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Uri Vool

Publications and source records attributed to Uri Vool.

At least 19 recordsLinked to original sources

Resolving unconventional gap structure in kagome superconductors with hybrid microwave circuits

Unconventional superconductivity is a hallmark of exotic quantum matter, where determining the pairing symmetry is essential for uncovering its microscopic origin. Kagome superconductors provide a fertile landscape for emergent phenomena arising from strong electronic correlations and nontrivial band topology, yet their superconducting pairing symmetry remains elusive. The superconducting gap structure is commonly probed via electrodynamic response, but such measurements are inapplicable to thin flakes due to their small volume and delicate nature. Superconducting microwave resonators offer a coherent and highly sensitive platform for probing electrodynamic responses, with versatile designs that enable incorporation of diverse materials and geometries. Here, we integrate flakes into microwave circuits, enabling noninvasive access to the superfluid response through contactless coupling that preserves structural integrity. By engineering the device geometry to suppress parasitic two-level-system losses that dominate dissipation in microwave circuits, we isolate the intrinsic material response. Remarkably, the temperature-dependent superfluid density exhibits linear behavior at low temperatures, consistent with a nodal gap structure. Our approach establishes a noninvasive platform for probing electrodynamic response of fragile superconducting flakes while advancing hybrid microwave architectures for quantum technologies.

cond-mat.supr-con

Power-Law Suppression of Superfluid Stiffness in High-Kinetic-Inductance NbN Films

Disorder is a powerful route to high kinetic inductance in superconducting ultrathin films, enabling compact high-impedance quantum circuits. This functionality, however, comes at the cost of reduced phase rigidity and potentially anomalous electrodynamics. Here, we use NbN microwave resonators with thicknesses down to 2.8 nm and sheet kinetic inductance up to 300 pH per square to probe how this trade-off reshapes the superconducting response. In the thinnest films, transport shows signatures of a Berezinskii-Kosterlitz-Thouless transition, while the microwave response reveals a pronounced low-temperature power-law suppression of the superfluid stiffness, inconsistent with Mattis-Bardeen theory. With increasing thickness, this anomalous regime is progressively suppressed, marking a continuous crossover toward conventional, gap-dominated electrodynamics. Cross-sectional transmission electron microscopy reveals a nanocrystalline twin-domain structure, pointing to oriented microstructural disorder as a crucial factor in the observed response. Overall, the crossover is governed by the ratio of superfluid stiffness to pairing energy, Theta(0)/Tc, identifying this ratio as a parameter governing the boundary between phase-fluctuation-dominated and gap-dominated superconducting electrodynamics in disordered nanofilms.

cond-mat.supr-con

Fraxonium: Fractional fluxon states for qudit encoding

We propose a superconducting circuit hosting $d$ low-lying states, well separated from the rest of the spectrum, that naturally realizes a qudit system protected from leakage errors. The system represents a generalization of the fluxonium and the low-energy states are constituted by fractional fluxon states, that we call {\it fraxons}, localized in the minima of a suitably designed Josephson potential. The latter is tailored through a Fourier engineering approach, that employs multi-harmonic Josephson building block elements composed by a Josephson junction and an inductance connected in series. We present the spectrum of a $d=4$ and a $d=5$ qudit system and study in detail the qutrit case. We analyze the dipole matrix elements for coupling to radiation and propose a non-Abelian, stimulated Raman adiabatic passage (STIRAP) protocol for single-qutrit gates, that is particularly suited for the present system. The proposed platform opens novel perspectives in circuit engineering and quantum computing beyond the qubit paradigm.

quant-ph

A Fourier-Space Approach to Physics-Informed Magnetization Reconstruction from Nitrogen-Vacancy Measurements

Reconstructing magnetization textures from nitrogen-vacancy (NV) magnetometry stray-field measurements is a challenging, fundamentally ill-posed inverse problem, further complicated by the unknown effective distance between sensor and magnetic material. Here we show that incorporating a micromagnetic energy functional directly into the inversion filters out unphysical, high-energy configurations, while Fourier-space upward continuation of the stray field allows us to simultaneously fit the distance. Applied to measurements of the van der Waals ferromagnet Fe$_{3-x}$GaTe$_2$, it recovers an effective distance estimate of approximately 81nm and low-energy configurations that reproduce the observed field. More broadly, embedding physics directly into the reconstruction turns ill-posed magnetic inverse problems into transparent, interpretable reconstructions, with applicability well beyond NV magnetometry.

cond-mat.mes-hall

Cuprate Twistronics for Quantum Hardware

Recent advances in the manipulation of complex oxide layers, particularly the fabrication of atomically thin cuprate superconducting films via molecular beam epitaxy, have revealed new ways in which nanoscale engineering can govern superconductivity and its interwoven electronic orders. In parallel, the creation of twisted cuprate heterostructures through cryogenic stacking techniques marks a pivotal step forward, exploiting cuprate superconductors to deepen our understanding of exotic quantum states and propel next-generation quantum technologies. This review explores over three decades of research in the emerging field of cuprate twistronics, examining both experimental breakthroughs and theoretical progress. It also highlights the methodologies poised to surmount the outstanding challenges in leveraging these complex quantum materials, underscoring their potential to expand the frontiers of quantum science and technology.

cond-mat.supr-con

Altermagnetic nanotextures revealed in bulk MnTe

With many candidate altermagnetic materials, MnTe has emerged as one of the most promising systems, with growing experimental evidence for altermagnetic phenomena. So far, the majority of measurements have been performed on thin-films, or have involved surface measurements. However, the question of altermagnetic order in the bulk system - in the absence of substrate or surface effects - remains. Here we show evidence for bulk altermagnetism in single crystal MnTe, through spectroscopic X-ray microscopy. By performing nanoscale X-ray magnetic circular dichroic (XMCD) imaging in transmission on a 200 nm thick lamella, we observe domains and magnetic textures with a spectroscopic signature characteristic of altermagnetic order, thereby confirming the intrinsic nature of altermagnetism in MnTe. Quantitative analysis of the XMCD signal reveals an excellent agreement with predicted signals, establishing that the altermagnetic order exists throughout the thickness of the lamella and confirming the intrinsic, bulk nature of the state. With these results, we demonstrate that transmission XMCD spectroscopic imaging is a robust, quantitative technique to probe altermagnetic order, providing a means to probe individual altermagnetic domains within complex configurations. This ability to investigate, and characterise altermagnetic order in bulk crystals represents an important tool for the exploration of altermagnetism across a wide range of candidate materials, of key importance for the development of future technologies.

cond-mat.mtrl-sci

Exploring van der Waals cuprate superconductors using a hybrid microwave circuit

The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. In this study, we investigate the superconducting properties of Bi2Sr2CaCu2O8+x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor. We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.

cond-mat.supr-con

Flux-Tunable Regimes and Supersymmetry in Twisted Cuprate Heterostructures

Van der Waals assembly allows for the creation of Josephson junctions in an atomically sharp interface between two exfoliated Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ (Bi-2212) flakes that are twisted relative to each other. In a narrow range of angles close to $45^\circ$, the junction exhibits a regime where time-reversal symmetry can be spontaneously broken and it can be used to encode an inherently protected qubit called flowermon. In this work we investigate the physics emerging when two such junctions are integrated in a SQuID circuit threaded by a magnetic flux. We show that the flowermon qubit regime is maintained up to a finite critical value of the magnetic field and, under appropriate conditions, it is protected against both charge and flux noise. For larger external fluxes, the interplay between the inherent twisted d-wave nature of the order parameter and the external magnetic flux enables the implementation of different artificial atoms, including a flux-biased protected qubit and a supersymmetric quantum circuit.

cond-mat.supr-con

Vortex motion in reconfigurable three-dimensional superconducting nanoarchitectures

When materials are patterned in three dimensions, there exist opportunities to tailor and create functionalities associated with an increase in complexity, the breaking of symmetries, and the introduction of curvature and non-trivial topologies. For superconducting nanostructures, the extension to the third dimension may trigger the emergence of new physical phenomena, as well as advances in technologies. Here, we harness three-dimensional (3D) nanopatterning to fabricate and control the emergent properties of a 3D superconducting nanostructure. Not only are we able to demonstrate the existence and motion of superconducting vortices in 3D but, with simulations, we show that the confinement leads to a well-defined bending of the vortices within the volume of the structure. Moreover, we experimentally observe a strong geometrical anisotropy of the critical field, through which we achieve the reconfigurable coexistence of superconducting and normal states in our 3D superconducting architecture, and the local definition of weak links. In this way, we uncover an intermediate regime of nanosuperconductivity, where the vortex state is truly three-dimensional and can be designed and manipulated by geometrical confinement. This insight into the influence of 3D geometries on superconducting properties offers a route to local reconfigurable control for future computing devices, sensors, and quantum technologies.

cond-mat.mes-hall

Current Induced Hidden States in Josephson Junctions

Josephson junctions enable dissipation-less electrical current through metals and insulators below a critical current. Despite being central to quantum technology based on superconducting quantum bits and fundamental research into self-conjugate quasiparticles, the spatial distribution of super current flow at the junction and its predicted evolution with current bias and external magnetic field remain experimentally elusive. Revealing the hidden current flow, featureless in electrical resistance, helps understanding unconventional phenomena such as the nonreciprocal critical current, i.e., Josephson diode effect. Here we introduce a platform to visualize super current flow at the nanoscale. Utilizing a scanning magnetometer based on nitrogen vacancy centers in diamond, we uncover competing ground states electrically switchable within the zero-resistance regime. The competition results from the superconducting phase re-configuration induced by the Josephson current and kinetic inductance of thin-film superconductors. We further identify a new mechanism for the Josephson diode effect involving the Josephson current induced phase. The nanoscale super current flow emerges as a new experimental observable for elucidating unconventional superconductivity, and optimizing quantum computation and energy-efficient devices.

cond-mat.mes-hall

Superconducting qubit based on twisted cuprate van der Waals heterostructures

Van-der-Waals (vdW) assembly enables the fabrication of novel Josephson junctions utilizing an atomically sharp interface between two exfoliated and relatively twisted $\rm{Bi_2Sr_2CaCu_2O_{8+x}}$ (Bi2212) flakes. In a range of twist angles around $45^\circ$, the junction provides a regime where the interlayer two-Cooper pair tunneling dominates the current-phase relation. Here we propose to employ this novel junction to realize a capacitively shunted qubit that we call flowermon. The $d$-wave nature of the order parameter endows the flowermon with inherent protection against charge-noise-induced relaxation and quasiparticle-induced dissipation. This inherently protected qubit paves the way to a new class of high-coherence hybrid superconducting quantum devices based on unconventional superconductors.

cond-mat.supr-con

Preturbulence in momentum-relaxing Navier-Stokes hydrodynamics

In a hydrodynamic regime of electronic fluids, the electron scattering on impurities and phonons inhibits the development of oscillating preturbulent phenomena (such as the K\'arm\'an vortex shedding) and enforces a laminar flow. Working in a local generalization of the Navier-Stokes hydrodynamics of incompressible two-dimensional fluids, we show that the critical relaxation time separating these two regimes is described by a surprisingly simple fractional power function of the Reynolds number. The critical exponent, $\alpha \simeq 4/3$, sets particular experimental conditions for the observation of preturbulent effects in electronic fluids.

physics.flu-dyn

Nanoscale Electric Field Imaging with an Ambient Scanning Quantum Sensor Microscope

Nitrogen-vacancy (NV) center in diamond is a promising quantum sensor with remarkably versatile sensing capabilities. While scanning NV magnetometry is well-established, NV electrometry has been so far limited to bulk diamonds. Here we demonstrate imaging external alternating (AC) and direct (DC) electric fields with a single NV at the apex of a diamond scanning tip under ambient conditions. A strong electric field screening effect is observed at low frequencies due to charge noise on the surface. We quantitatively measure its frequency dependence, and overcome this screening by mechanically oscillating the tip for imaging DC fields. Our scanning NV electrometry achieved an AC E-field sensitivity of 26 mV um^(-1) Hz^(-1/2), a DC E-field gradient sensitivity of 2 V um^(-2) Hz^(-1/2), and sub-100 nm resolution limited by the NV-sample distance. Our work represents an important step toward building a scanning-probe-based multimodal quantum sensing platform.

quant-ph

Nuclear Spin Assisted Magnetic Field Angle Sensing

Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications, predominantly used as a magnetometer. However, its magnetic field sensitivity vanishes when a bias magnetic field acts perpendicular to the NV axis. Here, we introduce a novel sensing strategy assisted by the nitrogen nuclear spin that uses the entanglement between the electron and nuclear spins to restore the magnetic field sensitivity. This, in turn, allows us to detect small changes in the magnetic field angle relative to the NV axis. Furthermore, based on the same underlying principle, we show that the NV coupling strength to magnetic noise, and hence its coherence time, exhibits a strong asymmetric angle dependence. This allows us to uncover the directional properties of the local magnetic environment and to realize maximal decoupling from anisotropic noise.

quant-ph

Imaging phonon-mediated hydrodynamic flow in WTe2

In the presence of interactions, electrons in condensed-matter systems can behave hydrodynamically, exhibiting phenomena associated with classical fluids, such as vortices and Poiseuille flow. In most conductors, electron-electron interactions are minimized by screening effects, hindering the search for hydrodynamic materials; however, recently, a class of semimetals has been reported to exhibit prominent interactions. Here we study the current flow in the layered semimetal tungsten ditelluride by imaging the local magnetic field using a nitrogen-vacancy defect in a diamond. We image the spatial current profile within three-dimensional tungsten ditelluride and find that it exhibits non-uniform current density, indicating hydrodynamic flow. Our temperature-resolve current profile measurements reveal a non-monotonic temperature dependence, with the strongest hydrodynamic effects at approximately 20 K. We also report ab initio calculations showing that electron-electron interactions are not explained by the Coulomb interaction alone, but are predominantly mediated by phonons. This provides a promising avenue in the search for hydrodynamic flow and prominent electron interactions in high-carrier-density materials.

cond-mat.mes-hall

High-Energy Quasiparticle Injection into Mesoscopic Superconductors

At nonzero temperatures, superconductors contain excitations known as Bogoliubov quasiparticles. The mesoscopic dynamics of quasiparticles inform the design of quantum information processors, among other devices. Knowledge of these dynamics stems from experiments in which quasiparticles are injected in a controlled fashion, typically at energies comparable to the pairing energy . Here we perform tunnel spectroscopy of a mesoscopic superconductor under high electric field. We observe quasiparticle injection due to field-emitted electrons with 10^6 times the pairing energy, an unexplored regime of quasiparticle dynamics. Upon application of a gate voltage, the quasiparticle injection decreases the critical current and, at sufficiently high electric field, the field-emission current (< 0.1 nA) switches the mesoscopic superconductor into the normal state, consistent with earlier results. We expect that high-energy injection will be useful for developing quasiparticle-tolerant quantum information processors, will allow rapid control of resonator quality factors, and will enable the design of electric-field-controlled superconducting devices with new functionality.

cond-mat.supr-con

Imaging viscous flow of the Dirac fluid in graphene

The electron-hole plasma in charge-neutral graphene is predicted to realize a quantum critical system whose transport features a universal hydrodynamic description, even at room temperature. This quantum critical "Dirac fluid" is expected to have a shear viscosity close to a minimum bound, with an inter-particle scattering rate saturating at the Planckian time $\hbar/(k_B T)$. While electrical transport measurements at finite carrier density are consistent with hydrodynamic electron flow in graphene, a "smoking gun" of viscous behavior remains elusive. In this work, we directly image viscous Dirac fluid flow in graphene at room temperature via measurement of the associated stray magnetic field. Nanoscale magnetic imaging is performed using quantum spin magnetometers realized with nitrogen vacancy (NV) centers in diamond. Scanning single-spin and wide-field magnetometry reveals a parabolic Poiseuille profile for electron flow in a graphene channel near the charge neutrality point, establishing the viscous transport of the Dirac fluid. This measurement is in contrast to the conventional uniform flow profile imaged in an Ohmic conductor. Via combined imaging-transport measurements, we obtain viscosity and scattering rates, and observe that these quantities are comparable to the universal values expected at quantum criticality. This finding establishes a nearly-ideal electron fluid in neutral graphene at room temperature. Our results pave the way to study hydrodynamic transport in quantum critical fluids relevant to strongly-correlated electrons in high-$T_c$ superconductors. This work also highlights the capability of quantum spin magnetometers to probe correlated-electronic phenomena at the nanoscale.

cond-mat.mes-hall

Schrodinger's catapult: Launching multiphoton quantum states from a microwave cavity memory

Encoding quantum states in complex multiphoton fields can overcome loss during signal transmission in a quantum network. Transmitting quantum information encoded in this way requires that locally stored states can be converted to propagating fields. Here we experimentally show the controlled conversion of multiphoton quantum states, like "Schr\"odinger cat" states, from a microwave cavity quantum memory into propagating modes. By parametric conversion using the nonlinearity of a single Josephson junction, we can release the cavity state in ~500 ns, about 3 orders of magnitude faster than its intrinsic lifetime. This `catapult' faithfully converts arbitrary cavity fields to traveling signals with an estimated efficiency of > 90%, enabling on-demand generation of complex itinerant quantum states. Importantly, the release process can be controlled precisely on fast time scales, allowing us to generate entanglement between the cavity and the traveling mode by partial conversion. Our system can serve as the backbone of a microwave quantum network, paving the way towards error-correctable distribution of quantum information and the transfer of highly non-classical states to hybrid quantum systems.

quant-ph