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Wilhelm Kadow

Publications and source records attributed to Wilhelm Kadow.

11 recordsLinked to original sources

Fractionalization from Kinetic Frustration in Doped Two-Dimensional SU(4) Quantum Magnets

Separating electrons into emergent fractional quasiparticles is a hallmark of exotic quantum phases of matter with strong interactions. Understanding under which circumstances fractionalized excitations appear is a major conceptual challenge and can help realize long sought-after states, such as quantum spin liquids. Here, we identify a distinct mechanism for fractionalization. Starting from the plaquette-ordered ground state of an SU(4) symmetric t-J model at quarter filling on frustrated triangular lattices, we reveal a compelling interplay between order and fractionalization as a function of doping. For hole doping, we find that the kinetic frustration can be relieved by fractionalizing the holes into fermionic spinons and bosonic holons: the holons minimize their kinetic energy when the spinons form a spinon Fermi surface. We support this mechanism analytically in the large-N limit as well as numerically by simulating the SU(4) case with matrix product states on cylinder geometries and with variational Monte Carlo methods on system sizes up to 40x40. Conversely, electron doping drives the system into a ferromagnetic phase, akin to Nagaoka's theorem. We discuss possible experimental realizations in moir\'e heterostructures as well as ultracold atoms, and propose dynamical probes to search for key characteristics of the fractionalized quasiparticles.

cond-mat.str-el

Digital quantum magnetism on a trapped-ion quantum computer

Digital quantum matter -- realized when discrete quantum gates approximate continuous time evolution -- is susceptible to heating into chaotic, structureless states. If digitization errors are adequately suppressed, a long-lived transient regime of approximately energy-conserving dynamics can be observed on gate-based quantum computers. Conservation of energy, in turn, enables the exploration of a wide variety of complex behaviors observed in equilibrium systems, ranging from the nontrivial microscopic origins of thermalization itself to the stabilization of effective models hosting exotic emergent properties. Here, we use Quantinuum's system model H2 quantum computer to simulate digitized dynamics of the quantum Ising model, suppressing digitization errors well enough to observe thermalization on timescales that severely challenge classical simulation methods. Relaxation of an inhomogeneous state reveals an emergent hydrodynamics due to approximate energy conservation, and we compute the associated diffusion constant. By reprogramming our simulations to take place on a triangular lattice with periodic boundary conditions, we observe thermalization consistent with emergent gauge and topological constraints resulting from lattice frustration. Our results were enabled by continued advances in two-qubit gate quality (native partial entangler fidelities of $99.94(1)\%$), and establish digital quantum computers as powerful tools for studying (effectively) continuous-time dynamics.

quant-ph

Gate-tunable Bose-Fermi mixture in a strongly correlated moir\'e bilayer electron system

Quantum gases consisting of species with distinct quantum statistics, such as Bose-Fermi mixtures, can behave in a fundamentally different way than their unmixed constituents. This makes them an essential platform for studying emergent quantum many-body phenomena such as mediated interactions and unconventional pairing. Here, we realize an equilibrium Bose-Fermi mixture in a bilayer electron system implemented in a WS$_{2}$/WSe$_{2}$ moir\'e heterobilayer with strong Coulomb coupling to a nearby moir\'e-free WSe$_{2}$ monolayer. Absent the fermionic component, the underlying bosonic phase manifests as a dipolar excitonic insulator. By injecting excess charges into it, we show that the bosonic phase forms a stable mixture with added electrons but abruptly collapses upon hole doping. We develop a microscopic model to explain the unusual asymmetric stability with respect to electron and hole doping. By studying the Bose-Fermi mixture via monitoring excitonic resonances from both layers, we demonstrate gate-tunability over a wide range in the boson/fermion density phase space, in excellent agreement with theoretical calculations. Our results further the understanding of phases stabilized in moir\'e bilayer electron systems and demonstrate their potential for exploring the exotic properties of equilibrium Bose-Fermi mixtures.

cond-mat.str-el

Single-particle spectral function of fractional quantum anomalous Hall states

Fractional quantum Hall states are the most prominent example of states with topological order, hosting excitations with fractionalized charge. Recent experiments in twisted $\text{MoTe}_2$ and graphene-based heterostructures provided evidence of fractional quantum anomalous Hall (FQAH) states, which spontaneously break time-reversal symmetry and persist even without an external magnetic field. Understanding the unique properties of these states requires the characterization of their low-energy excitations. To that end, we construct a parton theory for the energy and momentum-resolved single-particle spectral function of FQAH states. We explicitly consider several experimentally observed filling fractions as well as a composite Fermi liquid in the half-filled Chern band. The parton description qualitatively captures our numerical exact diagonalization results. Additionally, we discuss how the finite bandwidth of the Chern band and the non-ideal quantum geometry affect the fractionalized excitations. Our work demonstrates that the energy and momentum-resolved electronic single-particle spectral function provides a valuable tool to characterize fractionalized excitations of FQAH states in moir\'e lattices.

cond-mat.mes-hall

Tensor Network Python (TeNPy) version 1

TeNPy (short for 'Tensor Network Python') is a python library for the simulation of strongly correlated quantum systems with tensor networks. The philosophy of this library is to achieve a balance of readability and usability for new-comers, while at the same time providing powerful algorithms for experts. The focus is on MPS algorithms for 1D and 2D lattices, such as DMRG ground state search, as well as dynamics using TEBD, TDVP, or MPO evolution. This article is a companion to the recent version 1.0 release of TeNPy and gives a brief overview of the package.

cond-mat.str-el

Probing magnetism in moir\'e heterostructures with quantum twisting microscopes

Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum resolved spectrum of single-particle and collective excitations, can be used as a novel tool to distinguish between different types of magnetic order. To this end, we calculate the single-particle spectral function and the dynamical spin-structure factor for both a ferromagnetic and antiferromagnetic generalized Wigner crystal formed in fractionally filled moir\'e superlattices of transition metal dichalcogenide heterostructures. We demonstrate that magnetic order can be clearly identified in these response functions. Furthermore, we explore signatures of quantum phase transitions in the quantum twisting microscope response. We focus on the specific case of triangular moir\'e lattices at half filling, which have been proposed to host a topological phase transition between a chiral spin liquid and a 120 degree ordered state. Our work demonstrates the potential for quantum twisting microscopes to characterize quantum magnetism in moir\'e heterostructures.

cond-mat.str-el

Single-hole spectra of Kitaev spin liquids: from dynamical Nagaoka ferromagnetism to spin-hole fractionalization

The dynamical response of a quantum spin liquid upon injecting a hole is a pertinent open question. In experiments, the hole spectral function, measured momentum-resolved in angle-resolved photoemission spectroscopy (ARPES) or locally in scanning tunneling microscopy (STM), can be used to identify spin liquid materials. In this study, we employ tensor network methods to simulate the time evolution of a single hole doped into the Kitaev spin-liquid ground state. Focusing on the gapped spin liquid phase, we reveal two fundamentally different scenarios. For ferromagnetic spin couplings, the spin liquid is highly susceptible to hole doping: a Nagaoka ferromagnet forms dynamically around the doped hole, even at weak coupling. By contrast, in the case of antiferromagnetic spin couplings, the hole spectrum demonstrates an intricate interplay between charge, spin, and flux degrees of freedom, best described by a parton mean-field ansatz of fractionalized holons and spinons. Moreover, we find a good agreement of our numerical results to the analytically solvable case of slow holes. Our results demonstrate that dynamical hole spectral functions provide rich information on the structure of fractionalized quantum spin liquids.

cond-mat.str-el

Kinetic Ferromagnetism and Topological Magnons of the Hole-Doped Kitaev Spin Liquid

We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange $K$ the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group (DMRG) simulations on finite systems, we uncover that the introduction of a single hole with a hopping strength of just $t\sim{}0.28K$ is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic spin exchange $\varGamma$ drives the polarization towards the [111] direction via a reorientation transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic spinons/magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental signatures and implications for Kitaev candidate materials.

cond-mat.str-el

Isometric tensor network representations of two-dimensional thermal states

Tensor networks provide a useful tool to describe low-dimensional complex many-body systems. Finding efficient algorithms to use these methods for finite-temperature simulations in two dimensions is a continuing challenge. Here, we use the class of recently introduced isometric tensor network states, which can also be directly realized with unitary gates on a quantum computer. We utilize a purification ansatz to efficiently represent thermal states of the transverse field Ising model. By performing an imaginary-time evolution starting from infinite temperature, we find that this approach offers a different way with low computational complexity to represent states at finite temperatures.

cond-mat.str-el

Chiral Pseudo Spin Liquids in Moire Heterostructures

We propose multi-layer moire structures in strong external magnetic fields as a novel platform for realizing highly-tunable, frustrated Hubbard physics with topological order. Identifying the layer degree of freedom as a pseudo spin, allows us to retain SU(2) symmetry while controlling ring-exchange processes and concurrently quenching the kinetic energy by large external magnetic fields. This way, a broad class of interacting Hubbard-Hofstadter states and their transitions can be studied. Remarkably, in the limit of strong interactions the system becomes Mott insulating and we find chiral pseudo spin liquid phases which are induced by the magnetic field. We find that this topologically ordered state remains exceptionally stable towards relevant perturbations. We discuss how layer pseudo-spin can be probed in near-term experiments. As the magnetic flux can be easily tuned in moire systems, our approach provides a promising route towards the experimental realization and control of topologically ordered phases of matter.

cond-mat.str-el

Hole Spectral Function of a Chiral Spin Liquid in the Triangular Lattice Hubbard Model

Quantum spin liquids are fascinating phases of matter, hosting fractionalized spin excitations and unconventional long-range quantum entanglement. These exotic properties, however, also render their experimental characterization challenging, and finding ways to diagnose quantum spin liquids is therefore a pertinent challenge. Here, we numerically compute the spectral function of a single hole doped into the half-filled Hubbard model on the triangular lattice using techniques based on matrix product states. At half-filling the system has been proposed to realize a chiral spin liquid at intermediate interaction strength, surrounded by a magnetically ordered phase at strong interactions and a superconducting/metallic phase at weak interactions. We find that the spectra of these phases exhibit distinct signatures. By developing appropriate parton mean-field descriptions, we gain insight into the relevant low-energy features. While the magnetic phase is characterized by a dressed hole moving through the ordered spin background, we find indications of spinon dynamics in the chiral spin liquid. Our results suggest that the hole spectral function, as measured by angle-resolved photoemission spectroscopy, provides a useful tool to characterize quantum spin liquids.

cond-mat.str-el