arXiv subjects

Umberto Marini Bettolo Marconi

Publications and source records attributed to Umberto Marini Bettolo Marconi.

At least 37 records · Page 2Linked to original sources

arXiv2022

Active particles driven by competing spatially dependent self-propulsion and external force

We investigate how the competing presence of a nonuniform motility landscape and an external confining field affects the properties of active particles. We employ the active Ornstein-Uhlenbeck particle (AOUP) model with a periodic swim velocity profile to derive analytical approximations for the steady-state probability distribution of position and velocity, encompassing both the Unified Colored Noise Approximation and the theory of potential-free active particles with spatially dependent swim velocity recently developed. We test the theory by confining an active particle in a harmonic trap, which gives rise to interesting properties, such as a transition from a unimodal to a bimodal (and, eventually multimodal) spatial density, induced by decreasing the spatial period of the self propulsion. Correspondingly, the velocity distribution shows pronounced deviations from the Gaussian shape, even displaying a bimodal profile in the high-motility regions. Our results can be confirmed by real-space experiments on active colloidal Janus particles in external fields.

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arXiv2021

Dynamics of active particles with space-dependent swim velocity

We study the dynamical properties of an active particle subject to a swimming speed explicitly depending on the particle position. The oscillating spatial profile of the swim velocity considered in this paper takes inspiration from experimental studies based on Janus particles whose speed can be modulated by an external source of light. We suggest and apply an appropriate model of an active Ornstein Uhlenbeck particle to the present case. This allows us to predict the stationary properties, by finding the exact solution of the steady-state probability distribution of particle position and velocity. From this, we obtain the spatial density profile and show that its form is consistent with the one found in the framework of other popular models. The reduced velocity distribution highlights the emergence of non-Gaussianity in our generalized AOUP model which becomes more evident as the spatial dependence of the velocity profile becomes more pronounced. Then, we focus on the time-dependent properties of the system. Velocity autocorrelation functions are studied in the steady-state combining numerical and analytical methods derived under suitable approximations. We observe a non-monotonic decay in the temporal shape of the velocity autocorrelation function which depends on the ratio between the persistence length and the spatial period of the swim velocity. Finally, we numerically and analytically study the mean square displacement and the long-time diffusion coefficient. The ballistic regime, observed in the small-time region, is deeply affected by the properties of the swim velocity landscape which induces also a crossover to a sub-ballistic but superdiffusive regime for intermediate times. Finally, the long-time diffusion coefficient decreases as the amplitude of the swim velocity oscillations increases because the diffusion is determined by those regions where the particles are slow.

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arXiv2021

Correlated escape of active particles across a potential barrier

We study the dynamics of one-dimensional active particles confined in a double-well potential, focusing on the escape properties of the system, such as the mean escape time from a well. We first consider a single-particle both in near and far-from-equilibrium regimes by varying the persistence time of the active force and the swim velocity. A non-monotonic behavior of the mean escape time is observed with the persistence time of the activity, revealing the existence of an optimal choice of the parameters favoring the escape process. For small persistence times, a Kramers-like formula with an effective potential obtained within the Unified Colored Noise Approximation is shown to hold. Instead, for large persistence times, we developed a simple theoretical argument based on the first passage theory which explains the linear dependence on the escape time with the persistence of the active force. In the second part of the work, we consider the escape of two active particles mutually repelling. Interestingly, the subtle interplay of active and repulsive forces may lead to a correlation between particles favoring the simultaneous jump across the barrier. This mechanism cannot be observed in the escape process of two passive particles. Finally, we find that, in the small-persistence regime, the repulsion favors the escape, like in passive systems, in agreement with our theoretical predictions, while for large persistence times, the repulsive and active forces produce an effective attraction which hinders the barrier crossing.

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arXiv2021

Hydrodynamics of simple active liquids: the emergence of velocity correlations

We derive the Hydrodynamics for a system of N active, spherical, underdamped particles, interacting through conservative forces. At the microscopic level, we represent the evolution of the particles in terms of the Kramers equation for the probability density distribution of their positions, velocities, and orientations, while at a mesoscopic level we switch to a coarse-grained description introducing an appropriate set of hydrodynamic fields given by the lower-order moments of the distribution. In addition to the usual density and polarization fields, the Hydrodynamics developed in this paper takes into account the velocity and kinetic temperature fields, which are crucial to understanding new aspects of the behavior of active liquids. By imposing a suitable closure of the hydrodynamic moment equations and truncation of the Born-Bogolubov-Green-Kirkwood-Yvon hierarchy, we obtain a closed set of mesoscopic balance equations. At this stage, we focus our interest on the small deviations of the hydrodynamic fields from their averages and apply the methods of the theory of linear hydrodynamic fluctuations. Our treatment sheds light on the peculiar properties of isotropic active liquids and their emergent dynamical collective phenomena, such as the spontaneous alignment of the particle velocities. We predict the existence within the liquid phase of spatial equal-time Ornstein-Zernike-like velocity correlations both for the longitudinal and the transverse modes. At variance with active solids, in active liquids, the correlation length of the transverse velocity fluctuations is sensibly shorter than the length of the longitudinal fluctuations. In particular, the latter depends on the sound speed and increases with the persistence time, while the former displays a weaker dependence on these parameters. Finally, within the same framework, we derive the dynamical structure factors ...

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arXiv2021

Collective effects in confined Active Brownian Particles

We investigate a two-dimensional system of active particles confined to a narrow annular domain. Despite the absence of explicit interactions among the velocities or the active forces of different particles, the system displays a transition from a disordered and stuck state to an ordered state of global collective motion where the particles rotate persistently clockwise or anticlockwise. We describe this behavior by introducing a suitable order parameter, the velocity polarization, measuring the global alignment of the particles' velocities along the tangential direction of the ring. We also measure the spatial velocity correlation function and its correlation length to characterize the two states. In the rotating phase, the velocity correlation displays an algebraic decay that is analytically predicted together with its correlation length while in the stuck regime the velocity correlation decays exponentially with a correlation length that increases with the persistence time. In the first case, the correlation (and, in particular, its correlation length) does not depend on the active force but the system size only. The global collective motion, an effect caused by the interplay between finite-size, periodicity, and persistent active forces, disappears as the size of the ring becomes infinite, suggesting that this phenomenon does not correspond to a phase transition in the usual thermodynamic sense.

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arXiv2020

Spatial velocity correlations in inertial systems of Active Brownian Particles

Recently, it has been discovered that systems of Active Brownian particles (APB) at high density organise their velocities into coherent domains showing large spatial structures in the velocity field. Such a collective behavior occurs spontaneously, i.e. is not caused by any specific interparticle force favoring the alignment of the velocities. This phenomenon was investigated in the absence of thermal noise and in the overdamped regime where inertial forces could be neglected. In this work, we demonstrate through numerical simulations and theoretical analysis that the velocity alignment is a robust property of ABP and persists even in the presence of inertial forces and thermal fluctuations. We also show that a single dimensionless parameter, such as the Péclet number customarily employed in the description of self-propelled particles, is not sufficient to fully characterize such a phenomenon neither in the regimes of large viscosity nor small mass. Indeed, the size of the velocity domains, measured through the correlation length of the spatial velocity correlation, remains constant when the swim velocity increases while decreases as the rotational diffusion becomes larger. We find that the spatial velocity correlation depends on the inertia but, contrary to common belief, are non-symmetrically affected by mass and inverse viscosity variations. We conclude that in self-propelled systems, at variance with passive systems, variations of the inertial time (mass over solvent viscosity) and mass act as independent control parameters. Finally, we highlight the non-thermal nature of the spatial velocity correlations that are fairly insensitive both to solvent and active temperatures.

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arXiv2020

Activity-controlled clogging and unclogging of micro-channels

We propose a mechanism to control the formation of stable obstructions in two-dimensional micro-channels of variable sections taking advantage of the peculiar clustering property of active systems. Under the activation of the self-propulsion by external stimuli, the system behaves as a switch according to the following principle: by turning-on the self-propulsion the particles become active and even at very low densities stick to the walls and form growing layers eventually blocking the channel bottleneck, while the obstruction dissolves when the self-propulsion is turned off. We construct the phase diagram distinguishing clogged and open states in terms of density and bottleneck width. The study of the average clogging time, as a function of density and bottleneck width, reveals the marked efficiency of the active clogging that swiftly responds to the self-propulsion turning on. The resulting picture shows a profound difference with respect to the clogging obtained through the slow diffusive dynamics of attractive passive Brownian disks. This numerical work suggests a novel method to use particles with externally tunable self-propulsion to create or destroy plugs in micro-channels.

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arXiv2020

Inertial self-propelled particles

We study a self-propelled particle moving in a solvent with the active Ornstein Uhlenbeck dynamics in the underdamped regime to evaluate the influence of the inertia. We focus on the properties of potential-free and harmonically confined underdamped active particles, studying how the single-particle trajectories modify for different values of the drag coefficient. In both cases, we solve the dynamics in terms of correlation matrices and steady-state probability distribution functions revealing the explicit correlations between velocity and active force. We also evaluate the influence of the inertia on the time-dependent properties of the system, discussing the mean square displacement and the time-correlations of particle positions and velocities. Particular attention is devoted to the study of the Virial active pressure unveiling the role of the inertia on this observable.

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arXiv2020

Active Matter at high density: velocity distribution and kinetic temperature

We consider the solid or hexatic non-equilibrium phases of an interacting two-dimensional system of Active Brownian Particles at high density and investigate numerically and theoretically the properties of the velocity distribution function and the associated kinetic temperature. We obtain approximate analytical predictions for the shape of the velocity distribution and find a transition from a Mexican-hat-like to a Gaussian-like distribution as the persistence time of the active force changes from the small to the large persistence regime. Through a detailed numerical and theoretical analysis of the single-particle velocity variance, we report an exact analytical expression for the kinetic temperature of dense spherical self-propelled particles that holds also in the non-equilibrium regimes with large persistence times and discuss its range of validity.

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arXiv2020

Time-dependent properties of interacting active matter: dynamical behavior of one-dimensional systems of self-propelled particles

We study an interacting high-density one-dimensional system of self-propelled particles described by the Active Ornstein-Uhlenbeck particle (AOUP) model where, even in the absence of alignment interactions, velocity and energy domains spontaneously form in analogy with those already observed in two dimensions. Such domains are regions where the individual velocities are spatially correlated as a result of the interplay between self-propulsion and interactions. Their typical size is controlled by a characteristic correlation length. In the present work, we focus on a novel and lesser-known aspect of the model, namely its dynamical behavior. To this purpose, we investigate theoretically and numerically the time-dependent velocity autocorrelation and spatio-temporal velocity correlation functions. The study of these correlations provides a measure of the average life-time and, thus, the stability in time of the velocity domains.

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arXiv2020

Hidden velocity ordering in dense suspensions of self-propelled disks

Recent studies of the phase diagram for spherical, purely repulsive, active particles established the existence of a transition from a liquid-like to a solid-like phase analogous to the one observed in colloidal systems at thermal equilibrium, in particular in two dimensions an intermediate hexatic phase is observed. Here, we present evidence that the active dense phases (solid, hexatic and liquid) exhibit interesting dynamical anomalies. First, we unveil the growth - with density and activity - of ordered domains where the particles' velocities align in parallel or vortex-like patches. Second, when activity is strong, the spatial distribution of kinetic energy becomes heterogeneous with high energy regions correlated to defects of the crystalline structure. This spatial heterogeneity is accompanied by temporal intermittency, with sudden peaks in the time-series of kinetic energy. The observed dynamical anomalies are not present in a dense equilibrium system and cannot be detected by considering only the structural properties of the system.

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arXiv2019

Spontaneous velocity alignment in Motility-induced Phase Separation

We study a system of purely repulsive spherical self-propelled particles in the minimal set-up inducing Motility-Induced Phase Separation (MIPS). We show that, even if explicit alignment interactions are absent, a growing order in the velocities of the clustered particles accompanies MIPS. Particles arrange into aligned or vortex-like domains. Their sizes increase as the persistence of the self-propulsion grows, an effect that is quantified studying the spatial correlation function of the velocities. We explain the velocity-alignment by unveiling a hidden alignment interaction of the Vicsek-like form, induced by the interplay between steric interactions and self-propulsion. As a consequence, we argue that the MIPS transition cannot be fully understood in terms of a scalar field, the density, since the collective orientation of the velocities should be included in effective coarse-grained descriptions.

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arXiv2019

A comparative study between two models of active cluster-crystals

We study a system of active particles with soft repulsive interactions that lead to an active cluster-crystal phase in two dimensions. We use two different modelizations of the active force - Active Brownian particles (ABP) and Ornstein-Uhlenbeck particles (AOUP) - and focus on analogies and differences between them. We study the different phases appearing in the system, in particular, the formation of ordered patterns drifting in space without being altered. We develop an effective description which captures some properties of the stable clusters for both ABP and AOUP. As an additional point, we confine such a system in a large channel, in order to study the interplay between the cluster crystal phase and the well-known accumulation near the walls, a phenomenology typical of active particles. For small activities, we find clusters attached to the walls and deformed, while for large values of the active force they collapse in stripes parallel to the walls.

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arXiv2019

Transport of active particles in an open-wedge channel

The transport of independent active Brownian particles within a two-dimensional narrow channel, modeled as an open-wedge, is studied both numerically and theoretically. We show that the active force tends to localize the particles near the walls thus reducing the effect of the entropic force which, instead, is prevailing in the case of passive particles. As a consequence, the exit of active particles from the smaller side of the channel is facilitated with respect to their passive counterpart. By continuously re-injecting particles in the middle of the wedge, we obtain a steady regime whose properties are investigated with and without the presence of an external constant driving field. We characterize the statistics and properties of the exit process from the two opposite sides of the channel, also by making a comparison between the active and passive case. Our study reveals the existence of an optimal value of the persistence time of the active force which is able to guarantee the maximal efficiency in the transport process.

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arXiv2019

The Entropy Production of Ornstein-Uhlenbeck Active Particles: a path integral method for correlations

By employing a path integral formulation, we obtain the entropy production rate for a system of active Ornstein-Uhlenbeck particles (AOUP) both in the presence and in the absence of thermal noise. The present treatment clarifies some contraddictions concerning the definition of the entropy production rate in the AOUP model, recently appeared in the literature. We derive explicit formulas for three different cases: overdamped Brownian particle, AOUP with and without thermal noise. In addition, we show that it is not necessary to introduce additional hypotheses concerning the parity of auxiliary variables under time reversal transformation. Our results agree with those based on a previous mesoscopic approach.

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arXiv2018

Active escape dynamics: the effect of persistence on barrier crossing

We study a system of non-interacting active particles, propelled by colored noises, characterized by an activity time $τ$, and confined by a double-well potential. A straightforward application of this system is the problem of barrier crossing of active particles, which has been studied only in the limit of small activity. When $τ$ is sufficiently large, equilibrium-like approximations break down in the barrier crossing region. In the model under investigation, it emerges a sort of "negative temperature" region, and numerical simulations confirm the presence of non-convex local velocity distributions. We propose, in the limit of large $τ$, approximate equations for the typical trajectories which successfully predict many aspects of the numerical results. The local breakdown of detailed balance and its relation with a recent definition of non-equilibrium heat exchange is also discussed.

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arXiv2018

Active chiral particles under confinement: surface currents and bulk accumulation phenomena

In this work, we study the stationary behavior of an assembly of independent chiral active particles under confinement by employing an extension of the active Ornstein-Uhlenbeck model. The chirality modeled by means of an effective torque term leads to a drastic reduction of the accumulation near the walls with respect to the case without handedness and to the appearance of currents parallel to the container walls accompanied by a large accumulation of particles in the inner region. In the case of two-dimensional chiral particles confined by harmonic walls, we determine the analytic form of the distribution of positions and velocities in two different situations: a rotationally invariant confining potential and an infinite channel with parabolic walls. Both these models display currents and chirality induced inner accumulation. These phenomena are further investigated by means of a more realistic description of a channel, where the wall and bulk regions are clearly separated. The corresponding current and density profiles are obtained by numerical simulations. At variance with the harmonic models, the third model shows a progressive emptying of the wall regions and the simultaneous enhancement of the bulk population. We explain such a phenomenology in terms of the combined effect of wall repulsive forces and chiral motion and provide a semiquantitative description of the current profile in terms of an effective viscosity of the chiral gas.

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arXiv2018

Active particles under confinement and effective force generation among surfaces

We consider the effect of geometric confinement on the steady-state properties of a one-dimensional active suspension subject to thermal noise. The random active force is modeled by an Ornstein-Uhlenbeck process and the system is studied both numerically, by integrating the Langevin governing equations, and analytically by solving the associated Fokker-Planck equation under suitable approximations. The comparison between the two approaches displays a fairly good agreement and in particular, we show that the Fokker-Planck approach can predict the structure of the system both in the wall region and in the bulk-like region where the surface forces are negligible. The simultaneous presence of thermal noise and active forces determines the formation of a layer, extending from the walls towards the bulk, where the system exhibits polar order. We relate the presence of such ordering to the mechanical pressure exerted on the container's walls and show how it depends on the separation of the boundaries and determines a Casimir-like attractive force mediated by the active suspension.

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