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Uwe Sterr

Publications and source records attributed to Uwe Sterr.

At least 19 recordsLinked to original sources

Laser stabilized to a room temperature cavity with AlGaAs coatings reaching $4.2 \times 10^{-17}$ fractional frequency instability

We present a laser system referenced to a room-temperature ultrastable cavity employing crystalline AlGaAs coatings. We demonstrate a fractional frequency instability of $4.2 \times 10^{-17}$, which is one of the lowest for room temperature systems and surpasses the limit imposed by Brownian noise if dielectric coatings were employed. For the first time in a room temperature system we identified the spontaneous fluctuations of the coating birefringence as a leading contribution to frequency instability. At optimized conditions we achieve an ultrastable cavity with an eigenfrequency that is highly immune to power fluctuations. As acceleration noise is the main noise contribution, we demonstrated that a feed-forward method can reduce the influence of accelerations on the cavity-stabilized laser frequency by a factor of four.

physics.optics

Ultra-stable transportable ultraviolet clock laser using cancellation between photo-thermal and photo-birefringence noise

Optical clocks require an ultra-stable laser to probe and precisely measure the frequency of the narrow-linewidth clock transition. We introduce a portable ultraviolet (UV) laser system for use in an aluminum quantum logic clock, demonstrating a fractional frequency instability of approximately $\mathrm{mod}\,σ_\mathrm{y} = 2 \times 10^{-16}$. The system is based on an ultra-stable cavity with crystalline AlGaAs/GaAs mirror coatings, alongside with a frequency quadrupling system employing two single-pass second harmonic generation (SHG) stages. Its acceleration sensitivity, measured in all three axes, does not exceed $4(2) \times 10^{-12}$/(ms$^{-2}$) and is among the lowest recorded for transportable systems to date. Additionally, partial cancellation between photo-thermal noise and photo-birefringence noise is used to effectively mitigate noise induced by intra-cavity optical power fluctuation at lower Fourier frequencies.

physics.optics

Lunar Silicon Cavity

The Moon's permanently shadowed regions (PSRs) are among the coldest places in the Solar System and are expected to become key landing sites for upcoming international space agency missions. Their proximity to peaks of perpetual solar power and potential resource richness makes them prime candidates for lunar exploration and future Moon bases. Here we propose to deploy a passive, ultrastable optical resonator in these regions that will enable laser systems with unprecedented phase-coherence. The unique physical environment of lunar PSRs greatly benefits the construction of a cryogenic monolithic silicon cavity that exhibits low $10^{-18}$ thermal noise-limited stability and coherence time exceeding 1 minute, more than a decade better than the current best terrestrial system. Such a stable laser will form an enabling infrastructure for quantum technology in space to serve many applications, including establishing a lunar time standard, building long-baseline optical interferometry, distribution of stable optical signals across networks of satellites, testing general relativity and gravitational physics, and forming the backbone for space-based quantum networks.

quant-ph

Photo-birefringent effects in crystalline AlGaAs mirror coatings

High-reflective crystalline $GaAs/Al_{0.92}Ga_{0.08}As$ coatings show reduced Brownian noise compared to conventional dielectric coatings. However, several ultra stable laser systems observed additional noise sources that hinder the realization of the expected improvements in frequency stability. These additional noise sources are related to the birefringence of the coatings and its modification by intracavity light. The origin of the birefringence is not yet well understood and its modification via illumination remains unexplained. Here we present an extensive study on the steady-state and transient modification of the birefringence by intracavity light and by uniform illumination at various wavelengths using an optical cavity at room temperature. We find a unified description that suggests a primary two-photon process for photon energies below the bandgap of GaAs, or a single-photon process at higher energies. Adding external illumination allows to reduce noise induced by laser power fluctuations by balancing the photo-thermal-optic response of the mirrors and the photo-birefringent effect at a more favorable low intracavity power.

physics.optics

Frequency stability of $2.5\times10^{-17}$ in a Si cavity with AlGaAs crystalline mirrors

Developments in ultrastable lasers have fueled remarkable advances in optical frequency metrology and quantum science. A key ingredient in further improving laser frequency stability is the use of low-noise mirror materials such as AlGaAs crystalline coatings. However, excess noise observed with these coatings limits the performance of cryogenic silicon cavities with AlGaAs mirrors to similar levels achieved with conventional dielectric coatings. With a new pair of crystalline coated mirrors in a 6-cm-long cryogenic silicon cavity operated at 17 K, we demonstrate a clear advantage of crystalline coatings over dielectric coatings. The achieved fractional frequency stability of $2.5 \times 10^{-17}$ at 10 s is four times better than expected for dielectric mirrors and corresponds to more than tenfold reduction in the coating mechanical loss factor. We also combine two silicon cavities to demonstrate optical frequency averaging for enhanced stability. In addition, we present a long-term frequency drift record of four cryogenic silicon cavities measured over several years. These results open up realistic prospects for cavity-stabilized lasers with $10^{-18}$ fractional stability, as well as an all-optical timescale with continuously operating optical local oscillators.

physics.optics

Coordinated international comparisons between optical clocks connected via fiber and satellite links

Optical clocks provide ultra-precise frequency references that are vital for international metrology as well as for tests of fundamental physics. To investigate the level of agreement between different clocks, we simultaneously measured the frequency ratios between ten optical clocks in six different countries, using fiber and satellite links. This is the largest coordinated comparison to date, from which we present a subset of 38 optical frequency ratios and an evaluation of the correlations between them. Four ratios were measured directly for the first time, while others had significantly lower uncertainties than previously achieved, supporting the advance towards a redefinition of the second and the use of optical standards for international time scales.

physics.atom-ph

Guidelines for designs for ultrastable laser with $\mathbf{10^{-17}}$ fractional frequency instability

Lasers with long coherence time and narrow linewidth are an essential tool for quantum sensors and clocks. Ultrastable cavities and laser systems are now commercially available with fractional frequency instabilities in the mid $10^{-16}$ range. This document aims to provide technical guidance for researchers starting in the field of ultrastable lasers and to give an outlook toward the next generation of improved ultrastable lasers. These guidelines have arisen from the scope of the EMPIR project ``Next generation ultrastable lasers'' ( https://www.ptb.de/empir2021/nextlasers ) with contributions from the European project partners.

physics.optics

Excess noise and photo-induced effects in highly reflective crystalline mirror coatings

Thermodynamically induced length fluctuations of high-reflectivity mirror coatings put a fundamental limit on sensitivity and stability of precision optical interferometers like gravitational wave detectors and ultra-stable lasers. The main contribution - Brownian thermal noise - is related to the mechanical loss of the coating material. Owing to their low mechanical losses, Al\textsubscript{0.92}Ga\textsubscript{0.08}As/GaAs crystalline mirror coatings are expected to reduce this limit. At room temperature they have demonstrated lower Brownian thermal noise than with conventional amorphous coatings. %However, no detailed study on the noise constituents from these coatings in optical interferometers has been conducted. We present a detailed study on the spatial and temporal noise properties of such coatings by using them in two independent cryogenic silicon optical Fabry-Perot resonators operated at 4 K, 16 K and 124 K. We confirm the expected low Brownian thermal noise, but also discover two new noise sources that exceed the Brownian noise: birefringent noise that can be canceled via polarization averaging and global excess noise (10 dB above Brownian noise). These new noise contributions are a barrier to improving ultra-stable lasers and the related performance of atomic clocks, and potentially limit the sensitivity of third-generation gravitational wave detectors. Hence, they must be considered carefully in precision interferometry experiments using similar coatings based on semiconductor materials.

physics.optics

Frequency stability of cryogenic silicon cavities with semiconductor crystalline coatings

State-of-the-art optical oscillators employing cryogenic reference cavities are limited in performance by the Brownian thermal noise associated with the mechanical dissipation of the mirror coatings. Recently, crystalline Al$_{1-x}$Ga$_{x}$As/GaAs coatings have emerged as a promising candidate for improved coating thermal noise. We present measurements of the frequency noise of two fully crystalline cryogenic reference cavities with Al$_{0.92}$Ga$_{0.08}$As/GaAs optical coatings. We report on previously unmeasured birefringent noise associated with anti-correlated frequency fluctuations between the polarization modes of the crystalline coatings, and identify variables that affect its magnitude. Comparing the birefringent noise between the two cryogenic reference cavities reveals a phenomenological set of scalings with intracavity power and mode area. We implement an interrogation scheme that cancels this noise by simultaneous probing of both polarization modes. The residual noise remaining after this cancellation is larger than both cavities thermal noise limits, but still lower than the instabilities previously measured on equivalent resonators with dielectric coatings. Though the source of these novel noise mechanisms is unclear, we demonstrate that crystalline coatings can provide stability and sensitivity competitive with resonators employing dielectric coatings.

physics.optics

Ultimate stability of active optical frequency standards

Active optical frequency standards provide interesting alternatives to their passive counterparts. Particularly, such a clock alone continuously generates highly-stable narrow-line laser radiation. Thus a local oscillator is not required to keep the optical phase during a dead time between interrogations as in passive clocks, but only to boost the active clock's low output power to practically usable levels with the current state of technology. Here we investigate the spectral properties and the stability of active clocks, including homogeneous and inhomogeneous broadening effects. We find that for short averaging times the stability is limited by photon shot noise from the limited emitted laser power and at long averaging times by phase diffusion of the laser output. Operational parameters for best long-term stability were identified. Using realistic numbers for an active clock with $^{87}$Sr we find that an optimized stability of $σ_y(τ) \approx 4\times10^{-18}/\sqrt{τ[\mathrm{s}]}$ is achievable.

physics.atom-ph

A transportable clock laser system with an instability of $1.6 \times 10^{-16}$

We present a transportable ultra-stable clock laser system based on a Fabry-Pérot cavity with crystalline Al$_{0.92}$Ga$_{0.08}$As/GaAs mirror coatings, fused silica (FS) mirror substrates and a 20~cm-long ultra-low expansion (ULE\textsuperscript{\textregistered}) glass spacer with a predicted thermal noise floor of $\mathrm{mod}\,σ_\mathrm{y} = 7 \times 10^{-17}$ in modified Allan deviation at one second averaging time. The cavity has a cylindrical shape and is mounted at ten points. Its measured sensitivity of the fractional frequency to acceleration for the three Cartesian directions are $2(1) \times 10^{-12}$/(ms$^{-2}$), $3(3) \times 10^{-12}$/(ms$^{-2}$) and $3(1) \times 10^{-12}$/(ms$^{-2}$), which belong to the lowest acceleration sensitivities published for transportable systems. The laser system's instability reaches down to $\mathrm{mod}\,σ_\mathrm{y} = 1.6 \times 10^{-16}$

physics.optics

Thermal noise and mechanical loss of SiO$_2$/Ta$_2$O$_5$ optical coatings at cryogenic temperatures

Mechanical loss of dielectric mirror coatings sets fundamental limits for both gravitational wave detectors and cavity-stabilized optical local oscillators for atomic clocks. Two approaches are used to determine the mechanical loss: ringdown measurements of the coating quality factor and direct measurement of the coating thermal noise. Here we report a systematic study of the mirror thermal noise from room temperature to 4 K by operating reference cavities at these temperatures. The directly measured thermal noise is used to extract the corresponding mechanical loss for SiO$_2$/Ta$_2$O$_5$ coatings, which are compared with previously reported values.

physics.ins-det

Simple and compact diode laser system stabilized to Doppler-broadened iodine-lines at 633 nm

We present a compact iodine-stabilized laser system at 633 nm, based on a distributed-feedback laser diode. Within a footprint of $27\times 15$ cm$^2$ the system provides 5 mW of frequency stabilized light from a single-mode fiber. Its performance was evaluated in comparison to Cs clocks representing primary frequency standards, realizing the SI unit Hz via an optical frequency comb. With the best suited absorption line the laser reaches a fractional frequency instability below $10^{-10}$ for averaging times above 10 s. The performance was investigated at several iodine lines and a model was developed to describe the observed stability on the different lines.

physics.optics

Optical frequency ratio of a ${}^{171}\mathrm{Yb}^+$ single-ion clock and a ${}^{87}\mathrm{Sr}$ lattice clock

We report direct measurements of the frequency ratio of the 642 THz ${}^2S_{1/2} (F=0)$--${}^2F_{7/2} (F=3)$ electric octupole transition in ${}^{171}\mathrm{Yb}^+$ and the 429 THz ${}^1S_0$--${}^3P_0$ transition in ${}^{87}\mathrm{Sr}$. A series of 107 measurements has been performed at the Physikalisch-Technische Bundesanstalt between December 2012 and October 2019. Long-term variations of the ratio are larger than expected from the individual measurement uncertainties of few $10^{-17}$. The cause of these variations remains unknown. Even taking these into account, we find a fractional uncertainty of the frequency ratio of $2.5 \times 10^{-17}$, which improves upon previous knowledge by one order of magnitude. The average frequency ratio is $ν_{\mathrm{Yb}^+} / ν_{\mathrm{Sr}} = 1.495\,991\,618\,544\,900\,537(38)$. This represents one of the most accurate measurements between two different atomic species to date.

physics.atom-ph

Prospects and challenges for squeezing-enhanced optical atomic clocks

We have investigated the benefits of spin squeezed states for clocks operated with typical Brownian frequency noise-limited laser sources. Based on an analytic model of the closed servo-loop of an optical atomic clock, we can give quantitative predictions on the optimal clock stability for a given dead time and laser noise. Our analytic predictions are in very good agreement with numerical simulations of the closed servo-loop. We find that for usual cyclic Ramsey interrogation of single atomic ensembles with dead time, even with the current most stable lasers spin squeezing can only improve the clock stability for ensembles below a critical atom number of about one thousand in an optical Sr lattice clock. Even with a future improvement of the laser performance by one order of magnitude the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers.

quant-ph

A transportable interrogation laser system with an instability of $\mathrm{mod}\,σ_{\rm y} = 3\times10^{-16}$

We present an interrogation laser system for a transportable strontium lattice clock operating at 698 nm, which is based on an ultra-low-expansion glass reference cavity. Transportability is achieved by implementing a rigid, compact, and vibration insensitive mounting of the 12 cm-long reference cavity, sustaining shocks of up to 50 g. The cavity is mounted at optimized support points that independently constrain all degrees of freedom. This mounting concept is especially beneficial for cavities with a ratio of length $L$ over diameter $D$ $L/D>1$. Generally large $L$ helps to reduce thermal noise-induced laser frequency instability while small $D$ leads to small cavity volume. The frequency instability was evaluated, reaching its thermal noise floor of $\mathrm{mod}\,σ_{\rm y} \approx 3 \times 10^{-16}$ for averaging times between 0.5 s and 10 s. The laser system was successfully operated during several field studies.

physics.ins-det

End-to-end topology for fiber comb based optical frequency transfer at the $10^{-21}$ level

We introduce a simple and robust scheme for optical frequency transfer of an ultra-stable source light field via an optical frequency comb to a field at a target optical frequency, where highest stability is required, e.g. for the interrogation of an optical clock. The scheme relies on a topology for end-to-end suppression of the influence of optical path-length fluctuations, which is attained by actively phase-stabilized delivery, combined with common-path propagation. This approach provides a robust stability improvement without the need for additional isolation against environmental disturbances such as temperature, pressure or humidity changes. We measure residual frequency transfer instabilities by comparing the frequency transfers carried out with two independent combs simultaneously. Residual fractional frequency instabilities between two systems of $8\times10^{-18}$ at 1 s and $3\times10^{-21}$ at $10^5$ s averaging time are observed. We discuss the individual noise contributions to the residual instability. The presented scheme is technically simple, robust against environmental parameter fluctuations, and enables an ultra-stable frequency transfer, e.g. to optical clock lasers or to lasers in gravitational wave detectors.

physics.optics

Dynamic decoupling of laser phase noise in compound atomic clocks

The frequency stability achieved by an optical atomic clock ultimately depends on the coherence of its local oscillator. Even the best ultrastable lasers only allow interrogation times of a few seconds, at present. Here we present a universal measurement protocol that overcomes this limitation. Engineered dynamic decoupling of laser phase noise allows any optical atomic clock with high signal-to-noise ratio in a single interrogation to reconstruct the laser's phase well beyond its coherence limit. A compound clock is then formed in combination with another optical clock of any type, allowing the latter to achieve significantly higher frequency stability than on its own. We demonstrate implementation of the protocol in a realistic proof-of-principle experiment with a phase reconstruction fidelity of 99 %. The protocol enables minute-long interrogation for the best ultrastable laser systems. Likewise, it can improve clock performance where less stable local oscillators are used, such as in transortable systems.

physics.atom-ph