arXiv subjects

Urban F. P. Seifert

Publications and source records attributed to Urban F. P. Seifert.

31 records · Page 2Linked to original sources

arXiv2023

Topological and magnetic phase transitions in the bilayer Kitaev-Ising model

We investigate the phase diagram of a bilayer Kitaev honeycomb model with Ising interlayer interactions, deriving effective models via perturbation theory and performing Majorana mean-field theory calculations. We show that a diverse array of magnetic and topological phase transitions occur, depending on the direction of the interlayer Ising interaction and the relative sign of Kitaev interactions. When two layers have the same sign of the Kitaev interaction, a first-order transition from a Kitaev spin liquid to a magnetically ordered state takes place. The magnetic order points along the Ising axis and it is (anti)ferromagnetic for (anti)ferromagnetic Kitaev interactions. However, when two layers have opposite sign of the Kitaev interaction, we observe a notable weakening of magnetic ordering tendencies and the Kitaev spin liquid survives up to a remarkably larger interlayer exchange. Our mean-field analysis suggests the emergence of an intermediate gapped $\mathbb{Z}_2$ spin liquid state, which eventually becomes unstable upon vison condensation. The confined phase is described by a highly frustrated $120^\circ$ compass model. We furthermore use perturbation theory to study the model with the Ising axis pointing along $\hat{z}$-axis or lying in the $xy$-plane. In both cases, our analysis reveals the formation of 1D Ising chains, which remain decoupled in perturbation theory, resulting in a subextensive ground-state degeneracy. Our results highlight the interplay between topological order and magnetic ordering tendencies in bilayer quantum spin liquids.

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arXiv2023

Mott insulators in moiré transition metal dichalcogenides at fractional fillings: Slave-rotor mean-field theory

In this work, we study a slave-rotor mean-field theory of an extended Hubbard model, applicable to transition metal dichalcogenide moiré systems, that captures both the formation of Wigner crystals as well as exotic spin states on top of these charge backgrounds. Phase diagrams are mapped out for different choices of long-range Coulomb repulsion strength, reproducing several experimentally found Wigner crystal states. Assuming unbroken time reversal symmetry, we find several spin liquid states as well as dimer states at fractional fillings. While spin dimer states are always found to have the lowest mean field energy, several spin liquid states are energetically competitive and may be stabilized by including gauge fluctuations or further interaction terms. We further discuss possible experimental signatures of these states pertinent to two-dimensional moiré heterostructures.

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arXiv2022

Twisted bilayer U(1) Dirac spin liquids

When two layers of two-dimensional materials are assembled with a relative twist, moiré patterns arise, inducing a tremendous wealth of exotic phenomena. In this work, we consider twisting two triangular lattices hosting Dirac quantum spin liquids. A single decoupled layer is described by compact quantum electrodynamics in 2+1 dimensions (QED$_3$) with an emergent $\mathrm{U}(1)$ gauge field, which is assumed to flow to a strongly interacting fixed point in the IR with conformal symmetry. We use recent results for the quantum numbers of monopole operators, which tunnel $2 π$ fluxes of the compact gauge field. It is found that, in the bilayer system, interlayer monopole tunneling is a symmetry-allowed relevant perturbation which induces an (ordering) instability. We show using perturbation theory that upon twisting the two layers the system remains unstable under the interlayer interaction, but any finite twist angle softens this instability compared to the untwisted case. To analyse the resulting phase induced by the (twisted) interlayer tunneling, we use "conformal mean field theory", which reduces the interacting bilayer system to two copies of QED$_3$ coupled to background fields which are to be determined self-consistently. In the weak-coupling regime, where the interlayer coupling is weak compared to the energy scale set by the moiré lattice constant, we solve the self-consistency equations perturbatively. In the limit of strongly coupled layers, a local scaling approximation is used, and we find that the magnetically ordered state exhibits a lattice of magnetic vortices, with the lattice constant tunable through the twisting angle.

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arXiv2022

Phase diagrams and excitations of anisotropic $S=1$ quantum magnets on the triangular lattice

The $S=1$ bilinear-biquadratic Heisenberg exchange model on the triangular lattice with a single-ion anisotropy has previously been shown to host a number of exotic magnetic and nematic orders [Moreno-Cardoner $\textit{et al.}$, Phys. Rev. B $\textbf{90}$, 144409 (2014)], including an extensive region of "supersolid" order. In this work, we amend the model by an XXZ anisotropy in the exchange interactions. Tuning to the limit of an exactly solvable $S=1$ generalized Ising-/Blume-Capel-type model provides a controlled limit to access phases at finite transverse exchange. Notably, we find an additional macroscopically degenerate region in the phase diagram and study its fate under perturbation theory. We further map out phase diagrams as a function of the XXZ anisotropy parameter, ratio of bilinear and biquadratic interactions and single-ion anisotropy, and compute corrections to the total ordered moment in various phases using systematically constructed linear flavor-wave theory. We also present linear flavor-wave spectra of various states, finding that the lowest-energy band in three-sublattice generalized (i.e. with $S^z=\pm1,0$) Ising/Blume-Capel states, stabilized by strong exchange anisotropies, is remarkably flat, opening up the way to flat-band engineering of magnetic excitation via stabilizing non-trivial Ising-ordered ground states.

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arXiv2022

Ultrafast optical excitation of magnetic dynamics in van der Waals magnets: Coherent magnons and BKT dynamics in NiPS$_3$

Optical pump-probe experiments carried out in the time domain reveal both the intrinsic low energy dynamics and its connections to higher energy excitations in correlated electron systems. In this work, we propose two microscopic mechanisms for the optical generation of coherent magnetic modes in van der Waals magnets, and derive the corresponding effective light-spin interactions: either through pumping atomic orbital excitations resonantly or via a light-induced Floquet spin Hamiltonian, the ground state of the system is driven out of equilibrium. The subsequent long-time relaxational dynamics can then be probed using, e.g. the magneto-optical Kerr effect or transient grating spectroscopy. As an example, we apply our framework to NiPS$_3$, which is magnetically ordered in the bulk, and is conjectured to realize the XY model in the monolayer limit. Our theory makes explicit how the material's low-energy response depends sensitively on the microscopic details of the light-spin coupling as well as pump fluence, frequency and polarization. For the case of bulk NiPS$_3$, we find quantitative agreement with recent experiments by Afanasiev et al. [Science Advances 7, abf3096 (2021)]. We further propose pump-probe experiments for monolayer NiPS$_3$ and detail how anomalous relaxational behaviour may reveal excitations of a (proximate) BKT phase in a proposed effective XY model.

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arXiv2021

Phase diagrams of SO($N$) Majorana-Hubbard models: Dimerization, internal symmetry breaking, and fluctuation-induced first-order transitions

We study the zero-temperature phase diagrams of Majorana-Hubbard models with SO($N$) symmetry on two-dimensional honeycomb and $π$-flux square lattices, using mean-field and renormalization group approaches. The models can be understood as real counterparts of the SU($N$) Hubbard-Heisenberg models, and may be realized in Abrikosov vortex phases of topological superconductors, or in fractionalized phases of strongly-frustrated spin-orbital magnets. In the weakly-interacting limit, the models feature stable and fully symmetric Majorana semimetal phases. Increasing the interaction strength beyond a finite threshold for large $N$, we find a direct transition towards dimerized phases, which can be understood as staggered valence bond solid orders, in which part of the lattice symmetry is spontaneously broken and the Majorana fermions acquire a mass gap. For small to intermediate $N$, on the other hand, phases with spontaneously broken SO($N$) symmetry, which can be understood as generalized Néel antiferromagnets, may be stabilized. These antiferromagnetic phases feature fully gapped fermion spectra for even $N$, but gapless Majorana modes for odd $N$. While the transitions between Majorana semimetal and dimerized phases are strongly first order, the transitions between Majorana semimetal and antiferromagnetic phases are continuous for small $N \leq 3$ and weakly first order for intermediate $N \geq 4$. The weakly-first-order nature of the latter transitions arises from fixed-point annihilation in the corresponding effective field theory, which contains a real symmetric tensorial order parameter coupled to the gapless Majorana degrees of freedom, realizing interesting examples of fluctuation-induced first-order transitions.

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arXiv2021

Flux crystals, Majorana metals, and flat bands in exactly solvable spin-orbital liquids

Spin-orbital liquids are quantum disordered states in systems with entangled spin and orbital degrees of freedom. We study exactly solvable spin-orbital models in two dimensions with selected Heisenberg-, Kitaev-, and $Γ$-type interactions, as well as external magnetic fields. These models realize a variety of spin-orbital-liquid phases featuring dispersing Majorana fermions with Fermi surfaces, nodal Dirac or quadratic band touching points, or full gaps. In particular, we show that Zeeman magnetic fields can stabilize nontrivial flux patterns and induce metamagnetic transitions between states with different topological character. Solvable nearest-neighbor biquadratic spin-orbital perturbations can be tuned to stabilize zero-energy flat bands. We discuss in detail the examples of $\mathrm{SO}(2)$- and $\mathrm{SO}(3)$-symmetric spin-orbital models on the square and honeycomb lattices, and use group-theoretical arguments to generalize to $\mathrm{SO}(ν)$-symmetric models with arbitrary integer $ν> 1$. These results extend the list of exactly solvable models with spin-orbital-liquid ground states and highlight the intriguing general features of such exotic phases. Our models are thus excellent starting points for more realistic modellings of candidate materials.

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arXiv2020

Fractionalized fermionic quantum criticality in spin-orbital Mott insulators

We study transitions between topological phases featuring emergent fractionalized excitations in two-dimensional models for Mott insulators with spin and orbital degrees of freedom. The models realize fermionic quantum critical points in fractionalized Gross-Neveu$^\ast$ universality classes in (2+1) dimensions. They are characterized by the same set of critical exponents as their ordinary Gross-Neveu counterparts, but feature a different energy spectrum, reflecting the nontrivial topology of the adjacent phases. We exemplify this in a square-lattice model, for which an exact mapping to a $t$-$V$ model of spinless fermions allows us to make use of large-scale numerical results, as well as in a honeycomb-lattice model, for which we employ $ε$-expansion and large-$N$ methods to estimate the critical behavior. Our results are potentially relevant for Mott insulators with $d^1$ electronic configurations and strong spin-orbit coupling, or for twisted bilayer structures of Kitaev materials.

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arXiv2020

Microscopic models for Kitaev's sixteenfold way of anyon theories

In two dimensions, the topological order described by $\mathbb{Z}_2$ gauge theory coupled to free or weakly interacting fermions with a nonzero spectral Chern number $ν$ is classified by $ν\; \mathrm{mod}\; 16$ as predicted by Kitaev [Ann. Phys. 321, 2 (2006)]. Here we provide a systematic and complete construction of microscopic models realizing this so-called sixteenfold way of anyon theories. These models are defined by $Γ$ matrices satisfying the Clifford algebra, enjoy a global $\mathrm{SO}(ν)$ symmetry, and live on either square or honeycomb lattices depending on the parity of $ν$. We show that all these models are exactly solvable by using a Majorana representation and characterize the topological order by calculating the topological spin of an anyonic quasiparticle and the ground-state degeneracy. The possible relevance of the $ν=2$ and $ν=3$ models to materials with Kugel-Khomskii-type spin-orbital interactions is discussed.

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arXiv2019

Optical excitation of magnons in an easy-plane antiferromagnet: Application to Sr$_2$IrO$_4$

We study the interaction of a (classical) light field with the magnetic degrees of freedom in the two-dimensional antiferromagnet Sr$_2$IrO$_4$. The reduced space group symmetry of the crystal allows for several channels for spin-operator bilinears to couple to the electric field. Integrating out high-energy degrees of freedom in a Keldysh framework, we derive induced effective fields which enter the equations of motion of the low-energy mode of in-plane rotations which couple to the out-of-plane magnetization. Considering a pump-probe protocol, these induced fields excite magnetization oscillations which can subsequently probed, e.g. using Kerr rotation. We discuss how the induced fields depend on polarization and frequency of the driving light, and our study applies to both resonant and non-resonant regimes. Crucially, the induced fields depend on the two-magnon density of states, thus allowing for further insight into properties of the magnetic excitation spectrum. Furthermore, these effects rely upon (weak) magnon-interactions, and so are beyond a "Floquet magnon" description.

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arXiv2019

Theory of partial quantum disorder in the stuffed honeycomb Heisenberg antiferromagnet

Recent numerical results [Gonzalez $\textit{et al.}$, Phys. Rev. Lett. $\textbf{122}$, 017201 (2019); Shimada $\textit{et al.}$, J. Phys. Conf. Ser. $\textbf{969}$, 012126 (2018)] point to the existence of a partial-disorder ground state for a spin-1/2 antiferromagnet on the stuffed honeycomb lattice, with 2/3 of the local moments ordering in an antiferromagnetic Néel pattern, while the remaining 1/3 of the sites display short-range correlations only, akin to a quantum spin liquid. We derive an effective model for this disordered subsystem, by integrating out fluctuations of the ordered local moments, which yield couplings in a formal $1/S$ expansion, with $S$ being the spin amplitude. The result is an effective triangular-lattice XXZ model, with planar ferromagnetic order for large $S$ and a stripe-ordered Ising ground state for small $S$, the latter being the result of frustrated Ising interactions. Within the semiclassical analysis, the transition point between the two orders is located at $S_c=0.646$, being very close to the relevant case $S=1/2$. Near $S=S_c$ quantum fluctuations tend to destabilize magnetic order. We conjecture that this applies to $S=1/2$, thus explaining the observed partial-disorder state.

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arXiv2018

Bilayer Kitaev models: Phase diagrams and novel phases

Kitaev's honeycomb-lattice spin-$1/2$ model has become a paradigmatic example for $\mathbb{Z}_2$ quantum spin liquids, both gapped and gapless. Here we study the fate of these spin-liquid phases in differently stacked bilayer versions of the Kitaev model. Increasing the ratio between the inter-layer Heisenberg coupling $J_\perp$ and the intra-layer Kitaev couplings $K^{x,y,z}$ destroys the topological spin liquid in favor of a paramagnetic dimer phase. We study phase diagrams as a function of $J_\perp/K$ and Kitaev coupling anisotropies using Majorana-fermion mean-field theory, and we employ different expansion techniques in the limits of small and large $J_\perp/K$. For strongly anisotropic Kitaev couplings, we derive effective models for the different layer stackings which we use to discuss the quantum phase transition out of the Kitaev phase. We find that the phase diagrams depend sensitively on the nature of the stacking and anisotropy strength. While in some stackings and at strong anisotropies we find a single transition between the Kitaev and dimer phases, other stackings are more involved: Most importantly, we prove the existence of two novel macro-spin phases which can be understood in terms of Ising chains which can be either coupled ferromagnetically or remain degenerate, thus realizing a classical spin liquid. In addition, our results suggest the existence of a flux phase with spontaneous inter-layer coherence.

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arXiv2018

Fractionalized Fermi liquids and exotic superconductivity in the Kitaev-Kondo lattice

Fractionalized Fermi liquids (FL$^\ast$) have been introduced as non-Fermi-liquid metallic phases, characterized by coexisting electron-like charge carriers and local moments which itself form a fractionalized spin liquid. Here we investigate a Kondo lattice model on the honeycomb lattice with compass interactions among the local moments, a concrete model hosting FL$^\ast$ phases based on Kitaev's $\mathbb{Z}_2$ spin liquid. We characterize the FL$^\ast$ phases via perturbation theory, and we employ a Majorana-fermion mean-field theory to map out the full phase diagram. Most remarkably we find triplet superconducting phases which mask the quantum phase transition between fractionalized and conventional Fermi liquid phases. Their pairing structure is inherited from the Kitaev spin liquid, i.e., superconductivity is driven by Majorana glue.

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