arXiv subjects

Teresa Puig

Publications and source records attributed to Teresa Puig.

6 recordsLinked to original sources

arXiv2026

Non-Linear Dynamics Induced by Strong Radio-Frequency Fields in ReBCO High Temperature Superconductors

Probing the dynamics of superconducting transitions induced by strong electromagnetic fields is vital to designing high power devices leveraging these materials. The development of high temperature superconductors (HTS) is particularly interesting due to critical temperatures ($T_c$) approaching 90\,K, the ability to support high current densities, and their ability to operate in strong static magnetic fields. This work aims to determine the transition dynamics of these materials at radio-frequencies (rf) in the microwave range where they have enormous potential for new applications ranging from particle accelerators to dark matter searches. We have tested two types of coatings formed from rare earth barium copper oxide (REBCO): a film deposited by electron-beam physical vapor deposition, and HTS conductor tapes soldered to a copper substrate with exposed REBCO surfaces. Testing was performed via a hemispherical transverse-electric mode cavity that maximizes the surface rf magnetic field and minimizes the surface electric field on a 2-inch diameter sample. We report on steady-state measurements at low rf power, as well as fully time-resolved transition dynamics on the microsecond timescale seen for the first time with strong surface rf fields.

physics.acc-ph↗

arXiv2025

Fast track to the overdoped regime of superconducting YBa2Cu3O7-δ thin films via electrochemical oxidation

High temperature superconductors, especially YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO), are considered a key enabling technology towards a clean energy future. Hole doping in YBCO is a prerequisite for the emergence of its unchallenged superconducting properties. Up to now, research was focused on the under- and optimally doped region, due to practical limitations in reaching the overdoped state, despite being highly interesting from fundamental and applied aspects as competing orders vanish and critical current densities are expected to peak. Here, we deploy for the first time an electrochemical method to access the mostly uncharted overdoped region. We demonstrate precise control over the bulk oxygen concentration in YBCO thin films across the full off-stoichiometry window (0$\leδ\le$1) using electrochemical oxidation combined with in situ XRD and electrical measurements. Resulting high doping states and critical current densities are confirmed using a multi modal approach, including x-ray diffraction, electrical, Hall and magnetic characterization. Thus, this work opens a promising pathway based on electrochemical oxidation towards electronically clean, oxygen overdoped cuprate superconductors and therefore will assist to further push the critical current density to its intrinsic limit.

cond-mat.supr-con↗

arXiv2025

Oxygen incorporation in YBa$_2$Cu$_3$O$_{7-δ}$ thin films: surface activation and degradation

The oxygen off-stoichiometry plays a pivotal role for the physical properties of superconducting oxides. Yet, there is a lack of knowledge on the fundamental processes of oxygen incorporation and correlated phenomena during oxygen post annealing treatments. Here, we deployed electrical probes ($ρ(T)$ and electrical conductivity relaxation (ECR) measurements) to gain a better understanding of the kinetics of the oxygen reduction reaction (ORR) in epitaxial YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) thin films. We identified a new indicator for the onset temperature of oxygen incorporation and report for the first time drastic kinetic deactivation in bare YBCO. We demonstrate that surface decoration using silver micro islands both catalytically activates oxygen incorporation and bypasses surface degradation processes. Our results suggest that the ORR in the studied YBCO samples is limited by a surface reaction. Additionally, weak XRD signatures of the formation of extended bulk defects were identified, which have to be considered in the designing of an optimal oxygenation treatment to obtain best performing superconducting YBCO.

cond-mat.supr-con↗

arXiv2024

Electron Beam Characterization of REBCO-Coated Conductors at Cryogenic Conditions

Particle accelerators with superconducting magnets operating at cryogenic temperatures use a beam screen (BS) liner that extracts heat generated by the circulating bunched charge particle beam before it can reach the magnets. The BS surface, commonly made of high-conductivity copper, provides a low impedance for beam stability reasons, low secondary electron yield (SEY)to mitigate the electron-cloud (EC) effect, and low electron-stimulated desorption yield (ESD) to limit the dynamic pressure rise due to EC. Rare-earth barium copper oxide (REBCO) high-temperature superconductors (HTs) recently reached technical maturity, are produced as coated conductor tapes (REBCO-CCs), and will be considered for application in future colliders to decrease the BS impedance and enable operation at around 50 K, consequently relaxing the cryogenic requirements. Aside from HTS properties, industry-grade REBCO-CCs also need qualification for EC and dynamic vacuum compatibility under accelerator-like conditions. Hence, we report the SEY and ESD measured at cryogenic temperatures of 12 K under low-energy electron irradiation of 0 - 1.4 keV. We also verify the sample compositions and morphologies using XPS, SEM, and EDS methods. The energy and dose dependencies of ESD are comparable to those of technical-grade metals and one sample reached SEY$_{MAX}=$1.2 after electron conditioning.

physics.acc-ph↗

arXiv2016

Diminish Electrostatic in Piezoresponse Force Microscopy through longer ultra-stiff tips

Piezoresponse Force Microscopy is a powerful but delicate nanoscale technique that measures the mechanical response resulting from the application of a highly localized electric field. Though mechanical response is normally due to piezoelectricity, other physical phenomena, especially electrostatic interaction, can contribute to the signal read. We address this problematic through the use of longer ultra-stiff probes providing state of the art sensitivity, with the lowest electrostatic interaction and avoiding working in high frequency regime. In order to find this solution we develop a theoretical description addressing the effects of electrostatic contributions in the total cantilever vibration and its quantification for different setups. The theory is subsequently tested in a Periodically Poled Lithium Niobate (PPLN) crystal, a sample with well-defined 0deg and 180deg domains, using different commercial available conductive tips. We employ the theoretical description to compare the electrostatic contribution effects into the total phase recorded. Through experimental data our description is corroborated for each of the tested commercially available probes. We propose that a larger probe length can be a solution to avoid electrostatic forces, so the cantilever-sample electrostatic interaction is reduced. For hard oxide samples we propose an ultra-stiff cantilever which avoids the use of high frequency voltage but still diminishing electrostatic forces. Our proposed commercially available solution have great implications into avoiding artifacts while studying soft biological samples, multiferroic oxides, and thin film ferroelectric materials and it opens a new window into tip engineering.

cond-mat.mtrl-sci↗

arXiv2016

Piezo-generated charge mapping revealed through Direct Piezoelectric Force Microscopy

While piezoelectrics and ferroelectrics are playing a key role in many everyday applications, there are still a number of open questions related to the physics of those materials. In order to foster the understanding of piezoelectrics and ferroelectric and pave the way to future applications, the nanoscale characterization of these materials is essential. In this light, we have developed a novel AFM based mode that obtains a direct quantitative analysis of the piezoelectric coefficient d33. This nanoscale tool is capable of detecting and reveal piezo-charge generation through the direct piezoelectric effect at the surface of the piezoelectric and ferroelectric materials. We report the first nanoscale images of the charge generated in a thick single crystal of Periodically Poled Lithium Niobate (PPLN) and a Bismuth Ferrite (BiFO3) thin film by applying a force and recording the current produced by the materials. The quantification of both d33 coefficients for PPLN and BFO are 13 +- 2 pC/N and 46 +- 7 pC/N respectively, in agreement with the values reported in the literature. This new mode can operate simultaneously with PFM mode providing a powerful tool for the electromechanical and piezo-charge generation characterization of ferroelectric and piezoelectric materials.

cond-mat.mtrl-sci↗