arXiv subjects

U. Welp

Publications and source records attributed to U. Welp.

At least 37 records · Page 2Linked to original sources

arXiv2019

Self-induced Magnetic Flux Structure in the Magnetic Superconductor RbEuFe$_4$As$_4$

We report an unusual enhancement of the magnetic induction in single crystals of the magnetic superconductor RbEuFe$_4$As$_4$ , highlighting the interplay between superconducting and magnetic subsystems in this material. Contrary to the conventional Meissner expulsion of magnetic flux below the superconducting transition temperature, we observe a substantial boost of the magnetic flux density upon approaching the magnetic transition temperature, Tm. Direct imaging of the flux evolution with a magneto-optical technique, shows that the magnetic subsystem serves as an internal magnetic flux pump, drawing Abrikosov vortices from the surface, while the superconducting subsystem controls their conveyance into the bulk of the magnetic superconductor via a peculiar self-organized critical state.

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arXiv2018

Competition between orthorhombic and re-entrant tetragonal phases in underdoped Ba$_{1-x}$K$_x$Fe$_2$As$_2$ probed by the response to controlled disorder

Low-temperature (22~K) irradiation with 2.5~MeV electrons was used to study the competition between stripe ${\rm C_2}$ and tetragonal ${\rm C_4}$ antiferromagnetic phases which exist in a narrow doping range around $x=$0.25 in hole-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$. In nearby compositions outside of this range, at $x=$0.22 and $x=$0.19, the temperatures of both the concomitant orthorhombic/stripe antiferromagnetic transition $T_{\rm C2}$ and the superconducting transition $T_{\rm c}$ are monotonically suppressed by added disorder at similar rates of about 0.1~K/$μΩ$cm, as revealed through using resistivity variation as an intrinsic measure of scattering rate. In a stark contrast, a rapid suppression of the ${\rm C_4}$ phase at the rate of 0.24 K/$μΩ\cdot$cm is found at $x=$0.25. Moreover, this suppression of the ${\rm C_4}$ phase is accompanied by unusual disorder-induced stabilization of the ${\rm C_2}$ phase, determined by resistivity and specific heat measurements. The rate of the ${\rm C_4}$ phase suppression is notably higher than the suppression rate of the spin-vortex phase in the Ni-doped CaKFe$_4$As$_4$ (0.16 K/$μΩ$cm).

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arXiv2018

Anisotropic superconductivity and magnetism in single-crystal RbEuFe$_4$As$_4$

We investigate the anisotropic superconducting and magnetic properties of single-crystal RbEuFe$_4$As$_4$ using magnetotransport and magnetization measurements. We determine a magnetic ordering temperature of the Eu-moments of $T_m$ = 15 K and a superconducting transition temperature of $T_c$ = 36.8 K. The superconducting phase diagram is characterized by high upper critical field slopes of -70 kG/K and -42 kG/K for in-plane and out-of-plane fields, respectively, and a surprisingly low superconducting anisotropy of $Γ$ = 1.7. Ginzburg-Landau parameters of $κ_c \sim 67$ and $κ_{ab} \sim 108$ indicate extreme type-II behavior. These superconducting properties are in line with those commonly seen in optimally doped Fe-based superconductors. In contrast, Eu-magnetism is quasi-two dimensional as evidenced by highly anisotropic in-plane and out-of-plane exchange constants of 0.6 K and $<$ 0.04 K. A consequence of the quasi-2D nature of the Eu-magnetism are strong magnetic fluctuation effects, a large suppression of the magnetic ordering temperature as compared to the Curie-Weiss temperature, and a cusp-like anomaly in the specific heat devoid of any singularity. Magnetization curves reveal a clear magnetic easy-plane anisotropy with in-plane and out-of-plane saturation fields of 2 kG and 4 kG.

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arXiv2017

Superconducting and normal-state anisotropy of the doped topological insulator Sr$_{0.1}$Bi$_2$Se$_3$

Sr$_x$Bi$_2$Se$_3$ and the related compounds Cu$_x$Bi$_2$Se$_3$ and Nb$_x$Bi$_2$Se$_3$ have attracted considerable interest, as these materials may be realizations of unconventional topological superconductors. Superconductivity with T$_c$ ~ 3 K in Sr$_x$Bi$_2$Se$_3$ arises upon intercalation of Sr into the layered topological insulator Bi$_2$Se$_3$. Here we elucidate the anisotropy of the normal and superconducting state of Sr$_{0.1}$Bi$_2$Se$_3$ with angular dependent magnetotransport and thermodynamic measurements. High resolution x-ray diffraction studies underline the high crystalline quality of the samples. We demonstrate that the normal state electronic and magnetic properties of Sr$_{0.1}$Bi$_2$Se$_3$ are isotropic in the basal plane while we observe a large two-fold in-plane anisotropy of the upper critical field in the superconducting state. Our results support the recently proposed odd-parity nematic state characterized by a nodal gap of $E_u$ symmetry in Sr$_x$Bi$_2$Se$_3$.

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arXiv2017

Superconductivity, pairing symmetry, and disorder in the doped topological insulator Sn$_{1-x}$In$_x$Te for x $\geq$ 0.10

The temperature dependence of the London penetration depth $Δλ(T)$ in the superconducting doped topological crystalline insulator Sn$_{1-x}$In$_x$Te was measured down to 450 mK for two different doping levels, x $\approx$ 0.45 (optimally doped) and x $\approx$ 0.10 (underdoped), bookending the range of cubic phase in the compound. The results indicate no deviation from fully gapped BCS-like behavior, eliminating several candidate unconventional gap structures. Critical field values below 1 K and other superconducting parameters are also presented. The introduction of disorder by repeated particle irradiation with 5 MeV protons does not enhance $T_c$, indicating that ferroelectric interactions do not compete with superconductivity.

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arXiv2017

An increase in $T_c$ under hydrostatic pressure in the superconducting doped topological insulator Nb$_{0.25}$Bi$_2$Se$_3$

We report an unexpected positive hydrostatic pressure derivative of the superconducting transition temperature in the doped topological insulator \NBS via $dc$ SQUID magnetometry in pressures up to 0.6 GPa. This result is contrary to reports on the homologues \CBS and \SBS where smooth suppression of $T_c$ is observed. Our results are consistent with recent Ginzburg-Landau theory predictions of a pressure-induced enhancement of $T_c$ in the nematic multicomponent $E_u$ state proposed to explain observations of rotational symmetry breaking in doped Bi$_2$Se$_3$ superconductors.

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arXiv2017

Robust odd-parity superconductivity in the doped topological insulator Nb$_x$Bi$_2$Se$_3$

We present resistivity and magnetization measurements on proton-irradiated crystals demonstrating that the superconducting state in the doped topological superconductor Nb$_x$Bi$_2$Se$_3$ (x = 0.25) is surprisingly robust against disorder-induced electron scattering. The superconducting transition temperature $T_c$ decreases without indication of saturation with increasing defect concentration, and the corresponding scattering rates far surpass expectations based on conventional theory. The low-temperature variation of the London penetration depth $Δλ(T)$ follows a power law ($Δλ(T)\sim T^2$) indicating the presence of symmetry-protected point nodes. Our results are consistent with the proposed robust nematic $E_u$ pairing state in this material.

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arXiv2016

Evidence of nodes in the order parameter of the superconducting doped topological insulator Nb$_x$Bi$_2$Se$_3$ via penetration depth measurements

The low-temperature variation of the London penetration depth $λ(T)$ in the candidate topological superconductor Nb$_x$Bi$_2$Se$_3$ (x = 0.25) is reported for several crystals. The measurements were carried out by means of a tunnel-diode oscillator (TDO) technique in both field orientations ($H_{rf} \parallel$ $c$ and $H_{rf} \parallel$ $ab$ planes). All samples exhibited power law behavior at low temperatures ($Δλ\sim T^2$) clearly indicating the presence of point nodes in the superconducting order parameter. The results presented here are consistent with a nematic odd-parity spin-triplet $E_u$ pairing state in Nb$_x$Bi$_2$Se$_3$.

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arXiv2016

Decoupling and tuning competing effects of different types of defects on flux creep in irradiated YBa$_{2}$Cu$_{3}$O$_{7-δ}$ coated conductors

YBa$_{2}$Cu$_{3}$O$_{7-δ}$ coated conductors (CCs) have achieved high critical current densities ($\textit{J}_{c}$) that can be further increased through the introduction of additional defects using particle irradiation. However, these gains are accompanied by increases in the flux creep rate, a manifestation of competition between the different types of defects. Here, we study this competition to better understand how to design pinning landscapes that simultaneously increase $\textit{J}_{c}$ and reduce creep. CCs grown by metal organic deposition show non-monotonic changes in the temperature-dependent creep rate, $\textit{S}(\textit{T})$. Notably, in low fields, there is a conspicuous dip to low $\textit{S}$ as temperature ($\textit{T}$) increases from ~20 K to ~65 K. Oxygen-, proton-, and Au-irradiation substantially increase $\textit{S}$ in this temperature range. Focusing on an oxygen-irradiated CC, we investigate the contribution of different types of irradiation-induced defects to the flux creep rate. Specifically, we study $\textit{S}(\textit{T})$ as we tune the relative density of point defects to larger defects by annealing both an as-grown and an irradiated CC in O$_{2}$ at temperatures $\textit{T}_{A}$ = 250$°$C to 600$°$C. We observe a steady decrease in $\textit{S}$($\textit{T}$ > 20 K) with increasing $\textit{T}_{A}$, unveiling the role of pre-existing nanoparticle precipitates in creating the dip in $\textit{S}(\textit{T})$ and point defects and clusters in increasing $\textit{S}$ at intermediate temperatures.

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arXiv2016

Toward superconducting critical current by design

We present the new paradigm of critical current by design. Analogous to materials by design, it aims at predicting the optimal defect landscape in a superconductor for targeted applications by elucidating the vortex dynamics responsible for the bulk critical current. To highlight this approach, we demonstrate the synergistic combination of critical current measurements on commercial high-temperature superconductors containing self-assembled and irradiation tailored correlated defects by using large-scale time-dependent Ginzburg-Landau simulations for vortex dynamics.

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arXiv2015

Superconducting gap evolution in overdoped BaFe$_{2}$(As$_{1-x}$P$_x$)$_2$ single crystals through nanocalorimetry

We report on specific heat measurements on clean overdoped $\mathrm{BaFe_{2}(As_{1-x}P_x)_2}$ single crystals performed with a high resolution membrane-based nanocalorimeter. A nonzero residual electronic specific heat coefficient at zero temperature $γ_\mathrm{r}={C/T}|_{T \to 0}$ is seen for all doping compositions, indicating a considerable fraction of the Fermi surface ungapped or having very deep minima. The remaining superconducting electronic specific heat is analyzed through a two-band s-wave $α$ model in order to investigate the gap structure. Close to optimal doping we detect a single zero-temperature gap of $Δ_0 \sim 5.3\,\mathrm{meV}$, corresponding to $Δ_0 / k_\mathrm{B} T_\mathrm{c} \sim 2.2$. Increasing the phosphorus concentration $x$, the main gap reduces till a value of $Δ_0 \sim 1.9\,\mathrm{meV}$ for $x = 0.55$ and a second weaker gap becomes evident. From the magnetic field effect on $γ_\mathrm{r}$, all samples however show similar behavior [$γ_\mathrm{r}(H) - γ_\mathrm{r}(H=0) \propto H^n$, with $n$ between 0.6 and 0.7]. This indicates that, despite a considerable redistribution of the gap weights, the total degree of gap anisotropy does not change drastically with doping.

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arXiv2015

Microscopic Parameters from High-Resolution Specific Heat Measurements on Overdoped BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ Single Crystals

We investigate the electronic specific heat of overdoped BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals in the superconducting state using high-resolution nanocalorimetry. From the measurements, we extract the doping dependence of the condensation energy, superconducting gap $Δ$, and related microscopic parameters. We find that the anomalous scaling of the specific heat jump $ΔC \propto T_{\mathrm{c}}^3$, found in many iron-based superconductors, in this system originates from a $T_\mathrm{c}$-dependent ratio $Δ/k_\mathrm{B}T_\mathrm{c}$ in combination with a doping-dependent density of states $N(\varepsilon_\mathrm{F})$. A clear enhancement is seen in the effective mass $m^{*}$ as the composition approaches the value that has been associated with a quantum critical point at optimum doping. However, a simultaneous increase in the superconducting carrier concentration $n_\mathrm{s}$ maintains the superfluid density, yielding an apparent penetration depth $λ$ that decreases with increasing $T_\mathrm{c}$ without sharp divergence at the quantum critical point. Uemura scaling indicates that $T_\mathrm{c}$ is governed by the Fermi temperature $T_\mathrm{F}$ for this multi-band system.

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arXiv2014

Stripe Domains and First Order Phase Transition in the Vortex Matter of Anisotropic High-temperature Superconductors

We report the direct imaging of a novel modulated flux striped domain phase in a nearly twin-free YBCO crystal. These domains arise from instabilities in the vortex structure within a narrow region of tilted magnetic fields at small angles from the in-plane direction. By comparing the experimental and theoretically derived vortex phase diagrams we infer that the stripe domains emerge from a first order phase transition of the vortex structure. The size of domains containing vortices of certain orientations is controlled by the balance between the vortex stray field energy and the positive energy of the domain boundaries. Our results confirm the existence of the kinked vortex chain phase in an anisotropic high temperature superconductor and reveal a sharp transition in the state of this phase resulting in regular vortex domains.

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arXiv2013

Dirac Fermions and Superconductivity in Homologous Structures (AgxPb1-xSe)5(Bi2Se3)3m,m = 1,2

A newly discovered topological insulator (AgxPb1-xSe)5(Bi2Se3)3m, m=2, has a band gap of 0.5 eV, the largest value ever reported in topological insulators (TIs). We present a magnetoconductivity study of the Dirac electrons of this compound in the quantum diffusion regime. Two dimensional weak antilocalization was observed and identified as destructive interference caused by the Berry phase of this topological state. We find that the phase coherence length of the Dirac electrons is independent of doping and disorder levels. This provides proof for the absence of backscattering arising from the protection of time reversal invariance in TI (AgxPb1-xSe)5(Bi2Se3)3m, m=2. We further report that the homologous compound (AgxPb1-xSe)5(Bi2Se3)3m, m=1 is a superconductor with a transition temperature Tc = 1.7 K. The related structures of these two phases allow lateral intergrowth of crystals to occur naturally, offering an opportunity to observe the Majorana Fermion state at the boundary of two intergrown crystals.

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arXiv2013

Effect of heavy-ion irradiation on London penetration depth in over-doped Ba(Fe,Co)2As2

Irradiation with 1.4 GeV $^{208}$Pb ions was used to induce artificial disorder in single crystals of iron-arsenide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ and to study its effect on the temperature-dependent London penetration depth and transport properties. Study was undertaken on overdoped single crystals with $x$=0.108 and $x$=0.127 characterized by notable modulation of the superconducting gap. Irradiation with doses 2.22$\times10^{11}$$\textit{d}$/cm$^2$ and 2.4$\times10^{11}$$\textit{d}$/cm$^2$, corresponding to the matching fields of $B_ϕ = $6 T and 6.5 T, respectively, suppresses the superconducting $T_c$ by approximately 0.3 to 1 K. The variation of the low-temperature penetration depth in both pristine and irradiated samples is well described by the power-law, $Δλ(T)=AT^n$. Irradiation increases the magnitude of the pre-factor $A$ and decreases the exponent $n$, similar to the effect of irradiation in optimally doped samples. This finding supports universal $s_{\pm}$ pairing in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ compounds for the whole Co doping range.

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arXiv2013

Doubling the Critical Current Density of High Temperature Superconducting Coated Conductors through Proton Irradiation

The in-field critical current of commercial YBa2Cu3O7 coated conductors can be substantially enhanced by post-fabrication irradiation with 4 MeV protons. Irradiation to a fluence of 8x10^16 p/cm^2 induces a near doubling of the critical current in fields of 6 T || c at a temperature of 27 K, a field and temperature range of interest for applications such as rotating machinery. A mixed pinning landscape of preexisting precipitates and twin boundaries and small, finely dispersed irradiation induced defects may account for the improved vortex pinning in high magnetic fields. Our data indicate that there is significant head-room for further enhancements.

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arXiv2013

Powerful terahertz emission from Bi2Sr2CaCu2O8+delta mesa arrays

Stacks of intrinsic Josephson junctions (IJJs) in high-temperature superconductors enable the fabrication of compact sources of coherent terahertz radiation. Here we demonstrate that multiple stacks patterned on the same Bi2Sr2CaCu2O8+delta crystal can - under optimized conditions - be synchronized to emit high-power THz-radiation. For three synchronized stacks we achieved 610 microwatts of continuous-wave coherent radiation power at 0.51 THz. We suggest that synchronization is promoted by THz-waves in the base crystal. We note though that synchronization cannot be achieved in all samples. However, even in these cases powers on the 100-microwatt scale can be generated.

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arXiv2013

The chiral phase transition in charge ordered 1T-TiSe2

It was recently discovered that the low temperature, charge ordered phase of 1T-TiSe2 has a chiral character. This unexpected chirality in a system described by a scalar order parameter could be explained in a model where the emergence of relative phase shifts between three charge density wave components breaks the inversion symmetry of the lattice. Here, we present experimental evidence for the sequence of phase transitions predicted by that theory, going from disorder to non-chiral and finally to chiral charge order. Employing X-ray diffraction, specific heat, and electrical transport measurements, we find that a novel phase transition occurs ~7 K below the main charge ordering transition in TiSe2, in agreement with the predicted hierarchy of charge ordered phases.

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