Searcharxiv⌕ Search

arXiv subjects

Vladimir M. Shalaev

Publications and source records attributed to Vladimir M. Shalaev.

At least 91 records · Page 5Linked to original sources

Colloidal Plasmonic Titanium Nitride Nanoparticles: Properties and Applications

Optical properties of colloidal plasmonic titanium nitride nanoparticles are examined with an eye on their photothermal via transmission electron microscopy and optical transmittance measurements. Single crystal titanium nitride cubic nanoparticles with an average size of 50 nm exhibit plasmon resonance in the biological transparency window. With dimensions optimized for efficient cellular uptake, the nanoparticles demonstrate a high photothermal conversion efficiency. A self-passivating native oxide at the surface of the nanoparticles provides an additional degree of freedom for surface functionalization.

physics.optics↗

Ultra-compact modulators based on novel CMOS-compatible plasmonic materials

We propose several planar layouts of ultra-compact plasmonic waveguide modulators that utilize alternative CMOS-compatible materials. The modulation is efficiently achieved by tuning the carrier concentration in a transparent conducting oxide layer, thereby tuning the waveguide either in plasmonic resonance or off-resonance. Resonance significantly increases the absorption coefficient of the plasmonic waveguide, which enables larger modulation depth. We show that an extinction ratio of 86 dB/um can be achieved, allowing for a 3-dB modulation depth in less than one micron at the telecommunication wavelength. Our multilayer structures can potentially be integrated with existing plasmonic and photonic waveguides as well as novel semiconductor-based hybrid photonic/electronic circuits.

physics.optics↗

Broadband Transformation Optics Devices

Recently we have suggested that two-dimensional broadband transformation optics devices based on metamaterial designs may be built using tapered waveguides. Here we review application of this principle to broadband electromagnetic cloaking, trapped rainbow, and novel microscopy devices.

physics.optics↗

Trapped Rainbow Techniques for Spectroscopy on a Chip and Fluorescence Enhancement

We report on the experimental demonstration of the broadband "trapped rainbow" in the visible range using arrays of adiabatically tapered optical nano waveguides. Being a distinct case of the slow light phenomenon, the trapped rainbow effect could be applied to optical signal processing, and sensing in such applications as spectroscopy on a chip, and to providing enhanced light-matter interactions. As an example of the latter applications, we have fabricated a large area array of tapered nano-waveguides, which exhibit broadband "trapped rainbow" effect. Considerable fluorescence enhancement due to slow light behavior in the array has been observed.

physics.optics↗

Negative refraction in Al:ZnO/ZnO metamaterial in the near-infrared

Noble metals such as gold and silver are the primary metallic building blocks of metamaterial devices. Making subwavelength-sized structural elements from these metals seriously limits the optical performance of a device, however, and complicates the manufacturing process of nearly all metamaterial devices in the optical wavelength range. As an alternative to noble metals, we propose to use heavily-doped oxide semiconductors that offer both functional and fabrication advantages in the near-infrared. In this letter, we report an experimental demonstration of negative refraction in a near-infrared metamaterial device that is designed and fabricated using aluminum-doped zinc oxide.

physics.optics↗

Merging Nonlinear Optics and Negative-Index Metamaterials

The extraordinary properties of nonlinear optical propagation processes in double-domain positive/negative index metamaterials are reviewed. These processes include second harmonic generation, three- and four-wave frequency mixing, and optical parametric amplification. Striking contrasts with the properties of the counterparts in ordinary materials are shown. We also discuss the possibilities for compensating strong losses inherent to plasmonic metamaterials, which present a major obstacle in numerous exciting applications, and the possibilities for creation of unique ultracompact photonic devices such as data processing chips and nonlinear-optical sensors. Finally, we propose similar extraordinary three-wave mixing processes in crystals based on optical phonons with negative dispersion.

physics.optics↗

Imaging Properties of Two-Dimensional Microlenses

Despite strong experimental and theoretical evidence supporting superresolution imaging based on microlenses, imaging mechanisms involved are not well understood. Based on the transformation optics approach, we demonstrate that microlenses may act as two-dimensional fisheye or Eaton lenses. An asymmetric Eaton lens may exhibit considerable image magnification, which has been confirmed experimentally.

physics.optics↗

Searching for Better Plasmonic Materials

Plasmonics is a research area merging the fields of optics and nanoelectronics by confining light with relatively large free-space wavelength to the nanometer scale - thereby enabling a family of novel devices. Current plasmonic devices at telecommunication and optical frequencies face significant challenges due to losses encountered in the constituent plasmonic materials. These large losses seriously limit the practicality of these metals for many novel applications. This paper provides an overview of alternative plasmonic materials along with motivation for each material choice and important aspects of fabrication. A comparative study of various materials including metals, metal alloys and heavily doped semiconductors is presented. The performance of each material is evaluated based on quality factors defined for each class of plasmonic devices. Most importantly, this paper outlines an approach for realizing optimal plasmonic material properties for specific frequencies and applications, thereby providing a reference for those searching for better plasmonic materials.

physics.optics↗

Frequency-domain simulations of a negative-index material with embedded gain

We solve the equations governing light propagation in a negative-index material with embedded nonlinearly saturable gain material using a frequency-domain model. We show that available gain materials can lead to complete loss compensation only if they are located in the regions where the field enhancement is maximal. We study the increased enhancement of the fields in the gain composite as well as in the metal inclusions and show analytically that the effective gain is determined by the average near-field enhancement.

physics.optics↗

Tunable magnetic response of metamaterials

We demonstrate a thermally tunable optical metamaterial with negative permeability working in the visible range. By covering coupled metallic nanostrips with aligned nematic liquid crystals (NLCs), the magnetic response wavelength of the metamaterial is effectively tuned through control of the ambient temperature, changing the refractive index of LC via phase transitions. By increasing the ambient temperature from 20 degree to 50 degree, the magnetic response wavelength shifts from 650nm to 632nm. Numerical simulations confirm our tests and match the experimental observations well.

physics.optics↗

Yellow-light Negative-index Metamaterials

A well-established, silver fishnet design has been further miniaturized to function as a negative-index material at the shortest wavelength to date. By studying the transmittance, reflectance, and corresponding numerical simulations of the sample, we report in this paper a negative refractive index of -0.25 at the yellow-light wavelength of 580 nm.

physics.optics↗

Translation of Nanoantenna Hot-Spots by a Metal-Dielectric Composite Superlens

We employ numerical simulations to show that highly localized, enhanced electromagnetic fields, also known as "hot spots," produced by a periodic array of silver nanoantennas can be spatially translated to the other side of a metal-dielectric composite superlens. The proposed translation of the hot spots enables surface-enhanced optical spectroscopy without the undesirable contact of molecules with metal, and thus it broadens and reinforces the potential applications of sensing based on field-enhanced fluorescence and surface-enhanced Raman scattering.

physics.optics↗

Coherent Nonlinear Optics and Quantum Control in Negative-Index Metamaterials

The extraordinary properties of laser-induced transparency of a negative-index slab and parametric amplification for a backward-wave signal are investigated. The effects of the idler absorption and phase mismatch on the amplification of the signal are studied, and the feasibility of ensuring robust transparency for a broad range of control field intensities and slab thicknesses is shown. A particular option consisting of the independent engineering of a strong four-wave mixing response and the negative refractive index is proposed and its specific features are investigated. The feasibility of quantum control over the slab transparency in such a scheme is confirmed through numerical experiments. We thus show opportunities and conditions for the compensation of the strong absorption inherent to plasmonic negative-index metamaterials, and we further show achievable transparency through coherent energy transfer from the control optical field to the negative-index signal.

physics.optics↗

Anisotropic Metamaterials Emulated by Tapered Waveguides: Application to Optical Cloaking

We demonstrate that metamaterial devices requiring anisotropic dielectric permittivity and magnetic permeability may be emulated by specially designed tapered waveguides. This approach leads to low-loss, broadband performance. Based on this technique, we demonstrate broadband electromagnetic cloaking in the visible frequency range on a scale ~100 times larger than the wavelength.

physics.optics↗

Resonant nonlinear optics of backward waves in negative-index metamaterials

The extraordinary properties of resonant four-wave mixing of backward waves in doped negative-index materials are investigated. The feasibility of independent engineering of negative refractive index and nonlinear optical response as well as quantum control of the nonlinear propagation process in such composites is shown due to the coherent energy transfer from the control to the signal field. Laser-induced transparency, quantum switching, frequency-tunable narrow-band filtering, amplification, and realizing a miniature mirrorless optical parametric generator of the entangled backward and ordinary waves are among the possible applications of the investigated processes.

physics.optics↗

Mirrorless Negative-index Parametric Micro-oscillator

The feasibility and extraordinary properties of mirrorless parametric oscillations in strongly absorbing negative-index metamaterials are shown. They stem from the backwardness of electromagnetic waves inherent to this type of metamaterials.

physics.optics↗

Optical Metamagnetism and Negative Index Metamaterials

A new class of artificially structured materials called metamaterials makes it possible to achieve electromagnetic properties that do not exist in nature. In this paper we review the recent progress made in the area of optical metamaterials. It was predicted that nanostructured metamaterials could provide us with artificial magnetic response and negative refractive index at optical frequencies. To date, optical metamagnetics have been already fabricated to demonstrate artificial magnetic response in the infrared and across the entire visible spectrum, while metamaterials showing negative refractive index, also called negative index materials (NIM), have been demonstrated in the infrared and at the border with the visible spectral range. Here we report the results of a sample that displays NIM behavior for red light at a wavelength of 710 nm. This is the shortest wavelength so far at which NIM behavior has been observed for light (excluding a device built on surface plasmon polaritons). We also discuss the fabrication challenges and the impact of fabrication limitations, specifically surface roughness of the fabricated structures on the optical properties of the metamaterials.

physics.optics↗

From Positive- to Negative-Index Materials: Transitional Phenomena

Electromagnetic field propagation through a transition layer between the positive-index and negative-index materials with linearly changing dielectric permittivity and magnetic permeability was investigated. It is shown that at oblique incidence, the components of both TE- and TM-waves exhibit singular behavior in the vicinity of the point where both dielectric permittivity and magnetic permeability are equal to zero. In this case, finite dissipation of electromagnetic field energy takes place even at infinitesimally small values of losses. These results are applicable to a broader class of inhomogeneous metamaterials and may provide a new platform for the realization of low intensity nonlinear optics in metamaterials.

physics.optics↗