.

At least 19 recordsLinked to original sources

arXiv2026

A material-agnostic platform to probe spin-phonon interactions using high-overtone bulk acoustic wave resonators

Spin-phonon interactions have a dual role in emerging spin-based quantum technologies. While they can be a limitation to device performance through decoherence, they also serve as a critical resource for coherent spin control, detection, and the realization of spin-based quantum networks. However, their direct characterization remains a challenge and is usually material-dependent. Here, we introduce a technique to probe spin-phonon coupling at millikelvin temperatures and gigahertz frequencies, using high-overtone bulk acoustic wave resonators (HBARs) integrated with arbitrary crystals via visco-elastic transfer of thin-film lithium niobate transducers. By tuning the Larmor frequency of dilute spin ensembles into resonance with HBAR modes, we extract the anisotropy and strength of spin-phonon interactions from acoustic dispersion and dissipation measurements. We demonstrate this approach in calcium tungstate (CaWO4) and yttrium orthosilicate (Y2SiO5), achieving cooperativities up to 0.5 for erbium dopant ensembles. Our method enables the study of spin-phonon interactions in complex crystalline materials, with minimal fabrication constraints. These results will facilitate the design of hybrid quantum systems and the quest for ion-matrix combination with enhanced spin-phonon coupling.

cond-mat.mes-hall↗

arXiv2024

Electron Paramagnetic Resonance spectroscopy of a scheelite crystal using microwave photon counting

Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been introduced as a sensitive new method for electron paramagnetic resonance spectroscopy at millikelvin temperatures. Here, we apply this spin fluorescence method to a scheelite crystal of CaWO4, finding some known ($\mathrm{Er}^{3+}$, $\mathrm{Yb}^{3+}$, $\mathrm{Nd}^{3+}$ and $\mathrm{Fe}^{3+}$) and other unknown paramagnetic impurities. Investigating the zero nuclear spin isotope ($I=0$) transition of $\mathrm{Er}^{3+}:\mathrm{CaWO}_4$ as a model system, we provide a quantitative analysis of the time-dependent photon counting rate following an excitation pulse, as a function of its power. The achieved signal-to-noise ratio is found to be an order of magnitude higher than the one obtained by inductively-detected Hahn echo under identical conditions. Finally, we use spin fluorescence spectroscopy at low excitation power to probe the properties of rare-earth-ions close to a metallic wire deposited on the surface; our data reveal line distortion caused by the mechanical strain imparted by the thermal contractions of the metal relative to the underlying crystal. Coherent oscillations are also observed for the most highly strained ions.

quant-ph↗

arXiv2021

Hyperfine spectroscopy in a quantum-limited spectrometer

We report measurements of electron spin echo envelope modulation (ESEEM) performed at millikelvin temperatures in a custom-built high-sensitivity spectrometer based on superconducting micro-resonators. The high quality factor and small mode volume (down to 0.2pL) of the resonator allow to probe a small number of spins, down to $5\cdot 10^2$. We measure 2-pulse ESEEM on two systems: erbium ions coupled to $^{183}$W nuclei in a natural-abundance $\text{CaWO}_4$ crystal, and bismuth donors coupled to residual $^{29}$Si nuclei in a silicon substrate that was isotopically enriched in the $^{28}$Si isotope. We also measure 3- and 5-pulse ESEEM for the bismuth donors in silicon. Quantitative agreement is obtained for both the hyperfine coupling strength of proximal nuclei, and the nuclear spin concentration.

quant-ph↗

arXiv2020

Superhyperfine induced photon-echo collapse of erbium in Y$_2$SiO$_5$

We investigate the decoherence of Er$^{3+}$ in Y$_2$SiO$_5$ at low magnetic fields using the photon-echo technique. We reproduce accurately a variety of the decay curves with a unique coherence time by considering the so-called superhyperfine modulation induced by a large number of neighbouring spins. There is no need to invoke any characteristic time of the spin fluctuations to reproduce very different decay curves. The number of involved nuclei increases when the magnetic is lowered. The experiment is compared with a model associating 100 surrounding ions with their exact positions in the crystal frame. We also derive an approximate spherical model (angular averaging) to interpret the main feature the observed decay curves close to zero-field.

quant-ph↗

arXiv2020

Multimode storage of quantum microwave fields in electron spins over 100 ms

A long-lived multi-mode qubit register is an enabling technology for modular quantum computing architectures. For interfacing with superconducting qubits, such a quantum memory should be able to store incoming quantum microwave fields at the single-photon level for long periods of time, and retrieve them on-demand. Here, we demonstrate the partial absorption of a train of weak microwave fields in an ensemble of bismuth donor spins in silicon, their storage for 100 ms, and their retrieval, using a Hahn-echo-like protocol. The long storage time is obtained by biasing the bismuth donors at a clock transition. Phase coherence and quantum statistics are preserved in the storage.

quant-ph↗

arXiv2020

Spin fine-structure reveals bi-exciton geometry in an organic semiconductor

In organic semiconductors, bi-excitons are key intermediates in carrier-multiplication and exciton annihilation. Their local geometry governs their electronic properties and yet has been challenging to determine. Here, we access the structure of the recently discovered $S=2$ quintet bi-exciton state in an organic semiconductor using broadband optically detected magnetic resonance. We correlate the experimentally extracted spin structure with the molecular crystal geometry to identify the specific molecular pairings on which bi-exciton states reside.

cond-mat.mtrl-sci↗

arXiv2018

Optical study of the anisotropic erbium spin flip-flop dynamics

We investigate the erbium flip-flop dynamics as a limiting factor of the electron spin lifetime and more generally as an indirect source of decoherence in rare-earth doped insulators. Despite the random isotropic arrangement of dopants in the host crystal, the dipolar interaction strongly depends on the magnetic field orientation following the strong anisotropy of the $g$-factor. In Er$^{3+}$:Y$_2$SiO$_5$, we observe by transient optical spectroscopy a three orders of magnitude variation of the erbium flip-flop rate (10ppm dopant concentration). The measurements in two different samples, with 10ppm and 50ppm concentrations, are well-supported by our analytic modeling of the dipolar coupling between identical spins with an anisotropic $g$-tensor. The model can be applied to other rare-earth doped materials. We extrapolate the calculation to Er$^{3+}$:CaWO$_4$, Er$^{3+}$:LiNbO$_3$ and Nd$^{3+}$:Y$_2$SiO$_5$ at different concentrations.

quant-ph↗

arXiv2018

Storage of RF photons in minimal conditions

We investigate the minimal conditions to store coherently a RF pulse in a material medium. We choose a commercial quartz as memory support because it is a widely available component with a high Q-factor. Pulse storage is obtained by varying dynamically the light-matter coupling with an analog switch. This parametric driving of the quartz dynamics can be alternatively interpreted as a stopped light experiment. We obtain an efficiency of 26%, a storage time of 209$μ$s and a time-to-bandwidth product of 98 by optimizing the pulse temporal shape. The coherent character of the storage is demonstrated. Our goal is to connect different types of memories in the RF and optical domain for quantum information processing. Our motivation is essentially fundamental.

physics.class-ph↗

arXiv2017

Slow-light analogue with a ladder of RLC circuits

The linear susceptibility of an atomic sample is formally equivalent to the response of a RLC circuit. We use a ladder of lumped RLC circuits to observe an analogue of slow-light, a well-known phenomenon in atomic physics. We first characterize the radio-frequency response of the circuit in the spectral domain exhibiting a transparency window surrounded by two strongly absorptive lines. We then observe a delayed pulse whose group delay is comparable to the pulse duration corresponding to slow-light propagation. The large group delay is obtained by cascading in a ladder configuration doubly resonant RLC cells.

physics.class-ph↗

arXiv2015

Optical measurement of heteronuclear cross-relaxation interactions in Tm:YAG

We investigate cross-relaxation interactions between Tm and Al in Tm:YAG using two optical methods: spectral holeburning and stimulated echoes. These interactions lead to a reduction in the hyperfine lifetime at magnetic fields that bring the Tm hyperfine transition into resonance with an Al transition. We develop models for measured echo decay curves and holeburning spectra near a resonance, which are used to show that the Tm-Al interaction has a resonance width of 10~kHz and reduces the hyperfine lifetime to 0.5 ms. The antihole structure is consistent with an interaction dominated by the Al nearest neighbors at 3.0 Angstroms, with some contribution from the next nearest neighbors at 3.6 Angstroms.

cond-mat.mtrl-sci↗

arXiv2014

Photon echo with a few photons in two-level atoms

To store and retrieve signals at the single photon level, various photon echo schemes have resorted to complex preparation steps involving ancillary shelving states in multi-level atoms. For the first time, we experimentally demonstrate photon echo operation at such a low signal intensity without any preparation step, which allows us to work with mere two-level atoms. This simplified approach relies on the so-coined "Revival Of Silenced Echo" (ROSE) scheme. Low noise conditions are obtained by returning the atoms to the ground state before the echo emission. In the present paper we manage ROSE in photon counting conditions, showing that very strong control fields can be compatible with extremely weak signals, making ROSE consistent with quantum memory requirements.

quant-ph↗

arXiv2013

Quantum Memory with a controlled homogeneous splitting

We propose a quantum memory protocol where a input light field can be stored onto and released from a single ground state atomic ensemble by controlling dynamically the strength of an external static and homogeneous field. The technique relies on the adiabatic following of a polaritonic excitation onto a state for which the forward collective radiative emission is forbidden. The resemblance with the archetypal Electromagnetically-Induced-Transparency (EIT) is only formal because no ground state coherence based slow-light propagation is considered here. As compared to the other grand category of protocols derived from the photon-echo technique, our approach only involves a homogeneous static field. We discuss two physical situations where the effect can be observed, and show that in the limit where the excited state lifetime is longer than the storage time, the protocols are perfectly efficient and noise-free. We compare the technique to other quantum memories, and propose atomic systems where the experiment can be realized.

quant-ph↗

arXiv2013

Spin coherence lifetime extension in Tm$^{3+}$:YAG through dynamical decoupling

We report on spin coherence lifetime extension on Tm$^{3+}$:YAG obtained through dynamically decoupling the thulium spins from their magnetic environment. The coherence lifetime reached with a Carr-Purcell-Meiboom-Gill sequence revealed a 450-fold extension [$\sim$$(230 \pm 30)$ ms] with respect to previously measured values. Comparison to a simple theoretical model allowed us to estimate the correlation time of the fluctuations of the ground level transition frequency to $(172 \pm 30)$ $μ$s at 1.7 K. For attaining efficient decoupling sequences, we developed a strategy inspired by the \emph{zero-first-order Zeeman} effect to minimize the large inhomogeneous broadening of the ground level spin transition.

quant-ph↗

arXiv2012

Atomic Frequency Comb storage as a slow-light effect

Atomic Frequency Comb (AFC) protocol has been particularly successful recently to demonstrate the storage of quantum information in a solid medium (rare-earth doped crystals). The AFC is inspired by the photon-echo technique. We show in this paper that the AFC is actually closely related to the slow-light based storage protocols extensively used in atomic vapours. Experimental verifications are performed in thulium doped YAG (Tm3+:YAG). We clarify the interplay between absorption and dispersion and propose a classification of the existing protocols.

quant-ph↗

arXiv2011

Emission of photon echoes in a strongly scattering medium

We observe the two- and three-pulse photon echo emission from a scattering powder, obtained by grinding a Pr$^{3+}$:Y$_2$SiO$_5$ rare earth doped single crystal. We show that the collective emission is coherently constructed over several grains. A well defined atomic coherence can therefore be created between randomly placed particles. Observation of photon echo on powders as opposed to bulk materials opens the way to faster material development. More generally, time-domain resonant four-wave mixing offers an attractive approach to investigate coherent propagation in scattering media.

physics.optics↗

arXiv2011

Revival of Silenced Echo and Quantum Memory for Light

We propose an original quantum memory protocol. It belongs to the class of rephasing processes and is closely related to two-pulse photon echo. It is known that the strong population inversion produced by the rephasing pulse prevents the plain two-pulse photon echo from serving as a quantum memory scheme. Indeed gain and spontaneous emission generate prohibitive noise. A second $π$-pulse can be used to simultaneously reverse the atomic phase and bring the atoms back into the ground state. Then a secondary echo is radiated from a non-inverted medium, avoiding contamination by gain and spontaneous emission noise. However, one must kill the primary echo, in order to preserve all the information for the secondary signal. In the present work, spatial phase mismatching is used to silence the standard two-pulse echo. An experimental demonstration is presented.

quant-ph↗

arXiv2010

Highly multimode memory in a crystal

We experimentally demonstrate the storage of 1060 temporal modes onto a thulium-doped crystal using an atomic frequency comb (AFC). The comb covers 0.93 GHz defining the storage bandwidth. As compared to previous AFC preparation methods (pulse sequences i.e. amplitude modulation), we only use frequency modulation to produce the desired optical pumping spectrum. To ensure an accurate spectrally selective optical pumping, the frequency modulated laser is self-locked on the atomic comb. Our approach is general and should be applicable to a wide range of rare-earth doped material in the context of multimode quantum memory.

quant-ph↗

arXiv2009

Efficiency optimization for Atomic Frequency Comb storage

We study the efficiency of the Atomic Frequency Comb storage protocol. We show that for a given optical depth, the preparation procedure can be optimize to significantly improve the retrieval. Our prediction is well supported by the experimental implementation of the protocol in a \TMYAG crystal. We observe a net gain in efficiency from 10% to 17% by applying the optimized preparation procedure. In the perspective of high bandwidth storage, we investigate the protocol under different magnetic fields. We analyze the effect of the Zeeman and superhyperfine interaction.

quant-ph↗