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Théo Sépulcre

Publications and source records attributed to Théo Sépulcre.

9 recordsLinked to original sources

Forbidden transitions in superconducting artificial atoms

Artificial atoms built from Josephson junctions have become a powerful tool to explore the limits of quantum optics due to their strong coupling to electromagnetic fields and their sensitivity to changes at the single-photon level. This sensitivity to quantum fluctuations complements their metrological and computational use, which are based on the precise oscillating frequency of the underlying supercurrents. We present here a theory for Josephson junctions immersed in electromagnetic fields where focus is shifted from temporal correlations and towards spatial ones. Unlike the commonly used circuit and black-box descriptions, our work is based on a microscopic model that enables systematically accounting for the effect of the spatial and vectorial profile of an electromagnetic field over a junction. As an example of the interactions that emerge in such a setup, we investigate the possibility of driving a junction via a quadrupole transition, using typical experimental parameters in existing devices. With the transition being dependent on the gradient of the electric field -- rather than its intensity -- the junction can be excited in a region where the electric field vanishes.

quant-ph↗

Analytical phase boundary of a quantum driven-dissipative Kerr oscillator from classical stochastic instantons

The framework of Keldysh path integral concisely describes quantum systems driven away from thermal equilibrium, such as the two-photon driven Kerr oscillator. Within the thermodynamic limit of diverging photon occupation, we map it to a Martin-Siggia-Rose-Janssen-de Dominicis path integral, and obtain a purely classical, stochastic equivalent where photon self-interaction plays the role of temperature. This perspective sheds light on the difficulties encountered in the search for an effective thermodynamic potential to describe the bistability of the model. It allows us to estimate the bistable tunneling rates using a real-time instanton technique leading to an analytical expression of the phase boundary, the first to our knowledge. It opens the way to powerful semi-analytical techniques to be applied to various quantum optics models displaying bistability.

quant-ph↗

Experimental observation of multimode quantum phase transitions in a superconducting Bose-Hubbard simulator

The study of phase transitions and critical phenomena arising in quantum driven-dissipative systems, and whether a correspondence can be drawn to their equilibrium counterparts, is a pressing question in contemporary physics. The development of large-scale superconducting circuits provides an experimental platform for these theoretical models. We report an experimental study of a multi-mode dissipative first-order phase transition in a 1D Bose-Hubbard chain consisting of 21 superconducting resonators. This phase transition manifests itself as a simultaneous frequency jump in all resonator modes as the frequency or power of a pump tone is swept. By measuring the system's emission spectrum through the transition, we characterize the dim-to-bright phase transition and construct the full phase diagram. We further perform time-dependent measurements of the switching between the two phases in the transition region, from which we corroborate the transition line and extract transition times ranging from a few ms up to 143~s. Our model, based on single-mode mean-field theory and cross-Kerr interactions, captures the features at moderate pump powers and quantitatively reproduces the transition line. Our results open a new window into non-equilibrium quantum many-body physics and mark a step toward realizing and understanding dissipative phase transitions in the thermodynamic limit using superconducting quantum circuits.

cond-mat.quant-gas↗

Direct detection of down-converted photons spontaneously produced at a single Josephson junction

We study spontaneous photon decay into multiple photons triggered by strong non-linearities in a superconducting quantum simulator of the boundary sine-Gordon impurity model. Previously, spectroscopic signatures of photon-conversion were reported and evidenced as resonances in the many-body spectrum of these systems. Here, we report on the observation of multi-mode fluorescence of a small Josephson junction embedded in a high impedance superconducting transmission line. Measurement of the down-converted photons is achieved using state-of-the-art broadband parametric amplifiers. Photon triplet emission is explicitly demonstrated at a given frequency as the counterpart of inelastic photon decay at three-times the emission frequency. These results open exciting prospects for the burgeoning field of many-body quantum optics and offer a direct signature of the ultra-strong light-matter coupling.

cond-mat.mes-hall↗

Comment on "Absence versus Presence of Dissipative Quantum Phase Transition in Josephson Junctions''

In a recent Letter [Phys. Rev. Lett. 129, 087001, (2022)], Masuki, Sudo, Oshikawa, and Ashida studied a Josephson junction, with Josephson energy $E_{\rm J}$ and charging energy $E_{\rm C}$, shunted by an ohmic transmission line with conductance $α(2e)^2/h$. Their model includes a realistic high frequency cutoff of order $αE_c$, that is typically smaller than the plasma frequency $W$. The authors present a phase diagram showing surprising features, not anticipated in the established literature [eg. Schön and Zaikin, Phys. Reports 198, 237, (1990)]. For $E_{\rm J}/E_{\rm C}$ above a certain value, they find that the junction remains superconducting for all $α$, while below this value, they find that the insulating phase leads to re-entrant superconductivity at small $α$. In this Comment, we show that their Numerical Renormalization Group (NRG) implementation is uncontrolled, and that there is no evidence for the re-entrant superconductivity in the phase diagram presented in Fig. 1a of PRL 129, 087001.

cond-mat.supr-con↗

Universal control of a bosonic mode via drive-activated native cubic interactions

Linear bosonic modes offer a hardware-efficient alternative for quantum information processing but require access to some nonlinearity for universal control. The lack of nonlinearity in photonics has led to encoded measurement-based quantum computing, which rely on linear operations but requires access to resourceful ('nonlinear') quantum states, such as cubic phase states. In contrast, superconducting microwave circuits offer engineerable nonlinearities but suffer from static Kerr nonlinearity. Here, we demonstrate universal control of a bosonic mode composed of a superconducting nonlinear asymmetric inductive element (SNAIL) resonator, enabled by native nonlinearities in the SNAIL element. We suppress static nonlinearities by operating the SNAIL in the vicinity of its Kerr-free point and dynamically activate nonlinearities up to third order by fast flux pulses. We experimentally realize a universal set of generalized squeezing operations, as well as the cubic phase gate, and exploit them to deterministically prepare a cubic phase state in 60 ns. Our results initiate the experimental field of universal continuous-variables quantum computing.

quant-ph↗

Revealing the finite-frequency response of a bosonic quantum impurity

Quantum impurities are ubiquitous in condensed matter physics and constitute the most stripped-down realization of many-body problems. While measuring their finite-frequency response could give access to key characteristics such as excitations spectra or dynamical properties, this goal has remained elusive despite over two decades of studies in nanoelectronic quantum dots. Conflicting experimental constraints of very strong coupling and large measurement bandwidths must be met simultaneously. We get around this problem using cQED tools, and build a precisely characterized quantum simulator of the boundary sine-Gordon model, a non-trivial bosonic impurity problem. We succeeded to fully map out the finite frequency linear response of this system. Its reactive part evidences a strong renormalisation of the nonlinearity at the boundary in agreement with non-perturbative calculations. Its dissipative part reveals a dramatic many-body broadening caused by multi-photon conversion. The experimental results are matched quantitatively to a resummed diagrammatic calculation based on a microscopically calibrated model. Furthermore, we push the device into a regime where diagrammatic calculations break down, which calls for more advanced theoretical tools to model many-body quantum circuits. We also critically examine the technological limitations of cQED platforms to reach universal scaling laws. This work opens exciting perspectives for the future such as quantifying quantum entanglement in the vicinity of a quantum critical point or accessing the dynamical properties of non-trivial many-body problems.

quant-ph↗

Spin-boson quantum phase transition in multilevel superconducting qubits

Superconducting circuits are currently developed as a versatile platform for the exploration of many-body physics, by building on non-linear elements that are often idealized as two-level qubits. A classic example is given by a charge qubit that is capacitively coupled to a transmission line, which leads to the celebrated spin-boson description of quantum dissipation. We show that the intrinsic multilevel structure of superconducting qubits drastically restricts the validity of the spin-boson paradigm due to phase localization, which spreads the wavefunction over many charge states. Numerical Renormalization Group simulations also show that the quantum critical point moves out of the physically accessible range in the multilevel regime. Imposing charge discreteness in a simple variational state accounts for these multilevel effects, that are relevant for a large class of devices.

cond-mat.mes-hall↗

Particle Production in Ultra-Strong Coupling Waveguide QED

Understanding large-scale interacting quantum matter requires dealing with the huge number of quanta that are produced by scattering even a few particles against a complex quantum object. Prominent examples are found from high energy cosmic ray showers to the optical or electrical driving of degenerate Fermi gases. We tackle this challenge in the context of many-body quantum optics, as motivated by the recent developments of circuit quantum electrodynamics at ultrastrong coupling. The issue of particle production is addressed quantitatively with a simple yet powerful concept rooted in the quantum superposition principle. This key idea is illustrated by the study of multi-photon emission from a single two-level artificial atom coupled to a high impedance waveguide. We find surprisingly that the off-resonant inelastic emission lineshape is dominated by broadband particle production, due to the large phase space associated with contributions that do not conserve the number of excitations. Such frequency conversion processes produce striking signatures in time correlation measurements, which can be tested experimentally in quantum waveguides. These ideas open new directions for the simulation of a variety of physical systems, from polaron dynamics in solids to complex superconducting quantum architectures.

cond-mat.mes-hall↗