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V. Nosov

Publications and source records attributed to V. Nosov.

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First observation of neutral bremsstrahlung electroluminescence in liquid argon

A recent discovery of additional mechanism of electroluminescence (EL) in noble gases due to the neutral bremsstrahlung (NBrS) effect led to a prediction that NBrS EL should be present in noble liquids as well. A theoretical model of NBrS EL in noble liquids was developed accordingly in the frameworks of Cohen-Lekner and Atrazhev. In this work, we confirm this prediction: for the first time, visible-range EL has been observed in liquid argon at electric fields reaching 90~kV/cm, using Gas Electron Multiplier (GEM) and Thick GEM (THGEM) structures. Absolute light yields of the EL were measured and found to be in excellent agreement with the theory, provided that the momentum-transfer cross section of electron scattering is used for calculation of NBrS cross section (instead of the energy-transfer one).

physics.ins-det

Possible evidence for the production of Ar$_2^{*-}$ metastable negative molecular ions in gaseous argon of two-phase detectors for dark matter searches

Our recent studies of electroluminescence (EL) properties in two-phase argon detectors for dark matter searches have revealed the presence of unusual delayed pulses in the EL signal in the form of two slow components with time constants of about 5 and 50 $μ$s. These components were shown to be present in the charge signal itself, which clearly indicates that drifting electrons are temporarily trapped on two states of metastable negative argon ions which have never been observed before. In this work, using the pressure dependence of the ratio of slow component contributions measured in experiment, it is deduced that these states are those of two types of metastable negative molecular ions, $\mathrm{Ar}_2^{*-}(b \ ^4Σ_u^-)$ and $\mathrm{Ar}_2^{*-}(a \ ^4Σ_g^+)$ for the higher and lower energy level respectively.

physics.ins-det

Unraveling the puzzle of slow components in gaseous argon of two-phase detectors for dark matter searches using Thick Gas Electron Multiplier

The effect of proportional electroluminescence (EL) is used to record the primary ionization signal (S2) in the gas phase of two-phase argon detectors for dark matter particle (WIMP) searches and low-energy neutrino experiments. Our previous studies of EL time properties revealed the presence of two unusual slow components in S2 signal of two-phase argon detector, with time constants of about 4-5 $μ$s and 50 $μ$s. The puzzle of slow components is that their time constants and contributions to the overall signal increase with electric field (starting from a certain threshold), which cannot be explained by any of the known mechanisms of photon and electron emission in two-phase media. There are indications that these slow components result from delayed electrons, temporarily trapped during their drift in the EL gap on metastable negative argon ions of yet unknown nature. In this work, this hypothesis is confirmed by studying the time properties of electroluminescence in a Thick Gas Electron Multiplier (THGEM) coupled to the EL gap of two-phase argon detector. In particular, an unusual slow component in EL signal, similar to that observed in the EL gap, was observed in THGEM itself. In addition, with the help of THGEM operated in electron multiplication mode, the slow component was observed directly in the charge signal, confirming the effect of trapped electrons in S2 signal. These results will help to unravel the puzzle of slow components in two-phase argon detectors and thus to understand the background in low-mass WIMP searches.

physics.ins-det

Puzzling time properties of proportional electroluminescence in two-phase argon detectors for dark matter searches

Proportional electroluminescence (EL) in noble gases is a physical process routinely used in two-phase (liquid-gas) detectors for low-energy astroparticle-physics experiments. In this work, the time properties of visible-light EL in two-phase argon detectors have been systematically studied for the first time. In particular, two unusual slow components in the EL signal, with their contributions and time constants increasing with electric field, were observed. This puzzling property is not expected in any of the known mechanisms of photon and electron emission in two-phase media. Time constants of these components is about 4-5 $μ$s and 50 $μ$s. In addition, a specific threshold behavior of the slow components was revealed: they emerged at a threshold in reduced electric field of 4.8 $\pm$ 0.2 Td regardless of the gas phase density, which is about 1 Td above the onset of standard (excimer) EL. There is a conspicuous similarity between this threshold and reduced field threshold of EL in NIR occurring via higher atomic excited states Ar$^{*}(3p^{5}4p)$. An unexpected temperature dependence of slow components was also observed: their contribution decreased with temperature, practically disappearing at room temperature. We show that the puzzling properties of slow components can be explained in the framework of hypothesis that these are produced in the charge signal itself due to trapping of drifting electrons on metastable negative argon ions.

physics.ins-det

Study of visible-light emission in pure and methane-doped liquid argon

In liquid argon TPCs for dark matter search and neutrino detection experiments, primary scintillation light is used as a prompt signal of particle scattering, being intensively produced in the vacuum ultraviolet (VUV) due to excimer emission mechanism. On the other hand, there were indications on the production of visible-light emission in liquid argon, albeit at a much lower intensity, the origin of which is still not clear. The closely related issue is visible-light emission in liquid argon doped with methane, the interest in which is due to the possible use in neutron veto detectors for those experiments. In this work we study in detail the properties of such light emission in pure liquid argon and its mixtures with methane. In particular, the absolute photon yield of visible-light emission in pure liquid argon was measured to be about 200 and 90 photon/MeV for X-rays and alpha particles respectively. In liquid argon doped with methane the photon yield dropped down significantly, by about an order of magnitude at a methane molar content varying from 0.01 to 1%, and then almost did not change when further increasing the methane content up to 10%.

physics.ins-det

Observation of primary scintillations in the visible range in liquid argon doped with methane

Neutron veto detector based on liquid scintillator containing hydrogen atoms is an integral part of any underground experiment for dark matter search. So far, a flammable mixture of liquid hydrocarbons was used as a liquid scintillator in such detectors. A safe alternative might be a liquid scintillator based on liquid argon doped with methane. In this work, we have studied the primary scintillations in pure liquid argon and its mixtures with methane, the CH4 content varying from 100 ppm to 5%. The primary scintillations have for the first time been observed in liquid argon doped with methane, in the visible and near infrared range, and their relative light yields have been measured as a function of the CH4 content.

physics.ins-det

Neutral bremsstrahlung in two-phase argon electroluminescence: further studies and possible applications

We further study the effect of neutral bremsstrahlung (NBrS) in two-phase argon electroluminescence (EL), revealed recently in [1]. The absolute EL yield due to NBrS effect, in the visible and NIR range, was remeasured in pure gaseous argon in the two-phase mode, using a two-phase detector with EL gap read out directly by cryogenic PMTs and SiPMs. Possible applications of the NBrS effect in detection science are discussed, including those in two-phase dark matter detectors.

physics.ins-det

Revealing neutral bremsstrahlung in two-phase argon electroluminescence

Proportional electroluminescence (EL) in noble gases has long been used in two-phase detectors for dark matter search, to record ionization signals induced by particle scattering in the noble-gas liquid (S2 signals). Until recently, it was believed that proportional electroluminescence was fully due to VUV emission of noble gas excimers produced in atomic collisions with excited atoms, the latter being in turn produced by drifting electrons. In this work we consider an additional mechanism of proportional electroluminescence, namely that of bremsstrahlung of drifting electrons scattered on neutral atoms (so-called neutral bremsstrahlung); it is systemically studied here both theoretically and experimentally. In particular, the absolute EL yield has for the first time been measured in pure gaseous argon in the two-phase mode, using a dedicated two-phase detector with EL gap optically read out by cryogenic PMTs and SiPMs. We show that the neutral bremsstrahlung effect can explain two intriguing observations in EL radiation: that of the substantial contribution of the non-VUV spectral component, extending from the UV to NIR, and that of the photon emission at lower electric fields, below the Ar excitation threshold. Possible applications of neutral bremsstrahlung effect in two-phase dark matter detectors are discussed.

physics.ins-det

Characterization of a 109Cd gamma-ray source for the two-phase argon detector

At present, a two-phase argon detector is being developed in our laboratory for dark matter search and low-energy neutrino experiments. To calibrate its energy scale a $^{109}$Cd gamma-ray source was used. In this work a detailed emission spectrum of the $^{109}$Cd source was measured using YAP:Ce scintillator and high-purity germanium (HPGe) detectors. It is shown that the $^{109}$Cd source, equipped with a W substrate and a Cu filter, can provide a complete set of gamma-ray lines, ranging from 8 to 90 keV, for the energy calibration of two-phase detectors. These measurements allowed us to successfully quantify the shape of the amplitude spectra observed in the two-phase argon detector when irradiated with the $^{109}$Cd source.

physics.ins-det

Measurement of the ionization yield of nuclear recoils in liquid argon using a two-phase detector with electroluminescence gap

A measurement of ionization yields in noble-gas liquids is relevant to the energy calibration of nuclear recoil detectors for dark matter search and coherent neutrino-nucleus scattering experiments. In this work we further study the ionization yield of nuclear recoils in liquid Ar, using a two-phase detector with an electroluminescence gap and DD neutron generator. The ionization yields of nuclear recoils in liquid Ar were measured at 233 keV and electric fields of 0.56 and 0.62 kV/cm; their values amounted to 5.9 $\pm$ 0.8 and 7.4 $\pm$ 1 e$^-$/keV, respectively. The characteristic dependences of the ionization yield on energy and electric field were determined, while comparing the results obtained to those at lower energies and higher fields.

astro-ph.IM

Further studies of proportional electroluminescence in two-phase argon

The study of proportional electroluminescence in two-phase argon is relevant in the field of noble-gas liquid detectors for dark matter search and low-energy neutrino experiments. In this work, we continued to study proportional electroluminescence (EL) in two-phase argon doped with a minor (9 ppm) admixture of nitrogen, in the VUV, UV and visible spectral ranges. We confirmed the effect of enhancement of the EL yield, as well as the presence of non-VUV component in addition to that of VUV, in proportional electroluminescence in two-phase Ar. On the other hand, the contribution of non-VUV component determined here within the model of N2 emission in the UV, turned out to be insufficient to explain the EL yield enhancement effect. Accordingly, the problem of proportional electroluminescence in two-phase Ar remains unresolved.

astro-ph.IM

Study of cryogenic photomultiplier tubes for the future two-phase cryogenic avalanche detector

We report the results of a characterization study of several types of cryogenic photomultipliers manufactured by Hamamatsu Photonics and intended for operation in liquid Ar conditions, namely: compact 2-inch R6041-506MOD tubes, 3-inch R11065-10 and R11065-MOD tubes for operation in liquid Ar and 3-inch R11410-20 tubes originally designed for operation in liquid Xe. These types of PMT are proposed for installation into the future two-phase cryogenic avalanche detector that is developed in the Laboratory of Cosmology and Particle Physics of the Novosibirsk State University jointly with the Budker Institute of Nuclear Physics. Eight R11065 PMTs and seven R11410-20 tubes were tested and all demonstrated excellent performance in liquid Ar in terms of gain and relative single electron efficiency. All 3-inch PMTs showed a maximal gain in liquid Ar above 5x10^6 and relative single electron efficiency higher than 95%. Compact R6041-506MOD tubes have dynode system different from that of the 3-inch photomultipliers and thus their single electron energy resolution and relative efficiency is much worse than that of 3-inch tubes. From 21 2-inch PMTs only 12 tubes were selected with acceptable, i.e. higher than 75%, relative single electron efficiency and the maximal gain higher than 5x10^6. However, these PMTs are very attractive because they are the only compact type of tubes that can operate in liquid Ar.

astro-ph.IM

Two-phase Cryogenic Avalanche Detector with electroluminescence gap operated in argon doped with nitrogen

A two-phase Cryogenic Avalanche Detector (CRAD) with electroluminescence (EL) gap, operated in argon doped with a minor (49$\pm$7 ppm) admixture of nitrogen, has been studied. The EL gap was optically read out using cryogenic PMTs located on the perimeter of the gap. We present the results of the measurements of the N$_2$ content, detector sensitivity to X-ray-induced signals, EL gap yield and electron lifetime in the liquid. The detector sensitivity, at a drift field in liquid Ar of 0.6 kV/cm, was measured to be 9 and 16 photoelectrons recorded at the PMTs per keV of deposited energy at 23 and 88 keV respectively. Such two-phase detectors, with enhanced sensitivity to the S2 (ionization-induced) signal, are relevant in the field of argon detectors for dark matter search and low energy neutrino detection.

physics.ins-det

Proportional electroluminescence in two-phase argon and its relevance to rare-event experiments

Proportional electroluminescence (EL) in gaseous Ar has for the first time been systematically studied in the two-phase mode, at 87 K and 1.00 atm. Liquid argon had a minor (56 ppm) admixture of nitrogen, which allowed to understand, inter alia, the effect of N2 doping on the EL mechanism in rare-event experiments using two-phase Ar detectors. The measurements were performed in a two-phase Cryogenic Avalanche Detector (CRAD) with EL gap located directly above the liquid-gas interface. The EL gap was optically read out in the Vacuum Ultraviolet (VUV), near 128 nm (Ar excimer emission), and in the near Ultraviolet (UV), at 300-450 nm (N2 Second Positive System emission), via cryogenic PMTs and a Geiger-mode APD (GAPD). Proportional electroluminescence was measured to have an amplification parameter of 109+-10 photons per drifting electron per kV overall in the VUV and UV, of which 51+-6% were emitted in the UV. The measured EL threshold, at an electric field of 3.7+-0.2 kV/cm, was in accordance with that predicted by the theory. The latter result is particularly relevant to DarkSide and SCENE dark matter search-related experiments, where the operation electric field was thereby on the verge of appearance of the S2 (ionization-induced) signal. The results obtained pave the way to the development of N2-doped two-phase Ar detectors with enhanced sensitivity to the S2 signal.

physics.ins-det

Characterization of photo-multiplier tubes for the Cryogenic Avalanche Detector

New Cryogenic Avalanche Detector (CRAD) with ultimate sensitivity, that will be able to detect one primary electron released in the cryogenic liquid, is under development in the Laboratory of Cosmology and Particle Physics of the Novosibirsk State University jointly with the Budker Institute of Nuclear Physics. The CRAD will use two sets of cryogenic PMTs in order to get trigger signal either from primary scintillations in liquid Ar or from secondary scintillations in high field gap above the liquid. Two types of cryogenic PMTs produced by Hamamatsu Photonics were tested and the results are presented in this paper. Low background 3 inch PMT R11065- 10 demonstrated excellent performance according to its specifications provided by the producer. The gain measured with single electron response (SER) in liquid Ar reached 10^7, dark count rate rate did not exceed 300 Hz and pulse height resolution of single electron signals was close to 50%(FWHM). However, two R11065-10 PMTs out of 7 tested stopped functioning after several tens minutes of operation immersed completely into liquid Ar. The remaining 5 devices and one R11065-MOD were operated successfully for several hours each with all the parameters according to the producer specifications. Compact 2 inch PMT R6041-506-MOD with metal-channel dynode structure is a candidate for side wall PMT system that will look at electroluminescence in high field region above liquid. Four of these PMTs were tested in liquid Ar and demonstrated gain up to 2x10^7, dark count rate rate below 100 Hz and pulse height resolution of single electron signals of about 110% (FWHM).

physics.ins-det