Searcharxiv⌕ Search

arXiv subjects

T. Eronen

Publications and source records attributed to T. Eronen.

At least 73 records · Page 4Linked to original sources

Total Absorption Spectroscopy Study of the Beta Decay of $^{86}$Br and $^{91}$Rb

The beta decays of $^{86}$Br and $^{91}$Rb have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the IGISOL facility in Jyväskylä and further purified using the JYFLTRAP. $^{86}$Br and $^{91}$Rb are considered to be major contributors to the decay heat in reactors. In addition $^{91}$Rb was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam {\it et al.} assuming that this decay was well known from high-resolution measurements. Our results show that both decays were suffering from the {\it Pandemonium} effect and that the results of Rudstam {\it et al.} should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated.

nucl-ex↗

Study of the $β$-decay of $^{100}$Tc with Total Absorption $γ$-Ray Spectroscopy

The \b{eta}-decay of 100 Tc has been studied using the Total Absorption γ-Ray Spectroscopy technique at IGISOL. In this work the new DTAS spectrometer in coincidence with a cylindrical plastic \b{eta} detector has been employed. The \b{eta}-intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random- phase approximation (QRPA) framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double \b{eta}-decay of 100 Mo.

nucl-ex↗

High-precision mass measurements for the isobaric multiplet mass equation at A = 52

Masses of $^{52}$Co, $^{52}$Co$^m$, $^{52}$Fe, $^{52}$Fe$^m$, and $^{52}$Mn have been measured with the JYFLTRAP double Penning trap mass spectrometer. Of these, $^{52}$Co and $^{52}$Co$^m$ have been experimentally determined for the first time and found to be more bound than predicted by extrapolations. The isobaric multiplet mass equation for the $T=2$ quintet at $A=52$ has been studied employing the new mass values. No significant breakdown (beyond the $3σ$ level) of the quadratic form of the IMME was observed ($χ^2/n=2.4$). The cubic coefficient was 6.0(32) keV ($χ^2/n=1.1$). The excitation energies for the isomer and the $T=2$ isobaric analogue state in $^{52}$Co have been determined to be 374(13) keV and 2922(13) keV, respectively. The $Q$ value for the proton decay from the $19/2^-$ isomer in $^{53}$Co has been determined with an unprecedented precision, $Q_{p} = 1558.8(17)$ keV. The proton separation energies of $^{52}$Co and $^{53}$Ni relevant for the astrophysical rapid proton capture process have been experimentally determined for the first time. \end{abstract}

nucl-ex↗

Characterization of a cylindrical plastic β-detector with Monte Carlo simulations of optical photons

In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic \b{eta}-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extensive simulations have to be done, as in the case of the calculation of the response function of the spectrometer in a total absorption γ-ray spectroscopy analysis.

physics.ins-det↗

Total Absorption Gamma-Ray Spectroscopy of 87Br, 88Br and 94Rb Beta-Delayed Neutron Emitters

We investigate the decay of 87Br, 88Br and 94Rb using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable gamma-intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the range 1 to 100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for gamma emission from neutron unbound states populated in the daughter nucleus. The gamma branching is compared to Hauser-Feshbach calculations which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94Rb, although much smaller, hints of the need to increase the radiative width by one order-of-magnitude. This leads to a similar increase in the calculated (n,gamma) cross section for this very neutron-rich nucleus with a potential impact on r-process abundance calculations.

nucl-ex↗

Mass of astrophysically relevant $^{31}$Cl and the breakdown of the isobaric multiplet mass equation

The mass of $^{31}$Cl has been measured with the JYFLTRAP double Penning trap mass spectrometer at the Ion-Guide Isotope Separator On-Line (IGISOL) facility. The determined mass-excess value, -7034.7(34) keV, is 15 times more precise than in the Atomic Mass Evaluation 2012. The quadratic form of the isobaric multiplet mass equation for the T=3/2 quartet at A=31 fails ($χ^2_n$=11.6) and a non-zero cubic term, d=-3.5(11) keV, is obtained when the new mass value is adopted. $^{31}$Cl has been found to be less proton-bound with a proton separation energy of $S_p$=265(4) keV. Energies for the excited states in $^{31}$Cl and the photodisintegration rate on $^{31}$Cl have been determined with significantly improved precision using the new $S_p$ value. The improved photodisintegration rate helps to constrain astrophysical conditions where $^{30}$S can act as a waiting point in the rapid proton capture process in type I x-ray bursts.

nucl-ex↗

Total Absorption Spectroscopy Study of $^{92}$Rb Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape

The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. $^{92}$Rb makes the dominant contribution to the reactor spectrum in the 5-8 MeV range but its decay properties are in question. We have studied $^{92}$Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.

nucl-ex↗

Enhanced Gamma-Ray Emission from Neutron Unbound States Populated in Beta Decay

Total absorption spectroscopy was used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in 87,88Br and 94Rb. Accurate results were obtained thanks to a careful control of systematic errors. An unexpectedly large gamma intensity was observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy was compared to Hauser-Feshbach model calculations. For 87Br and 88Br the gamma branching reaches 57% and 20% respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich 94Rb the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled introducing an enhancement of one order-of-magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proved to be correct, leads to a similar increase in the (n,gamma) cross section that would have an impact on r-process abundance calculations.

nucl-ex↗

Coulomb displacement energies as a probe for nucleon pairing in the $f_{7/2}$ shell

Coulomb displacement energies of $T=1/2$ mirror nuclei have been studied via a series of high-precision $Q_\mathrm{EC}$-value measurements with the double Penning trap mass spectrometer JYFLTRAP. Most recently, the $Q_\mathrm{EC}$ values of the $f_{7/2}$-shell mirror nuclei $^{45}$V ($Q_\mathrm{EC}=7123.82(22)$ keV) and $^{49}$Mn ($Q_\mathrm{EC}=7712.42(24)$ keV) have been measured with an unprecedented precision. The data reveal a 16-keV ($1.6σ$) offset in the adopted Atomic Mass Evaluation 2012 value of $^{49}$Mn suggesting the need for further measurements to verify the breakdown of the quadratic form of the isobaric multiplet mass equation. Precisely measured $Q_\mathrm{EC}$ values confirm that the pairing effect in the Coulomb energies is quenched when entering the $f_{7/2}$ shell and reaches a minimum in the midshell.

nucl-ex↗

Isomeric states close to doubly magic $^{132}$Sn studied with JYFLTRAP

The double Penning trap mass spectrometer JYFLTRAP has been employed to measure masses and excitation energies for $11/2^-$ isomers in $^{121}$Cd, $^{123}$Cd, $^{125}$Cd and $^{133}$Te, for $1/2^-$ isomers in $^{129}$In and $^{131}$In, and for $7^-$ isomers in $^{130}$Sn and $^{134}$Sb. These first direct mass measurements of the Cd and In isomers reveal deviations to the excitation energies based on results from beta-decay experiments and yield new information on neutron- and proton-hole states close to $^{132}$Sn. A new excitation energy of 144(4) keV has been determined for $^{123}$Cd$^m$. A good agreement with the precisely known excitation energies of $^{121}$Cd$^m$, $^{130}$Sn$^m$, and $^{134}$Sb$^m$ has been found.

nucl-ex↗

Precision Mass Measurements beyond $^{132}$Sn: Anomalous behaviour of odd-even staggering of binding energies

Atomic masses of the neutron-rich isotopes $^{121-128}$Cd, $^{129,131}$In, $^{130-135}$Sn, $^{131-136}$Sb, and $^{132-140}$Te have been measured with high precision (10 ppb) using the Penning trap mass spectrometer JYFLTRAP. Among these, the masses of four r-process nuclei $^{135}$Sn, $^{136}$Sb, and $^{139,140}$Te were measured for the first time. The data reveals a strong $N$=82 shell gap at $Z$=50 but indicates the importance of correlations for $Z>50$. An empirical neutron pairing gap expressed as the odd-even staggering of isotopic masses shows a strong quenching across $N$=82 for Sn, with the $Z$-dependence that is unexplainable by the current theoretical models.

nucl-ex↗

Q_EC values of the Superallowed beta-Emitters 10-C, 34-Ar, 38-Ca and 46-V

The Q_EC values of the superallowed beta+ emitters 10-C, 34-Ar, 38-Ca and 46-V have been measured with a Penning-trap mass spectrometer to be 3648.12(8), 6061.83(8), 6612.12(7) and 7052.44(10) keV, respectively. All four values are substantially improved in precision over previous results.

nucl-ex↗

Mass measurements in the vicinity of the doubly-magic waiting point 56Ni

Masses of 56,57Fe, 53Co^m, 53,56Co, 55,56,57Ni, 57,58Cu, and 59,60Zn have been determined with the JYFLTRAP Penning trap mass spectrometer at IGISOL with a precision of dm/m \le 3 x 10^{-8}. The QEC values for 53Co, 55Ni, 56Ni, 57Cu, 58Cu, and 59Zn have been measured directly with a typical precision of better than 0.7 keV and Coulomb displacement energies have been determined. The Q values for proton captures on 55Co, 56Ni, 58Cu, and 59Cu have been measured directly. The precision of the proton-capture Q value for 56Ni(p,gamma)57Cu, Q(p,gamma) = 689.69(51) keV, crucial for astrophysical rp-process calculations, has been improved by a factor of 37. The excitation energy of the proton emitting spin-gap isomer 53Co^m has been measured precisely, Ex = 3174.3(10) keV, and a Coulomb energy difference of 133.9(10) keV for the 19/2- state has been obtained. Except for 53Co, the mass values have been adjusted within a network of 17 frequency ratio measurements between 13 nuclides which allowed also a determination of the reference masses 55Co, 58Ni, and 59Cu.

nucl-ex↗

Mass Measurements and Implications for the Energy of the High-Spin Isomer in 94Ag

Nuclides in the vicinity of 94Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Separator On-Line. The masses of the two-proton-decay daughter 92Rh and the beta-decay daughter 94Pd of the high-spin isomer in 94Ag have been measured, and the masses of 93Pd and 94Ag have been deduced. When combined with the data from the one-proton or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in 94Ag, -46370(170) or -44970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.

nucl-ex↗

Electron-capture branch of 100Tc and tests of nuclear wave functions for double-beta decays

We present a measurement of the electron-capture branch of $^{100}$Tc. Our value, $B(\text{EC}) = (2.6 \pm 0.4) \times 10^{-5}$, implies that the $^{100}$Mo neutrino absorption cross section to the ground state of $^{100}$Tc is roughly one third larger than previously thought. Compared to previous measurements, our value of $B(\text{EC})$ prevents a smaller disagreement with QRPA calculations relevant to double-$β$ decay matrix elements.

nucl-ex↗

Mass measurements in the vicinity of the rp-process and the nu p-process paths with JYFLTRAP and SHIPTRAP

The masses of very neutron-deficient nuclides close to the astrophysical rp- and nu p-process paths have been determined with the Penning trap facilities JYFLTRAP at JYFL/Jyväskylä and SHIPTRAP at GSI/Darmstadt. Isotopes from yttrium (Z = 39) to palladium (Z = 46) have been produced in heavy-ion fusion-evaporation reactions. In total 21 nuclides were studied and almost half of the mass values were experimentally determined for the first time: 88Tc, 90-92Ru, 92-94Rh, and 94,95Pd. For the 95Pdm, (21/2^+) high-spin state, a first direct mass determination was performed. Relative mass uncertainties of typically $δm / m = 5 \times 10^{-8}$ were obtained. The impact of the new mass values has been studied in nu p-process nucleosynthesis calculations. The resulting reaction flow and the final abundances are compared to those obtained with the data of the Atomic Mass Evaluation 2003.

nucl-ex↗

Precise half-life measurement of the 26Si ground state

The beta-decay half-life of 26Si was measured with a relative precision of 1.4*10e3. The measurement yields a value of 2.2283(27) s which is in good agreement with previous measurements but has a precision that is better by a factor of 4. In the same experiment, we have also measured the non-analogue branching ratios and could determine the super-allowed one with a precision similar to the previously reported measurements. The experiment was done at the Accelerator Laboratory of the University of Jyvaskyla where we used the IGISOL technique with the JYFLTRAP facility to separate pure samples of 26Si.

nucl-ex↗

Evolution of the N=50 shell gap energy towards $^{78}$Ni

Atomic masses of the neutron-rich isotopes $^{76-80}$Zn, $^{78-83}$Ga, $^{80-85}Ge, $^{81-87}$As and $^{84-89}$Se have been measured with high precision using the Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. The masses of $^{82,83}$Ga, $^{83-85}$Ge, $^{84-87}$As and $^{89}$Se were measured for the first time. These new data represent a major improvement in the knowledge of the masses in this neutron-rich region. Two-neutron separation energies provide evidence for the reduction of the N=50 shell gap energy towards germanium Z=32 and a subsequent increase at gallium (Z=31). The data are compared with a number of theoretical models. An indication of the persistent rigidity of the shell gap towards nickel (Z=28) is obtained.

nucl-ex↗