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T. Eronen

Publications and source records attributed to T. Eronen.

At least 55 records · Page 3Linked to original sources

High-precision $Q$-value measurement and nuclear matrix elements for the double-$β$ decay of $^{98}$Mo

Neutrinoless double-beta ($0νββ$) decay and the standard two-neutrino double-beta ($2νββ$) decay of $^{98}$Mo have been studied. The double-beta decay $Q$-value has been determined as $Q_{ββ}=113.668(68)$ keV using the JYFLTRAP Penning trap mass spectrometer. It is in agreement with the literature value, $Q_{ββ}=109(6)$ keV, but almost 90 times more precise. Based on the measured $Q$-value, precise phase-space factors for $2νββ$ decay and $0νββ$ decay, needed in the half-life predictions, have been calculated. Furthermore, the involved nuclear matrix elements have been computed in the proton-neutron quasiparticle random-phase approximation (pnQRPA) and the microscopic interacting boson model (IBM-2) frameworks. Finally, predictions for the $2νββ$ decay are given, suggesting a much longer half-life than for the currently observed cases.

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Study of radial motion phase advance during motion excitations in a Penning trap and accuracy of JYFLTRAP mass spectrometer

Phase-imaging ion-cyclotron-resonance technique has been implemented at the Penning-trap mass spectrometer JYFLTRAP and is routinely employed for mass measurements of stable and short-lived nuclides produced at IGISOL facility. Systematic uncertainties that impose limitations on the accuracy of measurements are discussed. It was found out that the phase evolution of the radial motion of ions in a Penning trap during the application of radio-frequency fields leads to a systematic cyclotron frequency shift when more than one ion species is present in the trap during the cyclotron frequency measurement. An analytic expression was derived to correctly account for the shift. Cross-reference mass measurements with carbon-cluster ions have been performed providing the mass-dependent and residual uncertainties.

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Direct measurement of the mass difference of $^{72}$As-$^{72}$Ge rules out $^{72}$As as a promising $β$-decay candidate to determine the neutrino mass

We report the first direct determination of the ground-state to ground-state electron-capture $Q$-value for the $^{72}$As to $^{72}$Ge decay by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The $Q$-value was measured to be 4343.596(75)~keV, which is more than a 50-fold improvement in precision compared to the value in the most recent Atomic Mass Evaluation 2020. Furthermore, the new $Q$-value was found to be 12.4(40)~keV (3.1 $σ$) lower. With the significant reduction of the uncertainty of the ground-state to ground-state $Q$-value value combined with the level scheme of $^{72}$Ge from $γ$-ray spectroscopy, we confirm that the five potential ultra-low $Q$-value ${β^{+}}$-decay or electron capture transitions are energetically forbidden, thus precluding all the transitions as possible candidates for the electron neutrino mass determination. However, the discovery of small negative $Q$-values opens up the possibility to use $^{72}$As for the study of virtual $β$-$γ$ transitions.

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High-precision mass measurement of $^{168}$Yb for verification of nonlinear isotope shift

The absolute mass value of $^{168}$Yb has been directly determined with the JYFLTRAP Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. A more precise value of the mass of $^{168}$Yb is needed to extract possible signatures of beyond standard model physics from high-precision isotope shift measurements of Yb atomic transition frequencies. The measured mass-excess value, ME($^{168}$Yb) = $-$61579.846(94) keV, is 12 times more precise and deviates from the Atomic Mass Evaluation 2016 value by 1.7$σ$. The impact on precision isotope shift studies of the stable Yb isotopes is discussed.

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Novel Penning-trap techniques reveal isomeric states in $^{128}$In and $^{130}$In for the first time

Isomeric states in $^{128}$In and $^{130}$In have been studied with the JYFLTRAP Penning trap at the IGISOL facility. By employing novel ion manipulation techniques, different states were separated and masses of six beta-decaying states were measured. JYFLTRAP was also used to select the ions of interest for identification at a post-trap decay spectroscopy station. A new beta-decaying high-spin isomer feeding the $15^-$ isomer in $^{128}$Sn has been discovered in $^{128}$In at $1797.6(20)$ keV. Shell-model calculations employing a CD-Bonn potential re-normalized with the perturbative G-matrix approach suggest this new isomer to be a $16^+$ spin-trap isomer. In $^{130}$In, the lowest-lying $(10^-)$ isomeric state at $58.6(82)$ keV was resolved for the first time using the phase-imaging ion cyclotron resonance technique. The energy difference between the $10^-$ and $1^-$ states in $^{130}$In, stemming from parallel/antiparallel coupling of $(π0g_{9/2}^{-1})\otimes(ν0h_{11/2}^{-1})$, has been found to be around 200 keV lower than predicted by the shell model. Precise information on the energies of the excited states determined in this work is crucial for producing new improved effective interactions for the nuclear shell model description of nuclei near $^{132}$Sn.

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Determination of Beta Decay Ground State Feeding of Nuclei of Importance for Reactor Applications

In $β$-decay studies the determination of the decay probability to the ground state of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed $γ$-ray emission. In this work we revisit the $4πγ-β$ method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the $β$-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large ground state branches. The method is relevant for nuclear structure studies as well. Pertinent formulae are revised and extended to the special case of $β$-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain ground state feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.

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High-precision $Q$-value measurement confirms the potential of $^{135}$Cs for antineutrino-mass detection

The ground-state-to-ground-state $β$-decay $Q$-value of $^{135}\textrm{Cs}(7/2^+)\to\,^{135}\textrm{Ba}(3/2^+)$ was directly measured for the first time utilizing the Phase-Imaging Ion-Cyclotron Resonance (PI-ICR) technique at the JYFLTRAP Penning-trap setup. It is the first direct determination of this $Q$-value and its value of 268.66(30)\,keV is a factor of three more precise than the currently adopted $Q$-value in the Atomic Mass Evaluation 2016. Moreover, the $Q$-value deduced from the $β$-decay endpoint energy has been found to deviate from our result by approximately 6 standard deviations. The measurement confirms that the first-forbidden unique $β^-$-decay transition $^{135}\textrm{Cs}(7/2^+)\to\,^{135}\textrm{Ba}(11/2^-)$ is a candidate for antineutrino-mass measurements with an ultra-low $Q$-value of $0.44(31)$ keV. This $Q$-value is almost an order of magnitude smaller than in any presently running or planned direct (anti)neutrino-mass experiment.

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Exploring the mass surface near the rare-earth abundance peak via precision mass measurements at JYFLTRAP

The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capture process has been studied. The calculated abundance distribution results in a better agreement with the solar abundance pattern near the top of the rare-earth abundance peak at around $A\approx165$.

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Measurement of the $2^+\rightarrow 0^+$ ground-state transition in the $β$ decay of $^{20}$F

We report the first detection of the second-forbidden, non-unique, $2^+\rightarrow 0^+$, ground-state transition in the $β$ decay of $^{20}$F. A low-energy, mass-separated $^{20}\rm{F}^+$ beam produced at the IGISOL facility in Jyväskylä, Finland, was implanted in a thin carbon foil and the $β$ spectrum measured using a magnetic transporter and a plastic-scintillator detector. The $β$-decay branching ratio inferred from the measurement is $b_β = [ 0.41\pm 0.08\textrm{(stat)}\pm 0.07\textrm{(sys)}] \times 10^{-5}$ corresponding to $\log ft = 10.89(11)$, making this one of the strongest second-forbidden, non-unique $β$ transitions ever measured. The experimental result is supported by shell-model calculations and has significant implications for the final evolution of stars that develop degenerate oxygen-neon cores. Using the new experimental data, we argue that the astrophysical electron-capture rate on $^{20}$Ne is now known to within better than 25% at the relevant temperatures and densities.

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Discovery of an Exceptionally Strong $β$-Decay Transition of $^{20}$F and Implications for the Fate of Intermediate-Mass Stars

A significant fraction of stars between 7-11 solar masses are thought to become supernovae, but the explosion mechanism is unclear. The answer depends critically on the rate of electron capture on $^{20}$Ne in the degenerate oxygen-neon stellar core. However, due to the unknown strength of the transition between the ground states of $^{20}$Ne and $^{20}$F, it has not previously been possible to fully constrain the rate. By measuring the transition, we have established that its strength is exceptionally large and enhances the capture rate by several orders of magnitude. This has a decisive impact on the evolution of the core, increasing the likelihood that the star is (partially) disrupted by a thermonuclear explosion rather than collapsing to form a neutron star. Importantly, our measurement resolves the last remaining nuclear physics uncertainty in the final evolution of degenerate oxygen-neon stellar cores, allowing future studies to address the critical role of convection, which at present is poorly understood.

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Total absorption $γ$-ray spectroscopy of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb

The decays of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb have been studied with the total absorption $γ$-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyväskylä allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption $γ$-ray spectrometer, a segmented detector composed of eighteen NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt $γ$-rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of $β$-intensity to states above the neutron separation energy that de-excite by $γ$-rays, comparable to the neutron emission probability. The competition between $γ$ de-excitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the $β$-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties, and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.

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The MORA project

The MORA (Matter's Origin from the RadioActivity of trapped and oriented ions) project aims at measuring with unprecedented precision the D correlation in the nuclear beta decay of trapped and oriented ions. The D correlation offers the possibility to search for new CP-violating interactions, complementary to searches done at the LHC and with Electric Dipole Moments. Technically, MORA uses an innovative in-trap orientation method which combines the high trapping efficiency of a transparent Paul trap with laser orientation techniques. The trapping, detection, and laser setups are under development, for first tests at the Accelerator laboratory, JYFL, in the coming years.

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Total absorption $γ$-ray spectroscopy of niobium isomers

The $β$ intensity distributions of the decays of $^{100\text{gs},100\text{m}}$Nb and $^{102\text{gs},102\text{m}}$Nb have been determined using the Total Absorption $γ$-Ray Spectroscopy technique. The JYFLTRAP double Penning trap system was employed to disentangle the isomeric states involved, lying very close in energy, in a campaign of challenging measurements performed with the Decay Total Absorption $γ$-ray Spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. The low-spin isomeric state of each niobium case was populated through the decay of the zirconium parent, that was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained $β$ intensity distributions for these zirconium decays. The $β$-strength distributions evaluated with these results were compared with calculations in quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of $^{100,102}$Zr. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The $β$-intensities of the decay of $^{102\text{m}}$Nb were obtained for the first time. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported and here we detail the significant impact on decay heat calculations.

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A new off-line ion source facility at IGISOL

An off-line ion source station has been commissioned at the IGISOL (Ion Guide Isotope Separator On-Line) facility. It offers the infrastructure needed to produce stable ion beams from three off-line ion sources in parallel with the radioactive ion beams produced from the IGISOL target chamber. This has resulted in improved feasibility for new experiments by offering reference ions for Penning-trap mass measurements, laser spectroscopy and atom trap experiments.

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Isomeric fission yield ratios for odd-mass Cd and In isotopes using the Phase-Imaging Ion-Cyclotron-Resonance technique

Isomeric yield ratios for the odd-$A$ isotopes of $^{119-127}$Cd and $^{119-127}$In from 25-MeV proton-induced fission on natural uranium have been measured at the JYFLTRAP double Penning trap, by employing the Phase-Imaging Ion-Cyclotron-Resonance technique. With the significantly improved mass resolution of this novel method isomeric states separated by 140 keV from the ground state, and with half-lives of the order of 500 ms, could be resolved. This opens the door for obtaining new information on low-lying isomers, of importance for nuclear structure, fission and astrophysics. In the present work the experimental isomeric yield ratios are used for the estimation of the root-mean-square angular momentum ($J_\mathrm{rms}$) of the primary fragments. The results show a dependency on the number of unpaired protons and neutrons, where the odd-$Z$ In isotopes carry larger angular momenta. The deduced values of $J_\mathrm{rms}$ display a linear relationship when compared with the electric quadrupole moments of the fission products.

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First determination of $β$-delayed multiple neutron emission beyond A = 100 through direct neutron measurement: The P$_{2n}$ value of $^{136}$Sb

Background: $β$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $β$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyväskylä, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $β$- and neutron- growth-and-decay curves and the $β$-one-neutron and $β$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.14(3)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 32.2(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 44 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations.

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Characterization and performance of the DTAS detector

DTAS is a segmented total absorption γ-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption γ-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of \b{eta}-delayed neutron emitting nuclei.

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Precision mass measurements on neutron-rich rare-earth isotopes at JYFLTRAP - reduced neutron pairing and implications for the $r$-process calculations

The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear structure has been probed via two-neutron separation energies $S_{2n}$ and neutron pairing energy metrics $D_n$. The data do not support the existence of a subshell closure at $N=100$. Neutron pairing has been found to be weaker than predicted by theoretical mass models. The impact on the calculated $r$-process abundances has been studied. Substantial changes resulting in a smoother abundance distribution and a better agreement with the solar $r$-process abundances are observed.

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