arXiv subjects

Umberto Marini Bettolo Marconi

Publications and source records attributed to Umberto Marini Bettolo Marconi.

At least 19 recordsLinked to original sources

arXiv2026

Metastability and nucleation of bubbles in active chiral systems

Bubbles frequently emerge in dense chiral active fluids, yet it remains unclear whether they result from an instability of the homogeneous state or from rare nucleation events within a metastable phase. Here we develop a nucleation theory for chiral bubble formation by reducing the hydrodynamic equations to a single collective coordinate, the bubble radius. This reduction yields an effective nonlinear potential that captures the radial dynamics and predicts distinct stable, metastable, and unstable regimes of the homogeneous state. In the metastable regime, the theory identifies a critical bubble radius and an associated effective mechanical-work barrier, while its large-radius behavior determines whether bubble growth saturates at a finite size or becomes unbounded. We further analyze the stability of circular bubbles against noncircular perturbations, finding growing modes that can lead to elongation and breakup. The theoretical predictions are tested against event-driven molecular-dynamics simulations of chiral hard disks, which reproduce the predicted trends in the critical radius, nucleation barrier, and selected bubble size. Our results establish a unified framework for stability and nucleation in chiral active fluids and suggest routes to control bubble formation in experiments with spinning colloids and chiral spinners.

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arXiv2026

Kinetic Theory of Chiral Active Disks: Odd Transport and Torque Density

Parity-odd transport is a central signature of chiral fluids, yet analytical predictions are sparse. Here, we introduce a minimal two-dimensional hard-disk gas in which chirality arises solely from a collision-induced transverse impulse. Motivated by granular spinners, collisions are dissipative and inject orbital angular momentum through a fixed tangential ``kick'' at contact. Starting from a Boltzmann-Enskog description, we derive nonlinear hydrodynamic equations for density, momentum, and temperature, and show that chirality generates an antisymmetric homogeneous stress corresponding to a nonzero torque density. In the dilute limit, a Chapman-Enskog expansion yields analytical predictions for transport coefficients, including odd viscosity, odd thermal conductivity, and odd self-diffusivity, in good agreement with numerical simulations. This minimal kinetic model can serve as a foundation for systematic coarse-graining of chiral fluids and as a tractable benchmark for gaining insight into odd transport across a broader class of chiral systems.

cond-mat.stat-mech↗

arXiv2026

Curvature-driven wall accumulation in chiral active particles

We study a dilute system of non-motile chiral active particles confined in geometries ranging from straight channels to circular enclosures. Activity is introduced through chiral particle-wall interactions, modeled as tangential wall forces that generate the edge currents characteristic of chiral active matter. Remarkably, although the particles lack self-propulsion, these boundary currents induce density inhomogeneities. We show that boundary curvature drives a wall accumulation phenomenon: particles remain uniformly distributed in straight channels but accumulate near the boundaries of circular confinements. Numerical simulations and a hydrodynamic theory for the density and momentum fields consistently capture this curvature-induced wall-accumulation. These results identify boundary curvature as a fundamental control parameter for chiral edge transport and confinement-induced organization, with potential experimental relevance to spinning colloids and granular spinners.

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arXiv2026

Sparkling bubbles in chiral active fluids

We study an inertial chiral active fluid, formed by repulsive particles that transfer angular momentum through odd interactions, i.e. transverse forces. Chirality induces an inhomogeneous phase, consisting of rotating bubbles, whose formation is favored at an optimal packing fraction. In this regime, we discover that bubbles may be dynamically unstable, breaking up and reforming in the steady state, thereby showing a spontaneous sparkling-like behavior reminiscent of supersaturated liquids. Bubbles and sparkling bubbles are predicted by a coarse-grained hydrodynamic theory, revealing the intrinsic non-linearity of these collective phenomena, and call for experimental verifications in granular spinners or spinning colloids.

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arXiv2026

Emergent hydrodynamics of chiral active fluids: vortices, bubbles and odd diffusion

Starting from a microscopic multiparticle Langevin equation, we systematically derive a hydrodynamic description in terms of density and momentum fields for chiral active particles interacting via standard repulsive and nonlocal odd forces. These odd interactions are reciprocal but non-conservative: they are non-potential forces, as they act perpendicular to the vector joining any pair of particles. As a result, the torques that two particles exert on one another are non-reciprocal. The ensuing macroscopic continuum description consists of a continuity equation for the density and a generalized compressible Navier-Stokes equation for the fluid velocity. The latter includes a chirality-induced torque density term and an odd viscosity contribution. Our theory predicts the emergence of odd diffusivity, edge currents, and an inhomogeneous phase - characterized by bubble-like structures - recently observed in simulations. Specifically, the theory exhibits a linear instability arising from the interplay between odd viscosity and torque density, and admits steady-state inhomogeneous solutions featuring bubbles and vortices, in agreement with numerical simulations. Our findings can be tested experimentally in systems of granular spinners or rotating microorganisms suspended in a fluid.

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arXiv2025

Cooling mechanism controls motility-induced phase separation in inertial active liquids

Motility-induced phase separation (MIPS) is a central collective phenomenon in active matter, theoretically established in the overdamped regime. We discover that the dynamical origin of MIPS is fundamentally altered by inertia, which induces a cooling mechanism absent in overdamped active matter. This conclusion is supported by an active variant of the direct simulation Monte Carlo method and by a kinetic theory for inertial self-propelled hard spheres derived from the microscopic dynamics. In contrast to the overdamped case, both analyses demonstrate that inertial MIPS does not rely on volume exclusion but on a cooling mechanism involving density, polarization, and temperature fields. This mechanism emerges from the competition between activity and a density dependent collision rate, arising from spatial correlations between colliding particles. These findings open a pathway to fundamentally connect inertial active matter with granular physics.

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arXiv2025

Modeling chiral active particles: from circular motion to odd interactions

In this paper, we discuss microscopic models for chiral active particles, i.e., rotating active units that exhibit circular or spinning motion. While non-chiral active particles are typically governed by self-propulsion and conservative interactions, the rotating motion of chiral particles generates additional non-conservative forces that cannot be derived from a potential. These manifest as effective transverse forces, acting perpendicular to the line connecting the centres of two interacting particles, and are referred to as odd interactions, because they break the mirror symmetry of the system. Here, we demonstrate that odd interactions arise from a limiting case of a well-established model describing spinning granular objects. In addition, we show that these models for chiral active objects give rise to a novel collective phenomenon that emerges uniquely from transverse forces and, hence, chirality. Specifically, the system undergoes a transition from a homogeneous phase to an inhomogeneous one characterised by regions depleted of particles, referred to as bubbles. This collective behaviour, termed BIO (bubbles induced by odd interactions), is a general emergent phenomenon arising from chirality and odd interactions. In this work, we review theoretical approaches to this problem, including a scaling argument and predictions for spatial velocity correlations that account for the BIO phase. Finally, we outline perspectives and open challenges concerning this collective phenomenon.

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arXiv2025

Active thermodynamics of inertial chiral active gases: equation of state and edge currents

One of the most fundamental quests in the physics of active matter concerns the existence of a comprehensive theory for its macroscopic properties, i.e. an ``active thermodynamics''. Here, we derive and experimentally verify key elements of the active thermodynamics of ideal chiral active gases, unveiling edge currents and odd diffusivity as their peculiar features. Our main results are the derivation of an equation of state relating density and pressure via a chirality-dependent effective temperature, the derivation of Fick's law including the full diffusion matrix predicting odd diffusion, and the exact prediction of edge currents at container walls that nonmonotonically depend on chirality.

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arXiv2025

Active Gaussian Network Model: a non-equilibrium description of protein fluctuations and allosteric behavior

Understanding the link between structure and function in proteins is fundamental in molecular biology and proteomics. A central question in this context is whether allostery - where the binding of a molecule at one site affects the activity of a distant site - emerges as a further manifestation of the intricate interplay between structure, function, and intrinsic dynamics. This study explores how allosteric regulation is modified when intrinsic protein dynamics operate under out-of-equilibrium conditions. To this purpose, we introduce a simple nonequilibrium model of protein dynamics, inspired by active matter systems, by generalizing the widely employed Gaussian Network Model (GNM) to incorporate non-thermal effects. Our approach underscores the advantage of framing allostery as a causal process by using, as a benchmark system, the second PDZ domain of the human phosphatase hPT1E that mediates protein-protein interactions. We employ causal indicators, such as response functions and transfer entropy, to identify the network of PDZ2 residues through which the allosteric signal propagates across the protein structure. These indicators reveal specific regions that align well with experimental observations. Furthermore, our results suggest that deviations from purely thermal fluctuations can significantly influence allosteric communication by introducing distinct timescales and memory effects. This influence is particularly relevant when the allosteric response unfolds on timescales incompatible with relaxation to equilibrium. Accordingly, non-thermal fluctuations may become essential for accurately describing protein responses to ligand binding and developing a comprehensive understanding of allosteric regulation.

cond-mat.stat-mech↗

arXiv2025

Odd Active Solids: Vortices, Velocity Oscillations and Dissipation-Free Modes

A wide range of physical and biological systems, including colloidal magnets, granular spinners, and starfish embryos, are characterized by strongly rotating units that give rise to odd viscosity and odd elasticity. These active systems can be described using a coarse-grained model in which the pairwise forces between particles include a transverse component compared to standard interactions due to a central potential. These non-potential, additional forces, referred to as odd interactions, do not conserve energy or angular momentum and induce rotational motion. Here, we study a two-dimensional crystal composed of inertial Brownian particles that interact via odd forces and are in thermal contact with their environment. In the underdamped regime, the energy injected by odd forces can counteract dissipation due to friction, leading to quasi-dissipation-free excitations with finite frequency and wavelength. In the resulting non-equilibrium steady state, the system exhibits angular momentum and velocity correlations. When the strength of the odd forces exceeds a certain threshold or friction is too low, a crystal with only harmonic springs becomes linearly unstable due to transverse fluctuations. This instability can be mitigated by introducing nonlinear central interactions, which suppress the divergence of short-wavelength velocity fluctuations and allows us to numerically explore the linearly unstable regime. This is characterized by pronounced temporal oscillations in the velocity featuring the existence of vortex structures and kinetic temperature values larger than the thermal temperature.

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arXiv2024

Spontaneous generation of angular momentum in chiral active crystals

We study a two-dimensional chiral active crystal composed of underdamped chiral active particles. These particles, characterized by intrinsic handedness and persistence, interact via linear forces derived from harmonic potentials. Chirality plays a pivotal role in shaping the system's behavior: it reduces displacement and velocity fluctuations while inducing cross-spatial correlations among different Cartesian components of velocity. These features distinguish chiral crystals from their non-chiral counterparts, leading to the emergence of net angular momentum, as predicted analytically. This angular momentum, driven by the torque generated by the chiral active force, exhibits a non-monotonic dependence on the degree of chirality. Additionally, it contributes to the entropy production rate, as revealed through a path-integral analysis. We investigate the dynamic properties of the crystal in both Fourier and real space. Chirality induces a non-dispersive peak in the displacement spectrum, which underlies the generation of angular momentum and oscillations in time-dependent autocorrelation functions or mean-square displacement, all of which are analytically predicted.

cond-mat.soft↗

arXiv2024

Spontaneous self-wrapping in chiral active polymers

Biological organisms often have elongated, flexible structures with some degree of chirality in their bodies or movements. In nature, these organisms frequently take advantage of self-encapsulation mechanisms that create folded configurations, changing their functionality, such as for defensive purposes. Here, we explore the role of chirality in polymeric structures composed of chiral active monomers exhibiting circular motion. Through a combination of experiments and numerical simulations, we demonstrate a spontaneous unfolding-folding transition uniquely induced by chirality, a phenomenon not observed in passive polymers. This transition is driven by a self-wrapping mechanism, resulting in dynamic polymer collapse even without attractive interactions. Our findings, based on chiral polymers made from chiral active granular particles, present new opportunities in robotic applications taking advantage of the interplay between chirality and deformability.

cond-mat.soft↗

arXiv2024

Bubble phase induced by odd interactions

We study a repulsive thermal system governed by odd interactions. The interplay between oddness and inertia induces a non-equilibrium phase transition from a homogeneous to a non-homogeneous phase, characterized by bubbles induced by odd interactions. This phenomenon occurs in the absence of attractions and is generated by the competition between the standard pressure contribution due to particle repulsion and an effective surface tension generated by odd-induced centrifugal forces. As a signature of the phase transition, the system exhibits vortex structures and oscillating spatial velocity correlations, which emerge close to the analytically predicted transition point. Our findings can be verified in granular experiments governed by odd interactions, such as spinners and colloidal magnets, and could be key to characterizing the emerging properties of metamaterials.

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arXiv2024

Active fluctuations in the harmonic chain: phonons, entropons and velocity correlations

Non-equilibrium random fluctuations of non-thermal nature are a salient feature of active matter. In this work, we consider the collective excitations of active systems at high density, focusing on a one-dimensional chain of elastically coupled inertial particles, whose activity is modeled with an Ornstein-Uhlenbeck process. Their excitation spectrum shows the presence of two kinds of fluctuations: the first ones are thermally excited phonons analogous to those of a passive crystal while the second ones have been termed entropons because associated with the entropy production due to the active forces. These two types of fluctuations show different properties: in fact, only entropons generate spatial velocity correlations and fail to satisfy a standard fluctuation-response relation. We derive the exact expression for the equal-time velocity and displacement correlations as well as for the structure factor and in each case identify the phonon and entropon contributions. Finally, we investigate the dynamical properties of the excitations in terms of steady-state two-time correlations, such as the intermediate scattering function and the mean-square displacement, and show that both phonon and entropon fluctuations are characterized by a long wavelength overdamped regime and a short wavelength underdamped regime. In the large persistence case, entropons decay slower than phonons, and in general, activity tends to suppress the oscillations typical of the underdamped regime.

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arXiv2023

Entropy production and collective excitations of crystals out of equilibrium: the concept of entropons

We study the collective vibrational excitations of crystals under out-of-equilibrium steady conditions that give rise to entropy production. Their excitation spectrum comprises equilibrium-like phonons of thermal origin and additional collective excitations called entropons because each of them represents a mode of spectral entropy production. Entropons coexist with phonons and dominate over them when the system is far from equilibrium while they are negligible in near-equilibrium regimes. The concept of entropons has been recently introduced and verified in a special case of crystals formed by self-propelled particles. Here, we show that entropons exist in a broader class of active cyrstals that are intrinsically out of equilibrium and characterized by the lack of detailed balance. After a general derivation, several explicit examples are discussed, including crystals consisting of particles with alignment interactions and frictional contact forces.

cond-mat.stat-mech↗

arXiv2023

Chiral active matter in external potentials

We investigate the interplay between chirality and confinement induced by the presence of an external potential. For potentials having radial symmetry, the circular character of the trajectories induced by the chiral motion reduces the spatial fluctuations of the particle, thus providing an extra effective confining mechanism, that can be interpreted as a lowering of the effective temperature. In the case of non-radial potentials, for instance, with an elliptic shape, chirality displays a richer scenario. Indeed, the chirality can break the parity symmetry of the potential that is always fullfilled in the non-chiral system. The probability distribution displays a strong non-Maxwell-Boltzmann shape that emerges in cross-correlations between the two Cartesian components of the position, that vanishes in the absence of chirality or when radial symmetry of the potential is restored. These results are obtained by considering two popular models in active matter, i.e. chiral Active Brownian particles and chiral active Ornstein-Uhlenbeck particles.

cond-mat.soft↗

arXiv2023

Inhomogeneous entropy production in active crystals with point imperfections

The presence of defects in solids formed by active particles breaks their discrete translational symmetry. As a consequence, many of their properties become space-dependent and different from those characterizing perfectly ordered structures. Motivated by recent numerical investigations concerning the nonuniform distribution of entropy production and its relation to the configurational properties of active systems, we study theoretically and numerically the spatial profile of the entropy production rate when an active solid contains an isotopic mass defect. The theoretical study of such an imperfect active crystal is conducted by employing a perturbative analysis that considers the perfectly ordered harmonic solid as a reference system. The perturbation theory predicts a nonuniform profile of the entropy production extending over large distances from the position of the impurity. The entropy production rate decays exponentially to its bulk value with a typical healing length that coincides with the correlation length of the spatial velocity correlations characterizing the perfect active solids in the absence of impurities. The theory is validated against numerical simulations of an active Brownian particle crystal in two dimensions with Weeks-Chandler-Andersen repulsive interparticle potential.

cond-mat.stat-mech↗

arXiv2022

Entropons as collective excitations in active solids

The vibrational dynamics of solids is described by phonons constituting basic collective excitations in equilibrium crystals. Here we consider an active crystal composed of self-propelled particles which bring the system into a non-equilibrium steady-state governed by entropy production. Calculating the entropy production spectrum, we put forward the picture of "entropons", which are vibrational collective excitations responsible for entropy production. Entropons are purely generated by activity and coexist with phonons but dominate over them for large self-propulsion strength. The existence of entropons can be verified in experiments on dense self-propelled colloidal Janus-particles and granular active matter, as well as in living systems such as dense cell monolayers.

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