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Wolfgang Ketterle

Publications and source records attributed to Wolfgang Ketterle.

At least 19 recordsLinked to original sources
arXiv2026

Can Bose-Einstein condensates enhance radioactive decay?

This paper lays out the principles of how Bose-Einstein condensates can modify radioactive decay. We highlight the challenges of many modes and short coherence times due to the $\approx$ MeV energies of the emitted radiation. Recent proposals for gamma ray and neutrino lasers claim that using a Bose-Einstein condensate as a source would solve these issues. We show that this is not the case, and the proposed experiments would have a gain of only $10^{-16}$ or smaller. We also analyze proposals for gamma ray lasers based on stimulated annihilation of positronium Bose-Einstein condensates.

quant-ph↗
arXiv2026

Fringe visibility and which-way information in Young's double slit experiments with light scattered from single atoms

Young's double slit experiment has often been used to illustrate the concept of complementarity in quantum mechanics. If information can in principle be obtained about the path of the photon, then the visibility of the interference fringes is reduced or even destroyed. This Gedanken experiment discussed by Bohr and Einstein can be realized when the slit is replaced by individual atoms sensitive to the transferred recoil momentum of a photon which "passes through the slit". Early pioneering experiments were done with trapped ions and atom pairs created via photo-dissociation. Recently, it became possible to perform interference experiments with single neutral atoms cooled to the absolute ground state of a harmonic oscillator potential. The slits are now single atoms representing a two-level system, and the excitation in the harmonic oscillator potential is the which-way marker. In this note, we analyze and generalize two recent experiments performed with single atoms and emphasize the different ways they record which-way information.

quant-ph↗
arXiv2026

Fundamental impossibility of a superradiant neutrino laser

Here we address the fundamental question of whether an idealized system of $N$ atoms will show collective behavior and superradiance when it emits fermions instead of photons. We show that for single-fermion emission processes, the maximum emission is $\propto N$ and not $\propto N^2$, which proves the absence of superradiance and shows that the recent proposal to realize a superradiant neutrino laser is impossible. This can be understood as either destructive interference of fermionic transition amplitudes, or Pauli blockade by collective excitations with fermionic nature. We derive the exact solution of the fermionic Dicke problem and analyze the decay dynamics in various regimes. We extend the proof to arbitrary Hamiltonians and show that the jump rate operator for neutrino emission has a maximum eigenvalue of $N$ times the single-particle rate $Γ_0$. States with low excitation can show collective behavior and emit at a rate of $N Γ_0$.

quant-ph↗
arXiv2026

Suppression and enhancement of bosonic stimulation by atomic interactions

The tendency of identical bosons to bunch, seen in the Hanbury Brown-Twiss effect and Bose-Einstein condensation, is a hallmark of quantum statistics. This bunching can enhance the rates of fundamental processes such as atom-atom and atom-light scattering when atoms scatter into already occupied states. For non-interacting bosons, the enhancement of light scattering follows directly from the occupation of the atom's final momentum state. Here, we study scattering between off-resonant light and atoms in a quasi-homogeneous Bose gas with tunable interactions and show that even weak interactions, which do not significantly alter the momentum distribution, strongly affect atom-light scattering. Changes in local atomic correlations suppress the bosonic enhancement under weak repulsive interactions and increase the scattering rate under attractive ones. Moreover, if the interactions are rapidly tuned, light scattering reveals correlation dynamics that are orders of magnitude faster than the collisional dynamics of the momentum-space populations. Its extreme sensitivity to correlation effects makes off-resonant light scattering a powerful probe of many-body physics in ultracold atomic gases.

cond-mat.quant-gas↗
arXiv2025

Suppression of coherent light scattering in a three-dimensional atomic array

Understanding how atoms collectively interact with light is not only important for fundamental science, but also crucial for designing light-matter interfaces in quantum technologies. Over the past decades, numerous studies have focused on arranging atoms in ordered arrays and using constructive (destructive) interference to enhance (suppress) the coupling to electromagnetic fields, thereby tailoring collective light-matter interactions. These studies have mainly focused on one- and two-dimensional arrays. However, only three-dimensional (3D) arrays can demonstrate destructive interference of coherent light scattering in all directions. This omnidirectional suppression of coherent light scattering in 3D atomic arrays has thus far not been experimentally demonstrated. Here, we observe a strong reduction of light scattering in a 3D atomic array prepared in the form of a Mott insulator in optical lattices. The residual light scattering is shown to be caused by the delocalization of atoms, Raman scattering, and inelastic scattering associated with saturation. We also demonstrate how light scattering can be a sensitive probe for density fluctuations in many-body states in optical lattices, enabling us to characterize the superfluid-to-Mott insulator phase transition as well as defects generated by dynamical parameter ramps. The results of our work can be used to prepare subradiant states for photon storage and probe correlations for many-body systems in optical lattices.

cond-mat.quant-gas↗
arXiv2025

Probing quantum many-body dynamics using subsystem Loschmidt echos

The Loschmidt echo - the probability of a quantum many-body system to return to its initial state following a dynamical evolution - generally contains key information about a quantum system, relevant across various scientific fields including quantum chaos, quantum many-body physics, or high-energy physics. However, it is typically exponentially small in system size, posing an outstanding challenge for experiments. Here, we experimentally investigate the subsystem Loschmidt echo, a quasi-local observable that captures key features of the Loschmidt echo while being readily accessible experimentally. Utilizing quantum gas microscopy, we study its short- and long-time dynamics. In the short-time regime, we observe a dynamical quantum phase transition arising from genuine higher-order correlations. In the long-time regime, the subsystem Loschmidt echo allows us to quantitatively determine the effective dimension and structure of the accessible Hilbert space in the thermodynamic limit. Performing these measurements in the ergodic regime and in the presence of emergent kinetic constraints, we provide direct experimental evidence for ergodicity breaking due to fragmentation of the Hilbert space. Our results establish the subsystem Loschmidt echo as a novel and powerful tool that allows paradigmatic studies of both non-equilibrium dynamics and equilibrium thermodynamics of quantum many-body systems, applicable to a broad range of quantum simulation and computing platforms.

cond-mat.quant-gas↗
arXiv2024

In situ imaging of the thermal de Broglie wavelength in an ultracold Bose gas

We report the first in situ observation of density fluctuations on the scale of the thermal de Broglie wavelength in an ultracold gas of bosons. Bunching of $^{87}$Rb atoms in a quasi two-dimensional system is observed by single-atom imaging using a quantum gas microscope. Compared to a classical ensemble, we observe a 30 percent enhancement of the second-order correlation function. We show the spatial and thermal dependence of these correlations. The reported method of detecting in situ correlations can be applied to interacting many-body systems and to the study of critical phenomena near phase transitions.

cond-mat.quant-gas↗
arXiv2024

Coherent and incoherent light scattering by single-atom wavepackets

We study light scattering of single atoms in free space and discuss the results in terms of atom-photon entanglement and which-way information. Using ultracold atoms released from an optical lattice, we realize a Gedanken experiment which interferes single photons scattering off of Heisenberg uncertainty-limited wavepackets. We unify the free-space and trapped-atom pictures by measuring the light scattered during wavepacket expansion and show the coherence properties of the scattered light is independent of the presence of the trap. Our experiment demonstrates the potential of using atomic Mott insulators to create single-atom wavepackets for fundamental studies.

quant-ph↗
arXiv2024

Collisional Cooling of Ultracold Molecules

Since the original work on Bose-Einstein condensation, quantum degenerate gases of atoms have allowed the quantum emulation of important systems from condensed matter and nuclear physics, as well as the study of novel many-body states with no analog in other fields of physics. Ultracold molecules in the micro- and nano-Kelvin regimes promise to bring powerful new capabilities to quantum emulation and quantum computing, thanks to their rich internal degrees of freedom compared to atoms. They also open new possibilities for precision measurement and the study of quantum chemistry. Quantum gases of atoms were made possible by collision-based cooling schemes, such as evaporative cooling. For ultracold molecules, thermalization and collisional cooling have not been realized. With other techniques such as supersonic jets and cryogenic buffer gases, studies have been limited to temperatures above 10 mK. Here we show cooling of NaLi molecules at micro- and nano-Kelvin temperatures through collisions with ultracold Na atoms, both prepared in their stretched hyperfine spin states. We find a lower bound on the elastic to inelastic collision ratio between molecules and atoms greater than 50 -- large enough to support sustained collisional cooling. By employing two stages of evaporation, we increase the phase-space density (PSD) of the molecules by a factor of 20, achieving temperatures as low as 220 nK. The favorable collisional properties of a Na and NaLi mixture show great promise for making deeply quantum degenerate dipolar molecules and suggest the potential for such cooling in other systems.

cond-mat.quant-gas↗
arXiv2024

Observation of spin squeezing with contact interactions in one- and three-dimensional easy-plane magnets

Entanglement in a many-particle system can enable measurement sensitivities beyond that achievable by only classical correlations. For an ensemble of spins, all-to-all interactions are known to reshape the quantum projection noise, leading to a form of entanglement known as spin squeezing. Here, we demonstrate spin squeezing with strictly short-range contact interactions. In particular, working with ultracold lithium atoms in optical lattices, we utilize superexchange interactions to realize a nearest-neighbor anisotropic Heisenberg model. We investigate the resulting quench dynamics from an initial product state in both one and three dimensions. In 1D, we observe $1.9^{+0.7}_{-0.5}$ dB of spin squeezing in quantitative agreement with theory. However, in 3D, we observe a maximum of $2.0^{+0.7}_{-0.7}$ dB of squeezing, over an order of magnitude smaller than that expected. We demonstrate that this discrepancy arises from the presence of a finite density of holes; both the motion of the holes as well as direct coupling between spin and density qualitatively alter the spin dynamics. Our observations point to the importance of understanding the complex interplay between motional and spin degrees of freedom in quantum simulators.

quant-ph↗
arXiv2024

A conveyor-belt magneto-optical trap of CaF

We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $μ$m and a peak number density of $3.6(5) \times 10^{10}$ cm$^{-3}$, a 600-fold increase over the conventional red-detuned MOTs of CaF, and the densest molecular MOT observed to date. Subsequent loading of these molecules into an optical dipole trap yields up to $2.6 \times 10^4$ trapped molecules at a temperature of 14(2) $μ$K with a peak phase-space density of $\sim 2.4 \times 10^{-6}$. This opens new possibilities for a range of applications utilizing high-density, optically trapped ultracold molecules.

physics.atom-ph↗
arXiv2023

Raman sideband cooling of molecules in an optical tweezer array to the 3-D motional ground state

Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules. Further cooling of the molecules to near the motional ground state is crucial for reducing various dephasings in quantum and precision applications. In this work, we demonstrate Raman sideband cooling of CaF molecules in optical tweezers to near their motional ground state, with average motional occupation quantum numbers of $\bar{n}_{x}=0.16(12)$, $\bar{n}_{y}=0.17(17)$ (radial directions), $\bar{n}_{z}=0.22(16)$ (axial direction) and a 3-D motional ground state probability of $54\pm18\%$. This paves the way to increase molecular coherence times in optical tweezers for robust quantum computation and simulation applications.

physics.atom-ph↗
arXiv2023

Dynamics of Stripe Patterns in Supersolid Spin-Orbit-Coupled Bose Gases

Despite ground-breaking observations of supersolidity in spin-orbit-coupled Bose-Einstein condensates, until now the dynamics of the emerging spatially periodic density modulations has been vastly unexplored. Here, we demonstrate the nonrigidity of the density stripes in such a supersolid condensate and explore their dynamic behavior subject to spin perturbations. We show both analytically in infinite systems and numerically in the presence of a harmonic trap how spin waves affect the supersolid's density profile in the form of crystal waves, inducing oscillations of the periodicity as well as the orientation of the fringes. Both these features are well within reach of present-day experiments. Our results show that this system is a paradigmatic supersolid, featuring superfluidity in conjunction with a fully dynamic crystalline structure.

cond-mat.quant-gas↗
arXiv2023

Ab initio calculation of the spectrum of Feshbach resonances in NaLi + Na collisions

We present a combined experimental and theoretical study of the spectrum of magnetically tunable Feshbach resonances in NaLi $(a^3Σ^+)$ $+$ Na collisions. In the accompanying paper, we observe experimentally 8 and 17 resonances occur between $B=0$ and $1400$~G in upper and lower spin-stretched states, respectively. Here, we perform ab initio calculations of the NaLi $+$ Na interaction potential and describe in detail the coupled-channel scattering calculations of the Feshbach resonance spectrum. The positions of the resonances cannot be predicted with realistic uncertainty in the state-of-the-art ab initio potential, but our calculations yield a typical number of resonances that is in near-quantitative agreement with experiment. We show that the main coupling mechanism results from spin-rotation and spin-spin couplings in combination with the anisotropic atom-molecule interaction. The calculations furthermore explain the qualitative difference between the numbers of resonances in either spin state.

physics.atom-ph↗
arXiv2023

Can the dipolar interaction suppress dipolar relaxation?

Magnetic atoms in a thin layer have repulsive interactions when their magnetic moments are aligned perpendicular to the layer. We show experimentally and theoretically how this can suppress dipolar relaxation, the dominant loss process in spin mixtures of highly magnetic atoms. Using dysprosium, we observe an order of magnitude extension of the lifetime, and another factor of ten is within reach based on the models which we have validated with our experimental study. The loss suppression opens up many new possibilities for quantum simulations with spin mixtures of highly magnetic atoms.

cond-mat.quant-gas↗
arXiv2023

Spectrum of Feshbach resonances in NaLi $+$ Na collisions

Collisional resonances of molecules can offer a deeper understanding of interaction potentials and collision complexes, and allow control of chemical reactions. Here, we experimentally map out the spectrum of Feshbach resonances in collisions between ultracold triplet ro-vibrational ground-state NaLi molecules and Na atoms over a range of 1400 G. Preparation of the spin-stretched state puts the system initially into the non-reactive quartet potential. A total of 25 resonances are observed, in agreement with quantum-chemistry calculations using a coupled-channels approach. Although the theory cannot predict the positions of resonances, it can account for several experimental findings and provide unprecedented insight into the nature and couplings of ultracold, strongly interacting complexes. Previous work has addressed only weakly bound complexes. We show that the main coupling mechanism results from spin-rotation and spin-spin couplings in combination with the anisotropic atom-molecule interaction, and that the collisional complexes which support the resonances have a size of 30-40 $a_0$. This study illustrates the potential of a combined experimental and theoretical approach.

physics.atom-ph↗
arXiv2023

Atomic physics on a 50 nm scale: Realization of a bilayer system of dipolar atoms

Atomic physics has greatly advanced quantum science, mainly due to the ability to control the position and internal quantum state of atoms with high precision, often at the quantum limit. The dominant tool for this is laser light, which can structure and localize atoms in space (e.g., in optical tweezers, optical lattices, 1D tubes or 2D planes). Due to the diffraction limit of light, the natural length scale for most experiments with atoms is on the order of 500 nm or larger. Here we implement a new super-resolution technique which localizes and arranges atoms on a sub-50 nm scale, without any fundamental limit in resolution. We demonstrate this technique by creating a bilayer of dysprosium atoms, mapping out the atomic density distribution with sub-10 nm resolution, and observing dipolar interactions between two physically separated layers via interlayer sympathetic cooling and coupled collective excitations. At 50 nm, dipolar interactions are 1,000 times stronger than at 500 nm. For two atoms in optical tweezers, this should enable purely magnetic dipolar gates with kHz speed.

cond-mat.quant-gas↗