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Vo Tien Phong

Publications and source records attributed to Vo Tien Phong.

At least 19 recordsLinked to original sources

Multi-Knob Switchable Chiral Superconductivity Quartet in Rhombohedral Graphene

Chiral superconductors break orbital time-reversal symmetry and may host topological quasiparticles with non-Abelian statistics. In rhombohedral graphene, superconductivity develops from a spin-valley-polarized quarter-metal (QM) parent state and features unique magnetic hysteresis of resistance that indicates orbital time-reversal-symmetry-breaking. Exploring and controlling the full spin-valley flavors of such superconductivity could enable novel superconducting and topological devices, but have remained unexplored. Here we report transport measurements on rhombohedral hexalayer graphene (R6G), which reveal a new superconducting state (SCH) that is induced by an out-of-plane magnetic field, in addition to chiral superconductivity (CSC) similar to those observed in thinner layers. This SCH state emerges above 0.8 T, persists up to 1.6 T and can be switched on/off by magnetic field $H_\perp$, carrier density $n$, and gate displacement field $D$. Quantum oscillations and anomalous Hall measurements show that SCH stems from a field-induced quarter-metal (QM$'$) parent phase, which carries orbital magnetization opposite to that of the zero-field QM. Across the full $(n, D, H_\perp)$ parameter space, superconductivity can be realized from all four spin-valley isospin flavors, establishing a switchable chiral-superconductor quartet in R6G. We interpret the parent-state switching as arising from competition between a Kane-Mele-like spin-valley splitting and magnetic-field coupling to spin-valley-dependent magnetic moments. Our work establishes rhombohedral graphene as a multi-knob platform for different isospin-polarized superconductivities, which enables programmable superconducting networks with possible Majorana modes along domain walls.

cond-mat.supr-con↗

Valley Valves at Domain Walls in Symmetry-Broken Rhombohedral Graphene

Rhombohedral multilayer graphene polarized by a moderate perpendicular displacement field hosts a time-reversal-symmetry-breaking valley-and-spin-polarized metallic phase that may condense into a chiral superconductor. Recent magnetic imaging and transport measurements in this unconventional system suggest the presence of domain walls both in the metallic and superconducting phases. In this work, we show that valley domain walls are impenetrable barriers to transport in the metallic regime. Transmission through such a domain wall must therefore be mediated by intervalley interactions. We derive the symmetry-allowed terms and show via microscopic numerical simulations that they enable the transmission of electrons across the domain wall. In the superconducting phase, we find that intervalley mixing is crucial for supporting an appreciable supercurrent through a SNS' Josephson junction that connects opposite-chirality superconducting regions. Taken together, our work elucidates the nature of domain walls in these experimentally relevant multilayer systems and emphasizes the critical role of intervalley hybridization in governing their transport properties.

cond-mat.mes-hall↗

Family of High-Chern-Number Orbital Magnets in Twisted Rhombohedral Graphene

Realizing Chern insulators with Chern numbers greater than one remains a major goal in quantum materials research. Such platforms promise multichannel dissipationless chiral transport and access to correlated phases beyond the conventional C = 1 paradigm. Here, we discover a family of high-Chern-number orbital magnets in twisted monolayer-multilayer rhombohedral graphene, denoted (1+n) with n = 3, 4, and 5. Magnetotransport measurements show pronounced anomalous Hall effects at one and three electrons per moiré unit cell when they are polarized away from the moiré interface. Across the (1+n) systems, we observe a clear topological hierarchy C = n, revealed by the Středa trajectories and the quantized Hall resistance. Our experimental observations are supported by self-consistent mean-field calculations. Moreover, we realize both electrical and magnetic switching of the high-Chern-number states by flipping the valley polarization. Together, these results establish a tunable hierarchy of orbital Chern magnets in twisted rhombohedral graphene, offering systematic control of Chern number and topology through layer engineering in pristine graphene moiré systems.

cond-mat.mes-hall↗

Coulomb Interaction-Stabilized Isolated Narrow Bands with Chern Numbers $\mathcal{C} > 1$ in Twisted Rhombohedral Trilayer-Bilayer Graphene

Recently, fractional quantum anomalous Hall effects have been discovered in two-dimensional moiré materials when a topologically nontrivial band with Chern number $\mathcal{C}=1$ is partially doped. Remarkably, superlattice Bloch bands can carry higher Chern numbers that defy the Landau-level paradigm and may even host exotic fractionalized states with non-Abelian quasiparticles. Inspired by this exciting possibility, we propose twisted \textit{rhombohedral} trilayer-bilayer graphene at $θ\sim 1.2^\circ$ as a field-tunable quantum anomalous Chern insulator that features spectrally-isolated, kinetically-quenched, and topologically-nontrivial bands with $\mathcal{C} = 2,3$ favorable for fractional phases once fractionally doped, as characterized by their quantum geometry. Based on extensive self-consistent mean-field calculations, we show that these phases are stabilized by Coulomb interactions and are robust against variations in dielectric environment, tight-binding hopping parameters, and lattice relaxation.

cond-mat.mes-hall↗

Superconductivity from dual-surface carriers in rhombohedral graphene

Intrinsic rhombohedral graphene hosts an unusual low-energy electronic wavefunction, predominantly localized at its outer crystal faces with negligible presence in the bulk. Increasing the number of graphene layers amplifies the density of states near charge neutrality, greatly enhancing the susceptibility to symmetry-breaking phases. Here, we report superconductivity in rhombohedral graphene arising from an unusual charge-delocalized semimetallic normal state, characterized by coexisting valence- and conduction-band Fermi pockets split to opposite crystal surfaces. In octalayer graphene, the superconductivity appears in five apparently distinct pockets for each sign of an external electric displacement field ($D$). In a moiré superlattice sample where heptalayer graphene is aligned on one side to hexagonal boron nitride, two pockets of superconductivity emerge from a single sharp resistive feature. At higher $D$ the same resistive feature additionally induces an $h/e^{2}$-quantized anomalous Hall state at dopings near one electron per moiré unit cell. Our findings reveal a novel superconducting regime in multilayer graphene and create opportunities for coupling to nearby topological states.

cond-mat.mes-hall↗

Squeezing Quantum States in Three-Dimensional Twisted Crystals

A fundamental idea in wave mechanics is that propagation in a periodic medium can be described by Bloch waves whose conserved crystal momenta define their transformations when displaced by the set of discrete lattice translations. In ordered materials where incommensurate spatial periods compete, this general principle is rendered ineffective, often with dramatic consequences. Examples are crystals with broken symmetries from charge or spin density waves, quasiperiodic lattices that produce diffraction patterns with crystallographically forbidden point symmetries, and stacks of two-dimensional lattices with a relative rotation (twist) between layers. In special cases when there is a small difference between the competing periods, a useful work-around is a continuum description where a periodic long-wavelength field produces Bragg scattering that coherently mixes short-wavelength carrier waves. In this work, we advocate an alternative approach to study three-dimensional twisted crystals that replaces their spectrally congested momentum-space Bloch band structures with a representation using squeezed coherent states in a Fock space of free-particle vortex states. This reorganization of the Hilbert space highlights the crucial role of the Coriolis force in the equations of motion that leads to unconventional phase space dynamics and edge state structure generic to a family of complex crystals.

cond-mat.mes-hall↗

Optical Absorption and Emission from Wannier-Stark Spectra of Moiré Superlattices

Using a formalism based on the non-Abelian Berry connection, we explore quantum geometric signatures of Wannier-Stark spectra in two-dimensional superlattices. The Stark energy can be written as \textit{intraband} Berry phases, while Zener tunneling is given by \textit{interband} Berry connections. We suggest that the gaps induced by interband hybridization can be probed by THz optical absorption and emission spectroscopy. This is especially relevant to modern moiré materials wherein mini-bands are often spectrally entangled, leading to strong interband hybridization in the Wannier-Stark regime. Furthermore, owing to their large superlattice constants, both the low-field and high-field regimes can be accessed in these materials using presently available technology. Importantly, even at moderate electric fields, we find that stimulated emission can dominate absorption, raising the possibility of lasing at practically relevant parameter regimes.

cond-mat.mes-hall↗

Band Renormalization, Quarter Metals, and Chiral Superconductivity in Rhombohedral Tetralayer Graphene

Recently, exotic superconductivity emerging from a spin-and-valley-polarized metallic phase has been discovered in rhombohedral tetralayer graphene. To explain this observation, we study the role of electron-electron interactions in driving flavor symmetry breaking, using the Hartree-Fock (HF) approximation, and in stabilizing superconductivity mediated by repulsive interactions. Though mean-field HF correctly predicts the isospin flavors and reproduces the experimental phase diagram, it overestimates the band renormalization near the Fermi energy and suppresses superconducting instabilities. To address this, we introduce a physically motivated scheme that includes internal screening in the HF calculation. Using this formalism, we find superconductivity arising from the spin-valley polarized phase for a range of electric fields and electron dopings. Our findings reproduce the experimental observations and reveal a p-wave, finite-momentum, time-reversal-symmetry-broken superconducting state, encouraging further investigation into exotic phases in graphene multilayers.

cond-mat.str-el↗

Protected Fermionic Zero Modes in Periodic Gauge Fields

It is well-known that macroscopically-normalizable zero-energy wavefunctions of spin-$\frac{1}{2}$ particles in a two-dimensional inhomogeneous magnetic field are spin-polarized and exactly calculable with degeneracy equaling the number of flux quanta linking the whole system. Extending this argument to massless Dirac fermions subjected to magnetic fields that have \textit{zero} net flux but are doubly periodic in real space, we show that there exist \textit{only two} Bloch-normalizable zero-energy eigenstates, one for each spin flavor. This result is immediately relevant to graphene multilayer systems subjected to doubly-periodic strain fields, which at low energies, enter the Hamiltonian as periodic pseudo-gauge vector potentials. Furthermore, we explore various related settings including nonlinearly-dispersing band structure models and systems with singly-periodic magnetic fields.

cond-mat.mes-hall↗

Roses in the Nonperturbative Current Response of Artificial Crystals

In two-dimensional artificial crystals with large real-space periodicity, the nonlinear current response to a large applied electric field can feature a strong angular dependence, which encodes information about the band dispersion and Berry curvature of isolated electronic Bloch minibands. Within the relaxation-time approximation, we obtain analytic expressions up to infinite order in the driving field for the current in a band-projected theory with time-reversal and trigonal symmetry. For a fixed field strength, the dependence of the current on the direction of the applied field is given by rose curves whose petal structure is symmetry constrained and is obtained from an expansion in real-space translation vectors. We illustrate our theory with calculations on periodically-buckled graphene and twisted double bilayer graphene, wherein the discussed physics can be accessed at experimentally-relevant field strengths.

cond-mat.mes-hall↗

Quantum Geometric Oscillations in Two-Dimensional Flat-Band Solids

Two-dimensional van der Waals heterostructures can be engineered into artificial superlattices that host flat bands with significant Berry curvature and provide a favorable environment for the emergence of novel electron dynamics. In particular, the Berry curvature can induce an oscillating trajectory of an electron wave packet transverse to an applied static electric field. Though analogous to Bloch oscillations, this novel oscillatory behavior is driven entirely by quantum geometry in momentum space instead of band dispersion. While the orbits of Bloch oscillations can be localized by increasing field strength, the size of the geometric orbits saturates to a nonzero plateau in the strong-field limit. In non-magnetic materials, the geometric oscillations are even under inversion of the applied field, whereas the Bloch oscillations are odd, a property that can be used to distinguish these two co-existing effects.

cond-mat.mes-hall↗

Junctions and superconducting symmetry in twisted bilayer graphene

Junctions provide a wealth of information on the symmetry of the order parameter of superconductors. We analyze junctions between a scanning tunneling microscope (STM) tip and superconducting twisted bilayer graphene (TBG) and TBG Josephson junctions (JJs). We compare superconducting phases that are even or odd under valley exchange (s- or f-wave). The critical current in mixed (s- and f-) JJs strongly depends on the angle between the junction and the lattice. In STM-TBG junctions, due to Andreev reflection, f-wave leads to a prominent peak in subgap conductance, as seen in experiments.

cond-mat.supr-con↗

Superconductivity and correlated phases in non-twisted bilayer and trilayer graphene

Twisted bilayer graphene has a rich phase diagram, including superconductivity. Recently, an unexpected discovery has been the observation of superconductivity in non-twisted graphene bilayers and trilayers. In this Perspective, we give an overview of the search for uncommon phases in non-twisted graphene systems. We first contextualize these recent results within earlier work in the field, before examining the new experimental findings. Finally, we analyse the numerous theoretical models that study the underlying physical processes in these systems

cond-mat.mes-hall↗

Network model for periodically strained graphene

The long-wavelength physics of monolayer graphene in the presence of periodic strain fields has a natural chiral scattering network description. When the strain field varies slowly compared to the graphene lattice and the effective magnetic length of the induced valley pseudomagnetic field, the low-energy physics can be understood in terms of valley-polarized percolating domain-wall modes. Inspired by a recent experiment, we consider a strain field with threefold rotation and mirror symmetries but without twofold rotation symmetry, resulting in a system with the connectivity of the oriented kagome network. Scattering processes in this network are captured by a symmetry-constrained phenomenological $S$ matrix. We analyze the phase diagram of the kagome network, and show that the bulk physics of the strained graphene can be qualitatively captured by the network when we account for a percolation transition at charge neutrality. We also discuss the limitations of this approach to properly account for boundary physics.

cond-mat.mes-hall↗

Interaction-Enhanced Topological Hall Effects in Strained Twisted Bilayer Graphene

We analyze the effects of the long-range Coulomb interaction on the distribution of Berry curvature among the bands near charge neutrality of twisted bilayer graphene (TBG) closely aligned with hexagonal boron nitride (hBN). Due to the suppressed dispersion of the narrow bands, the band structure is strongly renormalized by electron-electron interactions, and thus, the associated topological properties of the bands are sensitive to filling. Using a Hartree formalism, we calculate the linear and nonlinear Hall conductivities, and find that for certain fillings, the remote bands contribute substantially to the Hall currents while the contribution from the central bands is suppressed. In particular, we find that these currents are generically substantial near regions of energies where the bands are highly entangled with each other, often featuring doping-induced band inversions. Our results demonstrate that topological transport in TBG/hBN is substantially modified by electron-electron interactions, which offer a simple explanation to recent experimental results.

cond-mat.mes-hall↗

Boundary Modes from Periodic Magnetic and Pseudomagnetic Fields in Graphene

Single-layer graphenes subject to periodic lateral strains are artificial crystals that can support boundary spectra with an intrinsic polarity. These are analyzed by comparing the effects of periodic magnetic fields and strain-induced pseudomagnetic fields that respectively break and preserve time-reversal symmetry. In the former case, a Chern classification of the superlattice minibands with zero total magnetic flux enforces {\it single} counter-propagating modes traversing each bulk gap on opposite boundaries of a nanoribbon. For the pseudomagnetic field, pairs of counter-propagating modes migrate to the {\it same} boundary where they provide well-developed valley-helical transport channels on a single zigzag edge. We discuss possible schemes for implementing this situation and their experimental signatures.

cond-mat.mes-hall↗

Superconductivity from Repulsive Interactions in Rhombohedral Trilayer Graphene: a Kohn-Luttinger-Like Mechanism

We study the emergence of superconductivity in rhombohedral trilayer graphene due purely to the long-range Coulomb repulsion. This repulsive-interaction-driven phase in rhombohedral trilayer graphene is significantly different from those found in twisted bilayer and trilayer graphenes. In the latter case, the nontrivial momentum-space geometry of the Bloch wavefunctions leads to an effective attractive electron-electron interaction; this allows for less modulated order parameters and for spin-singlet pairing. In rhombohedral trilayer graphene, we instead find spin-triplet superconductivity with critical temperatures up to 0.15 K. The critical temperatures strongly depend on electron filling and peak where the density of states diverge. The order parameter shows a significant modulation within each valley pocket of the Fermi surface.

cond-mat.mes-hall↗

Band Structure and Superconductivity in Twisted Trilayer Graphene

We study the symmetries of twisted trilayer graphene's band structure under various extrinsic perturbations, and analyze the role of long-range electron-electron interactions near the first magic angle. The electronic structure is modified by these interactions in a similar way to twisted bilayer graphene. We analyze electron pairing due to long-wavelength charge fluctuations, which are coupled among themselves via the Coulomb interaction and additionally mediated by longitudinal acoustic phonons. We find superconducting phases with either spin singlet/valley triplet or spin triplet/valley singlet symmetry, with critical temperatures of up to a few Kelvin for realistic choices of parameters.

cond-mat.mes-hall↗