arXiv subjects

T. Watanabe

Publications and source records attributed to T. Watanabe.

At least 37 records · Page 2Linked to original sources

arXiv2015

Electronic structure of Mott-insulator CaCu3Ti4O12: Photoemission and inverse photoemission study

We have performed the photoemission and inverse photoemission experiments to elucidate the origin of Mott insulating states in A-site ordered perovskite CaCu$_3$Ti$_4$O$_{12}$ (CCTO). Experimental results have revealed that Cu 3$d$-O 2$p$ hybridized bands, which are located around the Fermi level in the prediction of the local-density approximation (LDA) band calculations, are actually separated into the upper Hubbard band at $\sim$ 1.5 eV and the lower Hubbard band at $\sim$ $-$1.7 eV with a band gap of $\sim$ 1.5-1.8 eV. We also observed that Cu 3$d$ peak at $\sim$ $-$3.8 eV and Ti 3$d$ peak at $\sim$ 3.8 eV are further away from each other than as indicated in the LDA calculations. In addition, it is found that the multiplet strucutre around $-$9 eV includes a considerable number of O 2$p$ states. These observations indicate that the Cu 3$d$ and Ti 3$d$ electrons hybridized with the O 2$p$ states are strongly correlated, which originates in the Mott-insulating states of CCTO.

cond-mat.str-el↗

arXiv2015

Electron and ion heating characteristics during magnetic reconnection in MAST

Local electron and ion heating characteristics during merging reconnection startup on the MAST spherical tokamak have been revealed for the first time using a 130 channel YAG-TS system and a new 32 chord ion Doppler tomography diagnostic. 2D local profile measurement of $T_e$, $n_e$ and $T_i$ detect highly localized electron heating at the X point and bulk ion heating downstream. For the push merging experiment under high guide field condition, thick layer of closed flux surface formed by reconnected field sustains the heating profile for more than electron and ion energy relaxation time $τ^E_{ei}\sim4-10$ms, both heating profiles finally form triple peak structure at the X point and downstream. Toroidal guide field mostly contributes the formation of peaked electron heating profile at the X point. The localized heating increases with higher guide field, while bulk downstream ion heating is unaffected by the change in the guide field under MAST conditions ($B_t>3B_{rec}$).

physics.plasm-ph↗

arXiv2015

Single-crystal growth of underdoped Bi-2223

To investigate the origin of the enhanced Tc ({\approx} 110 K) of the trilayer cuprate superconductor Bi2Sr2Ca2Cu3O10+δ (Bi-2223), its underdoped single crystals are a critical requirement. Here, we demonstrate the first successful in-plane resistivity measurements of heavily underdoped Bi-2223 (zero-resistivity temperatures {\approx} 20~35 K). Detailed crystal growth methods, the annealing process, as well as X-ray diffraction (XRD) and magnetic susceptibility measurement results are also reported.

cond-mat.supr-con↗

arXiv2014

Temperature Dependence of the Electrical Transport Properties of Multilayer Graphene

Multilayer graphene (MLG) thin films are deposited on silicon oxide substrates by mechanical exfoliation (or 'scotch-tape method') from Kish graphite. The thickness and number of layers are determined from both Atomic Force Microscopy (AFM) and Raman Spectroscopy. Electrical terminals are deposited on MLGs in a four-probe configuration by electron-beam lithography, gold/titanium thermal evaporation, and lift-off. The electrical resistance is measured from room temperature down to 2 K. The electrical resistance of the MLGs shows an increase with decreasing temperature, and then decreases after reaching a maximum value. These results are compared with recent experimental and theoretical data from the literature.

cond-mat.mes-hall↗

arXiv2014

Clustering structure of nuclei in deep inelastic processes

A clustering aspect is explained for the $^9$Be nucleus in charged-lepton deep inelastic scattering. Nuclear modifications of the structure function $F_2$ are studied by the ratio $R_{\rm EMC} = F_2^A /F_2^D$, where $A$ and $D$ are a nucleus and the deuteron, respectively. In a JLab experiment, an unexpectedly large nuclear modification slope $|dR_{\rm EMC}/dx|$ was found for $^9$Be, which could be related to its clustering structure. We investigated a mean conventional part of a nuclear structure function $F_2^A$ by a convolution description with nucleon momentum distributions calculated by antisymmetrized (or fermionic) molecular dynamics (AMD) and also by a simple shell model. We found that clustering effects are small in the conventional part, so that the JLab result could be associated with an internal nucleon modification or a short-range nuclear correlation which is caused by high densities due to cluster formation.

hep-ph↗

arXiv2014

Cosmic ray tests of a GEM-based TPC prototype operated in Ar-CF4-isobutane gas mixtures: II

The spatial resolution along the pad-row direction was measured with a GEM-based TPC prototype for the future linear collider experiment in order to understand its performance for tracks with finite projected angles with respect to the pad-row normal. The degradation of the resolution due to the angular pad effect was confirmed to be consistent with the prediction of a simple calculation taking into account the cluster-size distribution and the avalanche fluctuation.

physics.ins-det↗

arXiv2014

Activity report of ILD-TPC Asia group

The purpose of ILD-TPC Asia group is realization of high precision Time Projection Chamber (TPC) with Gas Electron Multiplier (GEM) as a central tracker in International Linear Collider (ILC). We have been studying the many R&D items to build the real detector as a member of LCTPC collaboration. This paper describes the our efforts for realization of the ILD-TPC, the result of test beam using large prototype TPC, local field distortion, positive ion effects and gate devices, and cooling electronics which are key items to build ILD-TPC.

physics.ins-det↗

arXiv2013

Evidence for Hot Fast Flow above a Solar Flare Aracade

Solar flares are one of the main forces behind space weather events. However the mechanism that drives such energetic phenomena is not fully understood. The standard eruptive flare model predicts that magnetic reconnection occurs high in the corona where hot fast flows are created. Some imaging or spectroscopic observations have indicated the presence of these hot fast flows but there have been no spectroscopic scanning observation to date to measure the two-dimensional structure quantitatively. We analyzed a flare that occurred on the west solar limb on 27 January 2012 observed by the Hinode EUV Imaging Spectrometer (EIS) and found that the hot (~30MK) fast (>500 km/s) component was located above the flare loop. This is consistent with magnetic reconnection taking place above the flare loop.

astro-ph.SR↗

arXiv2013

Strong Correlation Effects of A-site Ordered Perovskite CaCu3Ti4O12 revealed by Angle-Resolved Photoemission Spectroscopy

We report angle-resolved photoemission spectroscopy (ARPES) results of A-site ordered perovskite CaCu$_3$Ti$_4$O$_{12}$. We have observed the clear band dispersions, which are shifted to the higher energy by 1.7 eV and show the band narrowing around 2 eV in comparison with the local density approximation calculations. In addition, the high energy multiplet structures of Cu 3$d^8$ final-states have been found around 8 - 13 eV. These results reveal that CaCu$_3$Ti$_4$O$_{12}$ is a Mott-type insulator caused by the strong correlation effects of the Cu 3$d$ electrons well hybridized with O 2$p$ states. Unexpectedly, there exist a very small spectral weight at the Fermi level in the insulator phase, indicating the existence of isolated metallic states.

cond-mat.str-el↗

arXiv2013

Simultaneous valence shift of Pr and Tb ions at the spin-state transition in ((Pr$_{1-y}$Tb$_{y})_{0.7}$Ca$_{0.3}$CoO$_{3}$

Temperature dependence of the X-ray absorption near-edge structure (XANES) spectra at the Pr $L_{3}$- and Tb $L_{3}$-edges was measured for the (Pr$_{1-y}$Tb$_{y})_{0.7}$Ca$_{0.3}$CoO$_{3}$ system, in which a metal-insulator (MI) and spin-state (SS) transition took place simultaneously at a critical temperature $T_{\rm MI}$. A small increase in the valence of the terbium ion was found below $T_{\rm MI}$, besides the enhancement of the praseodymium valence; the trivalent states, which are stable at room temperature, change to a 3+/4+ ionic mixture at low temperatures. In particular for the $y$=0.2 sample, the average valence determined at 8 K amounts to 3.03+ and 3.25+ for the Tb and Pr ion, respectively. In analogous (Pr$_{1-y}$RE$_{y})_{0.7}$Ca$_{0.3}$CoO$_{3}$ samples (RE=Sm and Eu), in which the MI-SS transition also took place, no valence shift of the RE ion was detected in the XANES spectra at the RE ion $L_{3}$-edge. The role of the substituted RE ion for the Pr-site on the MI-SS transition is discussed.

cond-mat.mtrl-sci↗

arXiv2012

Superconductivity in Fe1+dTe0.9Se0.1 induced by deintercalation of excess Fe using alcoholic beverage treatment

Superconductivity in polycrystalline Fe1+dTe0.9Se0.1 was enhanced by heating in alcoholic beverages. We found that part of the excess Fe was deintercalated from the interlayer sites by the treatment and the shielding volume fractions were increased with the reduction of excess Fe content in sample. This behavior is similar to the case of Fe1+dTe1-xSx. Thus the technique of alcoholic beverage treatment can be applied generally to the Fe-chalcogenide superconductors.

cond-mat.supr-con↗

arXiv2012

Evolution of superconductivity in LaO1-xFxBiS2 prepared by high pressure technique

Novel BiS2-based superconductors LaO1-xFxBiS2 prepared by the high pressure synthesis technique were systematically studied. It was found that the high pressure annealing strongly the lattice as compared to the LaO1-xFxBiS2 samples prepared by conventional solid state reaction at ambient pressure. Bulk superconductivity was observed within a wide F-concentration range of x = 0.2 ~ 0.7. On the basis of those results, we have established a phase diagram of LaO1-xFxBiS2.

cond-mat.supr-con↗

arXiv2012

Emergence of highly degenerate excited states in frustrated magnet MgCr$_2$O$_4$

High degeneracy in ground states leads to the generation of exotic zero-energy modes, a representative example of which is the formation of molecular spin liquid-like fluctuations in a frustrated magnet. Here we present single-crystal inelastic neutron scattering results for the frustrated magnet MgCr$_2$O$_4$, which show that a common set of finite-energy molecular spin excitation modes is sustained in both the liquid-like paramagnetic phase and a magnetically ordered phase with an extremely complex structure. Based on this finding, we propose the concept of high degeneracy in excited states, which promotes local resonant elementary excitations. This concept is expected to have ramifications on our understanding of excitations in many complex systems, including not only spin but also atomic liquids, complex order systems, and amorphous systems.

cond-mat.str-el↗

arXiv2012

Fermiological Interpretation of Superconductivity/Non-superconductivity of FeTe_{1-x}Se_{x} Thin Crystal Determined by Quantum Oscillation Measurement

We have successfully observed quantum oscillation (QO) for FeTe_{1-x}Se_{x}. QO measurements were performed using non-superconducting and superconducting thin crystals of FeTe_{0.65}Se_{0.35} fabricated by the scotch-tape method. We show that the Fermi surfaces (FS) of the non-superconducting crystal are in good agreement with the rigid band shift model based on electron doping by excess Fe while that of the superconducting crystal is in good agreement with the calculated FS with no shift. From the FS comparison of both crystals, we demonstrate the change of the cross-sectional area of the FS, suggesting that the suppression of the FS nesting with the vector Q_{s} = (π, π) due to excess Fe results in the disappearance of the superconductivity.

cond-mat.supr-con↗

arXiv2012

Phase diagram and oxygen annealing effect of FeTe1-xSex iron-based superconductor

Phase diagrams of as-grown and O2-annealed FeTe1-xSex determined from magnetic susceptibility measurement were obtained. For as-grown samples, the antiferromagnetic order was fully suppressed in the range region x \geq 0.15, and weak superconductivity appeared when x \geq 0.1. Beginning at x = 0.5, weak superconductivity was found to evolve into bulk superconductivity. Interestingly, for O2-annealed samples, complete suppression of magnetic order and the occurrence of bulk superconductivity were observed when x \geq 0.1. We found that O2-annealing induces bulk superconductivity for FeTe1-xSex. Oxygen probably plays a key role in the suppression of the magnetic order and the appearance of bulk superconductivity.

cond-mat.supr-con↗

arXiv2012

Evidence of Inhomogeneous Superconductivity in FeTe$_{1-x}$Se$_x$ Thin Film Using Scotch-Tape Method

We have fabricated thin films of FeTe$_{1-x}$Se$_x$ using a scotch-tape method. The superconductivities of the thin films are different from each other although these films were fabricated from the same bulk sample. The result clearly presents the inhomogeneous superconductivity in FeTe$_{1-x}$Se$_x$. The difference comes from inhomogeneity due to the excess Fe concentration. The resistivity of a thin film with low excess Fe shows good superconductivity with the sharp superconducting-transition width and more isotropic superconductivity.

cond-mat.supr-con↗

arXiv2012

Clarification as to why alcoholic beverages have the ability to induce superconductivity in Fe_{1+d}Te_{1-x}S_x

To elucidate the mechanism as to why alcoholic beverages can induce superconductivity in Fe_{1+d}Te_{1-x}S_x samples, we performed component analysis and found that weak acid such as organic acid has the ability to induce superconductivity. Inductively-coupled plasma spectroscopy was performed on weak acid solutions post annealing. We found that the mechanism of inducement of superconductivity in Fe_{1+d}Te_{1-x}S_x is the deintercalation of excess Fe from the interlayer sites.

cond-mat.supr-con↗

arXiv2011

Magnetic Reconnection in Non-Equilibrium Ionization Plasma

We have studied the effect of time-dependent ionization and recombination processes on magnetic reconnection in the solar corona. Petschek-type steady reconnection, in which model the magnetic energy is mainly converted at the slow-mode shocks, was assumed. We carried out the time-dependent ionization calculation in the magnetic reconnection structure. We only calculated the transient ionization of iron; the other species were assumed to be in ionization equilibrium. The intensity of line emissions at specific wavelengths were also calculated for comparison with {\it Hinode} or other observations in future. What we found is as follows: (1) iron is mostly in non-equilibrium ionization in the reconnection region, (2) the intensity of line emission estimated by the time-dependent ionization calculation is significantly different from that with the ionization equilibrium assumption, (3) the effect of time-dependent ionization is sensitive to the electron density in the case that the electron density is less than $10^{10}$ cm$^{-3}$, (4) the effect of thermal conduction lessens the time-dependent ionization effect, (5) the effect of radiative cooling is negligibly small even if we take into account time-dependent ionization.

astro-ph.SR↗