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Takuya Satoh

Publications and source records attributed to Takuya Satoh.

33 records · Page 2Linked to original sources

Efficient spin excitation via ultrafast damping-like torques in antiferromagnets

Damping effects form the core of many emerging concepts for high-speed spintronic applications. Important characteristics such as device switching times and magnetic domain-wall velocities depend critically on the damping rate. While the implications of spin damping for relaxation processes are intensively studied, damping effects during impulsive spin excitations are assumed to be negligible because of the shortness of the excitation process. Herein, we show that, unlike in ferromagnets, ultrafast damping plays a crucial role in antiferromagnets because of their strongly elliptical spin precession. In time-resolved measurements, we find that ultrafast damping results in an immediate spin canting along the short precession axis. The interplay between antiferromagnetic exchange and magnetic anisotropy amplifies this canting by several orders of magnitude towards large-amplitude modulations of the antiferromagnetic order parameter. This leverage effect discloses a highly efficient route towards the ultrafast manipulation of magnetism in antiferromagnetic spintronics.

cond-mat.mtrl-sci↗

Observation of terahertz magnon of Kaplan-Kittel exchange resonance in yttrium-iron garnet by Raman spectroscopy

Backscattering Raman spectroscopic investigations were performed on an yttrium-iron garnet single crystal using linearly and circularly polarized light. A terahertz (THz) magnon of the Kaplan-Kittel (KK) exchange resonance was discovered, which had been regarded as unobservable via optical methods. The KK exchange resonance had a 7.8-THz frequency at 80 K, and the polarization selection rule led to an antisymmetric Raman tensor of the $A_{2}$ mode. Moreover, the assignment of all the Raman-active phonon modes, $3A_{1g}$, $8E_{g}$, and $14T_{2g}$, was proposed. This study will stimulate further investigation of the coupling of THz magnons and phonons and pave the way toward THz optomagnonics.

physics.optics↗

Selective imaging of terahertz electric field of phonon-polariton in LiNbO$_3$

Coherent phonon-polaritons have attracted a considerable amount of interest owing to their relevance to nonlinear optics and terahertz (THz)-wave emissions. Therefore, it is important to analyze the THz electric-fields of phonon-polaritons. However, in the majority of previous measurements, only a single component of the THz electric field was detected. In this paper, we demonstrate that pump-probe electro-optical imaging measurements using the Stokes parameters of probe polarization enable the phase-resolved selective detection of THz electric-field components that are associated with the phonon-polariton. We experimentally distinguish the mode profiles of ordinary and extraordinary phonon-polaritons, and clarify the excitation mechanism as optical rectification. These results are explained by numerical calculations of Maxwell equations for the THz electric field. The technique of selectively observing the THz electric field components may be useful for designing efficient THz-wave emitters.

physics.optics↗

Observation of evanescent spin waves in the magnetic dipole regime

We observed spin-wave transmission through an air gap that works as a prohibited region. The spin waves were excited by circularly polarized pump pulses via the inverse Faraday effect, and their spatial propagation was detected through the Faraday effect of probe pulses using a pump-probe imaging technique. The experimentally observed spin-wave transmission was reproduced using numerical calculations with a Green's function method and micromagnetic simulation. We found that the amplitude of the spin waves decays exponentially in the air gap, which indicates the existence of evanescent spin waves in the magnetic dipole regime. This finding will pave the way for controllable amplitudes and phases of spin waves propagating through an artificial magnonic crystal.

physics.optics↗

Ultrafast Light-driven Simultaneous Excitation of Coherent Terahertz Magnons and Phonons in Multiferroic BiFeO$_3$

The ultrafast switching of magnetization in multiferroic materials by a femtosecond laser could provide various advantages in photonics and magnonics. An efficient approach to control the light matter interaction is the modulation of ultrafast coherent magnons and phonons in the high frequency range. Spontaneous Raman and infrared spectra reveal the excitation of magnons and optical phonons in multiferroic BiFeO3 in the sub few terahertz range. However, coherent control of such quasiparticles has not been achieved yet. In this study, we demonstrate that linearly polarized laser pulses simultaneously excite coherent magnons out of plane and in plane cyclone modes and optical phonon E mode in BiFeO3. Experimental results in conjugation with phenomenological theory, by considering three uniformly distributed magnetic domains reveal that impulsive stimulated Raman scattering is responsible for the generation of coherent magnons and phonons in BiFeO3. The observation of these terahertz magnon and optical phonon modes paves the way for the development of ultrafast magneto electro optical devices.

physics.optics↗

Excitation of coherent optical phonons in iron garnet by femtosecond laser pulses

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective excitation by a linearly polarized pump and detection by a circularly polarized probe confirm that impulsive stimulated Raman scattering (ISRS) is the driving force for the coherent phonons. Experimental results obtained from ISRS measurements reveal excellent agreement with spontaneous Raman spectroscopy data, analyzed by considering the symmetry of the phonon modes and corresponding excitation and detection selection rules.

cond-mat.mtrl-sci↗

Tracking the ultrafast motion of an antiferromagnetic order parameter

The unique functionalities of antiferromagnets offer promising routes to advance information technology. Their compensated magnetic order leads to spin resonances in the THz-regime, which suggest the possibility to coherently control antiferromagnetic (AFM) devices orders of magnitude faster than traditional electronics. However, the required time resolution, complex sublattice interations and the relative inaccessibility of the AFM order parameter pose serious challenges to studying AFM spin dynamics. Here, we reveal the temporal evolution of an AFM order parameter directly in the time domain. We modulate the AFM order in hexagonal YMnO$_\mathrm{3}$ by coherent magnon excitation and track the ensuing motion of the AFM order parameter using time-resolved optical second-harmonic generation (SHG). The dynamic symmetry reduction by the moving order parameter allows us to separate electron dynamics from spin dynamics. As transient symmetry reductions are common to coherent excitations, we have a general tool for tracking the ultrafast motion of an AFM order parameter.

cond-mat.mes-hall↗

Excitation of multiple phonon modes in copper metaborate CuB$_2$O$_4$ via non-resonant impulsive stimulated Raman scattering

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical birefringence using the balanced-detection (BD) technique. We compare the results of BD-ISRS experiment to the polarized spontaneous Raman scattering spectra. We show that the agreement between the two sets of data obtained by these allied techniques in a wide phonon frequencies range of 4-14 THz can be achieved by rigorously taking into account the symmetry of the phonon modes, and the corresponding excitation and detection selection rules. It is also important to account for the difference between incoherent and coherent phonons in terms of their contributions to the Raman scattering process. This comparative analysis highlights the importance of the ratio between the frequency of a particular mode, and the pump and probe spectral widths. We demonstrate analytically that the pump and probe pulse durations of 90 and 50 fs, respectively, used in our experiments, limit the highest frequency of the excited and detected coherent phonon modes to 12 THz, and define their relative amplitudes.

cond-mat.mtrl-sci↗

Optical determination of the exchange stiffness constant in an iron garnet

Brillouin light scattering measurements were performed in the backscattering geometry on a Bi-substituted rare earth iron garnet. We observed two different peaks, one attributed to a surface spin wave in the dipole-exchange regime. The other is referred to as a backscattering magnon mode, because the incident light in this case is scattered backward by exchange-dominated spin wave inside the material. We propose a method to estimate the exchange stiffness constant from the frequency of the backscattering magnon mode. The obtained value is comparable with the previously reported values for Y$ _3 $Fe$ _5 $O$ _{12} $.

physics.optics↗

Surface plasmon-mediated nanoscale localization of laser-driven sub-THz spin dynamics in magnetic dielectrics

Ultrafast all-optical control of spins with femtosecond laser pulses is one of the hot topics at the crossroads of photonics and magnetism with a direct impact on future magnetic recording. Unveiling light-assisted recording mechanisms for an increase of the bit density beyond the diffraction limit without excessive heating of the recording medium is an open challenge. Here we show that surface plasmon-polaritons in hybrid metal-dielectric structures can provide spatial confinement of the inverse Faraday effect, mediating the excitation of localized coherent spin precession with 0.41 THz frequency. We demonstrate a two orders of magnitude enhancement of the excitation efficiency at the surface plasmon resonance within the 100 nm layer in dielectric garnet. Our findings broaden the horizons of ultrafast spin-plasmonics and open pathways towards non-thermal opto-magnetic recording at the nano-scale.

physics.optics↗

Unidirectional control of optically induced spin waves

Unidirectional control of optically induced spin waves in a rare-earth iron garnet crystal is demonstrated. We observed the interference of two spin-wave packets with different initial phases generated by circularly polarized light pulses. This interference results in unidirectional propagation if the spin-wave sources are spaced apart at 1/4 of the wavelength of the spin waves and the initial phase difference is set to pi/2. The propagating direction of the spin wave is switched by the polarization helicity of the light pulses. Moreover, in a numerical simulation, applying more than two spin-wave sources with a suitable polarization and spot shape, arbitrary manipulation of the spin wave by the phased array method was replicated.

physics.app-ph↗

Ultrafast optical excitation of coherent magnons in antiferromagnetic NiO

In experiment and theory, we resolve the mechanism of ultrafast optical magnon excitation in antiferromagnetic NiO. We employ time-resolved optical two-color pump-probe measurements to study the coherent non-thermal spin dynamics. Optical pumping and probing with linearly and circularly polarized light along the optic axis of the NiO crystal scrutinizes the mechanism behind the ultrafast optical magnon excitation. A phenomenological symmetry-based theory links these experimental results to expressions for the optically induced magnetization via the inverse Faraday effect and the inverse Cotton-Mouton effect. We obtain striking agreement between experiment and theory that, furthermore, allows us to extract information about the spin domain distribution. We also find that in NiO the energy transfer into the magnon mode via the inverse Cotton-Mouton effect is about three orders of magnitude more efficient than via the inverse Faraday effect.

cond-mat.other↗

Two-Dimensional Propagation of a Photoinduced Spin Wave Packet

We report the two-dimensional propagation of photoinduced spin wave packets in Bi-doped rare-earth iron garnet. Spin waves were excited nonthermally and impulsively by a circularly polarized light pulse via the inverse Faraday effect. Space- and time resolved spin waves were detected with a magneto-optical pump-probe technique. We investigated propagation in two directions, parallel and perpendicular to the magnetic field. Backward volume magnetostatic waves (BVMSWs) were detected in both directions. The frequency of BVMSWs depends on the propagation direction. The experimental results agreed well with the dispersion relation of BVMSWs.

cond-mat.mes-hall↗

Spectral dependence of photoinduced spin precession in DyFeO3

Spin precession was nonthermally induced by an ultrashort laser pulse in orthoferrite DyFeO3 with a pump-probe technique. Both circularly and linearly polarized pulses led to spin precessions; these phenomena are interpreted as the inverse Faraday effect and the inverse Cotton-Mouton effect, respectively. For both cases, the same mode of spin precession was excited; the precession frequencies and polarization were the same, but the phases of oscillations were different. We have shown theoretically and experimentally that the analysis of phases can distinguish between these two mechanisms. We have demonstrated experimentally that in the visible region, the inverse Faraday effect was dominant, whereas the inverse Cotton-Mouton effect became relatively prominent in the near-infrared region.

cond-mat.str-el↗

Spin Oscillations in Antiferromagnetic NiO Triggered by Circularly Polarized Light

Coherent spin oscillations were non-thermally induced by circularly polarized pulses in fully compensated antiferromagnetic NiO. This effect is attributed to an entirely new mechanism of the action, on the spins, of the effective magnetic field generated by an inverse Faraday effect. The novelty of this mechanism is that spin oscillations are driven by the time derivative of the effective magnetic field acting even on "pure" antiferromagnets with zero net magnetic moment in the ground state. The measured frequencies (1.07 THz and 140 GHz) of the spin oscillations correspond to the out-of-plane and in-plane modes of antiferromagnetic magnons.

cond-mat.str-el↗