arXiv subjects

U. Welp

Publications and source records attributed to U. Welp.

At least 19 recordsLinked to original sources

arXiv2026

X-ray Fractional Orbital Angular Momentum from Coherent Magnetic Scattering

Artificial spin ice (ASI) based on a square lattice with a topological defect are known to generate orbital angular momentum (OAM) in diffracted X-ray beams. A previous investigation of ASI with even-charge topological defects showed both charge and magnetic X-ray scattering yield photon OAM, but these were confined to integer OAM values. However, the period of the square ASI's antiferromagnetic ground state is twice the period of the structural ground state, which should lead to fractional OAM from magnetic scattering when the topological defect has odd-charge. We employed photoemission electron microscopy to confirm that these ASIs order into antiferromagnetic ground states with protected superdomain walls that provide the phase discontinuity required for fractional OAM. Resonant, coherent X-ray scattering from ASIs with topological defects of charge 1 yields integer-valued X-ray OAM at structural charge peaks and fractional X-ray OAM at magnetic peaks. For thermally active ASIs, the fractional OAM beam exhibits fluctuations in the position of the phase discontinuity and thus dynamic rotation of the beam.

physics.optics↗

arXiv2026

High-resolution calorimetric sample platforms for cryogenic thermodynamic studies with multimodal synchrotron x-ray compatibility

X-ray calorimetric sample platforms combining specific heat and synchrotron x-ray measurements provide a powerful means to investigate fundamental material properties. Calorimeter cell designs featuring a compact heater and thermometer arranged in a sidecar geometry, with the sample positioned directly above the heater at the center of a silicon nitride membrane, are presented. High-yield, wafer-level batch fabrication of precision calorimetric sensor chips, beamline and laboratory cryostat plugins with sensor mounting and packaging are described. Using our calorimetric sensors, we present specific heat measurements on samples with masses ranging from 4 {\mu}g to 145 {\mu}g. The sample and reference cells are characterized with relaxation and ac steady-state measurements. The thermal response is captured using lock-in detection at carefully optimized measurement frequencies, with phase-lag correction ensuring precise extraction of heat capacity. The reference cell's background heat capacity was measured to be under 320 nJ/K at 300 K, decreasing to just 0.4 nJ/K at 0.7 K. The calorimeter performance is illustrated by studying the specific heat of small samples of superconducting Nb and a 4 {\mu}g piece of superconducting Al under different magnetic field strengths. The determination of fundamental thermodynamic quantities from low-temperature electronic and lattice specific heat measurements is discussed. These versatile, high-throughput sample platforms are engineered for small-sample calorimetry across a broad cryogenic temperature range, and they support scalable integration with a wide range of cryostats, including beamline cryostats at the Advanced Photon Source. They accommodate multimodal geometries and enable operation under ultra-high vacuum, millikelvin temperatures, magnetic fields, and x-ray illumination.

physics.ins-det↗

arXiv2024

Skyrmion Lattice Manipulation with Electric Currents and Thermal Gradients in MnSi

The skyrmion lattice (SkL) in MnSi was studied using small-angle neutron scattering and under the influence of a radial electric current in a Corbino geometry. In response to the applied current, the SkL undergoes an angular reorientation with respect to the MnSi crystal lattice. The reorientation is non-monotonic with increasing current, with the SkL rotating first in one direction and then the other. The SkL reorientation was studied at different sample locations and found to depend on the local current density as inferred from a finite element analysis. The non-monotonic response indicates the presence of two competing effects on the SkL, most likely due to the presence of both radial electric and thermal currents. Such a scenario is supported by micromagnetic simulations, which show how these effects can act constructively or destructively to drive the SkL rotation, depending on the direction of the electric current. In addition, the simulations also suggest how the direction of the skyrmion flow may affect the SkL orientation.

cond-mat.mes-hall↗

arXiv2024

Non-bulk Superconductivity in Pr$_4$Ni$_3$O$_{10}$ Single Crystals Under Pressure

Magneto-transport measurements of Pr$_4$Ni$_3$O$_{10}$ single crystals performed under externally applied pressures up to 73 GPa in diamond anvil cells with either KBr or Nujol oil as pressure media yield signatures of superconductivity with a maximum onset temperature of approximately 31 K. True zero resistance was not observed, consistent with a non-percolating superconducting volume fraction. Magnetization measurements provided corroborating evidence of superconductivity, with a pressure-dependent diamagnetic signal occurring below the onset temperature, and an estimate from the absolute value of the susceptibility suggests a superconducting volume fraction on the order of 10%. We observe sample-to-sample variations in the magnitude and pressure dependence of Tc as well as a dependence on the configuration of electrical contacts on a given sample. Possible causes of this behavior may be significant inhomogeneities in the pressure and/or damage to the samples induced by the pressure media as well as inhomogeneities in the crystals themselves. The results imply that our as-grown Pr$_4$Ni$_3$O$_{10}$ single crystals are not bulk superconductors but that there is a minority structure present within the crystals that is indeed superconducting.

cond-mat.supr-con↗

arXiv2024

Origin of anomalous magnetotransport in kagome superconductors AV$_{3}$Sb$_{5}$ (A=K,Rb,Cs)

Multiple anomalous features in electronic spectra of metals with kagome lattice structure -- van Hove singularities, Dirac points, and flat bands -- imply that materials containing this structural motif may lie at a nexus of topological and correlated electron physics. Due to the prospects of such exceptional electronic behavior, the recent discovery of superconductivity coexisting with charge-density wave (CDW) order in the layered kagome metals AV$_{3}$Sb$_{5}$ (A=K,Rb,Cs) has attracted considerable attention. Notably, these kagome metals express unconventional magnetotransport behavior, including a linear-in-H diagonal resistivity at low fields, and an even more peculiar, nonmonotonic sign-changing behavior of the Hall resistivity, which has been speculated to arise from a chiral CDW. We argue here that this unusual magnetotransport derives not from such unconventional phenomena, but rather from the unique fermiology of the AV$_{3}$Sb$_{5}$ materials. Specifically, it is caused by a large, concave hexagonal Fermi surface sheet formed in the close proximity to the van Hove singularities, which is backfolded into a small hexagonal sheet and two large triangular sheets in the CDW state. We introduce a model of the electronic structure of these Fermi surface sheets that allows for a full analytical treatment within Boltzmann kinetic theory and that enables semi-quantitative fits of our transport data. Specifically, we find that the anomalous magnetotransport behavior is caused by the confluence of strong reduction of the Fermi velocity near the van Hove singularities located near the vertices of the hexagonal sheet and sharp corners in Fermi surface generated by the CDW reconstruction.

cond-mat.supr-con↗

arXiv2022

Superconducting properties and gap structure of the topological superconductor candidate Ti_(3)Sb

We present a study of the superconducting properties of the candidate topological superconductor Ti_(3)Sb. Electrical transport measurements show zero resistance with a T_(c,onset) of ~ 5.9 K with a transition width ΔT_c~ 0.6 K. The superconducting phase boundaries as derived from magneto-transport and magnetic susceptibility measurements agree well. We estimate an upper critical field Bc2(0)~4.5 T. A Ginzburg-Landau (GL) analysis yields values of the coherence length and penetration depth of ζ = 6.2 nm and λ = 340 nm, respectively, and a GL parameter ~ 55, indicating extreme type-II behavior. Furthermore, we observed a step height in the specific heat (ΔC_e)/(γT_c )~1.61, a value larger than the Bardeen-Cooper-Schrieffer (BCS) value of 1.43, suggesting modest coupling. Measurements of the temperature dependence of the London penetration depth via the tunnel-diode oscillator (TDO) technique down to ~ 450 mK show a full superconducting gap, consistent with a conventional s-wave gap structure.

cond-mat.supr-con↗

arXiv2022

Large area photon calorimeter with Ir-Pt bilayer transition-edge sensor for the CUPID experiment

CUPID is a next-generation neutrinoless double-beta decay experiment that will require cryogenic light detectors to improve background suppression, via the simultaneous readout of heat and light channels from its scintillating crystals. In this work we showcase light detectors based on a novel Ir-Pt bilayer transition edge sensor. We have performed a systematic study to improve the thermal coupling between the photon absorber and the sensor, and thereby its responsivity. Our first devices meet CUPID's baseline noise requirement of <100~eV rms. Our detectors have risetimes of $\sim$180 $μ$s and measured timing jitter of <20 $μ$s for the expected signal-to-noise at the Q-value of the decay, which achieves the CUPID's criterion of rejecting two-neutrino double-beta decay pileup events. The current work will inform the fabrication of future devices, culminating in the final TES design and a scaleable readout scheme for CUPID.

physics.ins-det↗

arXiv2022

Key directions for research and development of superconducting radio frequency cavities

Radio frequency superconductivity is a cornerstone technology for many future HEP particle accelerators and experiments from colliders to proton drivers for neutrino facilities to searches for dark matter. While the performance of superconducting RF (SRF) cavities has improved significantly over the last decades, and the SRF technology has enabled new applications, the proposed HEP facilities and experiments pose new challenges. To address these challenges, the field continues to generate new ideas and there seems to be a vast room for improvements. In this paper we discuss the key research directions that are aligned with and address the future HEP needs.

physics.acc-ph↗

arXiv2022

Multimodal synchrotron X-ray diffraction across the superconducting transition of Sr$_{0.1}$Bi$_2$Se$_3$

In the doped topological insulator Sr$_x$Bi$_2$Se$_3$, a pronounced in-plane two-fold symmetry is observed in electronic properties below the superconducting transition temperature $T_c \sim$ 3 K, despite the three-fold symmetry of the observed $R\bar{3}m$ space group. The axis of two-fold symmetry is nominally pinned to one of three rotational equivalent directions and crystallographic strain has been proposed to be the origin of this pinning. We carried out multimodal synchrotron diffraction and resistivity measurements down to $\sim$0.68 K and in magnetic fields up to 45 kG on a single crystal of Sr$_{0.1}$Bi$_2$Se$_3$ to probe the effect of superconductivity on the crystallographic distortion. Our results indicate that there is no in-plane crystallographic distortion at the level of $1x10^{-5}$ associated with the superconducting transition. These results further support the model that the large two-fold in-plane anisotropy of superconducting properties of Sr$_x$Bi$_2$Sr$_3$ is not structural in origin but electronic, namely it is caused by a nematic superconducting order parameter of Eu symmetry.

cond-mat.supr-con↗

arXiv2022

Superconducting properties of the spin Hall candidate Ta3Sb with eightfold degeneracy

We report the synthesis and characterization of phase pure Ta3Sb, a material predicted to be topological with eightfold degenerate fermionic states [Science 353, aaf5037 (2016)] and to exhibit a large spin Hall effect [Sci. Adv. 5, eaav8575 (2019]. We observe superconductivity in Ta3Sb with Tc~ 0.67 K in both electrical resistivity \r{ho}(T) and specific heat C(T) measurements. Field dependent measurements yield the superconducting phase diagram with an upper critical field of Hc2(0) ~ 0.95 T, corresponding to a superconducting coherence length of ξ ~18.6 nm. The gap ratio deduced from specific heat anomaly, 2Δ0/kBTc is 3.46, a value close to the Bardeen-Cooper-Schrieffer (BCS) value of 3.53. From a detailed analysis of both the transport and thermodynamic data within the Ginsburg-Landau (GL) framework, a GL parameter of \k{appa} ~90 is obtained identifying Ta3Sb as an extreme type-II superconductor. The observation of superconductivity in an eightfold degenerate fermionic compound with topological surface states and predicted large spin Hall conductance positions Ta3Sb as an appealing platform to further explore exotic quantum states in multifold degenerate systems.

cond-mat.supr-con↗

arXiv2022

Full superconducting gap in the candidate topological superconductor In$_{1-x}$Pb$_x$Te for x = 0.2

High-pressure synthesis techniques have allowed for the growth of samples on the indium-rich side of (Pb,In)Te, which have increased superconducting transition temperatures compared to lead-rich compounds. In this study we present measurements of the temperature dependence of the London penetration depth $Δλ(T)$ in the compound In$_{0.8}$Pb$_{0.2}$Te, which shows a bulk $T_{c,onset}$ of $\sim4.75$ K. The results indicate fully gapped BCS-like behavior, ruling out odd-parity, topologically nontrivial $A_{2u}$ pairing; however, odd-parity $A_{1u}$ pairing is still possible. Critical field values measured below 1 K and other superconducting parameters are also presented.

cond-mat.supr-con↗

arXiv2021

Observing the suppression of superconductivity in RbEuFe$_4$As$_4$ by correlated magnetic fluctuations

In this letter, we describe quantitative magnetic imaging of superconducting vortices in RbEuFe$_4$As$_4$ in order to investigate the unique interplay between the magnetic and superconducting sublattices. Our scanning Hall microscopy data reveal a pronounced suppression of the superfluid density near the magnetic ordering temperature in good qualitative agreement with a recently-developed model describing the suppression of superconductivity by correlated magnetic fluctuations. These results indicate a pronounced exchange interaction between the superconducting and magnetic subsystems in RbEuFe\textsubscript{4}As\textsubscript{4} with important implications for future investigations of physical phenomena arising from the interplay between them.

cond-mat.supr-con↗

arXiv2020

Time-reversal invariant and fully gapped unconventional superconducting state in the bulk of the topological Nb0.25Bi2Se3

Recently, the niobium (Nb)-doped topological insulator Bi_2Se_3, in which the finite magnetic moments of the Nb atoms are intercalated in the van der Waals gap between the Bi_2Se_3 layers, has been shown to exhibit both superconductivity with T_c = 3 K and topological surface states. Here we report on muon spin rotation experiments probing the temperature-dependent of effective magnetic penetration depth Lambda_eff(T) in the layered topological superconductor candidate Nb_0.25Bi_2Se_3. The exponential temperature dependence of lambda_(eff)^(-2)(T) at low temperatures suggests a fully gapped superconducting state in the bulk with the superconducting transition temperature T_c = 2.9 K and the gap to T_c ratio 2Delta/k_BT_c = 3.95(19). We also revealed that the ratio T_c/lambda_(eff)^(-2) is comparable to those of unconventional superconductors, which hints at an unconventional pairing mechanism. Furthermore, time reversal symmetry breaking was excluded in the superconducting state with sensitive zero-field muSR experiments. We hope the present results will stimulate theoretical investigations to obtain a microscopic understanding of the relation between superconductivity and the topologically non-trivial electronic structure of Nb_0.25Bi_2Se_3.

cond-mat.supr-con↗

arXiv2020

Nodeless superconducting gap in the candidate topological superconductor Sn$_{1-x}$In$_x$Te for x = 0.7

High-pressure synthesis techniques have allowed for the growth of Sn$_{1-x}$In$_x$Te samples beyond the ambient In-saturation limit of $x$ = 0.5 (T$_c \sim$ 4.5 K). In this study, we present measurements of the temperature dependence of the London penetration depth $Δλ(T)$ in this superconducting doped topological insulator for $x$ = 0.7, where T$_{c,onset}\approx 5$ K. The results indicate fully gapped BCS-like behavior, ruling out odd-parity $A_{2u}$ pairing; however, odd-parity $A_{1u}$ pairing is still possible. Critical field values measured below 1 K and other superconducting parameters are also presented.

cond-mat.supr-con↗

arXiv2019

Melting of vortex lattice in magnetic superconductor $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$

The iron-based superconductors are characterized by strong fluctuations due to high transition temperatures and small coherence lengths. We investigate fluctuation behavior in the magnetic iron-pnictide superconductor $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$ by calorimetry and transport. We find that the broadening of the specific-heat transition in magnetic fields is very well described by the lowest-Landau-level scaling. We report calorimetric and transport observations for vortex-lattice melting, which is seen as a sharp drop of the resistivity and a step of the specific heat at the magnetic-field-dependent temperature. The melting line in the temperature/magnetic-field plane lies noticeably below the upper-critical-field line and its location is in quantitative agreement with theoretical predictions without fitting parameters. Finally, we compare the melting behavior of $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$ with other superconducting materials showing that thermal fluctuations of vortices are not as prevalent as in the high-temperature superconducting cuprates, yet they still noticeably influence the properties of the vortex matter.

cond-mat.supr-con↗

arXiv2019

Magnetic and superconducting anisotropy in Ni-doped RbEuFe$_4$As$_4$ single crystals

We investigate the effect of Ni doping on the Fe-site in single crystals of the magnetic superconductor RbEuFe$_4$As$_4$ for doping concentrations of up to 4%. A clear suppression in the superconducting transition temperature is observed in specific heat, resistivity and magnetization measurements. Upon Ni-doping, the resistivity curves shift up in a parallel fashion indicating a strong increase of the residual resistivity due to scattering by charged dopand atoms while the shape of the curve and thus the electronic structure appears largely unchanged. The observed step $ΔC/T_c$ at the superconducting transition decreases strongly for increasing Ni doping in agreement with expectations based on a model of multi-band superconductivity and strong inter-band pairing. The upper critical field slopes are reduced upon Ni doping for in- as well as out-of-plane fields leading to a small reduction in the superconducting anisotropy. The specific heat measurements of the magnetic transition reveal the same BKT behavior close to the transition temperature $T_m$ for all doping levels. The transition temperature is essentially unchanged upon doping. The in to out-of-plane anisotropy of Eu-magnetism observed at small magnetic fields is unaltered as compared to the undoped compound. All of these observations indicate a decoupling of the Eu magnetism from superconductivity and essentially no influence of Ni doping on the Eu magnetism in this compound.

cond-mat.supr-con↗

arXiv2019

Strongly fluctuating moments in the high-temperature magnetic superconductor RbEuFe$_4$As$_4$

We report detailed specific heat measurements on the recently discovered magnetic superconductor RbEuFe$_4$As$_4$. We investigated the superconducting transition at 37K and extract the phase boundary for in and out-of plane fields resulting in an anisotropy ratio of 1.8. An unusual cusp-like feature in the calorimetric data near 14.9K marks the onset of a magnetic phase. Studying the effect of small fields along the crystallographic $c$ axis, we resolve a shift in the cusp position moving to lower temperatures. For in-plane fields the cusp rapidly disappears and a broad shoulder that shifts to higher temperatures. We are able to reproduce our measured calorimetry data quantitatively by Monte-Carlo simulations of an anisotropic easy-plane 2D Heisenberg model. We can thus show that (i) the spins are preferably in plane, (ii) the cusp in specific heat is due to a Berezinskii-Kosterlitz-Thouless (BKT) transition, and (iii) the high-temperature hump in higher fields marks a crossover from a paramagnetically disordered to an ordered state. The extracted phase and crossover boundaries from experiment and simulations agree very well.

cond-mat.supr-con↗

arXiv2019

Anisotropic upper critical field of pristine and proton-irradiated single crystals of the magnetically ordered superconductor RbEuFe$_4$As$_4$

We present a study of the upper critical field, H$_{c2}$, of pristine and proton-irradiated RbEuFe$_4$As$_4$ crystals in pulsed magnetic fields of up to 65 T. The data for H$_{c2}$ reveal pronounced downwards curvature, particularly for the in-plane field orientation, and a superconducting anisotropy that decreases with decreasing temperature. These features are indicative of Pauli paramagnetic limiting. For the interpretation of these data, we use a model of a clean single-band superconductor with an open Fermi surface in the shape of a warped cylinder, which includes strong paramagnetic limiting. Fits to the data reveal that the in-plane upper critical field is Pauli paramagnetic limited, while the out-of-plane upper critical field is orbitally limited and that the orbital and paramagnetic fields have opposite anisotropies. A consequence of this particular combination is the unusual inversion of the anisotropy, $H_{c2}^{ab} < H_{c2}^c$, of the irradiated sample at temperatures below 10 K. The fits also yield an in-plane Maki parameter, $α_M^{110} \approx$ 2.6, exceeding the critical value for the formation of the Fulde-Ferrell-Larkin-Ovchinnikov state. Nevertheless, the current measurements did not reveal direct evidence for the occurrence of this state.

cond-mat.supr-con↗