arXiv subjects

T. Kuhn

Publications and source records attributed to T. Kuhn.

At least 37 records · Page 2Linked to original sources

arXiv2016

Evidence for a Strong Topological Insulator Phase in $\mathrm{ZrTe_5}$

The complex electronic properties of $\mathrm{ZrTe_5}$ have recently stimulated in-depth investigations that assigned this material to either a topological insulator or a 3D Dirac semimetal phase. Here we report a comprehensive experimental and theoretical study of both electronic and structural properties of $\mathrm{ZrTe_5}$, revealing that the bulk material is a strong topological insulator (STI). By means of angle-resolved photoelectron spectroscopy, we identify at the top of the valence band both a surface and a bulk state. The dispersion of these bands is well captured by ab initio calculations for the STI case, for the specific interlayer distance measured in our x-ray diffraction study. Furthermore, these findings are supported by scanning tunneling spectroscopy revealing the metallic character of the sample surface, thus confirming the strong topological nature of $\mathrm{ZrTe_5}$.

cond-mat.mtrl-sci↗

arXiv2016

Dynamics of excitons in individual InAs quantum dots revealed in four-wave mixing spectroscopy

A detailed understanding of the population and coherence dynamics in optically driven individual emitters in solids and their signatures in ultrafast nonlinear-optical signals is of prime importance for their applications in future quantum and optical technologies. In a combined experimental and theoretical study on exciton complexes in single semiconductor quantum dots we reveal a detailed picture of the dynamics employing three-beam polarization-resolved four-wave mixing (FWM) micro-spectroscopy. The oscillatory dynamics of the FWM signals in the exciton-biexciton system is governed by the fine-structure splitting and the biexciton binding energy in an excellent quantitative agreement between measurement and analytical description. The analysis of the excitation conditions exhibits a dependence of the dynamics on the specific choice of polarization configuration, pulse areas and temporal ordering of driving fields. The interplay between the transitions in the four-level exciton system leads to rich evolution of coherence and population. Using two-dimensional FWM spectroscopy we elucidate the exciton-biexciton coupling and identify neutral and charged exciton complexes in a single quantum dot. Our investigations thus clearly reveal that FWM spectroscopy is a powerful tool to characterize spectral and dynamical properties of single quantum structures.

cond-mat.mes-hall↗

arXiv2016

Fast and selective phonon-assisted state preparation of a quantum dot by adiabatic undressing

We investigate theoretically the temporal behavior of a quantum dot under off-resonant optical excitation targeted at fast acoustic phonon-assisted state preparation. We demonstrate that in a preparation process driven by short laser pulses three processes can be identified: a dressing of the states during the switch on of the laser pulse, a subsequent phonon-induced relaxation and an undressing at the end of the pulse. By analyzing excitation scenarios with different pulse shapes we highlight the decisive impact of an adiabatic undressing on the final state in short pulse protocols. Furthermore, we show that in exciton-biexciton systems the laser characteristics such as the pulse detuning and the pulse length as well as the biexciton binding energy can be used to select the targeted quantum dot state.

cond-mat.mes-hall↗

arXiv2015

Direct optical state preparation of the dark exciton in a quantum dot

Because of their weak coupling to the electromagnetic field dark excitons in semiconductor quantum dots possess extremely long lifetimes, which makes them attractive candidates for quantum information processing. On the other hand, preparation and manipulation of dark states is challenging, because commonly used optical excitation mechanisms are not applicable. We propose a new, efficient mechanism for the deterministic preparation of the dark exciton exploiting the application of a tilted magnetic field and the optical excitation with a chirped, i.e., frequency modulated, laser pulse.

cond-mat.mes-hall↗

arXiv2015

Coulomb mediated hybridization of excitons in artificial molecules

We report the Coulomb mediated hybridization of excitonic states in an optically active, artificial quantum dot molecule. By probing the optical response of the artificial molecule as a function of the static electric field applied along the molecular axis, we observe unexpected avoided level crossings that do not arise from the dominant single particle tunnel coupling. We identify a new few-particle coupling mechanism stemming from Coulomb interactions between different neutral exciton states. Such Coulomb resonances hybridize the exciton wave function over four different electron and hole single-particle orbitals. Comparisons of experimental observations with microscopic 8-band $k \cdot p$ calculations taking into account a realistic quantum dot geometry show good agreement and reveal that the Coulomb resonances arise from broken symmetry in the artificial molecule.

cond-mat.mes-hall↗

arXiv2014

Formulation of the twisted-light--matter interaction at the phase singularity: the twisted-light gauge

Twisted light is light carrying orbital angular momentum. The profile of such a beam is a ring-like structure with a node at the beam axis, where a phase singularity exits. Due to the strong spatial inhomogeneity the mathematical description of twisted-light--matter interaction is non-trivial, in particular close to the phase singularity, where the commonly used dipole-moment approximation cannot be applied. In this paper we show that, if the polarization and the orbital angular momentum of the twisted-light beam have the same sign, a Hamiltonian similar to the dipole-moment approximation can be derived. However, if the signs of polarization and orbital angular momentum differ, in general the magnetic parts of the light beam become of significant importance and an interaction Hamiltonian which only accounts for electric fields, as in the dipole-moment approximation, is inappropriate. We discuss the consequences of these findings for twisted-light excitation of a semiconductor nanostructures, e.g., a quantum dot, placed at the phase singularity.

physics.optics↗

arXiv2014

Higgs mode in the quench dynamics of a confined ultracold Fermi gas in the BCS regime

The Higgs amplitude mode of the order parameter of an ultracold confined Fermi gas in the BCS regime after a quench of the coupling constant is analyzed theoretically. Characteristic features are a damped oscillation which at a certain transition time changes into a rather irregular dynamics. We compare the numerical solution of the full set of nonlinear equations of motion for the normal and anomalous Bogoliubov quasiparticle excitations with a linearized approximation. In doing so the transition time as well as the difference between resonant systems, i.e., systems where the Fermi energy is close to a subband minimum, and off-resonant systems can be well understood and traced back to the system and geometry parameters.

cond-mat.quant-gas↗

arXiv2014

The role of phonons for exciton and biexciton generation in an optically driven quantum dot

For many applications of semiconductor quantum dots in quantum technology a well controlled state preparation of the quantum dot states is mandatory. Since quantum dots are embedded in the semiconductor matrix, the interaction with phonons plays often a major role in the preparation process. In this review, we discuss the influence of phonons on three basically different optical excitation schemes which can be used for the preparation of exciton, biexciton, and superposition states: a resonant excitation leading to Rabi rotations in the excitonic system, an excitation with chirped pulses exploiting the effect of adiabatic rapid passage, and an off-resonant excitation giving rise to a phonon-assisted state preparation. We give an overview over experimental and theoretical results showing the role of the phonons and compare the performance of the schemes for state preparation.

cond-mat.mes-hall↗

arXiv2014

Energy transport and coherence properties of acoustic phonons generated by optical excitation of a quantum dot

The energy transport of acoustic phonons generated by the optical excitation of a quantum dot as well as the coherence properties of these phonons are studied theoretically both for the case of a pulsed excitation and for a continuous wave (cw) excitation switched on instantaneously. For a pulsed excitation, depending on pulse area and pulse duration, a finite number of phonon wave packets is emitted, while for the case of a cw excitation a sequence of wave packets with decreasing amplitude is generated after the excitation has been switched on. We show that the energy flow associated with the generated phonons is partly related to coherent phonon oscillations and partly to incoherent phonon emission. The efficiency of the energy transfer to the phonons and the details of the energy flow depend strongly and in a non-monotonic way on the Rabi frequency exhibiting a resonance behavior. However, in the case of cw excitation it turns out that the total energy transferred to the phonons is directly linked in a monotonic way to the Rabi frequency.

cond-mat.mes-hall↗

arXiv2014

Light-hole transitions in quantum dots: realizing full control by highly focused optical-vortex beams

An optical-vortex is an inhomogeneous light beam having a phase singularity at its axis, where the intensity of the electric and/or magnetic field may vanish. Already well studied are the paraxial beams, which are known to carry well defined values of spin (polarization $σ$) and orbital angular momenta; the orbital angular momentum per photon is given by the topological charge $\ell$ times the Planck constant. Here we study the light-hole--to--conduction band transitions in a semiconductor quantum dot induced by a highly-focused beam originating from a $\ell=1$ paraxial optical vortex. We find that at normal incidence the pulse will produce two distinct types of electron--hole pairs, depending on the relative signs of $σ$ and $\ell$. When sign($σ$)$=$sign($\ell$), the pulse will create electron--hole pairs with band+spin and envelope angular momenta both equal to one. In contrast, for sign($σ$)$\neq$sign($\ell$), the electron-hole pairs will have neither band+spin nor envelope angular momenta. A tightly-focused optical-vortex beam thus makes possible the creation of pairs that cannot be produced with plane waves at normal incidence. With the addition of co-propagating plane waves or switching techniques to change the charge $\ell$ both the band+spin and the envelope angular momenta of the pair wave-function can be precisely controlled. We discuss possible applications in the field of spintronics that open up.

cond-mat.mes-hall↗

arXiv2013

Excitons in quantum dot molecules: Coulomb coupling, spin-orbit effects and phonon-induced line broadening

Excitonic states and the line shape of optical transitions in coupled quantum dots (quantum dot molecules) are studied theoretically. For a pair of electrically tunable, vertically aligned quantum dots we investigate the coupling between spatially direct and indirect excitons caused by different mechanisms such as tunnel coupling, Coulomb coupling, coupling due to the spin-orbit interaction and coupling induced by a structural asymmetry. The peculiarities of the different types of couplings are reflected in the appearance of either crossings or avoided crossings between direct and indirect excitons, the latter ones being directly visible in the absorption spectrum. We analyze the influence of the phonon environment on the spectrum by calculating the line shape of the various optical transitions including contributions due to both pure dephasing and phonon-induced transitions between different exciton states. The line width enhancement due to phonon-induced transitions is particularly pronounced in the region of an anticrossing and it strongly depends on the energy splitting between the two exciton branches.

cond-mat.mes-hall↗

arXiv2013

Adiabatic rapid passage in quantum dots: phonon-assisted decoherence and biexciton generation

We study the evolution of a quantum dot controlled by a frequency-swept (chirped), linearly polarized laser pulse in the presence of carrier-phonon coupling. The final occupation of the exciton state is limited both due to phonon-induced transitions between the adiabatic spectral branches and because of phonon-assisted transitions to the biexciton state. When the biexciton shift is large enough, the quantum dot can be modeled as a two-level system, which corresponds to excitation with circularly polarized light. For this case, we compare different methods of simulations: (i) a time convolutionless method, (ii) correlation expansion and (iii) path integrals. We show that results obtained from these methods agree perfectly at low temperatures.

cond-mat.mes-hall↗

arXiv2013

Competition between loss channels in quantum-dot cavity systems: unconventional consequences

We demonstrate that in quantum-dot cavity systems, the interplay between acoustic phonons and photon losses introduces novel features and characteristic dependencies in the system dynamics. In particular, the combined action of both loss mechanisms strongly affects the transition from the weak to the strong coupling regime as well as the shape of Mollow-type spectra in untypical ways. For weak coupling, where the spectra degenerate to a single line, we predict that their widths decrease with rising temperature.

cond-mat.mes-hall↗

arXiv2013

Spin dynamics in p-doped semiconductor nanostructures subject to a magnetic field tilted from the Voigt geometry

We develop a theoretical description of the spin dynamics of resident holes in a p-doped semiconductor quantum well (QW) subject to a magnetic field tilted from the Voigt geometry. We find the expressions for the signals measured in time-resolved Faraday rotation (TRFR) and resonant spin amplification (RSA) experiments and study their behavior for a range of system parameters. We find that an inversion of the RSA peaks can occur for long hole spin dephasing times and tilted magnetic fields. We verify the validity of our theoretical findings by performing a series of TRFR and RSA experiments on a p-modulation doped GaAs/Al_{0.3}Ga_{0.7}As single QW and showing that our model can reproduce experimentally observed signals.

cond-mat.mes-hall↗

arXiv2013

Optical signals of spin switching using the optical Stark effect in a Mn doped quantum dot

The optically induced spin dynamics of a single Mn atom embedded into a single semiconductor quantum dot can be strongly influenced by using the optical Stark effect. The exchange interaction gives rise to simultaneous spin flips between the quantum dot electron and Mn. In the time domain these flips correspond to exchange induced Rabi oscillations, which are typically off-resonant. By applying a detuned laser pulse, the states involved in the flipping can be brought into resonance by means of the optical Stark effect increasing the amplitude of the Rabi oscillations to one. In this paper we study theoretically how this spin dynamics can be monitored in time-resolved spectroscopy. In the spectrum the exchange interaction leads to a splitting of the exciton line into six lines, each corresponding to one of the six Mn spin states. The dynamical behavior of the Mn spin is reflected by the strength of the individual lines as a function of time. When an off-resonant optical pulse is applied the spectral positions of the lines shift, but still the flipping dynamics is visible.

cond-mat.mes-hall↗

arXiv2013

Phonon Effects on Population Inversion in Quantum Dots: Resonant, Detuned and Frequency-swept Excitations

The effect of acoustic phonons on different light-induced excitations of a semiconductor quantum dot is investigated. Resonant excitation of the quantum dot leads to Rabi oscillations, which are damped due to the phonon interaction. When the excitation frequency is detuned, an occupation can only occur due to phonon absorption or emission processes. For frequency-swept excitations a population inversion is achieved through adiabatic rapid passage, but the inversion is also damped by phonons. For all three scenarios the influence of the phonons depends non-monotonically on the pulse area.

cond-mat.mes-hall↗

arXiv2013

Fluctuation properties of acoustic phonons generated by ultrafast optical excitation of a quantum dot

We study theoretically the fluctuation properties of acoustic phonons created in a semiconductor quantum dot after ultrafast optical excitation. An excitation with a single ultrafast pulse creates an exciton confined to the quantum dot, which is coupled to longitudinal acoustic phonons. This leads to the formation of a polaron in the quantum dot accompanied by the emission of a phonon wave packet. We show that the fluctuations of the lattice displacement associated with the wave packet after a single laser pulse excitation in resonance with the exciton transition are always larger than their respective vacuum values. Manipulating the exciton with a second pulse can result in a reduction of the fluctuations below their vacuum limit, which means that the phonons are squeezed. We show that the squeezing properties of the wave packet strongly depend on the relative phase and the time delay between the two laser pulses.

cond-mat.mes-hall↗

arXiv2012

Biexciton state preparation in a quantum dot via adiabatic rapid passage: comparison between two control protocols and impact of phonon-induced dephasing

We investigate theoretically under which conditions a stable and high-fidelity preparation of the biexciton state in a quantum dot can be realized by means of adiabatic rapid passage in the presence of acoustic phonon coupling. Our analysis is based on a numerically complete real-time path integral approach and comprises different schemes of optical driving using frequency-swept (chirped) pulses. We show that depending on the size of the biexciton binding energy, resonant two-photon excitations or two-color schemes can be favorable. It is demonstrated that the carrier-phonon interaction strongly affects the efficiency of the protocols and that a robust preparation of the biexciton is restricted to positive chirps and low temperatures. A considerable increase of the biexciton yield can be achieved realizing temperatures below 4 K.

cond-mat.mes-hall↗