arXiv subjects

T. Taniguchi

Publications and source records attributed to T. Taniguchi.

At least 253 records · Page 14Linked to original sources

arXiv2019

Universal quantized thermal conductance in graphene

The universal quantization of thermal conductance provides information on the topological order of a state beyond electrical conductance. Such measurements have become possible only recently, and have discovered, in particular, that the value of the observed thermal conductance of the 5/2 state is not consistent with either the Pfaffian or the anti-Pfaffian model, motivating several theoretical articles. The analysis of the experiments has been made complicated by the presence of counter-propagating edge channels arising from edge reconstruction, an inevitable consequence of separating the dopant layer from the GaAs quantum well. In particular, it has been found that the universal quantization requires thermalization of downstream and upstream edge channels. Here we measure the thermal conductance in hexagonal boron nitride encapsulated graphene devices of sizes much smaller than the thermal relaxation length of the edge states. We find the quantization of thermal conductance within 5% accuracy for ν = 1, 4/3, 2 and 6 plateaus and our results strongly suggest the absence of edge reconstruction for fractional quantum Hall in graphene, making it uniquely suitable for interference phenomena exploiting paths of exotic quasiparticles along the edge.

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arXiv2019

Phonon scattering dominated electron transport in twisted bilayer graphene

Twisted bilayer graphene (tBLG) has recently emerged as a platform for hosting correlated phenomena, owing to the exceptionally flat band dispersion that results near interlayer twist angle $θ\approx1.1^\circ$. At low temperature a variety of phases are observed that appear to be driven by electron interactions including insulating states, superconductivity, and magnetism. Electrical transport in the high temperature regime has received less attention but is also highly anomalous, exhibiting gigantic resistance enhancement and non-monotonic temperature dependence. Here we report on the evolution of the scattering mechanisms in tBLG over a wide range of temperature and for twist angle varying from 0.75$^\circ$ - 2$^\circ$. We find that the resistivity, $ρ$, exhibits three distinct phenomenological regimes as a function of temperature, $T$. At low $T$ the response is dominated by correlation and disorder physics; at high $T$ by thermal activation to higher moiré subbands; and at intermediate temperatures $ρ$ varies linearly with $T$. The $T$-linear response is much larger than in monolayer graphenefor all measured twist angles, and increases by more than three orders of magnitude for $θ$ near the flat-band condition. Our results point to the dominant role of electron-phonon scattering in twisted layer systems, with possible implications for the origin of the observed superconductivity.

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arXiv2019

Absence of dissipationless transport in clean 2D superconductors

Dissipationless charge transport is one of the defining properties of superconductors (SC). The interplay between dimensionality and disorder in determining the onset of dissipation in SCs remains an open theoretical and experimental problem. In this work, we present measurements of the dissipation phase diagrams of SCs in the two dimensional (2D) limit, layer by layer, down to a monolayer in the presence of temperature (T), magnetic field (B), and current (I) in 2H-NbSe2. Our results show that the phase-diagram strongly depends on the SC thickness even in the 2D limit. At four layers we can define a finite region in the I-B phase diagram where dissipationless transport exists at T=0. At even smaller thicknesses, this region shrinks in area. In a monolayer, we find that the region of dissipationless transport shrinks towards a single point, defined by T=B=I=0. In applied field, we show that time-dependent-Ginzburg-Landau (TDGL) simulations that describe dissipation by vortex motion, qualitatively reproduce our experimental I-B phase diagram. Last, we show that by using non-local transport and TDGL calculations that we can engineer charge flow and create phase boundaries between dissipative and dissipationless transport regions in a single sample, demonstrating control over non-equilibrium states of matter.

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arXiv2019

Topological valley transport at the curved boundary of a folded bilayer graphene

The development of valleytronics demands long-range electronic transport with preserved valley index, a degree of freedom similar to electron spin. A promising structure for this end is a topological one-dimensional (1D) channel formed in bilayer graphene (BLG) under special electrostatic conditions or specific stacking configuration, called domain wall (DW). In these 1D channels, the valley-index defines the propagation direction of the charge carriers and the chiral edge states (kink states) are robust over many kinds of disorder. However, the fabrication of DWs is challenging, requiring the design of complex multi-gate structures or have been producing on rough substrates, showing a limited mean free path. Here, we report on a high-quality DW formed at the curved boundary of folded bilayer graphene (folded-BLG). At such 1D conducting channel we measured a two-terminal resistance close to the quantum resistance $R = e^2/4h$ at zero magnetic field, a signature of kink states. Our experiments reveal a long-range ballistic transport regime that occurs only at the DW of the folded-BLG, while the other regions behave like semiconductors with tunable band gap.

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arXiv2019

Photonic crystals for nano-light in moiré graphene superlattices

Graphene is an atomically thin plasmonic medium that supports highly confined plasmon polaritons, or nano-light, with very low loss. Electronic properties of graphene can be drastically altered when it is laid upon another graphene layer, resulting in a moiré superlattice. The relative twist angle between the two layers is a key tuning parameter of the interlayer coupling in thus obtained twisted bilayer graphene (TBG). We studied propagation of plasmon polaritons in TBG by infrared nano-imaging. We discovered that the atomic reconstruction occurring at small twist angles transforms the TBG into a natural plasmon photonic crystal for propagating nano-light. This discovery points to a pathway towards controlling nano-light by exploiting quantum properties of graphene and other atomically layered van der Waals materials eliminating need for arduous top-down nanofabrication.

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arXiv2019

Evidence for pairing states of composite fermions in double-layer graphene

Pairing interaction between fermionic particles leads to composite Bosons that condense at low temperature. Such condensate gives rise to long range order and phase coherence in superconductivity, superfluidity, and other exotic states of matter in the quantum limit. In graphene double-layers separated by an ultra-thin insulator, strong interlayer Coulomb interaction introduces electron-hole pairing across the two layers, resulting in a unique superfluid phase of interlayer excitons. In this work, we report a series of emergent fractional quantum Hall ground states in a graphene double-layer structure, which is compared to an expanded composite fermion model with two-component correlation. The ground state hierarchy from bulk conductance measurement and Hall resistance plateau from Coulomb drag measurement provide strong experimental evidence for a sequence of effective integer quantum Hall effect states for the novel two-component composite fermions (CFs), where CFs fill integer number of effective LLs (Lambda-level). Most remarkably, a sequence of incompressible states with interlayer correlation are observed at half-filled Lambda-levels, which represents a new type of order involving pairing states of CFs that is unique to graphene double-layer structure and beyond the conventional CF model.

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arXiv2019

Inducing out-of-plane precession of magnetization for microwave assisted magnetic recording using an oscillating polarizer in spin torque oscillator

We investigated the dynamics of a novel design of spin torque oscillator (STO) for microwave assisted magnetic recording. Using Ni$_{80}$Fe$_{20}$ (NiFe) as the polarizer and Fe$_{67}$Co$_{33}$ (FeCo) as the field generating layer, we experimentally observed the magnetization reversal of NiFe, followed by multiple signals in the power spectra as the bias voltage increased. The signals reflected the out-of-plane precession (OPP) mode oscillation of both FeCo and NiFe, as well as the magnetoresistance effect of the STO device, which had the frequency equal to the difference between the oscillation frequency of NiFe and FeCo. Such dynamics were reproduced by micromagnetic simulation. In addition to the merit of realizing the OPP mode oscillation with a simple and thin structure suitable for a narrow gap recording head, the experimental results using this design suggested that a large cone angle of $\sim$ 70$^{\circ}$ for the OPP mode oscillation of FeCo was achieved, which was estimated based on the macrospin model.

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arXiv2019

A corner reflector of graphene Dirac fermions as a phonon-scattering sensor

Dirac fermion optics exploits the refraction of chiral fermions across optics-inspired Klein-tunneling barriers defined by high-transparency p-n junctions. We consider the corner reflector (CR) geometry introduced in optics or radars. We fabricate Dirac fermion CRs using bottom-gate-defined barriers in hBN-encapsulated graphene. By suppressing transmission upon multiple internal reflections, CRs are sensitive to minute phonon scattering rates. We report on doping-independent CR transmission in quantitative agreement with a simple scattering model including thermal phonon scattering. As a new signature of CRs, we observe Fabry-Pérot oscillations at low temperature, consistent with single-path reflections. Finally, we demonstrate high-frequency operation which promotes CRs as fast phonon detectors. Our work establishes the relevance of Dirac fermion optics in graphene and opens a route for its implementation in topological Dirac matter.

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arXiv2019

Spin-orbit driven band inversion in bilayer graphene by van der Waals proximity effect

Spin orbit coupling (SOC) is the key to realizing time-reversal invariant topological phases of matter. Famously, SOC was predicted by Kane and Mele to stabilize a quantum spin Hall insulator; however, the weak intrinsic SOC in monolayer graphene has precluded experimental observation. Here, we exploit a layer-selective proximity effect---achieved via van der Waals contact to a semiconducting transition metal dichalcogenide--to engineer Kane-Mele SOC in ultra-clean \textit{bilayer} graphene. Using high-resolution capacitance measurements to probe the bulk electronic compressibility, we find that SOC leads to the formation of a distinct incompressible, gapped phase at charge neutrality. The experimental data agrees quantitatively with a simple theoretical model in which the new phase results from SOC-driven band inversion. In contrast to Kane-Mele SOC in monolayer graphene, the inverted phase is not expected to be a time reversal invariant topological insulator, despite being separated from conventional band insulators by electric field tuned phase transitions where crystal symmetry mandates that the bulk gap must close. Electrical transport measurements, conspicuously, reveal that the inverted phase has a conductivity $\sim e^2/h$, which is suppressed by exceptionally small in-plane magnetic fields. The high conductivity and anomalous magnetoresistance are consistent with theoretical models that predict helical edge states within the inversted phase, that are protected from backscattering by an emergent spin symmetry that remains robust even for large Rashba SOC. Our results pave the way for proximity engineering of strong topological insulators as well as correlated quantum phases in the strong spin-orbit regime in graphene heterostructures.

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arXiv2018

Magic Angle Spectroscopy

The electronic properties of heterostructures of atomically-thin van der Waals (vdW) crystals can be modified substantially by Moiré superlattice potentials arising from an interlayer twist between crystals. Moiré-tuning of the band structure has led to the recent discovery of superconductivity and correlated insulating phases in twisted bilayer graphene (TBLG) near the so-called "magic angle" of $\sim$1.1°, with a phase diagram reminiscent of high T$_c$ superconductors. However, lack of detailed understanding of the electronic spectrum and the atomic-scale influence of the Moiré pattern has so far precluded a coherent theoretical understanding of the correlated states. Here, we directly map the atomic-scale structural and electronic properties of TBLG near the magic angle using scanning tunneling microscopy and spectroscopy (STM/STS). We observe two distinct van Hove singularities (vHs) in the LDOS which decrease in separation monotonically through 1.1° with the bandwidth (t) of each vHs minimized near the magic angle. When doped near half Moiré band filling, the conduction vHs shifts to the Fermi level and an additional correlation-induced gap splits the vHs with a maximum size of 7.5 meV. We also find that three-fold (C$_3$) rotational symmetry of the LDOS is broken in doped TBLG with a maximum symmetry breaking observed for states near the Fermi level, suggestive of nematic electronic interactions. The main features of our doping and angle dependent spectroscopy are captured by a tight-binding model with on-site (U) and nearest neighbor Coulomb interactions. We find that the ratio U/t is of order unity, indicating that electron correlations are significant in magic angle TBLG. Rather than a simple maximization of the DOS, superconductivity arises in TBLG at angles where the ratio U/t is largest, suggesting a pairing mechanism based on electron-electron interactions.

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arXiv2018

Shubnikov-de Haas oscillations in optical conductivity of monolayer MoSe$_2$

We report polarization-resolved resonant reflection spectroscopy of a charge-tunable atomically-thin valley semiconductor hosting tightly bound excitons coupled to a dilute system of fully spin- and valley-polarized holes in the presence of a strong magnetic field. We find that exciton-hole interactions manifest themselves in hole-density dependent, Shubnikov-de Haas-like oscillations in the energy and line broadening of the excitonic resonances. These oscillations are evidenced to be precisely correlated with the occupation of Landau levels, thus demonstrating that strong interactions between the excitons and Landau-quantized itinerant carriers enable optical investigation of quantum-Hall physics in transition metal dichalcogenides.

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arXiv2018

Tunnel spectroscopy of localised electronic states in hexagonal boron nitride

Hexagonal boron nitride (hBN) is a large band gap layered crystal, frequently incorporated in van der Waals (vdW) heterostructures as an insulating or tunnel barrier. Localised states with energies within its band gap can emit visible light, relevant to applications in nanophotonics and quantum information processing. However, they also give rise to conducting channels, which can induce electrical breakdown when a large voltage is applied. Here we use gated tunnel transistors to study resonant electron tunnelling through the localised states in few atomic-layer hBN barriers sandwiched between two monolayer graphene electrodes. The measurements are used to determine the energy, linewidth, tunnelling transmission probability, and depth within the barrier of more than 50 distinct localised states. A three-step process of electron percolation through two spatially separated localised states is also investigated.

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arXiv2018

Resonant Terahertz Detection Using Graphene Plasmons

Plasmons, collective oscillations of electron systems, can efficiently couple light and electric current, and thus can be used to create sub-wavelength photodetectors, radiation mixers, and on-chip spectrometers. Despite considerable effort, it has proven challenging to implement plasmonic devices operating at terahertz frequencies. The material capable to meet this challenge is graphene as it supports long-lived electrically-tunable plasmons. Here we demonstrate plasmon-assisted resonant detection of terahertz radiation by antenna-coupled graphene transistors that act as both plasmonic Fabry-Perot cavities and rectifying elements. By varying the plasmon velocity using gate voltage, we tune our detectors between multiple resonant modes and exploit this functionality to measure plasmon wavelength and lifetime in bilayer graphene as well as to probe collective modes in its moiré minibands. Our devices offer a convenient tool for further plasmonic research that is often exceedingly difficult under non-ambient conditions (e.g. cryogenic temperatures and strong magnetic fields) and promise a viable route for various photonic applications.

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arXiv2018

The valley Zeeman effect in inter- and intra-valley trions in monolayer WSe$_2$

Monolayer transition metal dichalcogenides (TMDs) hold great promise for future information processing applications utilizing a combination of electron spin and valley pseudospin. This unique spin system has led to observation of the valley Zeeman effect in neutral and charged excitonic resonances under applied magnetic fields. However, reported values of the trion valley Zeeman splitting remain highly inconsistent across studies. Here, we utilize high quality hBN encapsulated monolayer WSe$_2$ to enable simultaneous measurement of both intervalley and intravalley trion photoluminescence. We find the valley Zeeman splitting of each trion state to be describable only by a combination of three distinct g-factors, one arising from the exciton-like valley Zeeman effect, the other two, trion specific, g-factors associated with recoil of the excess electron. This complex picture goes significantly beyond the valley Zeeman effect reported for neutral excitons, and eliminates the ambiguity surrounding the magneto-optical response of trions in tungsten based TMD monolayers.

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arXiv2018

Transport through a network of topological states in twisted bilayer graphene

We explore a network of electronic quantum valley Hall (QVH) states in the moiré crystal of minimally twisted bilayer graphene. In our transport measurements we observe Fabry-Pérot and Aharanov-Bohm oscillations which are robust in magnetic fields ranging from 0 to 8T, in strong contrast to more conventional 2D systems where trajectories in the bulk are bent by the Lorentz force. This persistence in magnetic field and the linear spacing in density indicate that charge carriers in the bulk flow in topologically protected, one dimensional channels. With this work we demonstrate coherent electronic transport in a lattice of topologically protected states.

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arXiv2018

Fine structure of $\mathrm{K}$-excitons in multilayers of transition metal dichalcogenides

Reflectance and magneto-reflectance experiments together with theoretical modelling based on the $\mathbf{k\cdot p}$ approach have been employed to study the evolution of direct bandgap excitons in MoS$_2$ layers with a thickness ranging from mono- to trilayer. The extra excitonic resonances observed in MoS$_2$ multilayers emerge as a result of the hybridization of Bloch states of each sub-layer due to the interlayer coupling. The properties of such excitons in bi- and trilayers are classified by the symmetry of corresponding crystals. The inter- and intralayer character of the reported excitonic resonances is fingerprinted with the magneto-optical measurements: the excitonic $g$-factors of opposite sign and of different amplitude are revealed for these two types of resonances. The parameters describing the strength of the spin-orbit interaction are estimated for bi- and trilayer MoS$_2$.

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arXiv2018

Phase change materials for nano-polaritonics: a case study of hBN/VO2 heterostructures

Polaritonic excitation and control in van der Waals (vdW) materials exhibit superior merits than conventional materials and thus hold new promise for exploring light matter interactions. In this work, we created vdW heterostructures combining hexagonal boron nitride (hBN) and a representative phase change material - vanadium dioxide (VO2). Using infrared nano-spectroscopy and nano-imaging, we demonstrated the dynamic tunability of hyperbolic phonon polaritons in hBN/VO2 heterostructures by temperature control in a precise and reversible fashion. The dynamic tuning of the polaritons stems from the change of local dielectric properties of the VO2 sublayer through insulator to metal transition by the temperature control. The high susceptibility of polaritons to electronic phase transitions opens possibilities for applications of vdW materials in combination with correlated phase change materials.

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arXiv2018

Proximity-Induced Spin-Orbit Coupling in Graphene-Bi$_{1.5}$Sb$_{0.5}$Te$_{1.7}$Se$_{1.3}$ Heterostructures

The weak intrinsic spin-orbit coupling in graphene can be greatly enhanced by proximity coupling. Here we report on the proximity-induced spin-orbit coupling in graphene transferred by hexagonal boron nitride (hBN) onto the topological insulator Bi$_{1.5}$Sb$_{0.5}$Te$_{1.7}$Se$_{1.3}$ (BSTS) which was grown on a hBN substrate by vapor solid synthesis. Phase coherent transport measurements, revealing weak localization, allow us to extract the carrier density-dependent phase coherence length $l_ϕ$. While $l_ϕ$ increases with increasing carrier density in the hBN/graphene/hBN reference sample, it decreases in BSTS/graphene due to the proximity-coupling of BSTS to graphene. The latter behavior results from D'yakonov-Perel-type spin scattering in graphene with a large proximity-induced spin-orbit coupling strength of at least 2.5 meV.

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