arXiv subjects

T. Szücs

Publications and source records attributed to T. Szücs.

At least 73 records · Page 4Linked to original sources

arXiv2014

A new study of the $^{22}$Ne(p,$γ$)$^{23}$Na reaction deep underground: Feasibility, setup, and first observation of the 186 keV resonance

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle is active in asymptotic giant branch stars as well as in novae and contributes to the nucleosythesis of neon and sodium isotopes. In order to reduce the uncertainties in the predicted nucleosynthesis yields, new experimental efforts to measure the $^{22}$Ne(p,$γ$)$^{23}$Na cross section directly at the astrophysically relevant energies are needed. In the present work, a feasibility study for a $^{22}$Ne(p,$γ$)$^{23}$Na experiment at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400\,kV accelerator deep underground in the Gran Sasso laboratory, Italy, is reported. The ion beam induced $γ$-ray background has been studied. The feasibility study led to the first observation of the $E_{\rm p}$ = 186\,keV resonance in a direct experiment. An experimental lower limit of 0.12\,$\times$\,10$^{-6}$\,eV has been obtained for the resonance strength. Informed by the feasibility study, a dedicated experimental setup for the $^{22}$Ne(p,$γ$)$^{23}$Na experiment has been developed. The new setup has been characterized by a study of the temperature and pressure profiles. The beam heating effect that reduces the effective neon gas density due to the heating by the incident proton beam has been studied using the resonance scan technique, and the size of this effect has been determined for a neon gas target.

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arXiv2014

Direct study of the alpha-nucleus optical potential at astrophysical energies using the 64Zn(p,alpha)61Cu reaction

In the model calculations of heavy element nucleosynthesis processes the nuclear reaction rates are taken from statistical model calculations which utilize various nuclear input parameters. It is found that in the case of reactions involving alpha particles the calculations bear a high uncertainty owing to the largely unknown low energy alpha-nucleus optical potential. Experiments are typically restricted to higher energies and therefore no direct astrophysical consequences can be drawn. In the present work a (p,alpha) reaction is used for the first time to study the alpha-nucleus optical potential. The measured 64Zn(p,alpha)61Cu cross section is uniquely sensitive to the alpha-nucleus potential and the measurement covers the whole astrophysically relevant energy range. By the comparison to model calculations, direct evidence is provided for the incorrectness of global optical potentials used in astrophysical models.

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arXiv2014

Alpha induced reaction cross section measurements on 162Er for the astrophysical gamma process

The cross sections of the 162Er(a,g,)166Yb and 162Er(a,n)165Yb reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m. = 16.09 down to Ec.m. = 11.21 MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The 162Er(a,n)165Yb reaction was studied above the reaction threshold between Ec.m. = 12.19 and 16.09 MeV. The fact that the 162Er(a,g)166Yb cross sections were measured below the (a,n) threshold at first time in this mass region opens the opportunity to study directly the a-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted.

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arXiv2013

Cross section and reaction rate of 92Mo(p,gamma)93Tc determined from thick target yield measurements

For the better understanding of the astrophysical gamma-process the experimental determination of low energy proton- and alpha-capture cross sections on heavy isotopes is required. The existing data for the 92Mo(p,gamma)93Tc reaction are contradictory and strong fluctuation of the cross section is observed which cannot be explained by the statistical model. In this paper a new determination of the 92Mo(p,gamma)93Tc and 98Mo(p,gamma)99mTc cross sections based on thick target yield measurements are presented and the results are compared with existing data and model calculations. Reaction rates of 92Mo(p,gamma)93Tc at temperatures relevant for the gamma-process are derived directly from the measured thick target yields. The obtained rates are a factor of 2 lower than the ones used in astrophysical network calculations. It is argued that in the case of fluctuating cross sections the thick target yield measurement can be more suited for a reliable reaction rate determination.

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arXiv2013

High precision $^{113}$In($α,α$)$^{113}$In elastic scattering at energies around the Coulomb barrier for the astrophysical $γ$ process

The $γ$ process in supernova explosions is thought to explain the origin of proton-rich isotopes between Se and Hg, the so-called $p$ nuclei. The majority of the reaction rates for $γ$ process reaction network studies has to be predicted in Hauser-Feshbach statistical model calculations using global optical potential parameterizations. While the nucleon+nucleus optical potential is fairly known, for the $α$+nucleus optical potential several different parameterizations exist and large deviations are found between the predictions calculated using different parameter sets. By the measurement of elastic $α$-scattering angular distributions at energies around the Coulomb barrier a comprehensive test for the different global $α$+nucleus optical potential parameter sets is provided. Between 20$^{\circ}$ and 175$^{\circ}$ complete elastic alpha scattering angular distributions were measured on the $^{113}$In \textit{p} nucleus with high precision at E$_{c.m.}$ = 15.59 and 18.82 MeV. The elastic scattering cross sections of the $^{113}$In($α$,$α$)$^{113}$In reaction were measured for the first time at energies close to the astrophysically relevant energy region. The high precision experimental data were used to evaluate the predictions of the recent global and regional $α$+nucleus optical potentials. Parameters for a local $α$+nucleus optical potential were derived from the measured angular distributions. Predictions for the reaction cross sections of $^{113}$In($α,γ$)$^{117}$Sb and $^{113}$In($α$,n)$^{116}$Sb at astrophysically relevant energies were given using the global and local optical potential parameterizations.

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arXiv2013

Investigation of alpha-induced reactions on the p nucleus 168Yb

Cross sections for the 168Yb(alpha,gamma)172Hf and 168Yb(alpha,n)171$Hf reactions were measured by means of the activation method using alpha particles with energies between 12.9 MeV and 15.1 MeV. The spectroscopy of the gamma rays emitted by the reaction products was performed using three different HPGe detector types, namely clover-type high-purity germanium detectors, a low-energy photon spectrometer detector, and a coaxial high-purity germanium detector. The results were compared to Hauser-Feshbach statistical model calculations. Within certain assumptions, astrophysical conclusions could be drawn concerning the production of the p nucleus 168Yb. The data in this work can serve as a contribution to the current very fragmentary experimental data base for charged-particle induced reactions. In addition, the absolute intensity for nine gamma-ray transitions following the electron capture decay of 171Hf could be derived.

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arXiv2013

Activation measurement of the 3He(a,g)7Be reaction cross section at high energies

The astrophysically important 3He(a,g)7Be reaction was studied at high energies where the available experimental data are in contradiction. A thin window 3He gas cell was used and the cross section was measured with the activation method. The obtained cross sections at energies between Ec.m. = 1.5 and 2.5 MeV are compared with the available data and theoretical calculations. The present results support the validity of the high energy cross section energy dependence observed by recent experiments.

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arXiv2013

Neutron-induced background by an alpha-beam incident on a deuterium gas target and its implications for the study of the 2H(alpha,gamma)6Li reaction at LUNA

The production of the stable isotope Li-6 in standard Big Bang nucleosynthesis has recently attracted much interest. Recent observations in metal-poor stars suggest that a cosmological Li-6 plateau may exist. If true, this plateau would come in addition to the well-known Spite plateau of Li-7 abundances and would point to a predominantly primordial origin of Li-6, contrary to the results of standard Big Bang nucleosynthesis calculations. Therefore, the nuclear physics underlying Big Bang Li-6 production must be revisited. The main production channel for Li-6 in the Big Bang is the 2H(alpha,gamma)6Li reaction. The present work reports on neutron-induced effects in a high-purity germanium detector that were encountered in a new study of this reaction. In the experiment, an α-beam from the underground accelerator LUNA in Gran Sasso, Italy, and a windowless deuterium gas target are used. A low neutron flux is induced by energetic deuterons from elastic scattering and, subsequently, the 2H(d,n)3He reaction. Due to the ultra-low laboratory neutron background at LUNA, the effect of this weak flux of 2-3 MeV neutrons on well-shielded high-purity germanium detectors has been studied in detail. Data have been taken at 280 and 400 keV alpha-beam energy and for comparison also using an americium-beryllium neutron source.

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arXiv2012

First Direct Measurement of the ^{17}O(p,γ)^{18}F Reaction Cross-Section at Gamow Energies for Classical Novae

Classical novae are important contributors to the abundances of key isotopes, such as the radioactive ^{18}F, whose observation by satellite missions could provide constraints on nucleosynthesis models in novae. The ^{17}O(p,γ)^{18}F reaction plays a critical role in the synthesis of both oxygen and fluorine isotopes but its reaction rate is not well determined because of the lack of experimental data at energies relevant to novae explosions. In this study, the reaction cross section has been measured directly for the first time in a wide energy range Ecm = 200 - 370 keV appropriate to hydrogen burning in classical novae. In addition, the E=183 keV resonance strength, ωγ=1.67\pm0.12 \mueV, has been measured with the highest precision to date. The uncertainty on the ^{17}O(p,γ)^{18}F reaction rate has been reduced by a factor of 4, thus leading to firmer constraints on accurate models of novae nucleosynthesis.

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arXiv2012

Preparation and characterisation of isotopically enriched Ta$_2$O$_5$ targets for nuclear astrophysics studies

The direct measurement of reaction cross sections at astrophysical energies often requires the use of solid targets of known thickness, isotopic composition, and stoichiometry that are able to withstand high beam currents for extended periods of time. Here, we report on the production and characterisation of isotopically enriched Ta$_2$O$_5$ targets for the study of proton-induced reactions at the Laboratory for Underground Nuclear Astrophysics facility of the Laboratori Nazionali del Gran Sasso. The targets were prepared by anodisation of tantalum backings in enriched water (up to 66% in $^{17}$O and up to 96% in $^{18}$O). Special care was devoted to minimising the presence of any contaminants that could induce unwanted background reactions with the beam in the energy region of astrophysical interest. Results from target characterisation measurements are reported, and the conclusions for proton capture measurements with these targets are drawn.

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arXiv2012

Relation between total cross sections from elastic scattering and alpha-induced reactions: the example of 64Zn

The total reaction cross section is related to the elastic scattering angular distribution by a basic quantum-mechanical relation. We present new experimental data for alpha-induced reaction cross sections on 64Zn which allow for the first time the experimental verification of this simple relation at low energies by comparison of the new experimental reaction data to the result obtained from 64Zn(alpha,alpha)64Zn elastic scattering.

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arXiv2012

Investigation of alpha-induced reactions on 127I for the astrophysical gamma process

(Shorten version of the PRC abstract) Alpha-induced reactions on 127I have been studied using the activation technique in order to provide cross section data for the modeling of the astrophysical gamma process. The relative intensity of the 536.1 keV gamma transition was measured precisely, its uncertainty was reduced from 13% to 4%. By measuring the yield of the characteristic X-rays, the cross sections of the 127I(alpha,gamma)131Cs reaction have been determined for the first time close to the astrophysically relevant energy region, at energies 9.50 < Ec.m. < 15.15$ MeV. The 127I(alpha,n)130Cs reaction was studied in the range 9.62 < Ec.m. < 15.15 MeV by measuring the yield of the 536.1 keV gamma-ray and at the lower part of this energy range by counting the characteristic X-rays. A comparison of the resulting cross sections to predictions of statistical model calculations confirmed the predictions of the astrophysically relevant averaged alpha width. Nevertheless, the newly derived stellar reaction rates at gamma process temperatures for 127I(alpha,gamma)131$Cs and its reverse reaction are factors 4-10 faster than previous calculations, due to improvements in the reaction model.

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arXiv2012

Investigation of alpha-induced reactions on 130Ba and 132Ba and their importance for the synthesis of heavy p nuclei

Captures of alpha particles on the proton-richest Barium isotope, 130Ba, have been studied in order to provide cross section data for the modeling of the astrophysical gamma process. The cross sections of the 130Ba(alpha,gamma)134Ce and 130Ba(alpha,n)133Ce reactions have been measured with the activation technique in the center-of mass energy range between 11.6 and 16 MeV, close above the astrophysically relevant energies. As a side result, the cross section of the 132Ba(alpha,n)135Ce reaction has also been measured. The results are compared with the prediction of statistical model calculations, using different input parameters such as alpha+nucleus optical potentials. It is found that the (alpha,n) data can be reproduced employing the standard alpha+nucleus optical potential widely used in astrophysical applications. Assuming its validity also in the astrophysically relevant energy window, we present new stellar reaction rates for 130Ba(alpha,gamma)134Ce and 132Ba(alpha,gamma)136Ce and their inverse reactions calculated with the SMARAGD statistical model code. The highly increased 136Ce(gamma,alpha)132Ba rate implies that the p nucleus 130Ba cannot directly receive contributions from the Ce isotopic chain. Further measurements are required to better constrain this result.

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arXiv2011

Experimental study of alpha-induced reactions on 64Zn for the astrophysical gamma-process

For the synthesis of the heavy, proton rich isotopes in the astrophysical gamma-process the precise knowledge of alpha-induced cross sections is of high importance. We have initiated a comprehensive study of the 64Zn+alpha system involving the cross section measurement of different reaction channels as well as the elastic scattering at low, astrophysically relevant energies. In this paper the experimental technique and some preliminary results of the 64Zn(alpha,p)67Ga cross section measurement are presented.

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arXiv2011

Half-life measurement of 66Ga with gamma-spectroscopy

The half-life of 66Ga, an isotope very important for high-energy efficiency calibration of gamma-detectors, has been measured using gamma-spectroscopy. In order to reduce systematic uncertainties, different source production methods and gamma-counting conditions have been applied. A half-life value of 9.312 +- 0.032 h has been obtained in agreement with a recent measurement but in contradiction with some of the earlier results.

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arXiv2011

Target characterization for the 130Ba(alpha,gamma)134Ce gamma-process experiment

In order to extend the available experimental database for the astrophysical gamma-process, the cross section measurement of the 130Ba(alpha,gamma)134Ce and 130Ba(alpha,n)133Ce reactions is in progress. The measurements are carried out using thin layers of evaporated BaCO3 as target. Since the target thickness enters directly into the calculation of the cross sections, the reliability of its determination is of crucial importance. Three different methods have been used to determine the target thickness. Details of these experiments and the obtained results are presented.

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arXiv2010

Determining reaction cross sections via characteristic X-ray detection: α-induced reactions on 169Tm for the astrophysical γ -process

The cross sections of the 169Tm(α, γ)173Lu and 169Tm(α,n)172Lu reactions have been measured first time using a new method, by detecting the characteristic X-ray radiation following the electron capturedecay of 172,173Lu. Despite the relatively long half-life of the reaction products (T1/2 = 500 and 6.7 days, respectively) it was possible to measure the cross section of the 169Tm(α,γ)173Lu reaction close to the Gamow window (T9 = 3.5 GK), between Ec.m. = 13.16 and 17.08 MeV. The 169Tm(α,n)172Lu reaction cross section was measured from Ec.m. = 11.21 MeV up to Ec.m. = 17.08 MeV. The experimental results have been compared to theoretical predictions

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arXiv2010

Alpha-induced reaction cross section measurements on 151Eu for the astrophysical gamma-process

In order to extend the experimental database relevant for the astrophysical gamma-process towards the unexplored heavier mass region, the cross sections of the 151Eu(alpha,gamma)155Tb and 151Eu(alpha,n)154Tb reactions have been measured at low energies between 12 and 17 MeV using the activation technique. The results are compared with the predictions of statistical model calculations and it is found that the calculations overestimate the cross sections by about a factor of two. A sensitivity analysis shows that this discrepancy is caused by the inadequate description of the alpha+nucleus channel. A factor of two reduction of the reaction rate of 151Eu(alpha,gamma)155Tb in gamma-process network calculations with respect to theoretical rates using the optical potential by McFadden and Satchler (1966) is recommended.

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