arXiv subjects

T. Kurosawa

Publications and source records attributed to T. Kurosawa.

33 records · Page 2Linked to original sources

arXiv2019

Link between magnetism and resistivity upturn in cuprates: a thermal conductivity study of La$_{2-x}$Sr$_x$CuO$_4$

A key unexplained feature of cuprate superconductors is the upturn in their normal state electrical resistivity $ρ(T)$ seen at low temperature inside the pseudogap phase. We examined this issue via measurements of the thermal conductivity $κ(T)$ down to 50 mK and in fields up to 17 T on the cuprate La$_{2-x}$Sr$_x$CuO$_4$ at dopings $p = 0.13$, 0.136, 0.143 and 0.18. At $p$ = 0.136, 0.143, and 0.18, we observe an initial increase of the electronic thermal conductivity $κ_0/T$ as a function of field, as expected in a $d$-wave superconductor. For $p$ = 0.136 and 0.143, further increasing the field then leads to a decrease of $κ_0/T$, which correlates with the onset of spin density-wave order as observed in neutron scattering experiments on the same samples. This decrease of $κ_0/T$ with field is imposed by the Wiedemann-Franz law and the high value of the resistivity in the high-field normal state of these samples. Our study therefore provides a direct link between magnetism and the resistivity upturn in the pseudogap phase of cuprates. We discuss this scenario in the broader context of other cuprates.

cond-mat.supr-con↗

arXiv2018

Incommensurate Chiral CDW in $1T$-VSe$_2$

We have investigated the chiral charge-density wave (CDW) in $1T$-VSe$_2$ using scanning tunneling microscopy (STM) measurements and optical polarimetry measurements. With the STM mesurements, we revealed that the CDW intensities along each triple-$q$ directions are different. Thus the rotational symmetry of $1T$-VSe$_2$ is lower than that in typical two-dimentional triple-$q$ CDWs. We found that the CDW peaks form a kagome lattice rather than a triangular lattice. The Friedel oscillations have the chirality and the periodicity reflected properties of the background CDW. With the optical measurements in $1T$-VSe$_2$, we also observed a lower rotational symmetry with the polarization dependence of the transient reflectivity variation, which is consistent with the STM result on a microscopic scale. Both $1T$-TiSe$_2$ and $1T$-VSe$_2$ show chiral CDWs, which implies that such waves are usual for CDWs with the condition $H_\mathrm{CDW} \equiv q_{1}\cdot(q_{2} \times q_{3}) \neq0$.

cond-mat.str-el↗

arXiv2018

Direct Observation of Orbital Hybridisation in a Cuprate Superconductor

The minimal ingredients to explain the essential physics of layered copper-oxide (cuprates= materials remains heavily debated. Effective low energy single-band models of the copper-oxygen orbitals are widely used because there exists no strong experimental evidence supporting multiband structures. Here we report angle-resolved photoelectron spectroscopy experiments on La-based cuprates that provide direct observation of a two-band structure. This electronic structure, qualitatively consistent with density functional theory, is parametrised by a two-orbital ($d_{x^2-y^2}$ and $d_{z^2}$) tight-binding model. We quantify the orbital hybridisation which provides an explanation for the Fermi surface topology and the proximity of the van-Hove singularity to the Fermi level. Our analysis leads to a unification of electronic hopping parameters for single-layer cuprates and we conclude that hybridisation, restraining d-wave pairing, is an important optimisation element for superconductivity.

cond-mat.supr-con↗

arXiv2017

Pseudogap phase of cuprate superconductors confined by Fermi surface topology

The properties of cuprate high-temperature superconductors are largely shaped by competing phases whose nature is often a mystery. Chiefly among them is the pseudogap phase, which sets in at a doping $p^*$ that is material-dependent. What determines $p^*$ is currently an open question. Here we show that the pseudogap cannot open on an electron-like Fermi surface, and can only exist below the doping $p_{FS}$ at which the large Fermi surface goes from hole-like to electron-like, so that $p^*$ $\leq$ $p_{FS}$. We derive this result from high-magnetic-field transport measurements in La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ under pressure, which reveal a large and unexpected shift of $p^*$ with pressure, driven by a corresponding shift in $p_{FS}$. This necessary condition for pseudogap formation, imposed by details of the Fermi surface, is a strong constraint for theories of the pseudogap phase. Our finding that $p^*$ can be tuned with a modest pressure opens a new route for experimental studies of the pseudogap.

cond-mat.supr-con↗

arXiv2017

Dynamics of the superconducting order parameter through ultrafast normal-to-superconducting phase transition in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ from multi-pulse polarization-resolved transient optical reflectivity

A systematic temperature dependent study of the femtosecond optical superconducting (SC) state destruction and recovery in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ cuprate superconductor by means of the all-optical polarization-sensitive multi-pulse spectroscopy is presented. At low temperatures and a partial SC state suppression an anisotropic SC-gap recovery-timescale is suggested by the data. The SC state destruction and recovery dynamics are compared to the recent TR-ARPES-inferred SC-gap dynamics and a qualitative agreement is found. Using a phenomenological response function the experimental data are also compared to time dependent Ginzburg-Landau model simulations.

cond-mat.supr-con↗

arXiv2017

Damped spin excitations in a doped cuprate superconductor with orbital hybridization

A resonant inelastic x-ray scattering (RIXS) study of overdamped spin-excitations in slightly underdoped La$_{2-x}$Sr$_{x}$CuO$_4$ (LSCO) with $x=0.12$ and $0.145$ is presented. Three high-symmetry directions have been investigated: (1) the antinodal $(0,0)\rightarrow (1/2,0)$, (2) the nodal $(0,0)\rightarrow (1/4,1/4)$ and (3) the zone boundary direction $(1/2,0)\rightarrow (1/4,1/4)$ connecting these two. The overdamped excitations exhibit strong dispersions along (1) and (3), whereas a much more modest dispersion is found along (2). This is in strong contrast to the undoped compound La$_{2}$CuO$_4$ (LCO) for which the strongest dispersions are found along (1) and (2). The $t-t^{\prime}-t^{\prime\prime}-U$ Hubbard model used to explain the excitation spectrum of LCO predicts $-$ for constant $U/t$ $-$ that the dispersion along (3) scales with $(t^{\prime}/t)^2$. However, the diagonal hopping $t^{\prime}$ extracted on LSCO using single-band models is low ($t^{\prime}/t\sim-0.16$) and decreasing with doping. We therefore invoked a two-orbital ($d_{x^2-y^2}$ and $d_{z^2}$) model which implies that $t^{\prime}$ is enhanced. This effect acts to enhance the zone-boundary dispersion within the Hubbard model. We thus conclude that hybridization of $d_{x^2-y^2}$ and $d_{z^2}$ states has a significant impact on the zone-boundary dispersion in LSCO.

cond-mat.supr-con↗

arXiv2017

Rotation symmetry breaking in La2-xSrxCuO4 revealed by ARPES

Using angle-resolved photoemission spectroscopy it is revealed that in the vicinity of optimal doping the electronic structure of La2-xSrxCuO4 cuprate undergoes an electronic reconstruction associated with a wave vector q_a=(pi, 0). The reconstructed Fermi surface and folded band are distinct to the shadow bands observed in BSCCO cuprates and in underdoped La2-xSrxCuO4 with x <= 0.12, which shift the primary band along the zone diagonal direction. Furthermore the folded bands appear only with q_a=(pi, 0) vector, but not with q_b= (0, pi). We demonstrate that the absence of q_b reconstruction is not due to the matrix-element effects in the photoemission process, which indicates the four-fold symmetry is broken in the system.

cond-mat.supr-con↗

arXiv2016

Origin of the metal-to-insulator crossover in cuprate superconductors

Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprates at low temperature, but its origin has remained a puzzle. Here we propose that this 'metal-to-insulator crossover' is due to a drop in carrier density n associated with the onset of the pseudogap phase at a critical doping p*. We use high-field resistivity measurements on LSCO to show that the upturns are quantitatively consistent with a drop from n=1+p above p* to n=p below p*, in agreement with high-field Hall data in YBCO. We demonstrate how previously reported upturns in the resistivity of LSCO, YBCO and Nd-LSCO are explained by the same universal mechanism: a drop in carrier density by 1.0 hole per Cu atom.

cond-mat.supr-con↗

arXiv2015

Electron scattering, charge order, and pseudogap physics in La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$: An angle resolved photoemission spectroscopy study

We report an angle-resolved photoemission study of the charge stripe ordered La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ system. A comparative and quantitative line shape analysis is presented as the system evolves from the overdoped regime into the charge ordered phase. On the overdoped side ($x=0.20$), a normal state anti-nodal spectral gap opens upon cooling below ~ 80 K. In this process spectral weight is preserved but redistributed to larger energies. A correlation between this spectral gap and electron scattering is found. A different lineshape is observed in the antinodal region of charge ordered Nd-LSCO $x=1/8$. Significant low-energy spectral weight appears to be lost. These observations are discussed in terms of spectral weight redistribution and gapping %of spectral weight originating from charge stripe ordering.

cond-mat.supr-con↗

arXiv2013

Dynamics of broken symmetry nodal and anti-nodal excitations in Bi_{2} Sr_{2} CaCu_{2} O_{8+δ} probed by polarized femtosecond spectroscopy

The dynamics of excitations with different symmetry is investigated in the superconducting (SC) and normal state of the high-temperature superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ (Bi2212) using optical pump-probe (Pp) experiments with different light polarizations at different doping levels. The observation of distinct selection rules for SC excitations, present in A$_{\rm 1g}$ and B$_{\rm 1g}$ symmetries, and for the PG excitations, present in A$_{\rm 1g}$ and B$_{\rm 2g}$ symmetries, by the probe and absence of any dependence on the pump beam polarization leads to the unequivocal conclusion of the existence of a spontaneous spatial symmetry breaking in the pseudogap (PG) state.

cond-mat.supr-con↗

arXiv2012

Ni-impurity effects on the superconducting gap of La$_{2-x}$Sr$_{x}$CuO$_4$ studied from the magnetic field and temperature dependence of the electronic specific heat

The magnetic field and temperature dependence of the electronic specific heat $C_{\rm el}$ have been systematically investigated in $\rm La_{2-{\it x}}Sr_{\it x}Cu_{1-{\it y}}Ni_{\it y}O_4$ (LSCNO) in order to study Ni-impurity effects on the superconducting (SC) gap. In LSCNO with $x$=0.15 and $y$=0.015, the value of $γ$ ($\equiv C_{\rm el}/T$) at $T$=0 K, $γ_0$, is enhanced under the magnetic field $H$ applied along the $\bm c$-axis. The increment of $γ_0$, $Δγ_0$, follows the Volovik relation $Δγ_0$=$A\sqrt{H}$, characteristic of the SC gap with line nodes, with prefactor $A$ similar to that of a pure sample. The $C_{\rm el}/T$ vs. $T$ curve under $H$=0 shows a d-wave-like SC anomaly with an abrupt increase at $T_{\rm c}$ and $T$-linear dependence at $T$$\ll$$T_{\rm c}$, although the $γ_0$-value in the $C_{\rm el}/T$ vs. $T$ curve increases with increasing Ni concentrations. Interestingly, as the SC part of $C_{\rm el}/T$, $C_{\rm el}/T$$-$$γ_0$$\equiv$$γ_{\rm s}$, decreases in LSCNO, $T_{\rm c}$ is reduced in proportion to the decrease of $γ_{\rm s}$. These findings can be explained phenomenologically by a simple model in which Ni impurities bring about strong pair breaking at the edges of the coherent nodal part of the Fermi surface but in the vicinity of the nodes of the SC gap. The reduction of the SC condensation energy $U_0$ in LSCNO, evaluated from $C_{\rm el}$ at $T$ {0.3em}\raisebox{0.4ex}{$<$} {-0.75em}\raisebox{-.7ex}{$\sim$} {0.3em}$T_{\rm c}$, is also understood by the same model.

cond-mat.supr-con↗

arXiv2012

Spin density wave induced disordering of the vortex lattice in superconducting La$_{2-x}$Sr$_x$CuO$_4$

We use small angle neutron scattering to study the superconducting vortex lattice in La$_{2-x}$Sr$_x$CuO$_4$ as a function of doping and magnetic field. We show that near optimally doping the vortex lattice coordination and the superconducting coherence length $ξ$ are controlled by a van-Hove singularity crossing the Fermi level near the Brillouin zone boundary. The vortex lattice properties change dramatically as a spin-density-wave instability is approached upon underdoping. The Bragg glass paradigm provides a good description of this regime and suggests that SDW order acts as a novel source of disorder on the vortex lattice.

cond-mat.supr-con↗

arXiv2010

STM/STS study on large pseudogap and nodal superconducting gap in Bi2201(La) and Bi2212

In the present work, scanning tunneling microscopy/spectroscopy (STM/STS) measurements were carried out on underdoped $\rm Bi_2Sr_{2-{\it x}}La_{\it x}CuO_{6+δ}$ and $\rm Bi_2Sr_2CaCu_2O_{8+δ}$ to clarify the origin of the pseudogap, in particular, the inhomogeneous large pseudogap. The nodal part of a d-wave pairing gap, which is under no influence of the inhomogeneous large pseudogap, was also examined by relating the homogeneous bottom part of the STS gap to a nodal d-wave gap in momentum space. We report that the inhomogeneous large pseudogap in the antinodal region links to a two-dimensional electronic charge order, and that the gap size of the nodal d-wave part $\rm Δ_{sc}$ scales with the superconducting critical temperature $\rm {\it T}_c$ in the pseudogap regime.

cond-mat.supr-con↗

arXiv2010

Chiral charge-density-waves

We discovered the chirality of charge density waves (CDW) in 1T-TiSe$_2$ by using scanning tunnelling microscopy (STM) and optical ellipsometry. We found that the CDW intensity becomes $I{a_1}:I{a_2}:I{a_3} = 1:0.7 \pm 0.1:0.5 \pm 0.1$, where $Ia_i$ (i =1, 2, 3) is the amplitude of the tunnelling current contributed by the CDWs. There were two states, in which the three intensity peaks of the CDW decrease \textit{clockwise} and \textit{anticlockwise} when we index each nesting vector in order of intensity in the Fourier transformation of the STM images. The chirality in CDW results in the three-fold symmetry breaking. Macroscopically, two-fold symmetry was indeed observed in optical measurement. We propose the new generalized CDW chirality $H_{CDW} \equiv {\boldmath $q_1$} \cdot ({\boldmath $q_2$}\times {\boldmath $q_3$})$, where ${\boldmath $q_i$}$ are the nesting vectors, which is independent of the symmetry of components. The nonzero $H_{CDW}$ - the triple-${\boldmath $q$}$ vectors do not exist in an identical plane in the reciprocal space - should induce a real-space chirality in CDW system.

cond-mat.other↗

arXiv2007

Electronic Charge Order in the Pseudogap State of $Bi_2 Sr_2 Ca Cu_2 O_{8+δ}$

Scanning tunneling microscopy/spectroscopy is used to examine the $4a$$\times$$4a$ electronic charge order (CO) in the pseudogap (PG) state above {\it T}$_{\rm c}$ on Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$. It is demonstrated that the static CO develops markedly in the inhomogeneous PG state, while it is very weak in the homogeneous PG state. We suggest that this static CO, which is considered to be stabilized by the pinning of the dynamically fluctuating CO, will remain below {\it T}$_{\rm c}$, together with the inhomogeneous gap structure, and coexist with the superconductivity.

cond-mat.supr-con↗