arXiv subjects

Takuya Satoh

Publications and source records attributed to Takuya Satoh.

At least 19 recordsLinked to original sources

arXiv2026

Circular Raman responses from angular-momentum inequivalence in CoSi

Circularly polarized Raman scattering in solids exhibits distinct phenomena such as Raman optical activity (ROA) and chiral-phonon-induced frequency splitting, whose relationship has remained unclear. Here we show that these seemingly different responses can be understood within a common framework based on the inequivalence of phonon states carrying opposite crystal angular momenta. Using helicity-resolved Raman spectroscopy of the chiral crystal CoSi, we find that ROA and frequency splitting arise from different symmetry channels, namely axial multipolar symmetry and structural chirality, respectively. First-principles calculations reproduce both effects and clarify their symmetry origins. These results establish angular-momentum inequivalence as a unifying principle of circular Raman responses and link helicity-resolved Raman spectroscopy to the angular-momentum structure of chiral phonons in topological materials.

physics.optics↗

arXiv2026

Quantifying chirality of phonons

Recent years have witnessed growing interest in chiral phonons, lattice vibrations carrying angular momentum and exhibiting handedness, as revealed by helicity-dependent optical phenomena. Despite this progress, a quantitative characterization of phonon chirality as a dynamical property has remained elusive. In this work, we propose a theoretical framework to quantify the dynamical chirality of lattice vibrations. We introduce two quantitative measures: momentum-resolved dynamical chirality, which provides a mode- and wave-vector-resolved picture of phonon chirality, and the bulk dynamical chirality, which characterizes the collective behavior of thermally populated chiral phonons. Using first-principles calculations for both chiral and achiral materials, we demonstrate how these quantities capture the handedness and population imbalance of phonon modes and serve as a means to distinguish the enantiomers of chiral crystals.

cond-mat.mtrl-sci↗

arXiv2026

Electric toroidal octupolar symmetry in pyrite FeS$_2$ probed by Raman optical activity

We report Raman optical activity in pyrite FeS$_2$, which hosts an electric toroidal octupolar symmetry. A clear and reproducible sign reversal of the circular intensity difference is observed between neighboring $\{111\}$ faces under cross-circular polarization. The signal appears only for the doubly degenerate $E_g$ phonon mode and is absent for other modes, consistent with symmetry analysis. First-principles calculations reproduce these features, establishing Raman optical activity as a probe of higher-rank axial multipolar symmetry.

cond-mat.mtrl-sci↗

arXiv2026

Chiral phonons in sixfold chiral CrSi$_2$: Raman spectroscopy and first-principles calculations

Chiral phonons have been identified in several chiral crystals, primarily in those with trigonal symmetry and threefold screw axes. In this study, chiral phonons in CrSi$_2$, a chiral crystal with a sixfold helical structure, were investigated. Circularly polarized Raman spectroscopy revealed a subtle splitting of doubly degenerate $E_2$ phonon modes between cross-circular polarization configurations. These observations, supported by first-principles phonon calculations, indicate the presence of chiral phonons in CrSi$_2$, expanding the scope of materials that exhibit chiral vibrational modes beyond the conventional trigonal class.

cond-mat.mtrl-sci↗

arXiv2025

Symmetry analysis of cross-circular and parallel-circular Raman optical activity

The Raman scattering regarding the circularly-polarized incident and scattered lights is closely related to the circular activity of a given system. We investigate the symmetry of its activity, called the cross-circular and parallel-circular Raman optical activity. The analysis is systematically performed with the magnetic point groups and indicates that the response allows for a useful diagnosis of the symmetry of materials like chirality and (magneto-)axiality. It is also shown that the Stokes and anti-Stokes processes are related to each other by the conserved antiunitary symmetry for the time-reversal operation and that combined with the mirror reflection.

cond-mat.mtrl-sci↗

arXiv2025

Raman Optical Activity Induced by Ferroaxial Order in NiTiO$_3$

Raman optical activity (ROA), the dependence of Raman intensity on the circular polarization of incident and scattered light, has traditionally been observed in chiral molecules and magnetic materials, where inversion or time-reversal symmetry is broken. Here we demonstrate that ROA can also arise in a centrosymmetric and non-magnetic ferroaxial crystal. Using circularly polarized Raman spectroscopy on single-crystalline NiTiO$_3$, we observed a pronounced ROA signal in the cross-circular polarization configurations, which correlates with the ferroaxial domain structure. Our symmetry analysis, first-principles calculations of phonons, and tight-binding model calculations reveal that the natural ROA originates from the ferroaxial order and persists even within the electric dipole approximation. These results establish ROA as a powerful probe of ferroaxial order in centrosymmetric systems.

cond-mat.mtrl-sci↗

arXiv2025

Polarization-dependent photocurrent in a quadrilateral-shaped bulk crystalline tellurium chip with near-infrared light excitation

We report the detection of zero-bias photocurrents induced by interband excitation using oblique near-infrared light ({\lambda}=0.780 {\mu}m) along the directions parallel and perpendicular to the helical axis in a millimeter-sized Te crystal. The photocurrent parallel to the helical axis exhibits a circular-polarization-dependent component, namely circular photogalvanic effect. We create a framework for estimating the gyrotropic photoconductivity tensor \b{eta}, the ratio between the circular-polarization-dependent photocurrent density and intensity of light, through which extrinsic \b{eta} values ranging from a few to a few tens of nA/W are obtained. Searching the \b{eta} values through existing literatures reveals that these values vary significantly with sample conditions, excitation wavelengths, and forms of crystallite samples. A particular interesting point found in our study is that the \b{eta} values for the interband excitation may be greater than those for intraband excitation as far as bulk Te is concerned.

cond-mat.mtrl-sci↗

arXiv2025

Anomalous Nernst effect in Co thin films under laser irradiation

The anomalous Nernst effect (ANE) generates electromotive forces transverse to temperature gradients and has attracted much attention for potential applications into alternative thermoelectric power generators. ANE efficiency is generally characterized by uniform temperature gradients in a steady state prepared by heaters. However, although focusing laser beams on a magnetic film can form much larger temperature gradients, the laser-irradiation method has not been sufficiently considered for quantifying the ANE coefficient due to the difficulty in estimating the localized in-homogeneous temperature gradients. In this study, we present a quantitative study of ANE in Ru(5 nm)/Co($t_{\mathrm{Co}}$) ($t_{\mathrm{Co}}$ = 3, 5, 7, 10, 20, 40, and 60 nm) bilayers on sapphire (0001) substrates by combining a laser irradiation approach with finite-element analysis of temperature gradients under laser excitation. We find that the estimated ANE coefficients are consistent with previously reported values and one independently characterized using a heater. Our results also reveal the advantages of the laser irradiation method over the conventional method using heaters. Intensity-modulated laser beams can create ac temperature gradients as large as approximately 10$^3$ K/mm at a frequency of tens of kilohertz in a micrometer-scale region.

cond-mat.mtrl-sci↗

arXiv2024

Magnetic resonance frequency of two-sublattice ferrimagnet with magnetic compensation temperature

Ferrimagnetic materials with a compensation temperature have recently attracted interest because of their unique combination of ferromagnetic and antiferromagnetic properties. However, their magnetization dynamics near the compensation temperature are complex and cannot be fully explained by conventional ferromagnetic resonance (FMR) or exchange resonance modes. Therefore, practical models are necessary to capture these dynamics accurately. In this study, we derived the analytical solutions for the magnetic resonance frequencies of compensated ferrimagnets over all temperature ranges, considering both the in-plane and out-of-plane orientations of the magnetization. Our solutions successfully reproduce the experimental data obtained from time-resolved magneto-optical Faraday rotation and Brillouin light scattering measurements for the in-plane and out-of-plane cases, respectively. This reproduction is achieved by incorporating the exchange stiffness and temperature dependence of the magnetic anisotropy into the free energy density. Additionally, at temperatures sufficiently far from the compensation temperature, our analytical solutions converge with the conventional FMR and exchange resonance models.

cond-mat.mtrl-sci↗

arXiv2024

Evidence of relativistic field-derivative torque in nonlinear THz response of magnetization dynamics

Understanding the complete light-spin interactions in magnetic systems is the key to manipulating the magnetization using optical means at ultrafast timescales. The selective addressing of spins by terahertz (THz) electromagnetic fields via Zeeman torque is one of the most successful ultrafast means of controlling magnetic excitations. Here we show that this traditional Zeeman torque on the spins is not sufficient, rather an additional relativistic field-derivative torque is essential to realize the observed magnetization dynamics. We accomplish this by exploring the ultrafast nonlinear magnetization dynamics of rare-earth, Bi-doped iron garnet when excited by two co-propagating THz pulses. First, by exciting the sample with an intense THz pulse and probing the magnetization dynamics using magneto-optical Faraday effect, we find the collective exchange resonance mode between rare-earth and transition metal sublattices at 0.48 THz. We further explore the magnetization dynamics via the THz time-domain spectroscopic means. We find that the observed nonlinear trace of the magnetic response cannot be mapped to the magnetization precession induced by the Zeeman torque, while the Zeeman torque supplemented by an additional field-derivative torque follows the experimental evidences. This breakthrough enhances our comprehension of ultra-relativistic effects and paves the way towards novel technologies harnessing light-induced control over magnetic systems.

cond-mat.mtrl-sci↗

arXiv2023

Sublattice-selective inverse Faraday effect in ferrimagnetic rare-earth iron garnet

We performed time-resolved pump--probe measurements using rare-earth iron garnet \ce{Gd3/2Yb1/2BiFe5O12} as a two-sublattice ferrimagnet. We measured the initial phases of the magnetic resonance modes below and above the magnetization compensation temperature to clarify the sublattice selectivity of the inverse Faraday effect in ferrimagnets. A comparison of the time evolution of magnetization estimated using the equations of motion revealed that the inverse Faraday effect occurring in ferrimagnetic materials has sublattice selectivity. This is in striking contrast to antiferromagnets, in which the inverse Faraday effect acts on each sublattice identically. The initial phase analysis can be applied to other ferrimagnets with compensation temperatures.

cond-mat.mtrl-sci↗

arXiv2023

Generation of third-harmonic spin oscillation from strong spin precession induced by terahertz magnetic near fields

The ability to drive a spin system to state far from the equilibrium is indispensable for investigating spin structures of antiferromagnets and their functional nonlinearities for spintronics. While optical methods have been considered for spin excitation, terahertz (THz) pulses appear to be a more convenient means of direct spin excitation without requiring coupling between spins and orbitals or phonons. However, room-temperature responses are usually limited to small deviations from the equilibrium state because of the relatively weak THz magnetic fields in common approaches. Here, we studied the magnetization dynamics in a HoFeO3 crystal at room temperature. A custom-made spiral-shaped microstructure was used to locally generate a strong multicycle THz magnetic near field perpendicular to the crystal surface; the maximum magnetic field amplitude of about 2 T was achieved. The observed time-resolved change in the Faraday ellipticity clearly showed second- and third-order harmonics of the magnetization oscillation and an asymmetric oscillation behaviour. Not only the ferromagnetic vector M but also the antiferromagnetic vector L plays an important role in the nonlinear dynamics of spin systems far from equilibrium.

physics.optics↗

arXiv2023

Sub-millimeter propagation of antiferromagnetic magnons via magnon-photon coupling

For the realization of magnon-based current-free technologies, referred to as magnonics, all-optical control of magnons is an important technique for both fundamental research and practical applications. Magnon-polariton is a coupled state of magnon and photon in a magnetic medium, expected to exhibit magnon-like controllability and photon-like high-speed propagation. While recent studies have observed magnon-polaritons as modulation of incident terahertz waves, the influence of magnon-photon coupling on magnon propagation properties remains unexplored. This study aimed to observe the spatiotemporal dynamics of coherent magnon-polaritons through time-resolved imaging measurements. BiFeO$_3$ was selected as the sample due to its anticipated strong coupling between magnons and photons. The observed dynamics suggest that antiferromagnetic magnons can propagate over long distances, up to hundreds of micrometers, through strong coupling with photons. These results enhance our understanding of the optical control of magnonic systems, thereby paving the way for terahertz opto-magnonics.

cond-mat.mtrl-sci↗

arXiv2022

Chiral phonons: circularly polarized Raman spectroscopy and $\textit{ab initio}$ calculations in a chiral crystal tellurium

Recently, phonons with chirality (chiral phonons) have attracted significant attention. Chiral phonons exhibit angular and pseudo-angular momenta. In circularly polarized Raman spectroscopy, the peak split of the $\Gamma_3$ mode is detectable along the principal axis of the chiral crystal in the backscattering configuration. In addition, peak splitting occurs when the pseudo-angular momenta of the incident and scattered circularly polarized light are reversed. Until now, chiral phonons in binary crystals have been observed, whereas those in unary crystals have not been observed. Here, we observe chiral phonons in a chiral unary crystal Te. The pseudo-angular momentum of the phonon is obtained in Te by an $\textit{ab initio}$ calculation. From this calculation, we verified the conservation law of pseudo-angular momentum in Raman scattering. From this conservation law, we determined the handedness of the chiral crystals. We also evaluated the true chirality of the phonons using a measure with symmetry similar to that of an electric toroidal monopole.

cond-mat.mtrl-sci↗

arXiv2022

Observation of quasi-elastic light scattering in BiFeO$_3$

We observed quasi-elastic light scattering (QELS) in BiFeO$_3$ using Raman spectroscopy over a temperature range of 300-860 K. The QELS has two components: a narrow and broad component. The temperature dependence of the intensity and linewidth of the broad component differed below and beyond the N\'eel point, and the broad QELS may have a magnetic origin.

cond-mat.mtrl-sci↗

arXiv2021

Truly chiral phonons in {\alpha}-HgS

Chirality is a manifestation of the asymmetry inherent in nature. It has been defined as the symmetry breaking of the parity of static objects, and the definition was extended to dynamic motion such that true and false chiralities were distinguished. Recently, rotating, yet not propagating, atomic motions were predicted and observed in two-dimensional materials, and they were referred to as "chiral phonons" . A natural development would be the discovery of truly chiral phonons that propagate while rotating in three-dimensional materials. Here, we used circularly polarised Raman scattering and first-principles calculations to identify truly chiral phonons in chiral bulk crystals. This approach enabled us to determine the chirality of a crystal in a non-contact and non-destructive manner. In addition, we demonstrated that the law of the conservation of pseudo-angular momentum holds between circularly polarised photons and chiral phonons. These findings are expected to help develop ways for transferring the pseudo-angular momentum from photons to electron spins via the propagating chiral phonons in opto-phononic-spintronic devices.

cond-mat.mtrl-sci↗

arXiv2021

Ultrafast Optomagnonics in Ferrimagnetic Multi-Sublattice Garnets

This review discusses the ultrafast magnetization dynamics within the gigahertz to terahertz frequency range in ferrimagnetic rare-earth iron garnets with different substitutions. In these garnets, the roles of spin-orbit and exchange interactions have been detected using femtosecond laser pulses via the inverse Faraday effect. The all-optical control of spin-wave and Kaplan-Kittel exchange resonance modes in different frequency ranges is shown. Generation and localization of the electric field distribution inside the garnet through the metal-bound surface plasmon-polariton strongly enhance the amplitude of the exchange resonance modes. The exchange resonance mode in yttrium iron garnets was observed using circularly polarized Raman spectroscopy. The results of this study may be utilized in the development of a wide class of optomagnonic devices in the gigahertz to terahertz frequency range.

cond-mat.mtrl-sci↗

arXiv2021

Fast acquisition of spin-wave dispersion by compressed sensing

For the realization of magnonic devices, spin-wave dispersions need to be identified. Recently, the time-resolved pump-probe imaging method combined with the Fourier transform was demonstrated for obtaining the dispersions in the lower-wavenumber regime. However, the measurement takes a long time when the sampling rate is sufficiently high. Here, we demonstrated the fast acquisition of spin-wave dispersions by using the compressed sensing technique. Further, we quantitatively evaluated the consistency of the results. Our results can be applied to other various pump-probe measurements, such as observations based on the electro-optical effects.

physics.optics↗