arXiv subjects

Violet Williams

Publications and source records attributed to Violet Williams.

5 recordsLinked to original sources

arXiv2026

Field-induced first order transitions and phase coexistence in the Kitaev quantum spin liquid candidate BaCo2(AsO4)2

BaCo2(AsO4)2 (BCAO) is an insulating Kitaev quantum spin liquid candidate with a rich low-temperature phase diagram. Below 5 K, it exhibits double-zigzag magnetic order. Upon application of an in-plane magnetic field, the magnetic structure first transforms into an up-up-down (UUD) state near 0.12 T and then enters a fully spin-polarized ferromagnetic (FM) state near 0.5 T. In the narrow field regime close to the polarized phase, a finite residual thermal conductivity has been reported, suggesting a possible field-induced quantum spin liquid phase. Using neutron scattering, we show that the field-induced double-zigzag-to-UUD transition near 0.15 T is accompanied by the emergence of a cluster of localized UUD spin excitations that coexist with conventional spin waves. Upon further increasing field, BCAO undergoes a first-order UUD-to-FM transition with coexistence of UUD and FM phases, accompanied by a sharp response in the spin Seebeck coefficient. These results do not support a quantum spin liquid scenario near the UUD-to-FM critical field. Instead, modeling indicates that the broad excitations arise from bound spin-flip pairs, while a low-lying dispersive branch near the FM phase boundary carries the same sign of magnetization as the FM order. These excitations naturally account for the observed sign of the spin Seebeck response and are likely relevant to the thermal conductivity near the critical field.

cond-mat.str-el↗

arXiv2025

Chemical potential of magnon polarons

Using a rotationally invariant formulation of spin-lattice coupling, we derive a rigorous definition of the chemical potential for magnon-polaron quasiparticles in collinear ferromagnets (FMs) and antiferromagnets (AFMs), valid when magnetoelastic scattering equilibrates magnons and acoustic phonons on timescales much shorter than those associated with quasiparticle-nonconserving relaxation processes. While our microscopic framework applies to generic magnon-phonon interactions, here we focus on high-symmetry crystals where the two transverse acoustic modes form a degenerate doublet. This doublet can combine into circularly polarized phonons, making the chiral selectivity of the coupling manifest: the FM magnon mode hybridizes only with the co-rotating phonon, whereas in collinear AFMs each magnon branch of opposite handedness couples to the phonon of the same chirality. We show that, in both FM and AFM systems, the nonequilibrium magnon-polaron gas is governed by a single chemical potential conjugate to the conserved axial angular momentum. In FMs, the two hybrid branches in the co-rotating sector share this chemical potential, weighted by their magnonic fractions; in AFMs, the four magnon-polaron branches split into two chiral sectors that carry opposite angular momenta and couple with opposite sign to the same chemical potential. Building on this microscopic thermodynamic framework, we formulate a Boltzmann transport theory for magnon-polarons and derive compact expressions for angular-momentum and heat currents that interpolate continuously to the decoupled regime and reproduce the phenomenological magnon-polaron transport framework underlying previous spin Seebeck analyses.

cond-mat.mes-hall↗

arXiv2025

Generating single- and many-body quantum magnonic states

The growing interest in quantum magnonics is driving the development of advanced techniques for generating, controlling, and detecting non-classical magnonic states. Here, we explore the potential of an ensemble of solid-state spin defects coupled to a shared magnetic bath as a source of such states. We establish a theoretical framework to characterize the quantum correlations among magnons emitted by the ensemble into the bath and investigate how these correlations depend on experimentally tunable parameters. Our findings show that the emitted magnons retain the quantum correlations inherent to the solid-state emitters, paving the way for the deterministic generation of quantum many-body magnonic states.

cond-mat.mes-hall↗

arXiv2025

Angular Momentum Fluctuations in the Phonon Vacuum of Symmetric Crystals

Although time-reversal and inversion symmetry constrain the angular momentum of each phonon mode to vanish, we show that the vacuum state of crystals with such symmetries can nevertheless exhibit finite angular momentum fluctuations, which persist at finite temperature. These fluctuations arise from quantum coherence between nondegenerate modes with noncollinear polarizations and are encoded in the off-diagonal components of the angular momentum operator. Their origin lies in the noncommutativity between the phonon Hamiltonian and angular momentum, which enables time-dependent rotational dynamics even in symmetric vacua. Using a minimal model, we provide an intuitive picture of this phenomenon in terms of beating between linearly polarized modes, which generates a finite instantaneous angular momentum while remaining symmetry-forbidden in the mean. We further show that these vacuum fluctuations give rise to distinct finite-frequency spectral signatures and outline a concrete route for their detection using time-resolved spectroscopic probes sensitive to lattice polarization and symmetry. Our results identify a previously unexplored regime of lattice dynamics, revealing that even the symmetric phonon vacuum can harbor structured, dynamical angular-momentum correlations.

cond-mat.mtrl-sci↗

arXiv2023

Layer-dependent magnetism and spin fluctuations in atomically thin van der Waals magnet CrPS4

van der Waals (vdW) magnets, an emerging family of two-dimensional (2D) materials, have received tremendous attention due to their rich fundamental physics and significant potential for cutting-edge technological applications. In contrast to the conventional bulk counterparts, vdW magnets exhibit significant tunability of local material properties, such as stacking engineered interlayer coupling and layer-number dependent magnetic and electronic interactions, which promise to deliver previously unavailable merits to develop multifunctional microelectronic devices. As a further ingredient of this emerging topic, here we report nanoscale quantum sensing and imaging of atomically thin vdW magnet chromium thiophosphate CrPS4, revealing its characteristic layer-dependent 2D static magnetism and dynamic spin fluctuations. We also show a large tunneling magnetoresistance in CrPS4-based spin filter vdW heterostructures. The excellent material stability, robust strategy against environmental degradation, in combination with tailored magnetic properties highlight the potential of CrPS4 in developing state-of-the-art 2D spintronic devices for next-generation information technologies.

cond-mat.mes-hall↗