arXiv subjects

Vittorio Pellegrini

Publications and source records attributed to Vittorio Pellegrini.

At least 55 records · Page 3Linked to original sources

arXiv2013

Artificial graphene as a tunable Dirac material

Artificial honeycomb lattices offer a tunable platform to study massless Dirac quasiparticles and their topological and correlated phases. Here we review recent progress in the design and fabrication of such synthetic structures focusing on nanopatterning of two-dimensional electron gases in semiconductors, molecule-by-molecule assembly by scanning probe methods, and optical trapping of ultracold atoms in crystals of light. We also discuss photonic crystals with Dirac cone dispersion and topologically protected edge states. We emphasize how the interplay between single-particle band structure engineering and cooperative effects leads to spectacular manifestations in tunneling and optical spectroscopies.

cond-mat.mes-hall↗

arXiv2012

Evidence of inter-layer interaction in magneto-luminescence spectra of electron bilayers

Magneto-luminescence studies in electron bilayers reveal the hallmarks of the even-denominator and other quantum Hall states in the intensities and energies of the inter-band optical recombination lines. In the presence of a small tunneling gap between the layers the magneto-optical emission from the lowest anti-symmetric subband, not populated in a single-electron picture, displays maxima at filling factors 1 and 2/3. These findings uncover a loss of pseudospin polarization, where the pseudospin describes the layer index degree of freedom, that is linked to an anomalous population of the anti-symmetric level due to excitonic correlations. The results demonstrate a new realm to probe the impact of inter-layer Coulomb interaction in quantum Hall bilayers.

cond-mat.mes-hall↗

arXiv2012

Prospects for hydrogen storage in graphene

Hydrogen-based fuel cells are promising solutions for the efficient and clean delivery of electricity. Since hydrogen is an energy carrier, a key step for the development of a reliable hydrogen-based technology requires solving the issue of storage and transport of hydrogen. Several proposals based on the design of advanced materials such as metal hydrides and carbon structures have been made to overcome the limitations of the conventional solution of compressing or liquefying hydrogen in tanks. Nevertheless none of these systems are currently offering the required performances in terms of hydrogen storage capacity and control of adsorption/desorption processes. Therefore the problem of hydrogen storage remains so far unsolved and it continues to represent a significant bottleneck to the advancement and proliferation of fuel cell and hydrogen technologies. Recently, however, several studies on graphene, the one-atom-thick membrane of carbon atoms packed in a honeycomb lattice, have highlighted the potentialities of this material for hydrogen storage and raise new hopes for the development of an efficient solid-state hydrogen storage device. Here we review on-going efforts and studies on functionalized and nanostructured graphene for hydrogen storage and suggest possible developments for efficient storage/release of hydrogen at ambient conditions.

cond-mat.mes-hall↗

arXiv2012

Plasmons and Coulomb drag in Dirac/Schroedinger hybrid electron systems

We show that the plasmon spectrum of an ordinary two-dimensional electron gas (2DEG) hosted in a GaAs heterostructure is significantly modified when a graphene sheet is placed on the surface of the semiconductor in close proximity to the 2DEG. Long-range Coulomb interactions between massive electrons and massless Dirac fermions lead to a new set of optical and acoustic intra-subband plasmons. Here we compute the dispersion of these coupled modes within the Random Phase Approximation, providing analytical expressions in the long-wavelength limit that shed light on their dependence on the Dirac velocity and Dirac-fermion density. We also evaluate the resistivity in a Coulomb-drag transport setup. These Dirac/Schroedinger hybrid electron systems are experimentally feasible and open new research opportunities for fundamental studies of electron-electron interaction effects in two spatial dimensions.

cond-mat.mes-hall↗

arXiv2012

Internal field induced enhancement and effect of resonance in Raman scattering of InAs nanowires

An internal field induced resonant intensity enhancement of Raman scattering of phonon excitations in InAs nanowires is reported. The experimental observation is in good agreement with the simulated results for the scattering of light under varying incident wavelengths, originating from the enhanced internal electric field in an infinite dielectric cylinder. Our analysis demonstrates the combined effect of the first higher lying direct band gap energy (E1) and the refractive index of the InAs nanowires in the internal field induced resonant Raman scattering. Furthermore, the difference in the relative contribution of electro-optic effect and deformation potential in Raman scattering of nanowires and bulk InAs over a range of excitation energies is discussed by comparing the intensity ratio of their LO and TO phonon modes.

cond-mat.mes-hall↗

arXiv2012

Raman Spectroscopy of magneto-phonon resonances in Graphene and Graphite

The magneto-phonon resonance or MPR occurs in semiconductor materials when the energy spacing between Landau levels is continuously tuned to cross the energy of an optical phonon mode. MPRs have been largely explored in bulk semiconductors, in two-dimensional systems and in quantum dots. Recently there has been significant interest in the MPR interactions of the Dirac fermion magnetoexcitons in graphene, and a rich splitting and anti-crossing phenomena of the even parity E2g long wavelength optical phonon mode have been theoretically proposed and experimentally observed. The MPR has been found to crucially depend on disorder in the graphene layer. This is a feature that creates new venues for the study of interplays between disorder and interactions in the atomic layers. We review here the fundamentals of MRP in graphene and the experimental Raman scattering works that have led to the observation of these phenomena in graphene and graphite.

cond-mat.mtrl-sci↗

arXiv2011

Raman sensitivity to crystal structure in InAs nanowires

We report a combined electron transmission and Raman spectroscopy study of InAs nanowires. We demonstrate that the temperature dependent behavior of optical phonon energies can be used to determine the relative wurtzite fraction in the InAs nanowires. Furthermore, we propose that the interfacial strain between zincblende and wurtzite phases along the length of the wires manifests in the temperature-evolution of the phonon linewidths. From these studies, temperature-dependent Raman measurements emerge has a non-invasive method to study polytypism in such nanowires.

cond-mat.mes-hall↗

arXiv2011

Controlled coupling of spin-resolved quantum Hall edge states

Topologically-protected edge states are dissipationless conducting surface states immune to impurity scattering and geometrical defects that occur in electronic systems characterized by a bulk insulating gap. One example can be found in a two-dimensional electron gas (2DEG) under high magnetic field in the quantum Hall regime. Based on the coherent control of the coupling between these protected states, several theoretical proposals for the implementation of information processing architectures were proposed. Here we introduce and experimentally demonstrate a new method that allows us to controllably couple co-propagating spin-resolved edge states of a QH insulator. The scheme exploits a spatially-periodic in-plane magnetic field that is created by an array of Cobalt nano-magnets placed at the boundary of the 2DEG. A maximum charge/spin transfer of about 28% is achieved at 250 mK. This result may open the way to the realization of scalable quantum-information architectures exploiting the spin degree of freedom of topologically-protected states.

cond-mat.mes-hall↗

arXiv2011

Probing the spin states of three interacting electrons in quantum dots

We observe a low-lying sharp spin mode of three interacting electrons in an array of nanofabricated AlGaAs/GaAs quantum dots by means of resonant inelastic light scattering. The finding is enabled by a suppression of the inhomogeneous contribution to the excitation spectra obtained by reducing the number of optically-probed quantum dots. Supported by configuration-interaction calculations we argue that the observed spin mode offers a direct probe of Stoner ferromagnetism in the simplest case of three interacting spin one-half fermions.

cond-mat.mes-hall↗

arXiv2011

Self-assembly and electron-beam-induced direct etching of suspended graphene nanostructures

We report on suspended single-layer graphene deposition by a transfer-printing approach based on polydimethylsiloxane stamps. The transfer printing method allows the exfoliation of graphite flakes from a bulk graphite sample and their residue-free deposition on a silicon dioxide substrate. This deposition system creates a blistered graphene surface due to strain induced by the transfer process itself. Single-layer-graphene deposition and its "blistering" on the substrate are demonstrated by a combination of Raman spectroscopy, scanning electron microscopy and atomic-force microscopy measurements. Finally, we demonstrate that blister-like suspended graphene are self-supporting single-layer structures and can be flattened by employing a spatially-resolved direct-lithography technique based on electron-beam induced etching.

cond-mat.mes-hall↗

arXiv2011

Quantum dot spectroscopy of proximity-induced superconductivity in a two-dimensional electron gas

We report the realization of a hybrid superconductor-quantum dot device by means of top-down nanofabrication starting from a two dimensional electron gas in a InGaAs/InAlAs semiconductor heterostructure. The quantum dot is defined by electrostatic gates placed within the normal region of a planar Nb-InGaAs quantum well-Nb junction. Measurements in the regime of strong Coulomb blockade as well as cotunneling spectroscopy allow to directly probe the proximity-induced energy gap in a ballistic two-dimensional electron gas coupled to superconductors.

cond-mat.mes-hall↗

arXiv2011

Proximity effect in a two dimensional electron gas probed with a lateral quantum dot

We report low-temperature transport measurements performed on a planar Nb-InGaAs-Nb proximity Josephson junction hosting a gate-defined lateral quantum dot in the weak-link. We first study quasiparticle and Josephson transport through the open junction, when all gates are grounded. When the quantum dot is defined in the normal region by electrostatic depletion, cotunneling spectroscopy allows us to directly probe the energy gap induced in the two dimensional electron gas. Our data show good qualitative agreement with a model describing resonant tunneling through an Anderson impurity connected to superconducting electrodes. These results demonstrate the feasibility of top-gated nanodevices based on a two-dimensional electron gas coupled to a superconductor.

cond-mat.mes-hall↗

arXiv2011

Reversible hydrogen storage by controlled buckling of graphene layers

We propose a multi-layer graphene-based device in which storage and release of atomic hydrogen is obtained by exploiting and controlling the corrugation of the layers. The proposal is based on density-functional simulations of hydrogen chemisorption on graphene with superimposed corrugation. We report a tunability of the binding energies of more than 2 eV by changing the sheet out-of-plane deformation up to \pm 0.2 Å, the convex regions allocating the energetically favored hydrogen binding sites. We discuss an optimized process of curvature inversion that can lead to efficient and fast hydrogen release and H2 formation. Our corrugated graphene device can potentially reach gravimetric capacities of ~8 wt % and reversibly store and release atomic hydrogen by application of external fields without the need of modifying temperature and pressure.

cond-mat.mes-hall↗

arXiv2010

Correlated electrons in optically-tunable quantum dots: Building an electron dimer molecule

We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we identify the inter-shell excitations in the one-electron regime and the distinct spin and charge modes in the interacting few-body configuration. In the case of two electrons a comparison with configuration-interaction calculations allows us to link the observed excitations with the breathing mode of the molecular dimer and to determine the singlet-triplet energy splitting.

cond-mat.mes-hall↗

arXiv2009

Electronic structure and Peierls instability in graphene nanoribbons sculpted in graphane

Graphene nanoribbons are semiconductor nanostructures with great potentials in nanoelectronics. Their realization particularly with small lateral dimensions below a few nanometers, however, remains challenging. Here we theoretically analyze zig-zag graphene nanoribbons created in a graphane substrate (a fully saturated two-dimensional hydrocarbon with formula CH) and predict that they are stable down to the limit of a single carbon chain. We exploit density functional theory with B3LYP functional that accurately treats exchange and correlation effects and demonstrate that at small widths below a few chains these zig-zag nanoribbons are semiconducting due to the Peierls instability similar to the case of polyacetylene. Graphene nanoribbons in graphane might represent a viable strategy for the realization of ultra-narrow semiconducting graphene nanoribbons with regular edges and controlled chemical termination and open the way for the exploration of the competition between Peierls distortion and spin effects in artificial one-dimensional carbon structures.

cond-mat.mes-hall↗

arXiv2009

A Phase Diagram for Quantum Hall Bilayers with Strong Inter-layer Correlation

Inter-layer excitonic coherence in a quantum Hall bilayer with negligible tunneling is monitored by measurements of low-lying spin excitations. At $ν_T =1$ new quasiparticle excitations are observed above a transition temperature revealing a competing metallic phase. For magnetic fields above an onset Zeeman energy this metallic phase has full spin polarization. A phase diagram in the parameter space of temperature and Zeeman energy reveals that the transition temperature increases at higher fields. This unexpected result suggests intriguing impacts of spin polarization in the highly correlated phases.

cond-mat.other↗

arXiv2009

Tuning non-linear charge transport between integer and fractional quantum Hall states

Controllable point junctions between different quantum Hall phases are a necessary building block for the development of mesoscopic circuits based on fractionally-charged quasiparticles. We demonstrate how particle-hole duality can be exploited to realize such point-contact junctions. We show an implementation for the case filling factors $ν=1$ and $ν^*\le1$ in which both the fractional filling $ν^*$ and the coupling strength can be finely and independently tuned. A peculiar crossover from insulating to conducting behavior as $ν^*$ goes from 1/3 to 1 is observed. These results highlight the key role played on inter-edge tunneling by local charge depletion at the point contact.

cond-mat.mes-hall↗

arXiv2009

A molecular state of correlated electrons in a quantum dot

Correlation among particles in finite quantum systems leads to complex behaviour and novel states of matter. One remarkable example is predicted to occur in a semiconductor quantum dot (QD) where at vanishing density the Coulomb correlation among electrons rigidly fixes their relative position as that of the nuclei in a molecule. In this limit, the neutral few-body excitations are roto-vibrations, which have either rigid-rotor or relative-motion character. In the weak-correlation regime, on the contrary, the Coriolis force mixes rotational and vibrational motions. Here we report evidence of roto-vibrational modes of an electron molecular state at densities for which electron localization is not yet fully achieved. We probe these collective modes by inelastic light scattering in QDs containing four electrons. Spectra of low-lying excitations associated to changes of the relative-motion wave function -the analogues of the vibration modes of a conventional molecule- do not depend on the rotational state represented by the total angular momentum. Theoretical simulations via the configuration-interaction (CI) method are in agreement with the observed roto-vibrational modes and indicate that such molecular excitations develop at the onset of short-range correlation.

cond-mat.mes-hall↗