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V. Korenivski

Publications and source records attributed to V. Korenivski.

At least 19 recordsLinked to original sources

Thermally-controlled interlayer exchange and field-induced anisotropy in synthetic antiferromagnets

Interlayer exchange in synthetic antiferromagnets incorporating thin paramagnetic spacers can be controlled thermally. The spacer provides an additional ferromagnetic contribution that renormalizes the otherwise temperature-independent interlayer coupling. As a result, the system shows antiferromagnetic alignment at high temperatures and ferromagnetic alignment at low temperatures. This behavior is observed in Fe(2 nm)/Cr(0.4 nm)/Fe$_{17.5}$Cr$_{82.5}$(0.9 nm)/Cr(0.4 nm)/Fe(2 nm) multilayers with the inner spacer Fe$_{17.5}$Cr$_{82.5}$ paramagnetic at and above room temperature, and is shown to be due to the spacer being significantly magnetically polarized on lowering the temperature toward its Curie point. Although the Fe layers lack intrinsic magnetocrystalline anisotropy, the magnetization reversal demonstrates a field-induced uniaxial anisotropy of antiferromagnetic character. The resulting reversal process resembles that of a metamagnet with a spin-flip transition.

cond-mat.mes-hall

Nonlinear spin dynamics across Néel phase transition in ferromagnetic/antiferromagnetic multilayers

We observe strongly nonlinear spin dynamics in ferro-/antiferro-magnetic multilayers, controlled by the number of bilayers in the system, layer thicknesses, as well as temperature, peaking in magnitude near the Néel point of the antiferromagnetic layers just above room temperature. Well above the Néel transition, the individual ferromagnetic layers are exchange decoupled and resonate independently. As the temperature is lowered toward the Néel point, the ferromagnetic proximity effect through the thin antiferromagnetic spacers transforms the system into a weakly coupled macrospin chain along the film normal, which exhibits pronounced standing spin-wave resonance modes, comparable in intensity to the uniform resonance in the ferromagnetic layers. These findings are supported by our micromagnetic simulations showing clear spin-wave profiles with precessional phase lag along the macrospin chain. Well below the Néel transition, the FeMn layers order strongly antiferromagnetically and exchange-pin the ferromagnetic layers to effectively make the multilayer one macrospin. The appearance and intensity of the high-frequency spin-wave modes can thus be conveniently controlled by thermal gating the multilayer. The nonlinearity in the microwave response of the demonstrated material can approach 100\%, large compared to nonlinear materials used in e.g. optics, with second-harmonic generation often at the single percentage level.

cond-mat.mes-hall

Spin waves in Co$_2$FeGe films

The dynamic magnetic properties of Full Heusler alloy thin films of Co$_2$FeGe, grown on MgO (001) substrates under different thermal conditions, were investigated. Brillouin light scattering and ferromagnetic resonance measurements revealed that depositing at room temperature followed by annealing at 300 deg C for 1 hour produces the best results for maximizing magnetization, exchange stiffness, and minimizing spin-dynamic dissipation in the films, which are desirable characteristics for high-speed spintronic devices. Additionally, strong hybridization of spin waves in the Damon-Eshbach geometry was observed, which is attractive for applications in magnonic signal processing circuits.

cond-mat.mtrl-sci

Ferromagnetic resonance in Y3AlFe4O12 garnets

Spin dynamics in Al-substituted yttrium iron garnets is investigated using broadband ferromagnetic resonance measurements in the temperature range T=200-360 K. Using the measured data, the resonance field and linewidth as well as their temperature dependence are determined, with implications for the uniformity and overall quality of the samples prepared via different chemical fabrication routes. These key parameters governing the spin dynamics in the material are important for its applications in high-speed spintronic and magnonic devices.

cond-mat.mtrl-sci

Fast barrier-free switching in synthetic antiferromagnets

We analytically solve the Landau-Lifshitz equations for the collective magnetization dynamics in a synthetic antiferromagnet (SAF) nanoparticle and uncover a regime of barrier-free switching under a short small-amplitude magnetic field pulse applied perpendicular to the SAF plane. We give examples of specific implementations for forming such low-power and ultra-fast switching pulses. For fully optical, resonant, barrier-free SAF switching we estimate the power per write operation to be $ \sim 100 $ pJ, 10-100 times smaller than for conventional quasi-static rotation, which should be attractive for memory applications.

cond-mat.mes-hall

Ultrafast inertia-free switching of double magnetic tunnel junctions

We investigate the switching of a magnetic nanoparticle comprising the middle free layer of a memory cell based on a double magnetic tunnel junction under the combined effect of spin-polarized current and weak on-chip magnetic field. We obtain the timing and amplitude parameters for the current and field pulses needed to achieve 100 ps range \emph{inertia-free} switching under \emph{least-power} dissipation. The considered method does not rely on the stochastics of thermal agitation of the magnetic nanoparticle typically accompanying spin-torque switching. The regime of ultimate switching speed-efficiency found in this work is promising for applications in high-performance nonvolatile memory.

cond-mat.mes-hall

Antiferromagnet-mediated interlayer exchange: hybridization versus proximity effect

We investigate the interlayer coupling between two thin ferromagnetic (F) films mediated by an antiferromagnetic (AF) spacer in F*/AF/F trilayers and show how it transitions between different regimes on changing the AF thickness. Employing layer-selective Kerr magnetometry and ferromagnetic-resonance techniques in a complementary manner enables us to distinguish between three functionally distinct regimes of such ferromagnetic interlayer coupling. The F layers are found to be individually and independently exchange-biased for thick FeMn spacers - the first regime of no interlayer F-F* coupling. F-F* coupling appears on decreasing the FeMn thickness below 9 nm. In this second regime found in structures with 6.0-9.0 nm thick FeMn spacers, the interlayer coupling exists only in a finite temperature interval just below the effective Néel temperature of the spacer, which is due to magnon-mediated exchange through the thermally softened antiferromagnetic spacer, vanishing at lower temperatures. The third regime, with FeMn thinner than 4 nm, is characterized by a much stronger interlayer coupling in the entire temperature interval, which is attributed to a magnetic-proximity induced ferromagnetic exchange. These experimental results, spanning the key geometrical parameters and thermal regimes of the F*/AF/F nanostructure, complemented by a comprehensive theoretical analysis, should broaden the understanding of the interlayer exchange in magnetic multilayers and potentially be useful for applications in spin-thermionics.

cond-mat.mes-hall

Oscillatory Exchange Bias Controlled by RKKY in Magnetic Multilayers

Ferromagnetic/antiferromagnetic bilayers are interfaced with normal metal/ferromagnetic bilayers to form F*/AF/N/F valves. The N-spacer thickness is chosen such that it mediates strong indirect exchange (RKKY) between the outer magnetic layers, which varies in strength/direction depending on the N thickness and in direction on switching F. The system exhibits a strong modulation of the F*/AF exchange bias, oscillating in strength syncronously with the oscillation in the interlayer RKKY exchange across the normal metal spacer. The effect is explained as due to a superposition taking place within the antiferromagnetic layer of the direct-exchange proximity effect from the F*/AF interface and the indirect RKKY exchange from F penetrating AF via N. The modulation, expressed via the strength of the F*/AF bias field, reaches 400% at the first RKKY peak.

cond-mat.mes-hall

Magnetocaloric effect in multilayers studied by membrane-based calorimetry

We study magnetic multilayers, incorporating dilute ferromagnetic spacers between strongly-ferromagnetic layers exhibiting a proximity-enhanced magnetocaloric effect. Using magnetometry and direct measurements of the adiabatic temperature change based on a nanomembrane-calorimetry, we find that the magnetocaloric effect in the studied multilayer is indeed enhanced compared to that in the bulk spacer material. We develop a phenomenological numerical model of the studied trilayer and find that a long-range exchange interaction through the weakly-ferromagnetic spacer is required to adequately describe the magnetic and magnetocaloric properties of the system.

cond-mat.mes-hall

Inverse magnetocaloric effect in synthetic antiferromagnets

The magnetocaloric effect in exchange-coupled synthetic-antiferromagnet multilayers is investigated experimentally and theoretically. We observe a temperature-controlled inversion of the effect, where the entropy increases on switching the individual ferromagnetic layers from anti-parallel to parallel alignment near their Curie point. Using a microscopic analytical model as well as numerical atomistic-spin simulations of the system, we explain the observed effect as due to the interplay between the intra- and inter-layer exchange interactions, which either add up or counteract to effectively modulate the Curie temperature of the dilute ferromagnetic layers. The proposed method of designing tunable, strongly magneto-caloric materials should be of interest for such applications as heat-assisted spintronics and magnetic refrigeration.

cond-mat.mes-hall

Higher-order ferromagnetic resonances in periodic arrays of synthetic-antiferromagnet nanodiscs

We investigate spin dynamics in nanodisc arrays of synthetic-antiferromagnets (SAF) made of Py/NiCu/Py trilayers, where the NiCu spacer undergoes a Curie transition at about 200 K. The observed ferromagnetic resonance spectra have three distinct resonance modes at room temperature, which are fully recreated in our micromagnetic simulations showing also how the intra-SAF asymmetry can be used to create and control the higher-order resonances in the structure. Below the Curie temperature of the spacer, the system effectively transitions into a single-layer nanodisc array with only two resonance modes. Our results show how multi-layering of nano-arrays can add tunable GHz functionality relevant for such rapidly developing fields as magnetic meta-materials, magnonic crystals, arrays of spin-torque oscillators and neuromorphic junctions.

cond-mat.mes-hall

Temperature and thickness dependent magnetostatic properties of [Fe/Py]/FeMn/Py multilayers

The magnetic properties of thin-film multilayers [Fe/Py]/FeMn/Py are investigated as a function of temperature and thickness of the antiferromagnetic FeMn spacer using SQUID magnetometry. The observed behavior differs substantially for the structures with 6-nm and 15-nm FeMn spacers. While the 15-nm-FeMn structure exhibits exchange pinning of both ferromagnetic layers in the entire measurement temperature interval from 5 to 300 K, the 6-nm-FeMn structure becomes exchange de-pinned in the vicinity of room temperature. The de-pinned state is characterized by a single hysteresis loop centered around zero field and having enhanced magnetic coercivity. The observed properties are explained in terms of finite-size effects and possibly ferromagnetic interlayer coupling through the thin antiferromagnetic spacer.

cond-mat.mtrl-sci

Effects of asymmetry in strongly coupled spin vortex pairs

Effects of magnetic asymmetry on strongly coupled spin-vortex pairs with parallel core polarization and antiparallel chirality in synthetic nanomagnets are investigated. This includes vortex-core length asymmetry, biasing field asymmetry, and pinning of one of the two vortex cores. Our experimental observations as well as analytical and micromagnetic modeling show how magnetic asymmetry can be used to differentiate magneto-resistively otherwise degenerate multiple stable states of a vortex pair. These results expand the knowledge base for spin vortex arrays in nanostructures and should be useful in light of the recent proposals on coding information into multiple topological spin states, such as single and multiple vortex core/chirality states.

cond-mat.mes-hall

Giant magnetocaloric effect driven by indirect exchange in magnetic multilayers

Indirect exchange coupling in magnetic multilayers, also known as the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, is known to be highly effective in controlling the interlayer alignment of the magnetization. This coupling is typically fixed at the stage of the multilayer fabrication and does not allow ex-situ control needed for device applications. It is highly desirable, in addition to the orientational control, to also control the magnitude of the intralayer magnetization, ideally switch it on/off by switching the relevant RKKY coupling. Here we demonstrate a magnetic multilayer material, incorporating thermally -- as well as field-controlled RKKY exchange, focused on to a dilute ferromagnetic alloy layer and driving it though it's Curie transition. Such on/off magnetization switching of a thin ferromagnet, performed repeatably and fully reproducibly within a low-field sweep, results in a giant magnetocaloric effect, with the estimated isothermal entropy change of -10 mJ/K cm^3 under an external field of ~10 mT, which greatly exceeds the performance of the best rare-earth based materials used in the adiabatic-demagnetization refrigeration systems.

cond-mat.mtrl-sci

Magnetic hysteresis in nanostructures with thermally-controlled RKKY coupling

Mechanisms of the recently demonstrated ex-situ thermal control of the indirect exchange coupling in magnetic multilayer are discussed for different designs of the spacer layer. Temperature-induced changes in the hysteresis of magnetization are shown to be associated with different types of competing interlayer exchange interactions. Theoretical analysis indicates that the measured step-like shape and hysteresis of the magnetization loops is due to local in-plane magnetic anisotropy of nano-crystallites within the strongly ferromagnetic films. Comparison of the experiment and theory is used to contrast the mechanisms of the magnetization switching based on the competition of (i) indirect (RKKY) and direct (non-RKKY) interlayer exchange interactions as well as (ii) indirect ferromagnetic and indirect antiferromagnetic (both of RKKY type) interlayer exchange.

cond-mat.mes-hall

Transient dynamics of strongly coupled spin vortex pairs: effects of anharmonicity and resonant excitation on inertial switching

Spin vortices in magnetic nanopillars are used as GHz oscillators, with frequency however essentially fixed in fabrication. We demonstrate a model system of a two-vortex nanopillar, in which the resonance frequency can be changed by an order of magnitude, without using high dc magnetic fields. The effect is due to switching between the two stable states of the vortex pair, which we show can be done with low-amplitude fields of sub-ns duration. We detail the relevant vortex-core dynamics and explain how field anharmonicity and phase control can be used to enhance the performance.

cond-mat.mes-hall

Resonant pinning spectroscopy with spin-vortex pairs

Vortex pairs in magnetic nanopillars with strongly coupled cores and pinning of one of the cores by a morphological defect, are used to perform resonant pinning spectroscopy, in which a microwave excitation applied to the nanopillar produces pinning or depinning of the cores only when the excitation is in resonance with the rotational or gyrational eigenmodes of the specific initial state of the core-core pair. The shift in the eigenmode frequencies between the pinned and depinned states is determined experimentally and explained theoretically, and illustrates the potential for multi-core spin-vortex memory with resonant writing of information on to various stable vortex pair states. Further, it is shown how the same resonant spectroscopy techniques applied to a vortex pair can be used as a sensitive nanoscale probe for characterizing morphological defects in magnetic films.

cond-mat.mes-hall

Chaotic dynamics in spin-vortex pairs

We report on spin-vortex pair dynamics measured at temperatures low enough to suppress stochastic core motion, thereby uncovering the highly non-linear intrinsic dynamics of the system. Our analysis shows that the decoupling of the two vortex cores is resonant and can be enhanced by dynamic chaos. We detail the regions of the relevant parameter space, in which the various mechanisms of the resonant core-core dynamics are activated. We show that the presence of chaos can reduce the thermally-induced spread in the switching time by up to two orders of magnitude.

cond-mat.mes-hall