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Tian Hui Zhang

Publications and source records attributed to Tian Hui Zhang.

8 recordsLinked to original sources

Escape of an Active Ring from an Attractive Surface: Behaving Like a Self-Propelled Brownian Particle

Escape of active agents from metastable states is of great interest in statistical and biological physics. In this study, we investigate the escape of a flexible active ring, composed of active Brownian particles, from a flat attractive surface using Brownian dynamics simulations. To systematically explore the effects of activity, persistence time, and the shape of attractive potentials, we calculate escape time and effective temperature. We observe two distinct escape mechanisms: Kramers-like thermal activation at small persistence times and the maximal force problem at large persistence time, where escape time is determined by persistence time. The escape time explicitly depends on the shape of the potential barrier at high activity and large persistence time. Moreover, when the propulsion force is biased along the ring's contour, escape becomes more difficult and is primarily driven by thermal noise. Our findings highlight that, despite its intricate configuration, the active ring can be effectively modeled as a self-propelled Brownian particle when studying its escape from a smooth surface.

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Constrained motion of self-propelling eccentric disks linked by a spring

It has been supposed that the interplay of elasticity and activity plays a key role in triggering the non-equilibrium behaviors in biological systems. However, the experimental model system is missing to investigate the spatiotemporally dynamical phenomena. Here, a model system of an active chain, where active eccentric-disks are linked by a spring, is designed to study the interplay of activity, elasticity, and friction. Individual active chain exhibits longitudinal and transverse motion, however, it starts to self-rotate when pinning one end, and self-beats when clamping one end. Additionally, our eccentric-disk model can qualitatively reproduce such behaviors and explain the unusual self-rotation of the first disk around its geometric center. Further, the structure and dynamics of long chains were studied via simulations without steric interactions. It was found that hairpin conformation emerges in free motion, while in the constrained motions, the rotational and beating frequencies scale with the flexure number (the ratio of self-propelling force to bending rigidity), ~4/3. Scaling analysis suggests that it results from the balance between activity and energy dissipation. Our findings show that topological constraints play a vital role in non-equilibrium synergy behavior.

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Activity Waves in Condensed Phases of Quincke Rollers

Wave-exciting is a universal phenomenon in physical and biological excitable systems. Here we show that colloidal systems of Quincke rollers which are driven periodically can condense into active liquids and active crystals, in which waves can be excited. In active liquids, the waves propagate antiparallel to local density gradients via the splitting of dense bands, and cross over each other in collision as sound waves do. The waves in active crystals have a sharp front like that of shock waves, and propagate parallel to local density gradients. The shock waves annihilate or converge as they collide. Detailed investigations on microscopic dynamics reveal that in sound waves, the dynamics of rollers is dominated by electrostatic repulsions; in shock waves, the dynamics is encoded with a density-dependent collective memory. These findings demonstrate a realization of excitable colloidal systems with tunable dynamics. This is of great interests in exploring the principles of self-organization and the fabrication of active functional materials.

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Tunable Memory and Activity of Quincke Particles in Micellar Fluid

Memory can remarkably modify the collective behaviors of active particles. We show that in a micellar fluid, Quincke particles driven by a square-wave electric field exhibit a frequency-dependent memory. Upon increasing the frequency, a memory of directions emerges whereas the activity of particles decreases. As the activity is dominated by interaction, Quincke particles aggregate and form dense clusters in which the memory of the direction is further enhanced due to the stronger electric interactions. The density-dependent memory and activity result in dynamic heterogeneity in flocking and offer new opportunity for study of collective motions.

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Modulated Collective Behaviors and Condensation of Bacteria

Bacteria can spontaneously develop collective motions by aligning their motions in dense systems. Here, we show that bacteria can also respond collectively to an alternating electrical field and form dynamic clusters oscillating at the same frequency of the field. As the dynamic clusters go beyond a critical size, they split into smaller ones spontaneously. The critical size for splitting depends on the frequency of electric field and the concentration of bacteria. We show that instead of their biological activity, the physical properties of bacteria as charged particles are responsible for the formation of dynamic clusters. Electroconvective flows across the system play the key role in stabilizing the clusters. However, to form clusters, collective hydrodynamic cooperation between bacteria is important such that no aggregation occurs in dilute suspensions. The findings in this study illustrate that bio-systems can respond collectively to an external field, promising an effective way to control and modulate the behavior of organisms. Moreover, the controlled aggregation and condensation of bacteria offer a robust approach to improve the local concentration of bacteria for early and rapid detection, which has wide applications in clinics.

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Emergence of Self-dual Patterns in Active Colloids with Periodical Feedback to Local Density

The central task in the study of self-organization is to explore the general mechanism of emergences. However, this is inhibited by the missing of a full knowledge of the microscopic dynamics of emergence. Here, in this study, the microscopic dynamics of self-organization for patterns is investigated and quantified in a periodically propelled Quincke system. The periodical coupling between propulsion and repulsion at the particle level leads to local directed oscillating particle flows and promises a loop of positive feedback to density fluctuations. Nevertheless, the global evolution of the resulting cluster phase is dominated by a global dual transformation. As stable attractors of the dual transformation, self-dual patterns including stripe patterns and square lattices can be achieved by tuning the strength and the frequency of propelling. However, stripes are possible only at strong propelling where boundary particle flows can form. The findings in this study show that the dynamics of emergence on different length scales are controlled by different mechanisms. The competition and the interplay between different microscopic dynamic processes play the central role in determining the product of emergence. Moreover, the periodically oscillating self-dual patterns demonstrate a classical approach to time crystals.

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Synchronized Fractionation and Phase Separation in Binary Colloids

Fractionation is necessary for self-assembly in multicomponent mixtures. Here, reversible fractionation and crystallization are realized and studied in a two-dimensional binary colloids which is supersaturated by enhancing the attraction between colloidal particles. As a deep and fast supersaturation results in gels with a uniform distribution of binary particles, a gradual quasistatic supersaturating process leads to a two-step crystallization in which small particles and large particles are fractionated as coexisting crystal and liquid phases respectively. Fractionation occurs as well in the quasistatic melting of gel. We show that the synchronized fractionation and phase separation arises from the competition between the size-dependent repulsion and the tunable attraction. The results in this study demonstrate a robust mechanism of fractionation via phase separation, and have important implication in understanding the reversible formation of membraneless organelles in living cells.

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Rotational averaging-out gravitational sedimentation of colloidal dispersions and phenomena

We report on the differences between colloidal systems left to evolve in the earth's gravitational field and the same systems for which a slow continuous rotation averaged out the effects of particle sedimentation on a distance scale small compared to the particle size. Several systems of micron-sized colloidal particles were studied: a hard sphere fluid, colloids interacting via long-range electrostatic repulsions above the freezing volume fraction, an oppositely charged colloidal system close to either gelation and/or crystallization, colloids with a competing short-range depletion attraction and a long-range electrostatic repulsion, colloidal dipolar chains, and colloidal gold platelets under conditions where they formed stacks. Important differences in the structure formation were observed between the experiments where the particles were allowed to sediment and those where sedimentation was averaged out. For instance, in the case of colloids interacting via long-range electrostatic repulsions, an unusual sequence of dilute-Fluid/dilute-Crystal/dense-Fluid/dense-Crystal phases was observed throughout the suspension under the effect of gravity, related to the volume fraction dependence of the colloidal interactions, whereas the system stayed homogeneously crystallized with rotation. For the oppositely charged colloids, a gel-like structure was found to collapse under the influence of gravity with a few crystalline layers grown on top of the sediment, whereas when the colloidal sedimentation was averaged out, the gel completely transformed into crystallites that were oriented randomly throughout the sample. Rotational averaging out gravitational sedimentation is an effective and cheap way to estimate the importance of gravity for colloidal self-assembly processes.

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