arXiv subjects

W. Nazarewicz

Publications and source records attributed to W. Nazarewicz.

At least 73 records · Page 4Linked to original sources

arXiv2016

Single-particle and collective motion in unbound deformed $ ^{39}\text{Mg} $

Background: Deformed neutron-rich magnesium isotopes constitute a fascinating territory where the interplay between collective rotation and single-particle motion is strongly affected by the neutron continuum. The unbound $fp$-shell nucleus $ ^{39}\text{Mg} $ is an ideal candidate to study this interplay. Purpose: In this work, we predict the properties of low-lying resonant states of $ ^{39}\text{Mg} $, using a suite of realistic theoretical approaches rooted in the open quantum system framework. Method: To describe the spectrum and decay modes of $ ^{39}\text{Mg} $ we use the conventional Shell Model, Gamow Shell Model, Resonating Group Method, Density Matrix Renormalization Group method, and the non-adiabatic Particle-Plus-Rotor model formulated in the Berggren basis. Results: The unbound ground state of $ ^{39}\text{Mg} $ is predicted to be either a $ J^π = {7/2}^- $ state or a $ {3/2}^- $ state. A narrow $ J^π = {7/2}^- $ ground-state candidate exhibits a resonant structure reminiscent of that of its one-neutron halo neighbor $ ^{37}\text{Mg} $, which is dominated by the $ f_{7/2} $ partial wave at short distances and a $ p_{3/2} $ component at large distances. A $ J^π={3/2}^- $ ground-state candidate is favored by the large deformation of the system. It can be associated with the $ {1/2}^- [321] $ Nilsson orbital dominated by the $\ell=1$ wave; hence its predicted width is large. The excited $J^π = {1/2}^-$ and $5/2^-$ states are expected to be broad resonances, while the $ J^π = {9/2}^- $ and $ {11/2}^- $ members of the ground-state rotational band are predicted to have very small neutron decay widths. Conclusion: We demonstrate that the subtle interplay between deformation, shell structure, and continuum coupling can result in a variety of excitations in an unbound nucleus just outside the neutron drip line.

nucl-th↗

arXiv2016

Resonant spectra of quadrupolar anions

In quadrupole-bound anions, an extra electron is attached at a sufficiently large quadrupole moment of a neutral molecule, which is lacking a permanent dipole moment. The nature of the bound states and low-lying resonances of such anions is of interest for understanding the threshold behavior of open quantum systems in general. In this work, we investigate the properties of quadrupolar anions as extreme halo systems, the formation of rotational bands, and the transition from a subcritical to supercritical electric quadrupole moment. We solve the electron-plus-molecule problem using a non-adiabatic coupled-channel formalism by employing the Berggren ensemble, which explicitly contains bound states, narrow resonances, and the scattering continuum. We demonstrate that binding energies and radii of quadrupolar anions strictly follow the scaling laws for two-body halo systems. Contrary to the case of dipolar anions, ground-state band of quadrupolar anions smoothly extend into the continuum, and many rotational bands could be identified above the detachment threshold. We study the evolution of a bound state of an anion as to dives into the continuum at a critical quadrupole moment and we show that the associated critical exponent is consistent with the second-order phase transition. Everything considered, quadrupolar anions represent a perfect laboratory for the studies of marginally bound open quantum systems.

physics.atm-clus↗

arXiv2016

Twist-averaged boundary conditions for nuclear pasta Hartree-Fock calculations

Background: Nuclear pasta phases, present in the inner crust of neutron stars, are associated with nucleonic matter at sub-saturation densities arranged in regular shapes. Those complex phases, residing in a layer which is approximately 100 m thick, impact many features of neutron stars. Theoretical quantum-mechanical simulations of nuclear pasta are usually carried out in finite 3D boxes assuming periodic boundary conditions (PBC). The resulting solutions are affected by spurious finite-size effects. Purpose: In order to remove spurious finite-size effects, it is convenient to employ twist-averaged boundary conditions (TABC) used in condensed matter, nuclear matter, and lattice QCD applications. In this work, we study the effectiveness of TABC in the context of pasta phases simulations within nuclear density functional theory. Methods: We perform Skyrme-Hartree-Fock calculations in three dimensions by implementing Bloch boundary conditions. The TABC averages are obtained by means of Gauss-Legendre integration over twist angles. Results: We benchmark the TABC for a free nucleonic gas and apply it to simple cases such as the rod and slab phases, as well as to more elaborate P-surface and gyroidal phases. Conclusions: We demonstrate that by applying TABC reliable results can be obtained from calculations performed in relatively small volumes. By studying various contributions to the total energy, we gain insights into pasta phases in mid-density range.

nucl-th↗

arXiv2016

Time-dependent density functional theory with twist-averaged boundary conditions

Time-dependent density functional theory is widely used to describe excitations of many-fermion systems. In its many applications, 3D coordinate-space representation is used, and infinite-domain calculations are limited to a finite volume represented by a box. For finite quantum systems (atoms, molecules, nuclei), the commonly used periodic or reflecting boundary conditions introduce spurious quantization of the continuum states and artificial reflections from boundary; hence, an incorrect treatment of evaporated particles. These artifacts can be practically cured by introducing absorbing boundary conditions (ABC) through an absorbing potential in a certain boundary region sufficiently far from the described system. But also the calculations of infinite matter (crystal electrons, quantum fluids, neutron star crust) suffer artifacts from a finite computational box. In this regime, twist- averaged boundary conditions (TABC) have been used successfully to diminish the finite-volume effects. In this work, we extend TABC to time-dependent framework and apply it to resolve the box artifacts for finite quantum systems using as test case small- and large-amplitude nuclear vibrations. We demonstrate that by using such a method, one can reduce finite volume effects drastically without adding any additional parameters. While they are almost equivalent in the linear regime, TABC and ABC differ in the nonlinear regime in their treatment of evaporated particles.

nucl-th↗

arXiv2016

Unexpectedly large charge radii of neutron-rich calcium isotopes

Despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain "magic" numbers of protons and neutrons. The calcium chain in particular is both unique and puzzling: evidence of doubly-magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known Ca isotopes have been successfully described by nuclear theory, it is still a challenge to predict their charge radii evolution. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectroscopy experiments at ISOLDE, CERN. The experimental results are complemented by state-of-the-art theoretical calculations. The large and unexpected increase of the size of the neutron-rich calcium isotopes beyond N = 28 challenges the doubly-magic nature of 52Ca and opens new intriguing questions on the evolution of nuclear sizes away from stability, which are of importance for our understanding of neutron-rich atomic nuclei.

nucl-ex↗

arXiv2016

Nuclear rotation in the continuum

${\textbf{Background:}}$ Atomic nuclei often exhibit collective rotational-like behavior in highly excited states, well above the particle emission threshold. What determines the existence of collective motion in the continuum region, is not fully understood. ${\textbf{Purpose:}}$ In this work, by studying the collective rotation of the positive-parity deformed configurations of the one-neutron halo nucleus $^{11}$Be, we assess different mechanisms that stabilize collective behavior beyond the limits of particle stability. ${\textbf{Method:}}$ To solve a particle-plus-core problem, we employ a non-adiabatic coupled-channel formalism and the Berggren single-particle ensemble, which explicitly contains bound states, narrow resonances, and the scattering continuum. We study the valence-neutron density in the intrinsic rotor frame to assess the validity of the adiabatic approach as the excitation energy increases. ${\textbf{Results:}}$ We demonstrate that collective rotation of the ground band of $^{11}$Be is stabilized by (i) the fact that the $\ell=0$ one-neutron decay channel is closed, and (ii) the angular momentum alignment, which increases the parentage of high-$\ell$ components at high spins; both effects act in concert to decrease decay widths of ground-state band members. This is not the case for higher-lying states of $^{11}$Be, where the $\ell=0$ neutron-decay channel is open and often dominates. ${\textbf{Conclusion:}}$ We demonstrate that long-lived collective states can exist at high excitation energy in weakly bound neutron drip-line nuclei such as $^{11}$Be.

nucl-th↗

arXiv2016

Nuclear charge and neutron radii and nuclear matter: trend analysis

Radii of charge and neutron distributions are fundamental nuclear properties. They depend on both nuclear interaction parameters related to the equation of state of infinite nuclear matter and on quantal shell effects, which are strongly impacted by the presence of nuclear surface. In this work, by studying the dependence of charge and neutron radii, and neutron skin, on nuclear matter parameters, we assess different mechanisms that drive nuclear sizes. We apply nuclear density functional theory using a family of Skyrme functionals obtained by means of different optimization protocols targeting specific nuclear properties. By performing the Monte-Carlo sampling of reasonable functionals around the optimal parametrization, we study correlations between nuclear matter paramaters and observables characterizing charge and neutron distributions. We demonstrate the existence of the strong converse relation between the nuclear charge radii and the saturation density of symmetric nuclear matter and also between the neutron skins and the slope of the symmetry energy. For functionals optimized to experimental binding energies only, proton and neutron radii are weakly correlated due to canceling trends from different nuclear matter parameters. We show that by requiring that the nuclear functional reproduces the empirical saturation point of symmetric nuclear matter practically fixes the charge (or proton) radii, and vice versa. The neutron skin uncertainty primarily depends on the slope of the symmetry energy. Consequently, imposing a constraint on both $ρ_0$ and $L$ practically determines the nuclear size, modulo small variations due to shell effects.

nucl-th↗

arXiv2015

Charge, neutron, and weak size of the atomic nucleus

What is the size of the atomic nucleus? This deceivably simple question is difficult to answer. While the electric charge distributions in atomic nuclei were measured accurately already half a century ago, our knowledge of the distribution of neutrons is still deficient. In addition to constraining the size of atomic nuclei, the neutron distribution also impacts the number of nuclei that can exist and the size of neutron stars. We present an ab initio calculation of the neutron distribution of the neutron-rich nucleus $^{48}$Ca. We show that the neutron skin (difference between radii of neutron and proton distributions) is significantly smaller than previously thought. We also make predictions for the electric dipole polarizability and the weak form factor; both quantities are currently targeted by precision measurements. Based on ab initio results for $^{48}$Ca, we provide a constraint on the size of a neutron star.

nucl-th↗

arXiv2015

Multipole modes in deformed nuclei within the finite amplitude method

Background: To access selected excited states of nuclei, within the framework of nuclear density functional theory, the quasiparticle random phase approximation (QRPA) is commonly used. Purpose: We present a computationally efficient, fully self-consistent framework to compute the QRPA transition strength function of an arbitrary multipole operator in axially-deformed superfluid nuclei. Methods: The method is based on the finite amplitude method (FAM) QRPA, allowing fast iterative solution of QRPA equations. A numerical implementation of the FAM-QRPA solver module has been carried out for deformed nuclei. Results: The practical feasibility of the deformed FAM module has been demonstrated. In particular, we calculate the quadrupole and octupole strength in a heavy deformed nucleus $^{240}$Pu, without any truncations in the quasiparticle space. To demonstrate the capability to calculate individual QRPA modes, we also compute low-lying negative-parity collective states in $^{154}$Sm. Conclusions: The new FAM implementation enables calculations of the QRPA strength function throughout the nuclear landscape. This will facilitate global surveys of multipole modes and beta decays, and will open new avenues for constraining the nuclear energy density functional.

nucl-th↗

arXiv2015

Accurate nuclear radii and binding energies from a chiral interaction

With the goal of developing predictive ab-initio capability for light and medium-mass nuclei, two-nucleon and three-nucleon forces from chiral effective field theory are optimized simultaneously to low-energy nucleon-nucleon scattering data, as well as binding energies and radii of few-nucleon systems and selected isotopes of carbon and oxygen. Coupled-cluster calculations based on this interaction, named NNLO$_{\rm sat}$, yield accurate binding energies and radii of nuclei up to $^{40}$Ca, and are consistent with the empirical saturation point of symmetric nuclear matter. In addition, the low-lying collective $J^π=3^-$ states in $^{16}$O and $^{40}$Ca are described accurately, while spectra for selected $p$- and $sd$-shell nuclei are in reasonable agreement with experiment.

nucl-th↗

arXiv2015

Benchmarking Nuclear Fission Theory

We suggest a small set of fission observables to be used as test cases for validation of theoretical calculations. The purpose is to provide common data to facilitate the comparison of different fission theories and models. The proposed observables are chosen from fission barriers, spontaneous fission lifetimes, fission yield characteristics, and fission isomer excitation energies.

nucl-th↗

arXiv2015

Recoil-alpha-fission and recoil-alpha-alpha-fission events observed in the reaction Ca-48 + Am-243

Products of the fusion-evaporation reaction Ca-48 + Am-243 were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung. Amongst the detected thirty correlated alpha-decay chains associated with the production of element Z=115, two recoil-alpha-fission and five recoil-alpha-alpha-fission events were observed. The latter are similar to four such events reported from experiments performed at the Dubna gas-filled separator. Contrary to their interpretation, we propose an alternative view, namely to assign eight of these eleven decay chains of recoil-alpha(-alpha)-fission type to start from the 3n-evaporation channel 115-288. The other three decay chains remain viable candidates for the 2n-evaporation channel 115-289.

nucl-ex↗

arXiv2015

Uncertainty Quantification for Nuclear Density Functional Theory and Information Content of New Measurements

Statistical tools of uncertainty quantification can be used to assess the information content of measured observables with respect to present-day theoretical models; to estimate model errors and thereby improve predictive capability; to extrapolate beyond the regions reached by experiment; and to provide meaningful input to applications and planned measurements. To showcase new opportunities offered by such tools, we make a rigorous analysis of theoretical statistical uncertainties in nuclear density functional theory using Bayesian inference methods. By considering the recent mass measurements from the Canadian Penning Trap at Argonne National Laboratory, we demonstrate how the Bayesian analysis and a direct least-squares optimization, combined with high-performance computing, can be used to assess the information content of the new data with respect to a model based on the Skyrme energy density functional approach. Employing the posterior probability distribution computed with a Gaussian process emulator, we apply the Bayesian framework to propagate theoretical statistical uncertainties in predictions of nuclear masses, two-neutron dripline, and fission barriers. Overall, we find that the new mass measurements do not impose a constraint that is strong enough to lead to significant changes in the model parameters. The example discussed in this study sets the stage for quantifying and maximizing the impact of new measurements with respect to current modeling and guiding future experimental efforts, thus enhancing the experiment-theory cycle in the scientific method.

nucl-th↗

arXiv2014

Nuclear Energy Density Optimization: UNEDF2

The parameters of the UNEDF2 nuclear energy density functional (EDF) model were obtained in an optimization to experimental data consisting of nuclear binding energies, proton radii, odd-even mass staggering data, fission-isomer excitation energies, and single particle energies. In addition to parameter optimization, sensitivity analysis was done to obtain parameter uncertainties and correlations. The resulting UNEDF2 is an all-around EDF. However, the sensitivity analysis also demonstrated that the limits of current Skyrme-like EDFs have been reached and that novel approaches are called for.

nucl-th↗

arXiv2014

Bound and resonance states of the dipolar anion of hydrogen cyanide: competition between threshold effects and rotation in an open quantum system

Bound and resonance states of the dipole-bound anion of hydrogen cyanide HCN$^-$ are studied using a non-adiabatic pseudopotential method and the Berggren expansion technique involving bound states, decaying resonant states, and non-resonant scattering continuum. We devise an algorithm to identify the resonant states in the complex energy plane. To characterize spatial distributions of electronic wave functions, we introduce the body-fixed density and use it to assign families of resonant states into collective rotational bands. We find that the non-adiabatic coupling of electronic motion to molecular rotation results in a transition from the strong-coupling to weak-coupling regime. In the strong coupling limit, the electron moving in a subthreshold, spatially extended halo state follows the rotational motion of the molecule. Above the ionization threshold, electron's motion in a resonance state becomes largely decoupled from molecular rotation. Widths of resonance-band members depend primarily on the electron orbital angular momentum.

physics.atm-clus↗

arXiv2014

Pairing-induced speedup of nuclear spontaneous fission

Collective inertia is strongly influenced at the level crossing at which quantum system changes diabatically its microscopic configuration. Pairing correlations tend to make the large-amplitude nuclear collective motion more adiabatic by reducing the effect of those configuration changes. Competition between pairing and level crossing is thus expected to have a profound impact on spontaneous fission lifetimes. To elucidate the role of nucleonic pairing on spontaneous fission, we study the dynamic fission trajectories of $^{264}$Fm and $^{240}$Pu using the state-of-the-art self-consistent framework. We employ the superfluid nuclear density functional theory with the Skyrme energy density functional SkM$^*$ and a density-dependent pairing interaction. Along with shape variables, proton and neutron pairing correlations are taken as collective coordinates. The collective inertia tensor is calculated within the nonperturbative cranking approximation. The fission paths are obtained by using the least action principle in a four-dimensional collective space of shape and pairing coordinates. Pairing correlations are enhanced along the minimum-action fission path. For the symmetric fission of $^{264}$Fm, where the effect of triaxiality on the fission barrier is large, the geometry of fission pathway in the space of shape degrees of freedom is weakly impacted by pairing. This is not the case for $^{240}$Pu where pairing fluctuations restore the axial symmetry of the dynamic fission trajectory. The minimum-action fission path is strongly impacted by nucleonic pairing. In some cases, the dynamical coupling between shape and pairing degrees of freedom can lead to a dramatic departure from the static picture. Consequently, in the dynamical description of nuclear fission, particle-particle correlations should be considered on the same footing as those associated with shape degrees of freedom.

nucl-th↗

arXiv2014

Structure of Superheavy Nuclei Along Element 115 Decay Chains

A recent high-resolution $α$, $X$-ray, and $γ$-ray coincidence-spectroscopy experiment offered first glimpse of excitation schemes of isotopes along $α$-decay chains of $Z=115$. To understand these observations and to make predictions about shell structure of superheavy nuclei below $^{288}115$, we employ two complementary mean-field models: self-consistent Skyrme Energy Density Functional approach and the macroscopic-microscopic Nilsson model. We discuss the spectroscopic information carried by the new data. In particular, candidates for the experimentally observed $E1$ transitions in $^{276}$Mt are proposed. We find that the presence and nature of low-energy $E1$ transitions in well-deformed nuclei around $Z=110, N=168$ strongly depends on the strength of the spin-orbit coupling; hence, it provides an excellent constraint on theoretical models of superheavy nuclei. To clarify competing theoretical scenarios, an experimental search for $E1$ transitions in odd-$A$ systems $^{275,277}$Mt, $^{275}$Hs, and $^{277}$Ds is strongly recommended.

nucl-th↗

arXiv2014

Excitation energy dependence of fission in the mercury region

Background: Recent experiments on beta-delayed fission reported an asymmetric mass yield in the neutron-deficient nucleus 180Hg. Earlier experiments in the mass region A=190-200 close to the beta-stability line, using the (p,f) and (α,f) reactions, observed a more symmetric distribution of fission fragments. While the beta-delayed fission of 180Hg can be associated with relatively low excitation energy, this is not the case for light-ion reactions, which result in warm compound nuclei. Purpose: To elucidate the roles of proton and neutron numbers and excitation energy in determining symmetric and asymmetric fission yields, we compute and analyze the isentropic potential energy surfaces of 174,180,198Hg and 196,210Po. Methods: We use the finite-temperature superfluid nuclear density functional theory, for excitation energies up to E*=30MeV and zero angular momentum. For our theoretical framework, we consider the Skyrme energy density functional SkM* and a density-dependent pairing interaction. Results: For 174,180Hg, we predict fission pathways consistent with asymmetric fission at low excitation energies, with the symmetric fission pathway opening very gradually as excitation energy is increased. For 198Hg and 196Po, we expect the nearly-symmetric fission channel to dominate. 210Po shows a preference for a slightly asymmetric pathway at low energies, and a preference for a symmetric pathway at high energies. Conclusions: Our self-consistent theory suggests that excitation energy weakly affects the fission pattern of the nuclei considered. The transition from the asymmetric fission in the proton-rich nuclei to a more symmetric fission in the heavier isotopes is governed by the shell structure of pre-scission configurations.

nucl-th↗