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T. Dong

Publications and source records attributed to T. Dong.

44 records · Page 3Linked to original sources

Nanoscale phase separation of antiferromagnetic order and superconductivity in K$_{0.75}$Fe$_{1.75}$Se$_2$

We report an in-plane optical spectroscopy study on the iron-selenide superconductor K$_{0.75}$Fe$_{1.75}$Se$_2$. The measurement revealed the development of a sharp reflectance edge below T$_c$ at frequency much smaller than the superconducting energy gap on a relatively incoherent electronic background, a phenomenon which was not seen in any other Fe-based superconductors so far investigated. Furthermore, the feature could be noticeably suppressed and shifted to lower frequency by a moderate magnetic field. Our analysis indicates that this edge structure arises from the development of a Josephson-coupling plasmon in the superconducting condensate. Together with the transmission electron microscopy analysis, our study yields compelling evidence for the presence of nanoscale phase separation between superconductivity and magnetism. The results also enable us to understand various seemingly controversial experimental data probed from different techniques.

cond-mat.supr-con↗

Optical study of the multiple charge density wave transitions in ErTe$_3$

We present an optical spectroscopy study on singe crystalline ErTe$_3$, a rare-earth-element tri-telluride which experiences two successive charge density wave (CDW) transitions at T$_{c1}$ = 267 K and T$_{c2}$ = 150 K. Two corresponding gap features, centered at 2770 \cm ($\sim$ 343 meV) and 890 \cm ($\sim$ 110 meV) respectively, are clearly seen in ordered state. A pronounced Drude component, which exists at all measurement temperatures, demonstrates the partial gap character of both CDW orders. About half of the unmodulated Fermi surface (FS) remains in the CDW state at the lowest measurement temperature. The study also reveals that fluctuation effect is still prominent in this two-dimensional (2D) material.

cond-mat.str-el↗

Infrared spectrum and its implications for the electronic structure of the semiconducting iron selenide K$_{0.83}$Fe$_{1.53}$Se$_2$

We report an infrared spectroscopy study on K$_{0.83}$Fe$_{1.53}$Se$_2$, a semiconducting parent compound of the new iron-selenide system. The major spectral features are found to be distinctly different from all other Fe-based superconducting systems. Our measurement revealed two peculiar spectral structures: a double peak structure between 4000-6000 cm$^{-1}$ and abundant phonon modes much more than those expected for a 122 structure. We elaborate that those features could be naturally explained from the blocked antiferromagnetism due to the presence of Fe vacancy ordering as determined by recent neutron diffraction experiments. The double peaks reflect the coexistence of ferromagnetic and antiferromagnetic couplings between the neighboring Fe sites.

cond-mat.supr-con↗

Optical spectroscopy study on CeTe$_3$: evidence for multiple charge-density-wave orders

We performed optical spectroscopy measurement on single crystal of CeTe$_3$, a rare-earth element tri-telluride charge density wave (CDW) compound. The optical spectra are found to display very strong temperature dependence. Besides a large and pronounced CDW energy gap being present already at room temperature as observed in earlier studies, the present measurement revealed the formation of another energy gap at smaller energy scale at low temperature. The second CDW gap removes the electrons near E$_F$ which undergo stronger scattering. The study yields evidence for the presence of multiple CDW orders or strong fluctuations in the light rare-earth element tri-telluride.

cond-mat.str-el↗

Three dimensionality of band structure and a large residual quasiparticle population in Ba$_{0.67}$K$_{0.33}$Fe$_2$As$_2$ as revealed by the c-axis polarized optical measurement

We report on a c-axis polarized optical measurement on a Ba$_{0.67}$K$_{0.33}$Fe$_2$As$_2$ single crystal. We find that the c-axis optical response is significantly different from that of high-T$_c$ cuprates. The experiments reveal an anisotropic three-dimensional optical response with the absence of the Josephson plasma edge in R($ω$) in the superconducting state. Furthermore, different from the ab-plane optical response, a large residual quasiparticle population down to $T\sim\frac{1}{5}T_c$ was observed in the c-axis polarized reflectance measurement. We elaborate that there exist nodes for the superconducting gap in regions of the 3D Fermi surface that contribute dominantly to the c-axis optical conductivity.

cond-mat.supr-con↗

Formation of partial energy gap below the structural phase transition and the rare-earth element substitution effect on infrared phonons in ReFeAsO (Re=La, Nd, and Sm)

Single crystals of LaFeAsO, NdFeAsO, and SmFeAsO have been prepared by means of a NaAs flux growth technique and studied by optical spectroscopy measurements. We show that the spectral features corresponding to the partial energy gaps in the spin-density-wave (SDW) state are present below the structural phase transition. This indicates that the electronic state below the structural phase transition is already very close to that in the SDW state. We also show that in-plane infrared phonon modes display systematic shifts towards high frequency upon rare-earth element substitutions for La, suggesting a strong enhancement of the bonding strength. Furthermore, an asymmetric line-shape of the in-plane phonon mode is observed, implying the presence of an electron-phonon coupling effect in Fe-pnictides.

cond-mat.supr-con↗

Measurement of the c-axis optical reflectance of AFe$_2$As$_2$ (A=Ba, Sr) single crystals: Evidence of different mechanisms for the formation of two energy gaps

We present the c-axis optical reflectance measurement on single crystals of BaFe$_2$As$_2$ and SrFe$_2$As$_2$, the parent compounds of FeAs based superconductors. Different from the ab-plane optical response where two distinct energy gaps were observed in the SDW state, only the smaller energy gap could be seen clearly for \textbf{E}$\parallel$c-axis. The very pronounced energy gap structure seen at a higher energy scale for \textbf{E}$\parallel$ab-plane is almost invisible. We propose a novel picture for the band structure evolution across the SDW transition and suggest different driving mechanisms for the formation of the two energy gaps.

cond-mat.supr-con↗

Optical spectroscopy study on single crystalline LaFeAsO

Millimeter-sized single crystals of LaFeAsO were grown from NaAs flux and the in-plane optical properties were studied over a wide frequency range. A sizable electronic correlation effect was indicated from the analysis of the free-carrier spectral weight. With decreasing temperature from 300 K, we observed a continuous suppression of the spectral weight near 0.6 eV. But a spin-density-wave gap formation at lower energy scale was seen only in the broken-symmetry state. We elaborate that both the itinerancy and local spin interactions of Fe\emph{3d} electrons are present for the FeAs-based systems; however, the establishment of the long-range magnetic order at low temperature has a dominantly itinerant origin.

cond-mat.supr-con↗