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T. Szücs

Publications and source records attributed to T. Szücs.

At least 55 records · Page 3Linked to original sources

Investigation of $α$-induced reactions on Sb isotopes relevant to the astrophysical $γ$-process

The aim of the present work is to measure the $^{121}$Sb($α,γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reaction cross sections. The $α$-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The ($α$,$γ$) cross sections of $^{121}$Sb were measured and are reported for first time. To determine the cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reactions, the yields of $γ$-rays following the $β$-decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic X-rays were counted with a LEPS (Low Energy Photon Spectrometer) detector. The cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I and $^{123}$Sb($α$,n)$^{126}$I reactions were measured with high precision in an energy range between 9.74 MeV to 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The ($α$,n) data show that the $α$ widths are predicted well for these reactions. The ($α$,$γ$) results are overestimated by the calculations but this is due to the applied neutron- and $γ$ widths. Relevant for the astrophysical reaction rate is the $α$ width used in the calculations.While for other reactions the $α$ widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.

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A high-efficiency gas target setup for underground experiments, and redetermination of the branching ratio of the 189.5 keV $\mathbf{^{22}Ne(p,γ)^{23}Na}$ resonance

The experimental study of nuclear reactions of astrophysical interest is greatly facilitated by a low-background, high-luminosity setup. The Laboratory for Underground Nuclear Astrophysics (LUNA) 400 kV accelerator offers ultra-low cosmic-ray induced background due to its location deep underground in the Gran Sasso National Laboratory (INFN-LNGS), Italy, and high intensity, 250-500 $μ$A, proton and $α$ ion beams. In order to fully exploit these features, a high-purity, recirculating gas target system for isotopically enriched gases is coupled to a high-efficiency, six-fold optically segmented bismuth germanate (BGO) $γ$-ray detector. The beam intensity is measured with a beam calorimeter with constant temperature gradient. Pressure and temperature measurements have been carried out at several positions along the beam path, and the resultant gas density profile has been determined. Calibrated $γ$-intensity standards and the well-known $E_p$ = 278 keV $\mathrm{^{14}N(p,γ)^{15}O}$ resonance were used to determine the $γ$-ray detection efficiency and to validate the simulation of the target and detector setup. As an example, the recently measured resonance at $E_p$ = 189.5 keV in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction has been investigated with high statistics, and the $γ$-decay branching ratios of the resonance have been determined.

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Nuclear physics uncertainties of the astrophysical gamma-process studied through the 64Zn(p,alpha)61Cu and 64Zn(p,gamma)65Ga reactions

In a recent work, the cross section measurement of the 64Zn(p,alpha)61Cu reaction was used to prove that the standard alpha-nucleus optical potentials used in astrophysical network calculation fail to reproduce the experimental data at energies relevant for heavy element nucleosynthesis. In the present paper the analysis of the obtained experimental data is continued by comparing the results with the predictions using different parameters. It is shown that the recently suggested modification of the standard optical potential leads to a better description of the data.

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Cross section of $α$-induced reactions on iridium isotopes obtained from thick target yield measurement for the astrophysical $γ$ process

The stellar reaction rates of radiative $α$-capture reactions on heavy isotopes are of crucial importance for the $γ$ process network calculations. These rates are usually derived from statistical model calculations, which need to be validated, but the experimental database is very scarce. This paper presents the results of $α$-induced reaction cross section measurements on iridium isotopes carried out at first close to the astrophysically relevant energy region. Thick target yields of $^{191}$Ir($α$,$γ$)$^{195}$Au, $^{191}$Ir($α$,n)$^{194}$Au, $^{193}$Ir($α$,n)$^{196m}$Au, $^{193}$Ir($α$,n)$^{196}$Au reactions have been measured with the activation technique between E$_α= 13.4$ MeV and 17 MeV. For the first time the thick target yield was determined with X-ray counting. This led to a previously unprecedented sensitivity. From the measured thick target yields, reaction cross sections are derived and compared with statistical model calculations. The recently suggested energy-dependent modification of the $α$+nucleus optical potential gives a good description of the experimental data.

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Astrophysical S-factor of the $^{14}\textrm{N(p,}γ\textrm{)}^{15}\textrm{O}$ reaction at 0.4 -- 1.3\,MeV

The $^{14}\textrm{N(p,}γ\textrm{)}^{15}\textrm{O}$ reaction is the slowest reaction of the carbon-nitrogen cycle of hydrogen burning and thus determines its rate. The precise knowledge of its rate is required to correctly model hydrogen burning in asymptotic giant branch stars. In addition, it is a necessary ingredient for a possible solution of the solar abundance problem by using the solar $^{13}$N and $^{15}$O neutrino fluxes as probes of the carbon and nitrogen abundances in the solar core. After the downward revision of its cross section due to a much lower contribution by one particular transition, capture to the ground state in $^{15}$O, the evaluated total uncertainty is still 8\%, in part due to an unsatisfactory knowledge of the excitation function over a wide energy range. The present work reports precise S-factor data at twelve energies between 0.357-1.292~MeV for the strongest transition, capture to the 6.79~MeV excited state in $^{15}$O, and at ten energies between 0.479-1.202~MeV for the second strongest transition, capture to the ground state in $^{15}$O. An R-matrix fit is performed to estimate the impact of the new data on astrophysical energies. The recently suggested slight enhancement of the 6.79~MeV transition at low energy could not be confirmed. The present extrapolated zero-energy S-factors are $S_{6.79}(0)$~=~1.24$\pm$0.11~keV~barn and $S_{\rm GS}(0)$~=~0.19$\pm$0.05~keV~barn.

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Cross section measurement of the astrophysically important 17O(p,gamma)18F reaction in a wide energy range

The 17O(p,g)18F reaction plays an important role in hydrogen burning processes in different stages of stellar evolution. The rate of this reaction must therefore be known with high accuracy in order to provide the necessary input for astrophysical models. The cross section of 17O(p,g)18F is characterized by a complicated resonance structure at low energies. Experimental data, however, is scarce in a wide energy range which increases the uncertainty of the low energy extrapolations. The purpose of the present work is therefore to provide consistent and precise cross section values in a wide energy range. The cross section is measured using the activation method which provides directly the total cross section. With this technique some typical systematic uncertainties encountered in in-beam gamma-spectroscopy experiments can be avoided. The cross section was measured between 500 keV and 1.8 MeV proton energies with a total uncertainty of typically 10%. The results are compared with earlier measurements and it is found that the gross features of the 17O(p,g)18F excitation function is relatively well reproduced by the present data. Deviation of roughly a factor of 1.5 is found in the case of the total cross section when compared with the only one high energy dataset. At the lowest measured energy our result is in agreement with two recent datasets within one standard deviation and deviates by roughly two standard deviations from a third one. An R-matrix analysis of the present and previous data strengthen the reliability of the extrapolated zero energy astrophysical S-factor. Using an independent experimental technique, the literature cross section data of 17O(p,g)18F is confirmed in the energy region of the resonances while lower direct capture cross section is recommended at higher energies. The present dataset provides a constraint for the theoretical cross sections.

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Origin of meteoritic stardust unveiled by a revised proton-capture rate of $^{17}$O

Stardust grains recovered from meteorites provide high-precision snapshots of the isotopic composition of the stellar environment in which they formed. Attributing their origin to specific types of stars, however, often proves difficult. Intermediate-mass stars of 4-8 solar masses are expected to contribute a large fraction of meteoritic stardust. However, no grains have been found with characteristic isotopic compositions expected from such stars. This is a long-standing puzzle, which points to serious gaps in our understanding of the lifecycle of stars and dust in our Galaxy. Here we show that the increased proton-capture rate of $^{17}$O reported by a recent underground experiment leads to $^{17}$O/$^{16}$O isotopic ratios that match those observed in a population of stardust grains, for proton-burning temperatures of 60-80 million K. These temperatures are indeed achieved at the base of the convective envelope during the late evolution of intermediate-mass stars of 4-8 solar masses, which reveals them as the most likely site of origin of the grains. This result provides the first direct evidence that these stars contributed to the dust inventory from which the Solar System formed.

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$α$-scattering and $α$-induced reaction cross sections of $^{64}$Zn at low energies

Background: alpha-nucleus potentials play an essential role for the calculation of alpha-induced reaction cross sections at low energies in the statistical model... Purpose: The present work studies the total reaction cross section sigma_reac of alpha-induced reactions at low energies which can be determined from the elastic scattering angular distribution or from the sum over the cross sections of all open non-elastic channels. Method: Elastic and inelastic 64Zn(a,a)64Zn angular distributions were measured at two energies around the Coulomb barrier at 12.1 MeV and 16.1 MeV. Reaction cross sections of the (a,g), (a,n), and (a,p) reactions were measured at the same energies using the activation technique. The contributions of missing non-elastic channels were estimated from statistical model calculations. Results: The total reaction cross sections from elastic scattering and from the sum of the cross sections over all open non-elastic channels agree well within the uncertainties. This finding confirms the consistency of the experimental data. At the higher energy of 16.1 MeV, the predicted significant contribution of compound-inelastic scattering to the total reaction cross section is confirmed experimentally. As a by-product it is found that most recent global alpha-nucleus potentials are able to describe the reaction cross sections for 64Zn around the Coulomb barrier. Conclusions: Total reaction cross sections of alpha-induced reactions can be well determined from elastic scattering angular distributions. The present study proves experimentally that the total cross section from elastic scattering is identical to the sum of non-elastic reaction cross sections. Thus, the statistical model can reliably be used to distribute the total reaction cross section among the different open channels.

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Direct measurement of low-energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction is the most uncertain process in the neon-sodium cycle of hydrogen burning. At temperatures relevant for nucleosynthesis in asymptotic giant branch stars and classical novae, its uncertainty is mainly due to a large number of predicted but hitherto unobserved resonances at low energy. Purpose: A new direct study of low energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances has been performed at the Laboratory for Underground Nuclear Astrophysics (LUNA), in the Gran Sasso National Laboratory, Italy. Method: The proton capture on $^{22}$Ne was investigated in direct kinematics, delivering an intense proton beam to a $^{22}$Ne gas target. $γ$ rays were detected with two high-purity germanium detectors enclosed in a copper and lead shielding suppressing environmental radioactivity. Results: Three resonances at 156.2 keV ($ωγ$ = (1.48\,$\pm$\,0.10)\,$\cdot$\,10$^{-7}$ eV), 189.5 keV ($ωγ$ = (1.87\,$\pm$\,0.06)\,$\cdot$\,10$^{-6}$ eV) and 259.7 keV ($ωγ$ = (6.89\,$\pm$\,0.16)\,$\cdot$\,10$^{-6}$ eV) proton beam energy, respectively, have been observed for the first time. For the levels at 8943.5, 8975.3, and 9042.4 keV excitation energy corresponding to the new resonances, the $γ$-decay branching ratios have been precisely measured. Three additional, tentative resonances at 71, 105 and 215 keV proton beam energy, respectively, were not observed here. For the strengths of these resonances, experimental upper limits have been derived that are significantly more stringent than the upper limits reported in the literature. Conclusions: Based on the present experimental data and also previous literature data, an updated thermonuclear reaction rate is provided in tabular and parametric form. The new reaction rate is significantly higher than previous evaluations at temperatures of 0.08-0.3 GK.

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Experimental study of the astrophysical gamma-process reaction 124Xe(alpha,gamma)128Ba

The synthesis of heavy, proton rich isotopes in the astrophysical gamma-process proceeds through photodisintegration reactions. For the improved understanding of the process, the rates of the involved nuclear reactions must be known. The reaction 128Ba(g,a)124Xe was found to affect the abundance of the p nucleus 124Xe. Since the stellar rate for this reaction cannot be determined by a measurement directly, the aim of the present work was to measure the cross section of the inverse 124Xe(a,g)128Ba reaction and to compare the results with statistical model predictions. Of great importance is the fact that data below the (a,n) threshold was obtained. Studying simultaneously the 124Xe(a,n)127Ba reaction channel at higher energy allowed to further identify the source of a discrepancy between data and prediction. The 124Xe + alpha cross sections were measured with the activation method using a thin window 124Xe gas cell. The studied energy range was between E = 11 and 15 MeV close above the astrophysically relevant energy range. The obtained cross sections are compared with statistical model calculations. The experimental cross sections are smaller than standard predictions previously used in astrophysical calculations. As dominating source of the difference, the theoretical alpha width was identified. The experimental data suggest an alpha width lower by at least a factor of 0.125 in the astrophysical energy range. An upper limit for the 128Ba(g,a)124Xe stellar rate was inferred from our measurement. The impact of this rate was studied in two different models for core-collapse supernova explosions of 25 solar mass stars. A significant contribution to the 124Xe abundance via this reaction path would only be possible when the rate was increased above the previous standard value. Since the experimental data rule this out, they also demonstrate the closure of this production path.

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Progress of the Felsenkeller shallow-underground accelerator for nuclear astrophysics

Low-background experiments with stable ion beams are an important tool for putting the model of stellar hydrogen, helium, and carbon burning on a solid experimental foundation. The pioneering work in this regard has been done by the LUNA collaboration at Gran Sasso, using a 0.4 MV accelerator. In the present contribution, the status of the project for a higher-energy underground accelerator is reviewed. Two tunnels of the Felsenkeller underground site in Dresden, Germany, are currently being refurbished for the installation of a 5 MV high-current Pelletron accelerator. Construction work is on schedule and expected to complete in August 2017. The accelerator will provide intense, 50 uA, beams of 1H+, 4He+, and 12C+ ions, enabling research on astrophysically relevant nuclear reactions with unprecedented sensitivity.

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Underground nuclear astrophysics: why and how

The goal of nuclear astrophysics is to measure cross sections of nuclear physics reactions of interest in astrophysics. At stars temperatures, these cross sections are very low due to the suppression of the Coulomb barrier. Cosmic ray induced background can seriously limit the determination of reaction cross sections at energies relevant to astrophysical processes and experimental setups should be arranged in order to improve the signal-to-noise ratio. Placing experiments in underground sites, however, reduces this background opening the way towards ultra low cross section determination. LUNA (Laboratory for Underground Nuclear Astrophysics) was pioneer in this sense. Two accelerators were mounted at the INFN National Laboratories of Gran Sasso (LNGS) allowing to study nuclear reactions close to stellar energies. A summary of the relevant technology used, including accelerators, target production and characterisation, and background treatment is given.

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Three new low-energy resonances in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle affects the synthesis of the elements between $^{20}$Ne and $^{27}$Al in asymptotic giant branch stars and novae. The $^{22}$Ne(p,$γ$)$^{23}$Na reaction rate is very uncertain because of a large number of unobserved resonances lying in the Gamow window. At proton energies below 400\,keV, only upper limits exist in the literature for the resonance strengths. Previous reaction rate evaluations differ by large factors. In the present work, the first direct observations of the $^{22}$Ne(p,$γ$)$^{23}$Na resonances at 156.2, 189.5, and 259.7\,keV are reported. Their resonance strengths have been derived with 2-7\% uncertainty. In addition, upper limits for three other resonances have been greatly reduced. Data were taken using a windowless $^{22}$Ne gas target and high-purity germanium detectors at the Laboratory for Underground Nuclear Astrophysics in the Gran Sasso laboratory of the National Institute for Nuclear Physics, Italy, taking advantage of the ultra-low background observed deep underground. The new reaction rate is a factor of 5 higher than the recent evaluation at temperatures relevant to novae and asymptotic giant branch stars nucleosynthesis.

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Determination of gamma-ray widths in $^{15}$N using nuclear resonance fluorescence

The stable nucleus $^{15}$N is the mirror of $^{15}$O, the bottleneck in the hydrogen burning CNO cycle. Most of the $^{15}$N level widths below the proton emission threshold are known from just one nuclear resonance fluorescence (NRF) measurement, with limited precision in some cases. A recent experiment with the AGATA demonstrator array determined level lifetimes using the Doppler Shift Attenuation Method (DSAM) in $^{15}$O. As a reference and for testing the method, level lifetimes in $^{15}$N have also been determined in the same experiment. The latest compilation of $^{15}$N level properties dates back to 1991. The limited precision in some cases in the compilation calls for a new measurement in order to enable a comparison to the AGATA demonstrator data. The widths of several $^{15}$N levels have been studied with the NRF method. The solid nitrogen compounds enriched in $^{15}$N have been irradiated with bremsstrahlung. The $γ$-rays following the deexcitation of the excited nuclear levels were detected with four HPGe detectors. Integrated photon-scattering cross sections of ten levels below the proton emission threshold have been measured. Partial gamma-ray widths of ground-state transitions were deduced and compared to the literature. The photon scattering cross sections of two levels above the proton emission threshold, but still below other particle emission energies have also been measured, and proton resonance strengths and proton widths were deduced. Gamma and proton widths consistent with the literature values were obtained, but with greatly improved precision.

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Test of statistical model cross section calculations for $α$-induced reactions on $^{107}$Ag at energies of astrophysical interest

Astrophysical reaction rates, which are mostly derived from theoretical cross sections, are necessary input to nuclear reaction network simulations for studying the origin of $p$ nuclei. Past experiments have found a considerable difference between theoretical and experimental cross sections in some cases, especially for ($α$,$γ$) reactions at low energy. Therefore, it is important to experimentally test theoretical cross section predictions at low, astrophysically relevant energies. The aim is to measure reaction cross sections of $^{107}$Ag($α$,$γ$)$^{111}$In and $^{107}$Ag($α$,n)$^{110}$In at low energies in order to extend the experimental database for astrophysical reactions involving $α$ particles towards lower mass numbers. Reaction rate predictions are very sensitive to the optical model parameters and this introduces a large uncertainty into theoretical rates involving $α$ particles at low energy. We have also used Hauser-Feshbach statistical model calculations to study the origin of possible discrepancies between prediction and data. An activation technique has been used to measure the reaction cross sections at effective center of mass energies between 7.79 MeV and 12.50 MeV. Isomeric and ground state cross sections of the ($α$,n) reaction were determined separately. The measured cross sections were found to be lower than theoretical predictions for the ($α$,$γ$) reaction. Varying the calculated averaged widths in the Hauser-Feshbach model, it became evident that the data for the ($α$,$γ$) and ($α$,n) reactions can only be simultaneously reproduced when rescaling the ratio of $γ$- to neutron width and using an energy-dependent imaginary part in the optical $α$+$^{107}$Ag potential.......

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Cosmic-ray induced background intercomparison with actively shielded HPGe detectors at underground locations

The main background above 3\,MeV for in-beam nuclear astrophysics studies with $γ$-ray detectors is caused by cosmic-ray induced secondaries. The two commonly used suppression methods, active and passive shielding, against this kind of background were formerly considered only as alternatives in nuclear astrophysics experiments. In this work the study of the effects of active shielding against cosmic-ray induced events at a medium deep location is performed. Background spectra were recorded with two actively shielded HPGe detectors. The experiment was located at 148\,m below the surface of the Earth in the Reiche Zeche mine in Freiberg, Germany. The results are compared to data with the same detectors at the Earth's surface, and at depths of 45\,m and 1400\,m, respectively.

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Measurement of (alpha,n) reaction cross sections of erbium isotopes for testing astrophysical rate predictions

The $γ$-process in core-collapse and/or type Ia supernova explosions is thought to explain the origin of the majority of the so-called $p$ nuclei (the 35 proton-rich isotopes between Se and Hg). Reaction rates for $γ$-process reaction network studies have to be predicted using Hauser-Feshbach statistical model calculations. Recent investigations have shown problems in the prediction of $α$-widths at astrophysical energies which are an essential input for the statistical model. It has an impact on the reliability of abundance predictions in the upper mass range of the $p$ nuclei. With the measurement of the $^{164,166}$Er($α$,n)$^{167,169}$Yb reaction cross sections at energies close to the astrophysically relevant energy range we tested the recently suggested low energy modification of the $α$+nucleus optical potential in a mass region where $γ$-process calculations exhibit an underproduction of the $p$ nuclei. Using the same optical potential for the $α$-width which was derived from combined $^{162}$Er($α$,n) and $^{162}$Er($α$,$γ$) measurement makes it plausible that a low-energy modification of the optical $α$+nucleus potential is needed.

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KADoNiS-$p$: The astrophysical $p$-process database

The KADoNiS-$p$ project is an online database for cross sections relevant to the $p$-process. All existing experimental data was collected and reviewed. With this contribution a user-friendly database using the KADoNiS (Karlsruhe Astrophysical Database of Nucleosynthesis in Stars) framework is launched, including all available experimental data from (p,$γ$), (p,n), (p,$α$), ($α$,$γ$), ($α$,n) and ($α$,p) reactions in or close to the respective Gamow window with cut-off date of August 2012 (www.kadonis.org/pprocess).

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