arXiv subjects

Tim Schröder

Publications and source records attributed to Tim Schröder.

At least 19 recordsLinked to original sources

arXiv2026

A non-Markovian approach to spin-phonon coherence and the breakdown of the Markovian approximation

Qubit coherence is an essential figure of merit for quantum information processing applications such as quantum computing, or quantum repeaters. Understanding the coherence properties of the underlying physical qubits that facilitate such applications is therefore are often limited by coupling to lattice phonons, which in turn constrains operation temperature. Here we study phonon induced electronic spin decoherence in group-IV vacancy centers in diamond. We begin by modeling the spin-phonon interaction and then employ the widely used Born-Markov approximation, highlighting its inconsistencies in this setting and its deviations from experimental observations. To close the gap between theoretical predictions and experimental results, we relax certain approximations, investigate their contributions to the predicted coherence times, and identify the dominant sources of discrepancy. We further demonstrate that experimentally measured electronic spin coherence dynamics are consistently captured within a non-Markovian framework, and we show how the magnetic field orientation influences the qubit coherence time.

quant-ph↗

arXiv2026

High-cooperativity coupling and spin-resolved extinction of tin-vacancy centers in a diamond-like microcavity

The tin-vacancy (SnV) center in diamond is a promising spin-photon interface for quantum networks, combining favorable optical properties with spin coherence above 1K. Unfolding the full potential requires cavity enhancement to increase photon-emitter coupling efficiency. Here, we demonstrate cavity-enhanced light-matter coupling of SnV centers in a fully tunable Fabry-Pérot microcavity operating at temperatures down to 1K with in-situ magnetic field control. We access the diamond-like regime of hybrid cavity modes through integration of low-roughness diamond membranes, where the field is concentrated inside the diamond and Purcell enhancement is maximized. Diamond-like modes deliver a more than two-fold increase in the effective Purcell factor over air-like modes, reaching $C_0 = 4.1(1)$ compared to $C_0 = 1.85(5)$ in the air-like case, while simultaneously relaxing mechanical stability requirements. Resonant probing reveals coherent cavity-emitter coupling with 96% extinction contrast and a coherent cooperativity of $C = 4.0(14)$. By applying a magnetic field, we further achieve spin-resolved cavity extinction, observing spin-selective optical transitions with a contrast of ${\cal C}_{\rm spin} = 0.91$. These results establish SnV centers in diamond coupled to open Fabry-Pérot microcavities as a promising platform for efficient spin-photon interfaces.

quant-ph↗

arXiv2026

Engineering Nanodiamonds for Quantum Sensing: Material Constraints at the Nanoscale

Optically addressable solid-state spin defects have emerged as powerful multimodal quantum sensors, with nitrogen-vacancy (NV) centers in bulk diamond providing benchmark quantum control and sensitivity under ambient conditions. Embedding such defects in nanodiamonds (NDs) extends these capabilities to mobile probes capable of accessing complex biological and nanoscale environments. Reduced dimensions, however, introduce constraints beyond volumetric spin impurities, notably enhanced lattice strain and surface-induced noise sources, which shorten NV spin relaxation times (T1 and T2) and destabilize the NV charge state, as well as resulting in pronounced particle-to-particle variability in NDs typically produced by top-down approaches. These effects complicate both sensing performance and the quantitative interpretation of multimodal signals in realistic environments. This article provides a structured perspective on the physical mechanisms by which material properties constrain NV behavior in NDs, together with mitigation strategies that shape the robust use of these mobile quantum sensors for biosensing and nanoscale science.

quant-ph↗

arXiv2026

Quantum Secure Authentication with Color Centers in Diamond

We present a quantum token scheme in which the token is a quantum state that ensures secure authentication or payment. In our approach, rooted in Wiesner's quantum money concept, a token is encoded in a multi-qubit state generated by a single-photon source and transmitted to a user who holds a quantum memory register. By leveraging state-dependent reflection from a highly efficient sawfish nanophotonic crystal cavity and implementing high-fidelity fractional quantum gates through a pulse train of optical pi/8 pulses, our design achieves gate fidelities exceeding 99% under realistic operating conditions. We also analyze microwave control, which extends the viability to longer storage times, albeit at reduced operational rates. We rigorously examine the impact of finite photon bandwidth, cavity design parameters, spectral diffusion, and control imperfections on overall performance. Our comprehensive model indicates that, with near-term improvements in device efficiency and conversion rates, the token acceptance rate can approach the MHz regime for short-distance communication links while remaining robust against optimal cloning attacks. These findings pave the way for integrating unforgeable quantum tokens into larger-scale quantum networks, thereby significantly enhancing the security of future quantum network applications.

quant-ph↗

arXiv2026

Optical probing of phononic properties of a tin-vacancy color center in diamond

The coherence characteristics of a tin-vacancy color center (SnV) in diamond are investigated through optical means, including linewidth broadening effects and coherent population trapping (CPT) between the ground state orbital levels. Spectral analysis is required as due to the large spin-orbit splitting of the orbital ground states, thermalization between the ground states occurs at rates that are impractical to measure directly in the time domain. First, by implementing a temperature-dependent linewidth broadening measurement, including the challenging-to-measure D transition, phononic coupling coefficients are determined. These measurements are performed on an emitter with a lifetime-limited linewidth and atom-like properties, making the measurement representative for high-quality SnVs. Next, a CPT-type experiment is carried out to independently analyze thermal decoherence processes at 4 K. The spectral information is transformed into its conjugate variable time, providing picosecond resolution and revealing an orbital depolarization timescale of ${\sim30{\rm~ps}}$. Consequences of the investigated dynamics are then used to estimate spin dephasing times limited by thermal effects.

quant-ph↗

arXiv2026

Quantum Networks Using Color Defects in Diamond: Principles, Progress, and Perspectives

Large-scale quantum networks will enable entirely new applications of quantum information science in fields such as quantum communication, distributed quantum computing, sensing, and metrology. To build nodes of such networks, diamond color defects are one of the promising candidates. Their excellent optical properties, fast spin-qubit control, and long spin coherence times make them well-suited for quantum information processing and quantum memory applications. Additionally, recent advances in the heterogeneous integration of diamond nanophotonic structures with photonic integrated circuits have made these systems more efficient and well-suited for scalable quantum processor architectures. In this comprehensive review, we discuss the optical and spin properties of these systems, recent progress in the building blocks of quantum networks, and demonstrations of metropolitan-scale quantum networks, as well as the challenges associated with these systems at both the fundamental and experimental levels, along with potential solutions.

quant-ph↗

arXiv2026

Spectral Diffusion Mitigation with a Laser Pulse Sequence

The optical spectrum of a quantum system is jointly determined by the properties of the emitter and the driving field. All-optical spectral control can hence be a promising method to engineer the properties of single photon emitters for quantum technological applications. It was proposed that driving a two-level system with a periodic sequence of optical pi-pulses during the excited state lifetime shifts the emission and absorption maximum to an arbitrarily detuned pulse carrier frequency, enabling the mitigation of spectral diffusion in noisy emitters. In this article, we report on the first experimental observation of this effect. We implement the protocol on a solid-state emitter and reduce its inhomogeneously broadened optical linewidth close to the lifetime limit. By detuning the excitation laser, we are able to concentrate approximately half of the absorption to a freely selectable target frequency. Our approach is solely based on properties of coherently evolving quantum systems, rendering it applicable to a wide range of individual and ensembles of quantum emitters.

quant-ph↗

arXiv2026

SUPER and femtosecond spin-conserving coherent excitation of a tin-vacancy color center in diamond

The coherent excitation of an optically active spin system is one of the key elements in the engineering of a spin-photon interface. Using the novel SUPER scheme, we coherently control the main optical transition of a tin-vacancy color center in diamond with nonresonant ultrashort optical pulses. Furthermore, we implement a femtosecond control scheme using resonant pulses for achieving record short quantum gates applied to diamond color centers. We simulate the applicability of the SUPER scheme to spin qubits and experimentally investigate spin mixing. Finally, we propose a spin-spin entanglement scheme in a scenario where the excitation with broadband pulses is incompatible with spin-selective excitation. The employed ultrafast quantum gates open up a new regime of quantum control with solid-state color centers, enabling multi-gate operations and efficient spectral filtering of the excitation laser from deterministically prepared coherent photons.

quant-ph↗

arXiv2026

Secure authentication via Quantum Physical Unclonable Functions: a review

Quantum Physical Unclonable Functions (QPUFs) offer a physically grounded approach to secure authentication, extending the capabilities of classical PUFs. This review covers their theoretical foundations and key implementation challenges - such as quantum memories and Haar-randomness -, and distinguishes QPUFs from Quantum Readout PUFs (QR-PUFs), more experimentally accessible yet less robust against quantum-capable adversaries. A co-citation-based selection method is employed to trace the evolution of QPUF architectures, from early QR-PUFs to more recent Hybrid PUFs (HPUFs). This method further supports a discussion on the role of information-theoretic analysis in mitigating inconsistencies in QPUF responses, underscoring the deep connection between secret-key generation and authentication. Despite notable advances, achieving practical and robust QPUF-based authentication remains an open challenge.

quant-ph↗

arXiv2026

Practical quantum tokens: challenges and perspectives

The concept of quantum tokens dates back alongside quantum cryptography to Stephen Wiesner's seminal work in 1983[1]. Already this initial work proposes society-relevant applications such as secure quantum banknotes, which can be exchanged between a bank and a customer. This quantum currency is based on various physical states that can be easily verified but is protected from being copied by the fundamental quantum laws. Four decades later, these ideas have flourished in the field of quantum information, and the concept of quantum banknotes has not only adopted many varying names, such as quantum money, quantum coins, quantum-digital payments, and quantum tokens, but also reached its first experimental demonstrations. In this perspective article, we discuss the current state-of-the-art of quantum tokens in the field of quantum information, as well as their future perspectives. We present a number of physical realizations of quantum tokens with integrated quantum memories and their applicability scenarios in detail. Finally, we discuss how quantum tokens fit into the information security ecosystem and consider their relationship to post-quantum cryptography.

quant-ph↗

arXiv2025

Waveguide-integrated colour centres in silicon carbide with broadband photonic crystal reflectors for efficient readout

Spin-active colour centres in 4H silicon carbide are promising candidates as building blocks for quantum information applications. To increase the photon count rate of the emitters at low temperatures, the colour centres must be integrated into nanophotonic structures and characterised under cryogenic conditions. Here, we design and fabricate waveguide structures attached with an efficient Dinosaur photonic crystal reflector at one side. The devices show broadband reflection over a range of 60 THz with a peak reflectance above 80 %. Additionally, colour centres were integrated into these structures and characterised at cryogenic conditions. The emission was collected by a tapered-waveguide-tapered-fibre interface. Although the spectral stability of the emitters must be further improved for high excitation powers, the saturation intensity in standard PLE measurements is about 104 kcps. The count rate can be further improved to about 125 kcps with a charge-resonance check measurement scheme. To highlight the relevance of our devices, we theoretically show that these count rates enable optical single-shot readout with a fidelity exceeding 98 %.

quant-ph↗

arXiv2025

Software Framework for Optically Accessible Quantum Memory Using Group-IV Color Centers in Diamond

In the rapidly evolving field of quantum technology, the precise and detailed description of quantum components is not just a necessity but the foundation for advancing research, development, and applications. Optically accessible quantum memories are key building blocks for devices such as quantum repeaters and two-factor authentication. The memory we describe here is based on a tin-vacancy color center coupled to a highly efficient cavity. It leverages state-dependent reflection from the cavity and implements high-fidelity fractional single qubit gates via a train of optical $π/8$ pulses. We also describe its operation under microwave control, further extending our analysis. Our primary contribution in this work is the integration of this device model into a standardized software framework for quantum memory architectures.

quant-ph↗

arXiv2025

Hybrid Quantum Repeater Chains with Semiconductor Quantum Dots and Group-IV-Vacancy Color Centers in Diamond

We propose and analyze a hybrid quantum repeater architecture that combines two leading hardware platforms: quantum dots (QDs) as bright, deterministic sources of entangled photon pairs and group-IV-vacancy centers in diamond as efficient, heralded quantum memories. This combination leverages high-rate entanglement generation together with long-lived storage, enabling scalable entanglement distribution over long distances. A key challenge is the large bandwidth mismatch between QD photons and the narrow optical transitions of the memories. We combine a comprehensive model of the spin-photon interface, including full spin-photon coupling dynamics, and explore mitigation strategies such as frequency filtering and optimized magnetic-field orientation. Our results show that with optimized designs, photon-to-memory transfer can be achieved with high efficiency and fidelity, supporting the feasibility of such hybrid systems. Finally, we analyze a full repeater chain using experimentally achievable parameters and find that a network with thousands of memories across several repeater nodes could achieve a secret-key rate of 500 bit/s over 1,000 km, demonstrating the strong potential of this approach for next-generation quantum networks.

quant-ph↗

arXiv2025

Dinosaur Photonic Crystal Cavity Interfaces for Color Center Coupling to Triangular Nanostructures

Waveguide-coupled photonic crystal cavities with a triangular cross section fabricated by angled etching are suitable to interface embedded color centers with flying photonic qubits in quantum information applications. Moreover, their fabrication requires fewer processing steps compared to nanostructures produced by quasi-isotropic undercutting. As an alternative to established hole-based photonic crystal cavities, we introduce corrugated triangular 'Dinosaur' photonic crystal cavities, and develop a tapered, quasi loss-free cavity-waveguide interface to adiabatically interconvert Bloch and waveguide modes. We optimize the cavity-waveguide interface to minimize photon losses and demonstrate that its adjustment allows precise tuning of the light-matter interaction.

physics.optics↗

arXiv2025

Quantum Electrometer for Time-Resolved Material Science at the Atomic Lattice Scale

The detection of individual charges plays a crucial role in fundamental material science and the advancement of classical and quantum high-performance technologies that operate with low noise. However, resolving charges at the lattice scale in a time-resolved manner has not been achieved so far. Here, we present the development of an electrometer with 60 ns acquisition steps, leveraging on the spectroscopy of an optically-active spin defect embedded in a solid-state material with a non-linear Stark response. By applying our approach to diamond, a widely used platform for quantum technology applications, we can distinguish the distinct charge traps at the lattice scale, quantify their impact on transport dynamics and noise generation, analyze relevant material properties, and develop strategies for material optimization.

physics.app-ph↗

arXiv2025

Optical spin readout of a silicon color center in the telecom L-band

Silicon-based quantum technologies have gained increasing attention due to their potential for large-scale photonic integration, long spin coherence times, and compatibility with CMOS fabrication. Efficient spin-photon interfaces are crucial for quantum networks, enabling entanglement distribution and information transfer over long distances. While several optically active quantum emitters in silicon have been investigated, no spin-active defect with optical transitions in the telecom L-band-a key wavelength range for low-loss fiber-based communication-has been experimentally demonstrated. Here, we demonstrate the optical detection of spin states in the C center, a carbon-oxygen defect in silicon that exhibits a zero-phonon line at 1571 nm. By combining optical excitation with microwave driving, we achieve optically detected magnetic resonance, enabling spin-state readout via telecom-band optical transitions. These findings provide experimental validation of recent theoretical predictions and mark a significant step toward integrating spin-based quantum functionalities into silicon photonic platforms, paving the way for scalable quantum communication and memory applications in the telecom L-band.

quant-ph↗

arXiv2025

Retrieving Lost Atomic Information: Monte Carlo-based Parameter Reconstruction of an Optical Quantum System

In regimes of low signal strengths and therefore a small signal-to-noise ratio, standard data analysis methods often fail to accurately estimate system properties. We present a method based on Monte Carlo simulations to effectively restore robust parameter estimates from large sets of undersampled data. This approach is illustrated through the analysis of photoluminescence excitation spectroscopy data for optical linewidth characterization of a nitrogen-vacancy color center in diamond. We evaluate the quality of parameter prediction using standard statistical data analysis methods, such as the median, and the Monte Carlo method. Depending on the signal strength, we find that the median can be precise (narrow confidence intervals) but very inaccurate. A detailed analysis across a broad range of parameters allows to identify the experimental conditions under which the median provides a reliable predictor of the quantum emitter's linewidth. We also explore machine learning to perform the same task, forming a promising addition to the parameter estimation toolkit. Finally, the developed method offers a broadly applicable tool for accurate parameter prediction from low signal data, opening new experimental regimes previously deemed inaccessible.

quant-ph↗

arXiv2024

The Influence of Experimental Imperfections on Photonic GHZ State Generation

While the advantages of photonic quantum computing, including direct compatibility with communication, are apparent, several imperfections such as loss and distinguishability presently limit actual implementations. These imperfections are unlikely to be completely eliminated, and it is therefore beneficial to investigate which of these are the most dominant and what is achievable under their presence. In this work, we provide an in-depth investigation of the influence of photon loss, multi-photon terms and photon distinguishability on the generation of photonic 3-partite GHZ states via established fusion protocols. We simulate the generation process for SPDC and solid-state-based single-photon sources using realistic parameters and show that different types of imperfections are dominant with respect to the fidelity and generation success probability. Our results indicate what are the dominant imperfections for the different photon sources and in which parameter regimes we can hope to implement photonic quantum computing in the near future.

quant-ph↗