arXiv subjects

Toru Sakai

Publications and source records attributed to Toru Sakai.

At least 37 records · Page 2Linked to original sources

arXiv2015

Magnetization Process of the Spin-S Kagome-Lattice Heisenberg Antiferromagnet

The magnetization process of the spin-S Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. Our numerical-diagonalization data for small finite-size clusters with S=1, 3/2, 2, and 5/2 suggest that a magnetization plateau appears at one-third of the height of the saturation in the magnetization process irrespective of S. We discuss the S dependences of the edge fields and the width of the plateau in comparison with recent results obtained by real-space perturbation theory.

cond-mat.mtrl-sci↗

arXiv2015

Instability of a ferrimagnetic state of a frustrated S=1/2 Heisenberg antiferromagnet in two dimensions

To clarify the instability of the ferrimagnetism which is the fundamental magnetism of ferrite, numerical-diagonalization study is carried out for the two-dimensional S=1/2 Heisenberg antiferromagnet with frustration. We find that the ferrimagnetic ground state has the spontaneous magnetization in small frustration; due to a frustrating interaction above a specific strength, the spontaneous magnetization discontinuously vanishes so that the ferrimagnetic state appears only under some magnetic fields. We also find that, when the interaction is increased further, the ferrimagnetism disappears even under magnetic field.

cond-mat.mtrl-sci↗

arXiv2014

Anomalous Behavior of the Magnetization Process of the S = 1/2 Kagome-Lattice Heisenberg Antiferromagnet at One-Third Height of the Saturation

The magnetization process of the S=1/2 Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. We successfully obtain a new result of the magnetization process of a 42-site cluster in the entire range. Our analysis clarifies that the critical behavior around one-third of the height of the saturation is different from the typical behavior of the well-known magnetization plateau in two-dimensional systems. We also examine the effect of the $\sqrt{3}\times\sqrt{3}$-type distortion added to the kagome lattice. We find at one-third of the height of the saturation in the magnetization process that the undistorted kagome point is just the boundary between two phases that show their own properties that are different from each other. Our results suggest a relationship between the anomalous critical behavior at the undistorted point and the fact that the undistorted point is the boundary.

cond-mat.str-el↗

arXiv2014

Spin-Flop Phenomenon of Two-Dimensional Frustrated Antiferromagnets without Anisotropy in Spin Space

Motivated by a recent finding of a spin-flop phenomenon in a system without anisotropy in spin space reported in the S=1/2 Heisenberg antiferromagnet on the square-kagome lattice, we study the S=1/2 Heisenberg antiferromagnets on two other lattices composed of vertex-sharing triangles by the numerical diagonalization method. One is a novel lattice including a shuriken shape with four teeth; the other is the kagome lattice with $\sqrt{3}\times\sqrt{3}$-structure distortion, which includes a shuriken shape with six teeth. We find in the magnetization processes of these systems that a magnetization jump accompanied by a spin-flop phenomenon occurs at the higher-field-side edge of the magnetization plateau at one-third the height of saturation. This finding indicates that the spin-flop phenomenon found in the isotropic system on the square-kagome lattice is not an exceptional case.

cond-mat.str-el↗

arXiv2014

Magnetization Process of the S=1/2 Heisenberg Antiferromagnet on the Cairo Pentagon Lattice

We study the S=1/2 Heisenberg antiferromagnet on the Cairo pentagon lattice by the numerical-diagonalization method. We tune the ratio of two antiferromagnetic interactions coming from two kinds of inequivalent sites in this lattice, examining the magnetization process of the antiferromagnet; particular attention is given to one-third of the height of the saturation. We find that quantum phase transition occurs at a specific ratio and that a magnetization plateau appears in the vicinity of the transition. The plateau is accompanied by a magnetization jump on one side among the edges due to the spin-flop phenomenon. Which side the jump appears depends on the ratio.

cond-mat.mtrl-sci↗

arXiv2014

Quantum spin-liquid behavior in the spin-1/2 random Heisenberg antiferromagnet on the triangular lattice

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts κ-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg antiferromagnets consisting of molecular dimers. These compounds exhibit no magnetic ordering nor the spin freezing down to very low temperature, while various physical quantities exhibit gapless behaviors. Recent dielectric measurements revealed the glassy dielectric response suggesting the random freezing of the electric polarization degrees of freedom. Inspired by this observation, we propose as a minimal model of the observed quantum spin-liquid behavior the S=1/2 antiferromagnetic Heisenberg on the triangular lattice with a quenched randomness in the exchange interaction. We study both zero- and finite-temperature properties of the model by an exact diagonalization method, to find that when the randomness exceeds a critical value the model exhibits a quantum spin-liquid ground state. This randomness-induced quantum spin-liquid state exhibits gapless behaviors including the temperature-linear specific heat. The results provide a consistent explanation of the recent experimental observations on organic salts.

cond-mat.str-el↗

arXiv2013

Edge Modes in the Intermediate-D and Large-D Phases of the S=2 Quantum Spin Chain with XXZ and On-Site Anisotropies

We investigate the edge modes at T=0 in the intermediate-D (ID) phase and the large-D (LD) phase of the S=2 quantum spin chain with the XXZ anisotropy and the generalized on-site anisotropies by use of the DMRG. There exists a gapless edge mode in the ID phase, while no gapless edge mode in the LD phase. These results are consistent with the physical pictures of these phases. We also show the ground-state phase diagrams obtained by use of the exact diagonalization and the level spectroscopy analysis.

cond-mat.str-el↗

arXiv2013

Long-Range Order of the Three-Sublattice Structure in the S = 1 Heisenberg Antiferromagnet on a Spatially Anisotropic Triangular Lattice

We study the S=1 Heisenberg antiferromagnet on a spatially anisotropic triangular lattice by the numerical diagonalization method. We examine the stability of the long-range order of a three-sublattice structure observed in the isotropic system between the isotropic case and the case of isolated one-dimensional chains. It is found that the long-range-ordered ground state with this structure exists in the range of 0.7 \simle J_2/J_1 \le 1, where J_1 is the interaction amplitude along the chains and J_2 is the amplitude of other interactions.

cond-mat.str-el↗

arXiv2012

Anomalous behavior of the spin gap of a spin-1/2 two-leg antiferromagnetic ladder with Ising-like rung interactions

Using mainly numerical methods, we investigate the width of the spin gap of a spin-1/2 two-leg ladder described by $\cH= J_\rl \sum_{j=1}^{N/2} [ \vS_{j,a} \cdot \vS_{j+1,a} + \vS_{j,b} \cdot \vS_{j+1,b} ] + J_\rr \sum_{j=1}^{N/2} [λ(S^x_{j,a} S^x_{j,b} + S^y_{j,a} S^y_{j,b}) + S^z_{j,a} S^z_{j,b}] $, where $S^α_{j,a(b)}$ denotes the $α$-component of the spin-1/2 operator at the $j$-th site of the $a (b)$ chain. We mainly focus on the $J_\rr \gg J_\rl > 0$ and $|λ| \ll 1$ case. The width of the spin gap as a function of $λ$ anomalously increases near $λ= 0$; for instance, for $-0.1 < λ< 0.1$ when $J_{\rm l}/J_{\rm r} = 0.1$. The gap formation mechanism is thought to be different for the $λ< 0$ and $λ> 0$ cases. Since, in usual cases, the width of the gap becomes zero or small at the point where the gap formation mechanism changes, the above gap-increasing phenomenon in the present case is anomalous. We explain the origin of this anomalous phenomenon by use of the degenerate perturbation theory. We also draw the ground-state phase diagram.

cond-mat.str-el↗

arXiv2012

Spin-Chirality Separation and S_3-Symmetry Breakings in the Magnetization Plateau of the Quantum Spin Tube

We study the magnetization plateau state of the three-leg spin-1/2 tube in the strong rung coupling region, where S_3-symmetry breakings and low-energy chirality degree of freedom play crucial roles. On the basis of the effective chirality model and density matrix renormalization group, we clarify that, as the leg coupling increases, the chirality liquid with gapless non-magnetic excitations, the spin imbalance phase and the vector-spin-chirality ordered phase emerge without closing the plateau spin gap. The relevance of these results to experiments is also discussed.

cond-mat.str-el↗

arXiv2011

Numerical-Diagonalization Study of Spin Gap Issue of the Kagome Lattice Heisenberg Antiferromagnet

We study the system size dependence of the singlet-triplet excitation gap in the $S=1/2$ kagome-lattice Heisenberg antiferromagnet by numerical diagonalization. We successfully obtain a new result of a cluster of 42 sites. The two sequences of gaps of systems with even-number sites and that with odd-number sites are separately analyzed. Careful examination clarifies that there is no contradiction when we consider the system to be gapless.

cond-mat.mtrl-sci↗

arXiv2011

How to distinguish the Haldane/Large-D state and the intermediate-D state in an S=2 quantum spin chain with the XXZ and on-site anisotropies

We numerically investigate the ground-state phase diagram of an S=2 quantum spin chain with the $XXZ$ and on-site anisotropies described by ${\mathcal H}=\sum_j (S_j^x S_{j+1}^x+S_j^y S_{j+1}^y+ΔS_j^z S_{j+1}^z) + D \sum_j (S_j^z)^2$, where $Δ$ denotes the XXZ anisotropy parameter of the nearest-neighbor interactions and $D$ the on-site anisotropy parameter. We restrict ourselves to the $Δ>0$ and $D>0$ case for simplicity. Our main purpose is to obtain the definite conclusion whether there exists or not the intermediate-$D$ (ID) phase, which was proposed by Oshikawa in 1992 and has been believed to be absent since the DMRG studies in the latter half of 1990's. In the phase diagram with $Δ>0$ and $D>0$ there appear the XY state, the Haldane state, the ID state, the large-$D$ (LD) state and the Néel state. In the analysis of the numerical data it is important to distinguish three gapped states; the Haldane state, the ID state and the LD state. We give a physical and intuitive explanation for our level spectroscopy method how to distinguish these three phases.

cond-mat.stat-mech↗

arXiv2011

Haldane, Large-D and Intermediate-D States in an S=2 Quantum Spin Chain with On-Site and XXZ Anisotropies

Using mainly numerical methods, we investigate the ground-state phase diagram of the S=2 quantum spin chain described by $H = \sum_j (S_j^x S_{j+1}^x + S_j^y S_{j+1}^y + ΔS_j^z S_{j+1}^z) + D \sum_j (S_j^z)^2$, where $Δ$ denotes the $XXZ$ anisotropy parameter of the nearest-neighbor interactions and $D$ the on-site anisotropy parameter. We restrict ourselves to the case with $Δ\ge 0$ and $D \ge 0$ for simplicity. Each of the phase boundary lines is determined by the level spectroscopy or the phenomenological renormalization analysis of numerical results of exact-diagonalization calculations. The resulting phase diagram on the $Δ$-$D$ plane consists of four phases; the XY 1 phase, the Haldane/large-$D$ phase, the intermediate-$D$ phase and the Néel phase. The remarkable natures of the phase diagram are: (1) the Haldane state and the large-$D$ state belong to the same phase; (2) there exists the intermediate-$D$ phase which was predicted by Oshikawa in 1992; (3) the shape of the phase diagram on the $Δ$-$D$ plane is different from that believed so far. We note that this is the first report of the observation of the intermediate-$D$ phase.

cond-mat.str-el↗

arXiv2011

Critical magnetization behaviors of the triangular and Kagome lattice quantum antiferromagnets

We investigate the $S=1/2$ quantum spin antiferromagnets on the triangular and Kagome lattices in magnetic field, using the numerical exact diagonalization. Particularly we focus on an anomalous magnetization behavior of each system at 1/3 of the saturation magnetization. The critical exponent analyses suggest that it is a conventional magnetization plateau on the triangular lattice, while an unconventional phenomenon, called the magnetization ramp, on the Kagome lattice.

cond-mat.mtrl-sci↗

arXiv2011

Collapse of Ferrimagnetism in Two-Dimensional Heisenberg Antiferromagnet due to Frustration

We study ferrimagnetism in the ground state of the antiferromagnetic Heisenberg model on the spatially anisotropic kagome lattice, in which ferrimagnetism of the conventional Lieb-Mattis type appears in the region of weak frustration whereas the ground state is nonmagnetic in the isotropic case. Numerical diagonalizations of small finite-size clusters are carried out to examine the spontaneous magnetization. We find that the spontaneous magnetization changes continuously in the intermediate region between conventional ferrimagnetism and the nonmagnetic phase. Local magnetization of the intermediate state shows strong dependence on the site position, which suggests non-Lieb-Mattis ferrimagnetism.

cond-mat.str-el↗

arXiv2010

Quantum spin nanotubes -- frustration, competing orders and criticalities

Recent developments of theoretical studies on spin nanotubes are reviewed, especially focusing on the $S=1/2$ three-leg spin tube. In contrast to the three-leg spin ladder, the tube has a spin gap in case of the regular-triangle unit cellwhen the rung interaction is sufficiently large. The effective theory based on the Hubbard Hamiltonian indicates a quantum phase transition to the gapless spin liquid due to the lattice distortion to an isosceles triangle. This is also supported by the numerical diagonalization and the density matrix renormalization group analyses. Furthermore, combining analytical and numerical approaches, we reveal several novel magnetic-field-induced phenomena: Néel, dimer, chiral and/or inhomogeneous orders, new mechanism for the magnetization plateau formation,and others. The recently synthesized spin tube materials are also briefly introduced.

cond-mat.stat-mech↗

arXiv2010

Magnetization Process of Kagome-Lattice Heisenberg Antiferromagnet

The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".

cond-mat.str-el↗

arXiv2007

Magnetic Field versus Temperature Phase Diagram of the Spin-1/2 Alternating Chain Compound F5PNN

We have measured the specific heat of the S = 1/2 alternating Heisenberg antiferromagnetic chain compound pentafluorophenyl nitronyl nitroxide in magnetic fields using a single crystal and powder. A sharp peak due to field-induced magnetic ordering (FIMO) is observed in both samples. The H-T phase boundary of the FIMO of the single crystal is symmetric with respect to the central field of the gapless field region HC1 < H < HC2, whereas it is distorted for the powder whose ordering temperatures are lower. An analysis employing calculations based on the finite temperature density matrix renormalization group indicates the possibility of novel incommensurate ordering due to frustration in the powder around the central field.

cond-mat.str-el↗