arXiv subjects

W. Nazarewicz

Publications and source records attributed to W. Nazarewicz.

At least 55 records · Page 3Linked to original sources

arXiv2020

Gamow Shell Model description of Li isotopes and their mirror partners

Background: Weakly bound and unbound nuclei close to particle drip lines are laboratories of new nuclear structure physics at the extremes of neutron/proton excess. The comprehensive description of these systems requires an open quantum system framework that is capable of treating resonant and nonresonant many-body states on equal footing. Purpose: In this work, we construct the minimal complex-energy configuration interaction approach to describe binding energies and spectra of selected 5 $\leq$ A $\leq$ 11 nuclei. Method: We employ the complex-energy Gamow shell model (GSM) assuming a rigid $^4$He core. The effective Hamiltonian, consisting of a core-nucleon Woods-Saxon potential and a simplified version of the Furutani-Horiuchi-Tamagaki interaction with the mass-dependent scaling, is optimized in the sp space. To diagonalize the Hamiltonian matrix, we employ the Davidson method and the Density Matrix Renormalization Group technique. Results: Our optimized GSM Hamiltonian offers a good reproduction of binding energies and spectra with the root-mean-square (rms) deviation from experiment of 160 keV. Since the model performs well when used to predict known excitations that have not been included in the fit, it can serve as a reliable tool to describe poorly known states. A case in point is our prediction for the pair of unbound mirror nuclei $^{10}$Li-$^{10}$N in which a huge Thomas-Ehrman shift dramatically alters the pattern of low-energy excitations. Conclusion: The new model will enable comprehensive studies of structure and reactions aspects of light drip-line nuclei.

nucl-th↗

arXiv2020

Energy Spectrum of Neutron-Rich Helium Isotopes: Complex Made Simple

We demonstrate that the intricate energy spectrum of neutron-rich helium isotopes can be straightforwardly described by taking advantage of the low-energy properties of neutron-neutron interaction and the scale separation that is present in diluted dripline systems. By using arguments based on the halo effective field theory, we carry out a parameter reduction of the complex-energy configuration interaction framework in the $spd$ space, including resonant and scattering states. By adjusting only one parameter, the strength of the spin-singlet central neutron-neutron interaction, we reproduce experimental energies and widths of $^{5-8}$He within tens of keV precision. We predict a parity inversion of narrow resonances in $^{9}$He and show that the ground state of $^{10}$He is an $s$-wave-dominated threshold configuration that could decay through two-neutron emission.

nucl-th↗

arXiv2020

Measurement and microscopic description of odd-even staggering of charge radii of exotic copper isotopes

The mesoscopic nature of the atomic nucleus gives rise to a wide array of macroscopic and microscopic phenomena. The size of the nucleus is a window into this duality: while the charge radii globally scale as $A^{1/3}$, their evolution across isotopic chains reveals unanticipated structural phenomena [1-3]. The most ubiquitous of these is perhaps the Odd-Even Staggering (OES) [4]: isotopes with an odd number of neutrons are usually smaller in size than the trend of their even-neutron neighbours suggests. This OES effect varies with the number of protons and neutrons and poses a significant challenge for nuclear theory [5-7]. Here, we examine this problem with new measurements of the charge radii of short-lived copper isotopes up to the very exotic $^{78}$Cu $(Z=29, N=49)$, produced at only 20 ions/s, using the highly-sensitive Collinear Resonance Ionisation Spectroscopy (CRIS) method at ISOLDE-CERN. Due to the presence of a single proton outside of the closed Z=28 shell, these measurements provide crucial insights into the single-particle proton structure and how this affects the charge radii. We observe an unexpected reduction in the OES for isotopes approaching the $N=50$ shell gap. To describe the data, we applied models based on nuclear Density Functional Theory [2,8] (DFT) and ab-initio Valence-Space In-Medium Similarity Renormalization Group (VS-IMSRG) theory [9,10]. Through these comparisons, we demonstrate a relation between the global behavior of charge radii and the saturation density of nuclear matter, and show that the local charge radii variations, which reflect the many-body polarization effects due to the odd neutron, naturally emerge from the VS-IMSRG calculations.

nucl-ex↗

arXiv2019

Beyond the charge radius: the information content of the fourth radial moment

Measurements of atomic transitions in different isotopes offer key information on the nuclear charge radius. The anticipated high-precision experimental techniques, augmented by atomic calculations, will soon enable extraction of the higher-order radial moments of the charge density distribution. To assess the value of such measurements for nuclear structure research, we study the information content of the fourth radial moment $\rf$ by means of nuclear density functional theory and a multiple correlation analysis. We show that $\rf$ can be directly related to the surface thickness of nuclear density, a fundamental property of the atomic nucleus that is difficult to obtain for radioactive systems. Precise knowledge of these radial moments is essential to establish reliable constraints on the existence of new forces from precision isotope shift measurements .

nucl-th↗

arXiv2019

Convenient location of a near-threshold proton-emitting resonance in $^{11}$B

The presence of cluster-like narrow resonances in the vicinity of reaction/decay thresholds is a ubiquitous phenomenon with profound consequences. We argue that the continuum coupling, present in the open quantum system description of the atomic nucleus, can profoundly impact the nature of near-threshold states. In this Letter, we discuss the structure of the recently observed near-threshold resonance in $^{11}$B, whose very existence explains the puzzling beta-delayed proton emission of the neutron-rich $^{11}$Be.

nucl-th↗

arXiv2019

First observation of unbound $^{11}$O, the mirror of the halo nucleus $^{11}$Li

The structure of the extremely proton-rich nucleus $^{11}_{~8}$O$_3$, the mirror of the two-neutron halo nucleus $^{11}_{~3}$Li$_8$, has been studied experimentally for the first time. Following two-neutron knockout reactions with a $^{13}$O beam, the $^{11}$O decay products were detected after two-proton emission and used to construct an invariant-mass spectrum. A broad peak of width $\sim$3\,MeV was observed. Within the Gamow coupled-channel approach, it was concluded that this peak is a multiplet with contributions from the four-lowest $^{11}$O resonant states: $J^π$=3/2$^-_1$, 3/2$^-_2$, 5/2$^+_1$, and 5/2$^+_2$. The widths and configurations of these states show strong, non-monotonic dependencies on the depth of the $p$-$^9$C potential. This unusual behavior is due to the presence of a broad threshold resonant state in $^{10}$N, which is an analog of the virtual state in $^{10}$Li in the presence of the Coulomb potential. After optimizing the model to the data, only a moderate isospin asymmetry between ground states of $^{11}$O and $^{11}$Li was found.

nucl-ex↗

arXiv2019

Structures and decay properties of extremely proton-rich nuclei $^{11,12}$O

${\rm \bf Background:}$ The recent observation of the unbound nucleus $^{11}$O offers the unique possibility to study how the structure and dynamics of two-proton ($2p$) decay is affected by the removal of one neutron from $^{12}$O, and provides important information on the Thomas-Ehrman effect in the mirror pairs $^{11}_{~8}$O$_3$-$^{11}_{~3}$Li$_8$ and $^{12}_{~8}$O$_4$-$^{12}_{~4}$Be$_8$, which involve the $2p$ emitters $^{11}$O and $^{12}$O. ${\rm \bf Purpose:}$ We investigate how continuum effects impact the structure and decay properties of $^{11}$O and $^{12}$O, and their mirror partners. ${\rm \bf Methods:}$ We solve the three-body core-nucleon-nucleon problem using the Gamow coupled-channel (GCC) method. The GCC Hamiltonian employs a realistic finite-range valence nucleon-nucleon interaction and the deformed cores of $^{9,10}$C, $^{9}$Li, and $^{10}$Be. ${\rm \bf Results:}$ We calculate the energy spectra and decay widths of $^{11}$O and $^{12}$O as well as those of their mirror nuclei. In particular, we investigate the dynamics of the $2p$ decay in the ground state of $^{12}$O by analyzing the evolution of the $2p$ configuration of the emitted protons as well as their angular correlations in the coordinate space. We also show how the analytic structure of the resonant states of $^{10}$Li and $^{10}$N impacts the low-lying states of $^{11}$Li and $^{11}$O. ${\rm \bf Conclusions:}$ We demonstrate that, in both nuclei $^{11}$O and $^{12}$O, there is a competition between direct and "democratic" $2p$ ground-state emission. The broad structure observed in $^{11}$O is consistent with four broad resonances, with the predicted $3/2^-_1$ ground state strongly influenced by the broad threshold resonant state in $^{10}$N, which is an isobaric analog of the antibound (or virtual) state in $^{10}$Li.

nucl-th↗

arXiv2019

Resonant spectra of multipole-bound anions

In multipole-bound anions, the excess electron is attached by a short-range multipole potential of a neutral molecule. Such anions are prototypical marginally-bound open quantum systems. In particular, around the critical multipole moment required to attach the valence electron, multipole-bound anions exhibit critical behavior associated with a transition from bound states dominated by low-$\ell$ partial waves to the electron continuum. In this work, multipole-bound anions are described using a nonadiabatic electron-plus-rotor model. The electron-molecule pseudo-potential is represented by a short-range multipole field with a Gaussian form-factor. The resulting coupled-channel Schrödinger equation is solved by means of the Berggren expansion method, in which the electron's wave function is decomposed into bound states, narrow resonances, and the non-resonant scattering continuum. We show that the Gaussian model predicts the critical transition at the detachment threshold. Resonant states, including bound states, decaying resonances, subthreshold resonances, and antibound states are studied, and exceptional points where two resonant states coalesce are predicted. We discuss the transition of rotational band structures around the threshold and study the effects of channel coupling on the decay width of resonant poles.

physics.atom-ph↗

arXiv2018

First observation of the competing fission modes in the neutron-deficient sub-lead region

Fragment mass distributions from fission of excited compound nucleus $^{178}$Pt have been deduced from the measured fragment velocities. The $^{178}$Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction $^{36}$Ar + $^{142}$Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of $\approx1/3$. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, $A_{L}/A_{H}\approx 79/99$, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.

nucl-ex↗

arXiv2018

FRIB and the GW170817 Kilonova

In July 2018 an FRIB Theory Alliance program was held on the implications of GW170817 and its associated kilonova for r-process nucleosynthesis. Topics of discussion included the astrophysical and nuclear physics uncertainties in the interpretation of the GW170817 kilonova, what we can learn about the astrophysical site or sites of the r process from this event, and the advances in nuclear experiment and theory most crucial to pursue in light of the new data. Here we compile a selection of scientific contributions to the workshop, broadly representative of progress in r-process studies since the GW170817 event.

astro-ph.HE↗

arXiv2018

r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context.

astro-ph.SR↗

arXiv2018

The puzzling two-proton decay of $^{67}$Kr

Two-proton (2$p$) radioactivity is a rare decay mode found in a few proton-unbound nuclei. The $2p$-decay lifetime and properties of emitted protons carry invaluable information on nuclear structure in the presence of low-lying proton continuum. The recently measured $2p$ decay of $^{67}$Kr [Phys. Rev. Lett. 117, 162501 (2016)] turned out to be unexpectedly fast. Since $^{67}$Kr is expected to be a deformed system, we investigate the impact of deformation effects on the $2p$ radioactivity. We apply the recently developed Gamow coupled-channel framework, which allows for a precise description of three-body systems in the presence of rotational and vibrational couplings. This is the first application of a three-body approach to a two-nucleon decay from a deformed nucleus. We show that deformation couplings significantly increase the $2p$ decay width of $^{67}$Kr; this finding explains the puzzling experimental data. The calculated angular proton-proton correlations reflect a competition between $1p$ and $2p$ decay modes in this nucleus.

nucl-th↗

arXiv2017

Quantified Gamow Shell Model interaction for $psd$-shell nuclei

The structure of weakly bound and unbound nuclei close to particle drip lines is one of the major science drivers of nuclear physics. A comprehensive understanding of these systems goes beyond the traditional configuration interactions approach formulated in the Hilbert space of localized states (nuclear shell model) and requires an open quantum system description. The complex-energy Gamow Shell Model (GSM) provides such a framework as it is capable of describing resonant and non-resonant many-body states on equal footing. To make reliable predictions, quality input is needed that allows for the full uncertainty quantification of theoretical results. In this study, we carry out the optimization of an effective GSM (one-body and two-body) interaction in the $psdf$ shell model space. The resulting interaction is expected to describe nuclei with $5 \leqslant A \leqslant 12$ at the $p-sd$-shell interface. The optimized one-body potential reproduces nucleon-$^4$He scattering phase shifts up to an excitation energy of 20 MeV. The two-body interaction built on top of the optimized one-body field is adjusted to the bound and unbound ground-state binding energies and selected excited states of the Helium, Lithium, and Beryllium isotopes up to $A=9$. A very good agreement with experiment was obtained for binding energies. First applications of the optimized interaction include predictions for two-nucleon correlation densities and excitation spectra of light nuclei with quantified uncertainties. The new interaction will enable comprehensive and fully quantified studies of structure and reactions aspects of nuclei from the $psd$ region of the nuclear chart.

nucl-th↗

arXiv2017

Search for excited states in $^{25}$O

Theoretical calculations suggest the presence of low-lying excited states in $^{25}$O. Previous experimental searches by means of proton knockout on $^{26}$F produced no evidence for such excitations. We search for excited states in $^{25}$O using the ${ {}^{24}\text{O} (d,p) {}^{25}\text{O} }$ reaction. The theoretical analysis of excited states in unbound $^{25,27}$O is based on the configuration interaction approach that accounts for couplings to the scattering continuum. We use invariant-mass spectroscopy to measure neutron-unbound states in $^{25}$O. For the theoretical approach, we use the complex-energy Gamow Shell Model and Density Matrix Renormalization Group method with a finite-range two-body interaction optimized to the bound states and resonances of $^{23-26}$O, assuming a core of $^{22}$O. We predict energies, decay widths, and asymptotic normalization coefficients. Our calculations in a large $spdf$ space predict several low-lying excited states in $^{25}$O of positive and negative parity, and we obtain an experimental limit on the relative cross section of a possible ${ {J}^π = {1/2}^{+} }$ state with respect to the ground-state of $^{25}$O at $σ_{1/2+}/σ_{g.s.} = 0.25_{-0.25}^{+1.0}$. We also discuss how the observation of negative parity states in $^{25}$O could guide the search for the low-lying negative parity states in $^{27}$O. Previous experiments based on the proton knockout of $^{26}$F suffered from the low cross sections for the population of excited states in $^{25}$O because of low spectroscopic factors. In this respect, neutron transfer reactions carry more promise.

nucl-ex↗

arXiv2017

Continuum effects in neutron-drip-line oxygen isotopes

The binding-energy pattern along the neutron-rich oxygen chain, governed by an interplay between shell effects and many-body correlations impacted by strong couplings to one- and two-neutron continuum, make these isotopes a unique testing ground for nuclear models. In this work, we investigate ground states and low-lying excited states of $^{23-28}$O using the complex-energy Gamow Shell Model and Density Matrix Renormalization Group method with a finite-range two-body interaction optimized to the bound states and resonances of $^{23-26}$O, assuming a core of $^{22}$O. Our results suggest that the ground-state of $^{28}$O has a threshold character, i.e., is very weakly bound or slightly unbound. We also predict narrow excited resonances in $^{25}$O and $^{27}$O. The inclusion of the large continuum space significantly impacts predicted binding energies of $^{26-28}$O. This implies that the careful treatment of neutron continuum is necessary prior to assessing the spectroscopic quality of effective interactions in this region.

nucl-th↗

arXiv2017

Structure and decays of nuclear three-body systems: the Gamow coupled-channel method in Jacobi coordinates

${\bf Background:}$ Weakly bound and unbound nuclear states appearing around particle thresholds are prototypical open quantum systems. Theories of such states must take into account configuration mixing effects in the presence of strong coupling to the particle continuum space. ${\bf Purpose:}$ To describe structure and decays of three-body systems, we developed a Gamow coupled-channel (GCC) approach in Jacobi coordinates by employing the complex-momentum formalism. We benchmarked the new framework against the complex-energy Gamow Shell Model (GSM). ${\bf Methods:}$ The GCC formalism is expressed in Jacobi coordinates, so that the center-of-mass motion is automatically eliminated. To solve the coupled-channel equations, we use hyperspherical harmonics to describe the angular wave functions while the radial wave functions are expanded in the Berggren ensemble, which includes bound, scattering and Gamow states. ${\bf Results:}$ We show that the GCC method is both accurate and robust. Its results for energies, decay widths, and nucleon-nucleon angular correlations are in good agreement with the GSM results. ${\bf Conclusions:}$ We have demonstrated that a three-body GSM formalism explicitly constructed in cluster-orbital shell model coordinates provides similar results to a GCC framework expressed in Jacobi coordinates, provided that a large configuration space is employed. Our calculations for $A=6$ systems and $^{26}$O show that nucleon-nucleon angular correlations are sensitive to the valence-neutron interaction. The new GCC technique has many attractive features when applied to bound and unbound states of three-body systems: it is precise, efficient, and can be extended by introducing a microscopic model of the core.

nucl-th↗

arXiv2017

Towards the global description of nuclear charge radii: exploring the Fayans energy density functional

In this work, we study the odd-even effect in binding energies and charge radii, and systematic behavior of differential radii, to identify the underlying components of the effective nuclear interaction. We apply nuclear density functional theory using a family of Fayans and Skyrme energy density functionals fitted to similar datasets but using different optimization protocols. We inspect various correlations between differential charge radii, odd-even staggering in energies and radii, and nuclear matter properties. Detailed analysis is carried out for medium-mass and heavy semi-magic nuclei with a particular focus on the Ca chain. By making the surface and pairing terms dependent on density gradients, the Fayans functional offers the superb simultaneous description of odd-even staggering effects in energies and charge radii. Conversely, when the data on differential radii are added to the pool of fit-observables, the coupling constants determining the strengths of the gradient terms of Fayans functional are increased by orders of magnitude. The Skyrme functional optimized in this work with the generalized Fayans pairing term offers results of similar quality. We quantify these findings by performing correlation analysis based on the statistical linear regression technique. The nuclear matter parameters characterizing Fayans and Skyrme functionals optimized to similar datasets are fairly close.

nucl-th↗

arXiv2017

Nucleon localization and fragment formation in nuclear fission

An electron localization measure was originally introduced to characterize chemical bond structures in molecules. Recently, a nucleon localization based on Hartree-Fock densities has been introduced to investigate $α$-cluster structures in light nuclei. Compared to the local nucleonic densities, the nucleon localization function has been shown to be an excellent indicator of shell effects and cluster correlations. Using the spatial nucleon localization measure, we investigate the emergence of fragments in fissioning heavy nuclei. To illustrate basic concepts of nucleon localization, we employ the self-consistent energy density functional method with a quantified energy density functional optimized for fission studies. We study the particle densities and spatial nucleon localization distributions along the fission pathways of $^{264}$Fm, $^{232}$Th and $^{240}$Pu. We demonstrate that the fission fragments are formed fairly early in the evolution, well before scission. We illustrate the usefulness of the localization measure by showing how the hyperdeformed state of $^{232}$Th can be understood in terms of a quasimolecular state made of $^{132}$Sn and $^{100}$Zr fragments. Compared to nucleonic distributions, the nucleon localization function more effectively quantifies nucleonic clustering: its characteristic oscillating pattern, traced back to shell effects, is a clear fingerprint of cluster/fragment configurations. This is of particular interest for studies of fragment formation and fragment identification in fissioning nuclei.

nucl-th↗