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Wenbin Zhang

Publications and source records attributed to Wenbin Zhang.

103 records · Page 6Linked to original sources

Disentangling the role of laser coupling in directional breaking of molecules

The directional control of molecular dissociation with the laser electric field waveform is a paradigm and was demonstrated for a variety of molecules. In most cases, the directional control occurs via a dissociative ionization pathway. The role of laser-induced coupling of electronic states in the dissociating ion versus selective ionization of oriented neutral molecules, however, could not be distinguished for even small heteronuclear molecules such as CO. Here, we introduce a technique, using elliptically polarized pump and linearly polarized two-color probe pulses that unambiguously distinguishes the roles of laser-induced state coupling and selective ionization. The measured photoelectron momentum distributions governed by the light polarizations allow us to coincidently identify the ionization and dissociation from the pump and probe pulses. Directional dissociation of CO+ as a function of the relative phase of the linearly polarized two-color pulse is observed for both parallel and orthogonally oriented molecules. We find that the laser-induced coupling of various electronic states of CO+ plays an important role for the observed directional bond breaking, which is verified by quantum calculations.

physics.optics↗

Molecular echoes in space and time

Mountain echoes are a well-known phenomenon, where an impulse excitation is mirrored by the rocks to generate a replica of the original stimulus, often with reverberating recurrences. For spin echoes in magnetic resonance and photon echoes in atomic and molecular systems the role of the mirror is played by a second, time delayed pulse which is able to reverse the ow of time and recreate the original event. Recently, laser-induced rotational alignment and orientation echoes were introduced for molecular gases, and discussed in terms of rotational-phase-space filamentation. Here we present, for the first time, a direct spatiotemporal analysis of various molecular alignment echoes by means of coincidence Coulomb explosion imaging. We observe hitherto unreported spatially rotated echoes, that depend on the polarization direction of the pump pulses, and find surprising imaginary echoes at negative times.

physics.optics↗

News-Based Group Modeling and Forecasting

In this paper, we study news group modeling and forecasting methods using quantitative data generated by our large-scale natural language processing (NLP) text analysis system. A news group is a set of news entities, like top U.S. cities, governors, senators, golfers, or movie actors. Our fame distribution analysis of news groups shows that log-normal and power-law distributions generally could describe news groups in many aspects. We use several real news groups including cities, politicians, and CS professors, to evaluate our news group models in terms of time series data distribution analysis, group-fame probability analysis, and fame-changing analysis over long time. We also build a practical news generation model using a HMM (Hidden Markov Model) based approach. Most importantly, our analysis shows the future entity fame distribution has a power-law tail. That is, only a small number of news entities in a group could become famous in the future. Based on these analysis we are able to answer some interesting forecasting problems - for example, what is the future average fame (or maximum fame) of a specific news group? And what is the probability that some news entity become very famous within a certain future time range? We also give concrete examples to illustrate our forecasting approaches.

cs.SI↗

A Multi-factor Adaptive Statistical Arbitrage Model

This paper examines the implementation of a statistical arbitrage trading strategy based on co-integration relationships where we discover candidate portfolios using multiple factors rather than just price data. The portfolio selection methodologies include K-means clustering, graphical lasso and a combination of the two. Our results show that clustering appears to yield better candidate portfolios on average than naively using graphical lasso over the entire equity pool. A hybrid approach of using the combination of graphical lasso and clustering yields better results still. We also examine the effects of an adaptive approach during the trading period, by re-computing potential portfolios once to account for change in relationships with passage of time. However, the adaptive approach does not produce better results than the one without re-learning. Our results managed to pass the test for the presence of statistical arbitrage test at a statistically significant level. Additionally we were able to validate our findings over a separate dataset for formation and trading periods.

q-fin.PM↗

Orbital stability of peakons for a generalized Camassa-Holm equation with both quadratic and cubic nonlinearity

In this paper, we investigate the orbital stability problem of peakons for a modified Camassa-Holm equation with both quadratic and cubic nonlinearity. This equation was derived from integrable theory and admits peaked soliton (peakon) and multipeakon solutions. By constructing two suitable piecewise functions, we establish the polynomial inequality relating to two conserved quantities and the maximum of the solution to this equation. The error estimate between the maximum of the solution and the peakon then follows from the structure of the polynomial inequality. Finally, we prove that a wave starting close to the peakon remains close to some translate of it at all later times, that is, the shapes of these peakons are stable under small perturbations.

math.AP↗

Nanoparticle enhanced evaporation of liquids: A case study of silicone oil and water

Evaporation is a fundamental physical phenomenon, of which many challenging questions remain unanswered. Enhanced evaporation of liquids in some occasions is of enormous practical significance. Here we report the enhanced evaporation of the nearly permanently stable silicone oil by dispersing with nanopariticles including CaTiO3, anatase and rutile TiO2. The results can inspire the research of atomistic mechanism for nanoparticle enhanced evaporation and exploration of evaporation control techniques for treatment of oil pollution and restoration of dirty water.

cond-mat.mes-hall↗

Group Operads and Homotopy Theory

We introduce the classical theory of the interplay between group theory and topology into the context of operads and explore some applications to homotopy theory. We first propose a notion of a group operad and then develop a theory of group operads, extending the classical theories of groups, spaces with actions of groups, covering spaces and classifying spaces of groups. In particular, the fundamental groups of a topological operad is naturally a group operad and its higher homotopy groups are naturally operads with actions of its fundamental groups operad, and a topological $K(π,1)$ operad is characterized by and can be reconstructed from its fundamental groups operad. Two most important examples of group operads are the symmetric groups operad and the braid groups operad which provide group models for $Ω^{\infty} Σ^{\infty} X$ (due to Barratt and Eccles) and $Ω^2 Σ^2 X$ (due to Fiedorowicz) respectively. We combine the two models together to produce a free group model for the canonical stabilization $Ω^2 Σ^2 X \hookrightarrow Ω^{\infty} Σ^{\infty} X$, in particular a free group model for its homotopy fibre.

math.AT↗

Operations on Spaces over Operads and Applications to Homotopy Groups

We establish certain smash operations on spaces over operads which are general analogues of the Samelson product on single loop spaces, and obtain a conceptual description of the structure of the homotopy groups of spaces $Y$ over a symmetric $K(π,1)$ operad: $π_*Y$ is a module over the free algebraic symmetric operad generated by operations on homotopy groups induced by these smash operations. In particular the homotopy groups of double loop spaces is a module over the free algebraic symmetric operad generated by the conjugacy classes of Brunnian braids modulo the conjugation action of pure braids.

math.AT↗

Pattern formation in weakly damped parametric surface waves driven by two frequency components

A quasi-potential approximation to the Navier-Stokes equation for low viscosity fluids is developed to study pattern formation in parametric surface waves driven by a force that has two frequency components. A bicritical line separating regions of instability to either one of the driving frequencies is explicitly obtained, and compared with experiments involving a frequency ratio of 1/2. The procedure for deriving standing wave amplitude equations valid near onset is outlined for an arbitrary frequency ratio following a multiscale asymptotic expansion of the quasi-potential equations. Explicit results are presented for subharmonic response to a driving force of frequency ratio 1/2, and used to study pattern selection. Even though quadratic terms are prohibited in this case, hexagonal or triangular patterns are found to be stable in a relatively large parameter region, a fact that is in qualitative agreement with experimental results.

patt-sol↗

Pattern formation in weakly damped Faraday waves

We present a theoretical study of nonlinear pattern formation in parametric surface waves for fluids of low viscosity, and in the limit of large aspect ratio. The analysis is based on a quasi-potential approximation to the equations governing fluid motion, followed by a multiscale asymptotic expansion in the distance away from threshold. Close to onset, the asymptotic expansion yields an amplitude equation which is of gradient form, and allows the explicit calculation of the functional form of the cubic nonlinearities. In particular, we find that three-wave resonant interactions contribute significantly to the nonlinear terms, and therefore are important for pattern selection. Minimization of the associated Lyapunov functional predicts a primary bifurcation to a standing wave pattern of square symmetry for capillary-dominated surface waves, in agreement with experiments. In addition, we find that patterns of hexagonal and quasi-crystalline symmetry can be stabilized in certain mixed capillary-gravity waves, even in this case of single frequency forcing. Quasi-crystalline patterns are predicted in a region of parameters readily accessible experimentally.

patt-sol↗

Square Patterns and Quasi-patterns in Weakly Damped Faraday Waves

Pattern formation in parametric surface waves is studied in the limit of weak viscous dissipation. A set of quasi-potential equations (QPEs) is introduced that admits a closed representation in terms of surface variables alone. A multiscale expansion of the QPEs reveals the importance of triad resonant interactions, and the saturating effect of the driving force leading to a gradient amplitude equation. Minimization of the associated Lyapunov function yields standing wave patterns of square symmetry for capillary waves, and hexagonal patterns and a sequence of quasi-patterns for mixed capillary-gravity waves. Numerical integration of the QPEs reveals a quasi-pattern of eight-fold symmetry in the range of parameters predicted by the multiscale expansion.

patt-sol↗

Secondary Instabilities and Spatiotemporal Chaos in Parametric Surface Waves

A two dimensional model is introduced to study pattern formation, secondary instabilities and the transition to spatiotemporal chaos (weak turbulence) in parametric surface waves. The stability of a periodic standing wave state above onset is studied against Eckhaus, zig-zag and transverse amplitude modulations (TAM) as a function of the control parameter $\varepsilon$ and the detuning. A mechanism leading to a finite threshold for the TAM instability is identified. Numerical solutions of the model are in agreement with the stability diagram, and also reveal the existence of a transition to spatiotemporal chaotic states at a finite $\varepsilon$. Power spectra of temporal fluctuations in the chaotic state are broadband, decaying as a power law of the frequency $ω^{-z}$ with $z \approx 4.0$.

patt-sol↗

Narrow band noise as a model of time-dependent accelerations: study of the stability of a fluid surface in a microgravity environment

We introduce a stochastic model to analyze in quantitative detail the effect of the high frequency components of the residual accelerations onboard spacecraft (often called g-jitter) on fluid motion. The residual acceleration field is modeled as a narrow band noise characterized by three independent parameters: its intensity $G^{2}$, a dominant frequency $Ω$, and a characteristic spectral width $τ^{-1}$. The white noise limit corresponds to $Ωτ\rightarrow 0$, with $G^{2} τ$ finite, and the limit of a periodic g-jitter (or deterministic limit) can be recovered for $Ωτ\rightarrow \infty$, $G^{2}$ finite. The analysis of the response of a fluid surface subjected to a fluctuating gravitational field leads to the stochastic Mathieu equation driven by both additive and multiplicative noise. We discuss the stability of the solutions of this equation in the two limits of white noise and deterministic forcing, and in the general case of narrow band noise. The results are then applied to typical microgravity conditions.

cond-mat↗