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Vikram V. Deshpande

Publications and source records attributed to Vikram V. Deshpande.

21 records · Page 2Linked to original sources

Spatially-Resolved Temperature Measurements of Electrically-Heated Carbon Nanotubes

Spatially-resolved Raman spectra of individual pristine suspended carbon nanotubes are observed under electrical heating. The Raman G+ and G- bands show unequal temperature profiles. The preferential heating is more pronounced in short nanotubes (2 um) than in long nanotubes (5 um). These results are understood in terms of the decay and thermalization of non-equilibrium phonons, revealing the mechanism of thermal transport in these devices. The measurements also enable a direct estimate of thermal contact resistances and the spatial variation of thermal conductivity.

cond-mat.mes-hall↗

Direct Observation of Born-Oppenheimer Approximation Breakdown in Carbon Nanotubes

Raman spectra and electrical conductance of individual, pristine, suspended, metallic single-walled carbon nanotubes are measured under applied gate potentials. The G- band is observed to downshift with small applied gate voltages, with the minima occurring at EF = +/- 1/2 Ephonon, contrary to adiabatic predictions. A subsequent upshift in the Raman frequency at higher gate voltages results in a 'W'-shaped Raman shift profile that agrees well with a non-adiabatic phonon renormalization model. This behavior constitutes the first experimental confirmation of the theoretically predicted breakdown of the Born-Oppenheimer approximation in individual single walled carbon nanotubes.

cond-mat.mes-hall↗

The One-Dimensional Wigner Crystal in Carbon Nanotubes

Electron-electron interactions strongly affect the behavior of low-dimensional systems. In one dimension (1D), arbitrarily weak interactions qualitatively alter the ground state producing a Luttinger liquid (LL) which has now been observed in a number of experimental systems. Interactions are even more important at low carrier density, and in the limit when the long-ranged Coulomb potential is the dominant energy scale, the electron liquid is expected to become a periodically ordered solid known as the Wigner crystal. In 1D, the Wigner crystal has been predicted to exhibit novel spin and magnetic properties not present in an ordinary LL. However, despite recent progress in coupled quantum wires, unambiguous experimental demonstration of this state has not been possible due to the role of disorder. Here, we demonstrate using low-temperature single-electron transport spectroscopy that a hole gas in low-disorder carbon nanotubes with a band gap is a realization of the 1D Wigner crystal. Our observation can lead to unprecedented control over the behavior of the spatially separated system of carriers, and could be used to realize solid state quantum computing with long coherence times.

cond-mat.str-el↗